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Chung, J.-H.*; Kwangwoo, S.*; Yokoo, Tetsuya R.; Ueta, Daichi*; Imai, Masaki; Kim, H.-S.; Kiem, D. H.; Han, M. J.*; Shamoto, Shinichi
Scientific Reports (Internet), 15, p.5978_1 - 5978_10, 2025/02
Times Cited Count:0 Percentile:0.00(Multidisciplinary Sciences)Yang, Q.*; Yang, X.*; Wang, Y.*; Fei, Y.*; Li, F.*; Zheng, H.*; Li, K.*; Han, Y.*; Hattori, Takanori; Zhu, P.*; et al.
Nature Communications (Internet), 15, p.7778_1 - 7778_9, 2024/09
Times Cited Count:11 Percentile:88.19(Multidisciplinary Sciences)Luminescent materials that simultaneously embody bright singlet and triplet excitons hold great potential in optoelectronics, signage, and information encryption. However, achieving high-performance white-light emission is severely hampered by their inherent unbalanced contribution of fluorescence and phosphorescence. Herein, we address this challenge by pressure treatment engineering via hydrogen bonding cooperativity effect to realize the mixture of n--
transitions, where the triplet state emission was boosted from 7% to 40% in isophthalic acid (IPA). A superior white-light emission based on hybrid fluorescence and phosphorescence was harvested in pressure-treated IPA, and the photoluminescence quantum yield was increased to 75% from the initial 19% (blue-light emission). In-situ high-pressure IR spectra, X ray diffraction, and neutron diffraction reveal continuous strengthening of the hydrogen bonds with the increase of pressure. Furthermore, this enhanced hydrogen bond is retained down to the ambient conditions after pressure treatment, awarding the targeted IPA efficient intersystem crossing for balanced singlet/triplet excitons population and resulting in efficient white-light emission. This work not only proposes a route for brightening triplet states in organic small molecule, but also regulates the ratio of singlet and triplet excitons to construct high-performance white-light emission.
Nguyen, T.-D.*; Singh, C.*; Kim, Y. S.*; Han, J. H.*; Lee, D.-H.*; Lee, K.*; Harjo, S.; Lee, S. Y.*
Journal of Materials Research and Technology, 31, p.1547 - 1556, 2024/07
Times Cited Count:3 Percentile:70.74(Materials Science, Multidisciplinary)Zeng, Z.*; Zhou, C.*; Zhou, H.*; Han, L.*; Chi, R.*; Li, K.*; Kofu, Maiko; Nakajima, Kenji; Wei, Y.*; Zhang, W.*; et al.
Nature Physics, 20(7), p.1097 - 1102, 2024/07
Times Cited Count:12 Percentile:94.31(Physics, Multidisciplinary)Kim, Y. S.*; Chae, H.*; Lee, D.-Y.*; Han, J. H.*; Hong, S.-K.*; Na, Y. S.*; Harjo, S.; Kawasaki, Takuro; Woo, W.*; Lee, S.-Y.*
Materials Science & Engineering A, 899, p.146453_1 - 146453_7, 2024/05
Times Cited Count:4 Percentile:79.11(Nanoscience & Nanotechnology)Park, P.*; Cho, W.*; Kim, C.*; An, Y.*; Kang, Y.-G.*; Avdeev, M.*; Sibille, R.*; Iida, Kazuki*; Kajimoto, Ryoichi; Lee, K. H.*; et al.
Nature Communications (Internet), 14, p.8346_1 - 8346_9, 2023/12
Times Cited Count:23 Percentile:86.45(Multidisciplinary Sciences)Tamii, Atsushi*; Pellegri, L.*; Sderstr
m, P.-A.*; Allard, D.*; Goriely, S.*; Inakura, Tsunenori*; Khan, E.*; Kido, Eiji*; Kimura, Masaaki*; Litvinova, E.*; et al.
European Physical Journal A, 59(9), p.208_1 - 208_21, 2023/09
Times Cited Count:8 Percentile:83.85(Physics, Nuclear)no abstracts in English
Boznar, M. Z.*; Charnock, T. W.*; Chouhan, S. L.*; Grsic, Z.*; Halsall, C.*; Heinrich, G.*; Helebrant, J.*; Hettrich, S.*; Kua, P.*; Mancini, F.*; et al.
IAEA-TECDOC-2001, 226 Pages, 2022/06
The IAEA organized a programme from 2012 to 2015 entitled Modelling and Data for Radiological Impact Assessments (MODARIA), which aimed to improve capabilities in the field of environmental radiation dose assessment by acquiring improved data, model testing and comparison of model inputs, assumptions and outputs, reaching a consensus on modelling philosophies, aligning approaches and parameter values, developing improved methods and exchanging information. This publication describes the activities of Working Group 2, Exposures in Contaminated Urban Environments and Effect of Remedial Measures.
Thiessen, K. M.*; Boznar, M. Z.*; Charnock, T. W.*; Chouhan, S. L.*; Federspiel, L.; Grai
, B.*; Grsic, Z.*; Helebrant, J.*; Hettrich, S.*; Hulka, J.*; et al.
