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Journal Articles

Development of new filter device removing a fine particle in high level liquid waste

Takahatake, Yoko; Goto, Ichiro*; Watanabe, So; Nakamura, Masahiro; Sano, Yuichi

Proceedings of International Conference on GLOBAL 2026 (Internet), p.722 - 731, 2026/08

Journal Articles

Enhancement of antioxidant function in various organs in mice using combined thermal and radon inhalation treatment

Miyanaga, Shogo*; Tanaka, Ayumi*; Takenaka, Reiju*; Naoe, Shota; Goto, Shuna*; Nagano, Mitsuki*; Tano, Kotaro*; Kanzaki, Norie; Sakoda, Akihiro; Yamaoka, Kiyonori*; et al.

Journal of Radiation Research (Internet), 67(4), p.538 - 549, 2026/07

 Times Cited Count:0 Percentile:0.00(Biology)

Journal Articles

Measurements of circular polarization from the 0.75-eV p-wave resonance of the $$^{139}$$La(n,$$gamma$$)$$^{140}$$La reaction

Endo, Shunsuke; Fujioka, Hiroyuki*; Goto, Yu*; Ino, Takashi*; Iwamoto, Osamu; Iwamoto, Nobuyuki; Kawamura, Shiori*; Kimura, Atsushi; Kitaguchi, Masaaki*; Kobayashi, Ryuju; et al.

JPS Conference Proceedings (Internet), 45, p.011056_1 - 011056_8, 2026/06

Journal Articles

J-PARC LINAC 50 Hz operation verification study

Kondo, Yasuhiro; Chimura, Motoki; Cicek, E.*; Fukui, Yuji*; Futatsukawa, Kenta*; Fuwa, Yasuhiro; Goto, Rikuto*; Hirano, Koichiro; Ishikawa, Masaki*; Ito, Takashi; et al.

Proceedings of 22nd Annual Meeting of Particle Accelerator Society of Japan (Internet), p.124 - 129, 2026/03

Various upgrade plans of the J-PARC linac are underway, and repetition-rate doubling project is one of the most important part. Currently, the linac supplies a 400~MeV H$$^-$$ ion beam to the 3~GeV synchrotron (RCS) at a repetition rate of 25~Hz. However, to deliver the beam to both RCS and proton-beam irradiation facility under planning, it is necessary to raise the repetition rate from 25~Hz to 50~Hz. Prior to construction of the beamline to the irradiation facility, we conducted a verification of the 50~Hz operation of all the linac apparatus simultaneously within the current operational limits in May 2025. And also, the verification of the 50~Hz operation of the particle counter system, which is one of the most important safety device of the J-PARC accelerator, was conducted. As a result, any significant problems were not found out, and it is now ready for the upcoming 50~Hz-beam acceleration demonstration. This paper describes this details of the demonstration of the 50~Hz operation, without beam acceleration, of the J-PARC linac.

Journal Articles

Complete genome sequences of ${it Micrococcus luteus}$ isolated from the radioactive element-containing water in Fukushima Daiichi Nuclear Power Station Unit 2

Dotsuta, Yuma; Taniguchi, Itsuki*; Goto, Yasuhiro*; Hayashi, Tetsuya*; Kurokawa, Ken*; Warashina, Tomoro*; Kanai, Akio*; Kitagaki, Toru

Microbiology Resource Announcements (Internet), 14(10), p.e00769-25_1 - e00769-25_3, 2025/10

Four bacteria strains with yellow-colored colonies which were Isolated from the radioactively element-containing water in Fukushima Daiichi Nuclear Power Station Unit 2 were identified as ${it Micrococcus luteus}$. Here, we present the complete genome sequences of these species assembled via a combination of short-read and long-read sequencing techniques.

Journal Articles

Development of fluorinated ligands for uranium recovery from radioactive liquid waste

Arai, Yoichi; Goto, Yasuhiro; Watanabe, So; Agou, Tomohiro*; Arai, Tsuyoshi*; Katsuki, Kenta*; Fukumoto, Hiroki*; Hoshina, Hiroyuki*; Seko, Noriaki*

Progress in Nuclear Science and Technology (Internet), 8, p.329 - 332, 2025/09

Journal Articles

Analysis of uranium, plutonium and fission product nuclides in process solution during flush-out for decommissioning of reprocessing plant

Yamamoto, Masahiko; Horigome, Kazushi; Goto, Yuichi; Taguchi, Shigeo; Kuno, Takehiko

Progress in Nuclear Science and Technology (Internet), 8, p.387 - 392, 2025/09

Flush-out of Tokai Reprocessing Plant was completed in February, 2024 for the preparation of process decontamination. Since remaining nuclear materials were contained in main process, purpose of the activities was to recover nuclear materials by transferring them to the highly radioactive liquid waste storage tank and converting uranium solution into uranium trioxide, and to rinse all related processes with nitric acid and water. During this activity, analysis of U and Pu was conducted for nuclear material control and accountancy. Appropriate analytical methods such as isotope dilution mass spectrometry, gravimetric method, spectrophotometry and alpha-ray counting methods were selected depending on the status of flush-out. Also, gamma-ray emitted nuclides in rinsing solution were detected by highly purified germanium detector. This paper describes analysis and its results related to flush-out activities of decommissioning in reprocessing plant.

