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Journal Articles

Secondary consolidation characteristic of bentonite by long-term consolidation tests of 2.7, 3.7 and 4 years

Takayama, Yusuke; Yamamoto, Yoichi*; Goto, Takahiro*

Jiban Kogaku Janaru (Internet), 18(3), p.317 - 330, 2023/09

It has been reported that the deformation greatly increased in the secondary consolidation process in the past long-term consolidation test of 1.8 years on Na-type bentonite/sand mixed soil. Therefore, we analyzed potential contributing factors in this behavior. A long-term consolidation test for about 10 years on bentonite and kaolinite was started using the test equipment with countermeasures against these factors. In this paper, the secondary consolidation behavior of bentonite was investigated based on the long-term consolidation test data for 2.7, 3.7 and 4 years. The results were generally consistent with the conventional findings on soil mechanics that the deformation due to secondary consolidation progresses linearly with respect to logarithm of time. This test will be continued for about 10 years and longer-term secondary consolidation behavior will be investigated.

JAEA Reports

Study on disposal of waste from reprocessing for commercial HTGR spent fuel

Fukaya, Yuji; Maruyama, Takahiro; Goto, Minoru; Ohashi, Hirofumi; Higuchi, Hideaki

JAEA-Research 2023-002, 19 Pages, 2023/06

JAEA-Research-2023-002.pdf:1.48MB

A study on disposal of waste derived from commercial High Temperature Gas-cooled Reactor ("HTGR") has been performed. Because of significant difference between the reprocessing of Light Water Reactor ("LWR") and that of HTGR due to difference in structures of the fuel, adoptability of the laws relating to reprocessing waste disposal, which is enacted for LWR, to HTGR waste should be confirmed. Then, we compared the technologies and waste of reprocessing and evaluated radioactivity concentration in graphite waste by activation and contamination based on whole core burn-up calculation. As a result, it was found that SiC residue waste should be disposed of into a geological repository as 2nd class designated radioactive waste in the Designated Radioactive Waste Final Disposal Act (Act No.117 of 2000), by way of amendment of the applicable order, same as hull and end-piece of LWR, and graphite waste should be shallowly disposed of than geological disposal as 2nd class waste for pit disposal in the Act on the Regulation of Nuclear Source Material, Nuclear Fuel Material and Reactors (Act No.166 of 1957) same as a channel box of LWR.

JAEA Reports

Development of "MOX weighing and Ball-mill blending" based on experience in operation and maintenance of MOX fuel manufacturing equipment

Kawasaki, Kohei; Ono, Takanori; Shibanuma, Kimikazu; Goto, Kenta; Aita, Takahiro; Okamoto, Naritoshi; Shinada, Kenta; Ichige, Hidekazu; Takase, Tatsuya; Osaka, Yuki; et al.

JAEA-Technology 2022-031, 91 Pages, 2023/02

JAEA-Technology-2022-031.pdf:6.57MB

The document for back-end policy opened to the public in 2018 by Japan Atomic Energy Agency (hereafter, JAEA) states the decommissioning of facilities of Nuclear Fuel Cycle Engineering Laboratories and JAEA have started gathering up nuclear fuel material of the facilities into Plutonium Fuel Production Facilities (hereafter, PFPF) in order to put it long-term, stable and safe storage. Because we planned to manufacture scrap assemblies almost same with Monju fuel assembly using unsealed plutonium-uranium mixed-oxide (hereafter, MOX) powder held in PFPF and transfer them to storage facilities as part of this "concentration" task of nuclear fuel material, we obtained permission to change the use of nuclear fuel material in response to the new regulatory Requirements in Japan for that. The amount of plutonium (which is neither sintered pellets nor in a lidded powder-transport container) that could be handled in the pellet-manufacturing process was limited to 50 kg Pu or less in order to decrease the facility risk in this manufacture. Therefore, we developed and installed the "MOX weighing and blending equipment" corresponding with small batch sizes that functioned in a starting process and the equipment would decrease handling amounts of plutonium on its downstream processes. The failure data based on our operation and maintenance experiences of MOX fuel production facilities was reflected in the design of the equipment to further improve reliability and maintainability in this development. The completed equipment started its operation using MOX powder in February 2022 and the design has been validated through this half-a-year operation. This report organizes the knowledge obtained through the development of the equipment, the evaluation of the design based on the half-a-year operation results and the issues in future equipment development.

JAEA Reports

Annual report for research on geosphere stability for long-term isolation of radioactive waste in fiscal year 2020

Ishimaru, Tsuneari; Ogata, Nobuhisa; Kokubu, Yoko; Shimada, Koji; Niwa, Masakazu; Shimada, Akiomi; Watanabe, Takahiro; Sueoka, Shigeru; Yokoyama, Tatsunori; Fujita, Natsuko; et al.

JAEA-Research 2021-007, 65 Pages, 2021/10

JAEA-Research-2021-007.pdf:4.21MB

This annual report documents the progress of research and development (R&D) in the 6th fiscal year during the JAEA 3rd Mid- and Long-term Plan (fiscal years 2015-2021) to provide the scientific base for assessing geosphere stability for long-term isolation of the high-level radioactive waste. The planned framework is structured into the following categories: (1) Development and systematization of investigation techniques, (2) Development of models for long-term estimation and effective assessment, (3) Development of dating techniques. The current status of R&D activities with previous scientific and technological progress is summarized.

JAEA Reports

Research plan on geosphere stability for long-term isolation of radioactive waste (Scientific program for fiscal year 2021)

Ishimaru, Tsuneari; Kokubu, Yoko; Shimada, Koji; Shimada, Akiomi; Niwa, Masakazu; Watanabe, Takahiro; Sueoka, Shigeru; Yokoyama, Tatsunori; Fujita, Natsuko; Ogita, Yasuhiro; et al.

JAEA-Review 2021-012, 48 Pages, 2021/08

JAEA-Review-2021-012.pdf:1.64MB

This report is a plan of research and development (R&D) on geosphere stability for long-term isolation of high-level radioactive waste (HLW) in Japan Atomic Energy Agency (JAEA), in fiscal year 2021. The objectives and contents in fiscal year 2021 are described in detail based on the JAEA 3rd Medium- and Long-term Plan (fiscal years 2015-2021). In addition, the background of this research is described from the necessity and the significance for site investigation and safety assessment, and the past progress. The plan framework is structured into the following categories: (1) Development and systematization of investigation techniques, (2) Development of models for long-term estimation and effective assessment, (3) Development of dating techniques.

Journal Articles

High temperature gas-cooled reactors

Takeda, Tetsuaki*; Inagaki, Yoshiyuki; Aihara, Jun; Aoki, Takeshi; Fujiwara, Yusuke; Fukaya, Yuji; Goto, Minoru; Ho, H. Q.; Iigaki, Kazuhiko; Imai, Yoshiyuki; et al.

High Temperature Gas-Cooled Reactors; JSME Series in Thermal and Nuclear Power Generation, Vol.5, 464 Pages, 2021/02

As a general overview of the research and development of a High Temperature Gas-cooled Reactor (HTGR) in JAEA, this book describes the achievements by the High Temperature Engineering Test Reactor (HTTR) on the designs, key component technologies such as fuel, reactor internals, high temperature components, etc., and operational experience such as rise-to-power tests, high temperature operation at 950$$^{circ}$$C, safety demonstration tests, etc. In addition, based on the knowledge of the HTTR, the development of designs and component technologies such as high performance fuel, helium gas turbine and hydrogen production by IS process for commercial HTGRs are described. These results are very useful for the future development of HTGRs. This book is published as one of a series of technical books on fossil fuel and nuclear energy systems by the Power Energy Systems Division of the Japan Society of Mechanical Engineers.