Journal Articles

Development trends of advanced reactor with a focus on fast reactor and high temperature gas-cooled reactor, 1; Development trends of fast reactor cycle (reactor system)

Ando, Masato; Goto, Shoji; Usui, Yukinori*

Nihon Genshiryoku Gakkai-Shi ATOMO$$Sigma$$, 67(8), p.471 - 475, 2025/08

no abstracts in English

JAEA Reports

Analysis of the radioactivity concentrations in radioactive waste stored at the Waste Storage Facility L as compressed packages

Aono, Ryuji; Goto, Katsunori*; Kinase, Akari; Sato, Yoshiyuki; Haraga, Tomoko; Iseda, Hirokatsu

JAEA-Data/Code 2025-006, 24 Pages, 2025/07

JAEA-Data-Code-2025-006.pdf:1.05MB

Radioactive wastes generated from nuclear research facilities in Japan Atomic Energy Agency are planned to be buried in the near surface disposal field as trench and pit. Therefore, it is required to establish the method to evaluate the radioactivity concentrations of radioactive wastes until the beginning of disposal. In order to contribute to this work, we collected and analyzed the samples stored at the waste storage facility L. In this report, we summarized the radioactivity concentrations of 12 radionuclides ($$^{3}$$H, $$^{14}$$C, $$^{60}$$Co, $$^{90}$$Sr, $$^{94}$$Nb, $$^{137}$$Cs, $$^{152}$$Eu, $$^{154}$$Eu, $$^{238}$$Pu, $$^{239}$$Pu, $$^{240}$$Pu, $$^{241}$$Am) which were obtained from radiochemical analysis of the samples in fiscal year 2020.

Journal Articles

Removal techniques for contaminated analytical Grove Box with nuclear fuel materials

Yokochi, Masaru; Goto, Yuichi; Kuno, Sorato; Suzuki, Yoshimasa; Yamamoto, Masahiko; Taguchi, Shigeo; Usui, Masato*; Onose, Taku*; Miyamoto, Toshihiko*; Mori, Eito*

Nihon Hozen Gakkai Dai-21-Kai Gakujutsu Koenkai Yoshishu, 4 Pages, 2025/07

Analysis facility in Tokai Reprocessing Plant, which is shifted to decommissioning stage, have been installed about 60 Grove Boxes to handling the nuclear fuel materials. Of these, progressing an aging accompanied by long use for 20 years more than half. This time, removal the special Grove Box that equipped the Thermal Ionization Mass Spectrometry, necessary safeguard analysis for nuclear fuel materials. This report summarized the removal techniques of the special Grove Box, the number of working days, workers and amount of waste generated in this removal work.

Journal Articles

Implementation of firebreaks as part of fire safety measures at the Tokai Reprocessing Plant

Tsuboi, Masatoshi; Takase, Yuki; Otsu, Shuya; Goto, Sho; Uno, Shota; Sakamoto, Gen; Mitoma, Kenshin; Yasuo, Kiyoshi

Nihon Hozen Gakkai Dai-21-Kai Gakujutsu Koenkai Yoshishu, 4 Pages, 2025/07

no abstracts in English

Journal Articles

Application of the spectral determination method to unified $$beta$$-, $$gamma$$- and X-ray spectra

Oshima, Masumi*; Goto, Jun*; Hayakawa, Takehito*; Asai, Masato; Shinohara, Hirofumi*; Suzuki, Katsuyuki*; Shen, H.*

Journal of Nuclear Science and Technology, 62(4), p.379 - 388, 2025/04

 Times Cited Count:1 Percentile:0.00(Nuclear Science & Technology)

The spectrum determination method (SDM) is the method to determine radioactivities by analyzing full spectral shape of $$beta$$- or $$gamma$$ rays through least-squares fitting by referring to standard $$beta$$- and $$gamma$$ spectra. In this paper, we have newly applied the SDM to a unified spectrum composed of two spectra measured with a Ge detector and a liquid scintillation counter. By analyzing the unified spectrum, uncertainties of deduced radioactivities have been improved. We applied this method to the unified spectrum including 40 radionuclides with equal intensities, and have deduced their radioactivities correctly.