Journal Articles

Methodology development and determination of solubility-limiting solid phases for a performance assessment of geological disposal of high-level radioactive and TRU wastes

Kitamura, Akira; Yoshida, Yasushi*; Goto, Takahiro*; Shibutani, Sanae*

Genshiryoku Bakkuendo Kenkyu (CD-ROM), 27(2), p.58 - 71, 2020/12

Evaluation and estimation of solubility values are required for a performance assessment of geological disposal of high-level radioactive and TRU wastes. Selection of solubility-limiting solid phases (SSPs) that control the solubility of radionuclides is necessary for the evaluation and estimation of solubility values. The authors have developed a methodology for selection of the SSP through a calculation of saturation indices (SIs) using thermodynamic database to show a transparent procedure for the selection. Literature survey should be performed to confirm decision of the SSP from candidate SSPs which generally have larger SIs from realistic point of view for precipitation and solubility control. The authors have selected the SSPs for the elements of interest for the latest Japanese performance assessment in bentonite and cement porewaters after grouping various water compositions.

JAEA Reports

Annual report for research on geosphere stability for long-term isolation of radioactive waste in fiscal year 2019

Ishimaru, Tsuneari; Ogata, Nobuhisa; Kokubu, Yoko; Shimada, Koji; Hanamuro, Takahiro; Shimada, Akiomi; Niwa, Masakazu; Asamori, Koichi; Watanabe, Takahiro; Sueoka, Shigeru; et al.

JAEA-Research 2020-011, 67 Pages, 2020/10

JAEA-Research-2020-011.pdf:3.87MB

This annual report documents the progress of research and development (R&D) in the 5th fiscal year during the JAEA 3rd Mid- and Long-term Plan (fiscal years 2015-2021) to provide the scientific base for assessing geosphere stability for long-term isolation of the high-level radioactive waste. The planned framework is structured into the following categories: (1) Development and systematization of investigation techniques, (2) Development of models for long-term estimation and effective assessment, (3) Development of dating techniques. The current status of R&D activities with previous scientific and technological progress is summarized.

JAEA Reports

Research plan on geosphere stability for long-term isolation of radioactive waste (Scientific program for fiscal year 2020)

Ishimaru, Tsuneari; Ogata, Nobuhisa; Shimada, Koji; Kokubu, Yoko; Niwa, Masakazu; Asamori, Koichi; Watanabe, Takahiro; Sueoka, Shigeru; Komatsu, Tetsuya; Yokoyama, Tatsunori; et al.

JAEA-Review 2020-010, 46 Pages, 2020/07

JAEA-Review-2020-010.pdf:1.89MB

This report is a plan of research and development (R&D) on geosphere stability for long-term isolation of high-level radioactive waste (HLW) in Japan Atomic Energy Agency (JAEA), in fiscal year 2020. The objectives and contents in fiscal year 2020 are described in detail based on the JAEA 3rd Medium- and Long-term Plan (fiscal years 2015-2021). In addition, the background of this research is described from the necessity and the significance for site investigation and safety assessment, and the past progress. The plan framework is structured into the following categories: (1) Development and systematization of investigation techniques, (2) Development of models for long-term estimation and effective assessment, (3) Development of dating techniques.

Journal Articles

Reactor physics experiment in graphite moderation system for HTGR, 1

Fukaya, Yuji; Nakagawa, Shigeaki; Goto, Minoru; Ishitsuka, Etsuo; Kawakami, Satoru; Uesaka, Takahiro; Morita, Keisuke; Sano, Tadafumi*

KURNS Progress Report 2018, P. 148, 2019/08

The Japan Atomic Energy Agency (JAEA) started the Research and Development (R&D) to improve nuclear prediction techniques for High Temperature Gas-cooled Reactors (HTGRs). The objectives are to introduce generalized bias factor method to avoid full mock-up experiment for the first commercial HTGR and to introduce reactor noise analysis to High Temperature Engineering Test Reactor (HTTR) experiment. To achieve the objectives, the reactor core of graphite moderation system named B7/4"G2/8"p8EUNU+3/8"p38EU(1) was newly composed in the B-rack of Kyoto University Critical Assembly (KUCA). The core plays a role of the reference core of the bias factor method, and the reactor noise was measured to develop the noise analysis scheme. In addition, training of operator of HTTR was also performed during the experiments.

Journal Articles

Development of performance assessment models for glass dissolution

Goto, Takahiro*; Mitsui, Seiichiro; Takase, Hiroyasu*; Kurosawa, Susumu*; Inagaki, Manabu*; Shibata, Masahiro; Ishiguro, Katsuhiko*

MRS Advances (Internet), 1(63-64), p.4239 - 4245, 2016/00

NUMO and JAEA have conducted a joint research since FY2011, which is designed to enhance the methodology of repository design and performance assessment in preliminary investigation stage for deep geological disposal of radioactive waste. As a part of this joint research, we have been developing glass dissolution models which consider various processes in EBS, such as precipitation of Fe-silicates associated with iron overpack corrosion, and Si transport through corrosion products in the cracked overpack. The objectives of the modeling work are to evaluate relative importance of relevant processes and to identify further R&D issues towards development of a convincing safety case. Sensitivity analyses suggested that predicted glass dissolution time ranges from 1$$times$$10$$^3$$ to 1$$times$$10$$^7$$ years or more due to uncertainties in the current understanding of the key processes, namely precipitation of Fe-silicates and transport characteristics of the altered glass layer.

JAEA Reports

Enhancement of the methodology of repository design and post-closure performance assessment for preliminary investigation stage, 3; Progress report on NUMO-JAEA collaborative research in FY2013 (Joint research)

Shibata, Masahiro; Sawada, Atsushi; Tachi, Yukio; Makino, Hitoshi; Wakasugi, Keiichiro; Mitsui, Seiichiro; Kitamura, Akira; Yoshikawa, Hideki; Oda, Chie; Ishidera, Takamitsu; et al.

JAEA-Research 2014-030, 457 Pages, 2015/03

JAEA-Research-2014-030.pdf:199.23MB

JAEA and NUMO have conducted a collaborative research work which is designed to enhance the methodology of repository design and post-closure performance assessment in preliminary investigation stage. With regard to (1) study on rock suitability in terms of hydrology, based on some examples of developing method of hydro-geological structure model, acquired knowledge are arranged using the tree diagram, and model uncertainty and its influence on the evaluation items were discussed. With regard to (2) study on scenario development, the developed approach for "defining conditions" has been reevaluated and improved from practical viewpoints. In addition, the uncertainty evaluation for the effect of use of cementitious material, as well as glass dissolution model, was conducted with analytical evaluation. With regard to (3) study on setting radionuclide migration parameters, based on survey of precedent procedures, multiple-approach for distribution coefficient of rocks was established, and the adequacy of the approach was confirmed though its application to sedimentary rock and granitic rock. Besides, an approach for solubility setting was developed including the procedure of selection of solubility limiting solid phase. The adequacy of the approach was confirmed though its application to key radionuclides.

JAEA Reports

Enhancement of the methodology of repository design and post-closure performance assessment for preliminary investigation stage, 2; Progress report on NUMO-JAEA collaborative research in FY2012 (Joint research)

Shibata, Masahiro; Sawada, Atsushi; Tachi, Yukio; Hayano, Akira; Makino, Hitoshi; Wakasugi, Keiichiro; Mitsui, Seiichiro; Oda, Chie; Kitamura, Akira; Osawa, Hideaki; et al.

JAEA-Research 2013-037, 455 Pages, 2013/12

JAEA-Research-2013-037.pdf:42.0MB

Following FY2011, JAEA and NUMO have conducted a collaborative research work which is designed to enhance the methodology of repository design and performance assessment in preliminary investigation stage. With regard to (1) study on rock suitability in terms of hydrology, the tree diagram of methodology of groundwater travel time has been extended for crystalline rock, in addition, tree diagram for sedimentary rock newly has been organized. With regard to (2) study on scenario development, the existing approach has been improved in terms of a practical task, and applied and tested for near field focusing on the buffer. In addition, the uncertainty of some important processes and its impact on safety functions are discussed though analysis. With regard to (3) study on setting radionuclide migration parameters, the approaches for parameter setting have been developed for sorption for rocks and solubility, and applied and tested through parameter setting exercises for key radionuclides.

Journal Articles

New result in the production and decay of an isotope, $$^{278}$$113 of the 113th element

Morita, Kosuke*; Morimoto, Koji*; Kaji, Daiya*; Haba, Hiromitsu*; Ozeki, Kazutaka*; Kudo, Yuki*; Sumita, Takayuki*; Wakabayashi, Yasuo*; Yoneda, Akira*; Tanaka, Kengo*; et al.