JAEA Reports

Analysis work on flush-out of plutonium and uranium for decommissioning of main plant in Tokai Reprocessing Plant

Sato, Hinata; Mori, Amami; Kuno, Sorato; Horigome, Kazushi; Goto, Yuichi; Yamamoto, Masahiko; Taguchi, Shigeo

JAEA-Technology 2024-011, 56 Pages, 2024/10

JAEA-Technology-2024-011.pdf:2.5MB

Flush-out, which recovers remaining nuclear materials in the process and transfer it to a highly radioactive liquid waste storage tank, has been performed at main plant of Tokai Reprocessing Plant. The flush-out has been composed from three steps: first step is to remove of spent fuel sheared powder, second step is to collect plutonium solution stored in the process, and third step is to convert uranium solution into uranium trioxide powder. The first step of flush-out activity has been completed in 2022. Second and third steps of flush-out have been completed from March 2023 to February 2024. Process control analysis has been performed for operation of the facility, and material accountancy analysis has been performed to control the accountancy of nuclear materials. In addition, related analytical work such as pretreatment for transporting inspection samples for safeguards analysis laboratories in IAEA has been also performed. This report describes results of analytical work performed in collections of plutonium and uranium solutions in second and third steps of the flush-out, including calibration of analytical equipment, waste generation, and education and training of analytical operator.

JAEA Reports

Neutron optics design of a neutron magnetic microscope using Wolter type I supermirror

Soyama, Kazuhiko; Hayashida, Hirotoshi*; Maruyama, Ryuji; Yamazaki, Dai; Goto, Yoshiki*; Kobayashi, Yuki*; Arakawa, Shohei*; Yamamoto, Yugo*; Suba, Kenta*; Yamamura, Kazuya*

JAEA-Research 2024-006, 15 Pages, 2024/10

JAEA-Research-2024-006.pdf:1.51MB

A neutron optics design has been conducted for a neutron magnetic microscope that utilize a Wolter type I multilayer supermirror for the purpose of magnetic fields imaging in magnetic materials. Ray trace simulation was performed for a magnifying imaging optical system with a magnification rate of 12.5 times. Based on classical model of Lamor precession, depolarization due to magnetic domains was simulated, and the effect of slope errors on the Wolter mirror created by the replica method on the spatial resolution of the microscope was investigated. As a result, reference data about the shape error required to obtain spatial resolution on the order of micrometers was obtained.

Journal Articles

Analysis of nuclear materials in process solution during flush-out activities for decommissioning of reprocessing plant

Yamamoto, Masahiko; Horigome, Kazushi; Goto, Yuichi; Taguchi, Shigeo

Proceedings of International Conference on Nuclear Fuel Cycle (GLOBAL2024) (Internet), 4 Pages, 2024/10

Flush-out activities of Tokai Reprocessing Plant were completed in February, 2024. Since it contained remaining nuclear materials in main process of the facility, purpose of activities was to flush-out them and to rinse with nitric acid solution. This paper describes analysis of nuclear materials related to flush-out activities.

Journal Articles

Hydroxyl group/fluorine disorder in deuterated magnesium hydroxyfluoride and behaviors of hydrogen bonds under high pressure

He, X.*; Kagi, Hiroyuki*; Komatsu, Kazuki*; Iizuka, Riko*; Okajima, Hajime*; Hattori, Takanori; Sano, Asami; Machida, Shinichi*; Abe, Jun*; Goto, Hirotada*; et al.

Journal of Molecular Structure, 1310, p.138271_1 - 138271_8, 2024/08

 Times Cited Count:0 Percentile:0.00(Chemistry, Physical)

High-pressure responses of the O-D$$cdotcdotcdot$$F hydrogen bonds in deuterated magnesium hydroxyfluoride were investigated using neutron powder diffraction and Raman spectroscopy. The Rietveld analysis at ambient conditions revealed a chemical formula of Mg(OD)$$_{0.920(12)}$$F$$_{1.080(12)}$$ and hydroxyl group/fluorine disorder (OD/F disorder) in the crystal structure, which gave rise to two hydrogen-bonding configurations. The Rietveld analysis showed the hydrogen-bonding geometries remains up to 9.8 GPa, indicating no pressure-induced strengthening of hydrogen bonds. The Raman spectra at ambient conditions showed three hydroxyl stretching bands at 2613, 2694, and 2718 cm$$^{-1}$$. The high frequencies of the O-D stretching modes indicated that the hydroxyls should be involved in weak or none hydrogen-bonding interactions. Up to 20.2 GPa, the mode initially centered at 2694 cm$$^{-1}$$ displayed a pressure-induced blue shift, revealing no strengthening of hydrogen bonds under compression. We discuss the existence of hydrogen bonds and the causes of the blue-shifting hydroxyls at ambient and at high pressures.