Journal of the Physical Society of Japan, 81(10), p.103201_1 - 103201_4, 2012/10

 Times Cited Count:167 Percentile:97.27(Physics, Multidisciplinary)

An isotope of the 113th element, $$^{278}$$113, was produced in a nuclear reaction with a $$^{70}$$Zn beam on a $$^{209}$$Bi target. We observed six consecutive $$alpha$$ decays following the implantation of a heavy particle in nearly the same position in the semiconductor detector, in extremely low background condition. The fifth and sixth decays are fully consistent with the sequential decays of $$^{262}$$Db and $$^{258}$$Lr both in decay energies and decay times. This indicates that the present decay chain consisted of $$^{278}$$113, $$^{274}$$Rg (Z = 111), $$^{270}$$Mt (Z = 109), $$^{266}$$Bh (Z = 107), $$^{262}$$Db (Z = 105), and $$^{258}$$Lr (Z = 103) with firm connections. This result, together with previously reported results from 2004 and 2007, conclusively leads the unambiguous production and identification of the isotope $$^{278}$$113, of the 113th element.

JAEA Reports

Enhancement of the methodology of repository design and post-closure performance assessment for preliminary investigation stage; Progress report on NUMO-JAEA collaborative research in FY2011 (Joint research)

Shibata, Masahiro; Sawada, Atsushi; Tachi, Yukio; Makino, Hitoshi; Hayano, Akira; Mitsui, Seiichiro; Taniguchi, Naoki; Oda, Chie; Kitamura, Akira; Osawa, Hideaki; et al.

JAEA-Research 2012-032, 298 Pages, 2012/09

JAEA-Research-2012-032.pdf:33.68MB

JAEA and NUMO have conducted a collaborative research work which is designed to enhance the methodology of repository design and performance assessment in preliminary investigation phase. The topics and the conducted research are follows; (1) Study on selection of host rock: in terms of hydraulic properties, items for assessing rock property, and assessment methodology of groundwater travel time has been organized with interaction from site investigation. (2) Study on development of scenario: the existing approach has been embodied, in addition, the phenomenological understanding regarding dissolution of and nuclide release from vitrified waste, corrosion of the overpack, long-term performance of the buffer are summarized. (3) Study on setting nuclide migration parameters: the approach for parameter setting has been improved for sorption and diffusion coefficient of buffer/rock, and applied and tested for parameter setting of key radionuclides. (4) Study on ensuring quality of knowledge: framework for ensuring quality of knowledge has been studied and examined aimed at the likely disposal facility condition.

Journal Articles

Sulfate complexation of element 104, Rf, in H$$_{2}$$SO$$_{4}$$/HNO$$_{3}$$ mixed solution

Li, Z.*; Toyoshima, Atsushi; Asai, Masato; Tsukada, Kazuaki; Sato, Tetsuya; Sato, Nozomi; Kikuchi, Takahiro; Nagame, Yuichiro; Sch$"a$del, M.; Pershina, V.*; et al.

Radiochimica Acta, 100(3), p.157 - 164, 2012/03

 Times Cited Count:13 Percentile:69.01(Chemistry, Inorganic & Nuclear)

Journal Articles

Identified charged hadron production in $$p + p$$ collisions at $$sqrt{s}$$ = 200 and 62.4 GeV

Adare, A.*; Afanasiev, S.*; Aidala, C.*; Ajitanand, N. N.*; Akiba, Yasuyuki*; Al-Bataineh, H.*; Alexander, J.*; Aoki, Kazuya*; Aphecetche, L.*; Armendariz, R.*; et al.

Physical Review C, 83(6), p.064903_1 - 064903_29, 2011/06

 Times Cited Count:184 Percentile:99.44(Physics, Nuclear)

Transverse momentum distributions and yields for $$pi^{pm}, K^{pm}, p$$, and $$bar{p}$$ in $$p + p$$ collisions at $$sqrt{s}$$ = 200 and 62.4 GeV at midrapidity are measured by the PHENIX experiment at the RHIC. We present the inverse slope parameter, mean transverse momentum, and yield per unit rapidity at each energy, and compare them to other measurements at different $$sqrt{s}$$ collisions. We also present the scaling properties such as $$m_T$$ and $$x_T$$ scaling and discuss the mechanism of the particle production in $$p + p$$ collisions. The measured spectra are compared to next-to-leading order perturbative QCD calculations.

Journal Articles

Azimuthal correlations of electrons from heavy-flavor decay with hadrons in $$p+p$$ and Au+Au collisions at $$sqrt{s_{NN}}$$ = 200 GeV

Adare, A.*; Afanasiev, S.*; Aidala, C.*; Ajitanand, N. N.*; Akiba, Yasuyuki*; Al-Bataineh, H.*; Alexander, J.*; Aoki, Kazuya*; Aphecetche, L.*; Aramaki, Y.*; et al.

Physical Review C, 83(4), p.044912_1 - 044912_16, 2011/04

 Times Cited Count:8 Percentile:49.7(Physics, Nuclear)

Measurements of electrons from the decay of open-heavy-flavor mesons have shown that the yields are suppressed in Au+Au collisions compared to expectations from binary-scaled $$p+p$$ collisions. Here we extend these studies to two particle correlations where one particle is an electron from the decay of a heavy flavor meson and the other is a charged hadron from either the decay of the heavy meson or from jet fragmentation. These measurements provide more detailed information about the interaction between heavy quarks and the quark-gluon matter. We find the away-side-jet shape and yield to be modified in Au+Au collisions compared to $$p+p$$ collisions.

Journal Articles

Anionic fluoro complex of element 105, Db

Kasamatsu, Yoshitaka*; Toyoshima, Atsushi; Asai, Masato; Tsukada, Kazuaki; Li, Z.; Ishii, Yasuo; Tome, Hayato*; Sato, Tetsuya; Kikuchi, Takahiro; Nishinaka, Ichiro; et al.

Chemistry Letters, 38(11), p.1084 - 1085, 2009/10

 Times Cited Count:15 Percentile:48.93(Chemistry, Multidisciplinary)

We report on the characteristic anion-exchange behavior of the superheavy element dubnium (Db) with atomic number Z = 105 in HF/HNO$$_{3}$$ solution at the fluoride ion concentration [F$$^{-}$$] = 0.003 M. The result clearly demonstrates that the fluoro complex formation of Db is significantly different from that of the group-5 homologue Ta in the 6th period of the periodic table while the behavior of Db is similar to that of the lighter homologue Nb in the 5th period.

Journal Articles

Attempt to produce the 3rd chain of $$^{278}$$113

Morimoto, Koji*; Morita, Kosuke*; Kaji, Daiya*; Akiyama, Takahiro*; Goto, Shinichi*; Haba, Hiromitsu*; Ideguchi, Eiji*; Katori, Kenji*; Koura, Hiroyuki; Kudo, Hisaaki*; et al.

RIKEN Accelerator Progress Report, Vol.42, P. 15, 2009/00

In 2003-2007, we had performed an experiment to synthesize an element 113 by a $$^{209}$$Bi$$+$$ $$^{70}$$Zn reaction using a gas-filled recoil ion separator (GARIS) at RIKEN Nishina-Center. In a total of 241 days of net irradiation time experiment, two decay chains were observed and assigned from an isotope $$^{278}$$113. The cross section of the $$^{209}$$Bi($$^{70}$$Zn,n)$$^{278}$$113 reaction was determined to be 31$$^{+40}_{-20}$$ fb at that time. In order to increase the statistics of the decay property, we continued to produce more decay chains. The experiment was carried out from January 7 to March 31, 2008. The experimental conditions were identical to those used in the previous experiment. $$^{70}$$Zn ion beam of 353 MeV was extracted from RILAC. The net irradiation time was 83 days and the total dose of $$^{70}$$Zn was 2.28$$times10^{19}$$. In the present expriment any candidate of $$^{278}$$113 was not observed. Then combining the results of the present and previous experiments, the production cross section of $$^{278}$$113 was determined to be 22$$^{+29}_{-19}$$ fb.

55 (Records 1-20 displayed on this page)