JAEA Reports

Analysis of the radioactivity concentrations in radioactive waste generated from JRR-2 and JRR-3 and Stored at the Waste Storage Facility L as compressed packages

Kinase, Akari; Goto, Katsunori*; Aono, Ryuji; Konda, Miki; Sato, Yoshiyuki; Haraga, Tomoko; Ishimori, Kenichiro; Kameo, Yutaka

JAEA-Data/Code 2024-004, 60 Pages, 2024/07

JAEA-Data-Code-2024-004.pdf:2.05MB

Radioactive wastes generated from nuclear research facilities in Japan Atomic Energy Agency are planning to be buried in the near surface disposal field as trench and pit. Therefore, it is required to establish the method to evaluate the radioactivity concentrations of radioactive wastes until the beginning of disposal. In order to contribute to this work, we collected and analyzed the samples generated from JRR-2 and JRR-3 and stored at the waste storage facility L. In this report, we summarized the radioactivity concentrations of 20 radionuclides ($$^{3}$$H, $$^{14}$$C, $$^{36}$$Cl, $$^{60}$$Co, $$^{63}$$Ni, $$^{90}$$Sr, $$^{94}$$Nb, $$^{99}$$Tc, $$^{108m}$$Ag, $$^{129}$$I, $$^{137}$$Cs, $$^{152}$$Eu, $$^{154}$$Eu, $$^{234}$$U, $$^{238}$$U, $$^{238}$$Pu, $$^{239}$$Pu, $$^{240}$$Pu, $$^{241}$$Am, $$^{244}$$Cm) which were obtained from radiochemical analysis of the samples in fiscal year 2022.

Journal Articles

Application of the spectral determination method to liquid scintillation spectra

Oshima, Masumi*; Goto, Jun*; Hayakawa, Takehito*; Shinohara, Hirofumi*; Suzuki, Katsuyuki*; Sano, Yuichi*; Asai, Masato; Haraga, Tomoko

Journal of Nuclear Science and Technology, 61(7), p.871 - 882, 2024/07

 Times Cited Count:2 Percentile:11.16(Nuclear Science & Technology)

Previously we reported a simple algorithmic method of spectral determination method (SDM), which is based on the first principle that a $$gamma$$-ray spectrum obtained for a sample is a linear superposition of individual spectra of the radioactive nuclides included in the sample and demonstrated that the method is valid for $$gamma$$-ray determination. Here we apply it to the spectra obtained by liquid scintillation counter (LSC). In LSC measurements quenching is generally observed and we at first developed its correction method to standard spectra. The SDM code reported in the previous investigation is used to analyze the LSC spectra. Based on the analyses done by using the measured spectra, we concluded that the SDM method is valid in the LSC spectra similarly to the $$gamma$$-ray spectra studied in the previous investigation.

Journal Articles

Sustainable thermoelectric materials; Utilizing Fukushima weathered biotite via molten salt treatment

Honda, Mitsunori; Kaneta, Yui; Muraguchi, Masakazu*; Hayakawa, Kosetsu*; Oda, Masato*; Iino, Chiaki*; Ishii, Hiroyuki*; Goto, Takuya*

AIP Advances (Internet), 14(5), p.055034_1 - 055034_6, 2024/05

 Times Cited Count:6 Percentile:45.46(Nanoscience & Nanotechnology)

This study examines the utilization of Fukushima weathered biotite(WB)as an alternative to conventional thermoelectric materials traditionally derived from rare and toxic substances. WB underwent milling, classification, and subsequent heat treatment via molten-salt treatment to produce crystals exhibiting conductivity akin to semiconductors within from 650$$^{circ}$$C to 850$$^{circ}$$C range. Evaluation of WB and the derived crystal's electrical conductivity and Seebeck coefficient showcased their viability for high-temperature thermoelectric applications. Consequently, WB attained a dimensionless figure of merit (ZT) of 0.015, signaling its potential as a thermoelectric material that surpasses 650$$^{circ}$$C.

Journal Articles

Optimization in granulation conditions for adsorbent of extraction chromatography

Hasegawa, Kenta; Goto, Ichiro*; Miyazaki, Yasunori; Ambai, Hiromu; Watanabe, So; Watanabe, Masayuki; Sano, Yuichi; Takeuchi, Masayuki

Mechanical Engineering Journal (Internet), 11(2), p.23-00407_1 - 23-00407_8, 2024/04

574 (Records 1-20 displayed on this page)