Journal of Radiological Protection, 42(2), p.020502_1 - 020502_8, 2022/06
Times Cited Count:5 Percentile:60.29(Environmental Sciences)Zhang, J.*; Chen, M.*; Chen, J.*; Yamamoto, Kei; Wang, H.*; Hamdi, M.*; Sun, Y.*; Wagner, K.*; He, W.*; Zhang, Y.*; et al.
Nature Communications (Internet), 12, p.7258_1 - 7258_8, 2021/12
Times Cited Count:21 Percentile:77.31(Multidisciplinary Sciences)Yan, S. Q.*; Li, X. Y.*; Nishio, Katsuhisa; Lugaro, M.*; Li, Z. H.*; Makii, Hiroyuki; Pignatari, M.*; Wang, Y. B.*; Orlandi, R.; Hirose, Kentaro; et al.
Astrophysical Journal, 919(2), p.84_1 - 84_7, 2021/10
Times Cited Count:5 Percentile:33.27(Astronomy & Astrophysics)Gao, D.*; Tang, X.*; Wang, X.*; Yang, X.*; Zhang, P.*; Che, G.*; Han, J.*; Hattori, Takanori; Wang, Y.*; Dong, X.*; et al.
Physical Chemistry Chemical Physics, 23(35), p.19503 - 19510, 2021/09
Times Cited Count:7 Percentile:42.22(Chemistry, Physical)Pressure-induced phase transition and polymerization of nitrogen-rich molecules are widely focused due to its extreme importance for the development of green high energy density materials. Here, we present a study of the phase transition and chemical reaction of 1H-tetrazole up to 100 GPa by using Raman, IR, X-ray diffraction, neutron diffraction techniques and theoretical calculation. A phase transition above 2.6 GPa was identified and the high-pressure structure was determined with one molecule in a unit cell. The 1H-tetrazole polymerizes reversibly below 100 GPa, probably through a carbon-nitrogen bonding instead of nitrogen-nitrogen bonding. Our studies updated the structure model of the high pressure phase of 1H-tetrazole, and presented the possible intermolecular bonding route for the first time, which gives new insights to understand the phase transition and chemical reaction of nitrogen-rich compounds, and benefit for designing new high energy density materials.
Yao, Y.*; Cai, R.*; Yang, S.-H.*; Xing, W.*; Ma, Y.*; Mori, Michiyasu; Ji, Y.*; Maekawa, Sadamichi; Xie, X.-C.*; Han, W.*
Physical Review B, 104(10), p.104414_1 - 104414_6, 2021/09
Times Cited Count:8 Percentile:41.33(Materials Science, Multidisciplinary)Soler, J. M.*; Meng, S.*; Moreno, L.*; Neretnieks, I.*; Liu, L.*; Kekl
inen, P.*; Hokr, M.*;
ha, J.*; Vete
n
k, A.*; Reimitz, D.*; et al.
SKB TR-20-17, 71 Pages, 2021/07
Task 9B of the SKB Task Force on Modelling of Groundwater Flow and Transport of Solutes in fractured rock focused on the modelling of experimental results from the LTDE-SD in situ tracer test performed at the sp
Hard Rock Laboratory in Sweden. Ten different modelling teams provided results for this exercise, using different concepts and codes. Three main types of modelling approaches were used: (1) analytical solutions to the transport-retention equations, (2) continuum-porous-medium numerical models, and (3) microstructure-based models accounting for small-scale heterogeneity (i.e. mineral grains and microfracture distributions). The modelling by the different teams allowed the comparison of many different model concepts, especially in terms of potential zonations of rock properties (porosity, diffusion, sorption), such as the presence of a disturbed zone at the rock and fracture surface, the potential effects of micro- and cm-scale fractures.
Tanaka, Junki*; Yang, Z.*; Typel, S.*; Adachi, Satoshi*; Bai, S.*; van Beek, P.*; Beaumel, D.*; Fujikawa, Yuki*; Han, J.*; Heil, S.*; et al.
Science, 371(6526), p.260 - 264, 2021/01
Times Cited Count:75 Percentile:99.30(Multidisciplinary Sciences)By employing quasi-free -cluster-knockout reactions, we obtained direct experimental evidence for the formation of
clusters at the surface of neutron-rich tin isotopes. The observed monotonous decrease of the reaction cross sections with increasing mass number, in excellent agreement with the theoretical prediction, implies a tight interplay between
-cluster formation and the neutron skin.
Kim, S.*; Lee, B.*; Reeder, J. T.*; Seo, S. H.*; Lee, S.-U.*; Hourlier-Fargette, A.*; Shin, J.*; Sekine, Yurina; Jeong, H.*; Oh, Y. S.*; et al.
Proceedings of the National Academy of Sciences of the United States of America, 117(45), p.27906 - 27915, 2020/11
Times Cited Count:109 Percentile:94.20(Multidisciplinary Sciences)In this study, we present a wireless, battery-free, skin-interfaced microfluidic system that combines lateral flow immunoassay for sweat cortisol assay, fluorometric imaging of glucose and ascorbic acid (vitamin C) assays, and digital tracking of sweat rate using electrodes that measure skin galvanic response. Systematic benchtop testing and on-body field studies on human subjects exercising in a gym environment highlight the key multifunctional features of this platform in tracking the biochemical correlates of physical stress.
El-Asaad, H.*; Nagai, Haruyasu; Sagara, Hiroshi*; Han, C. Y.*
Annals of Nuclear Energy, 141, p.107292_1 - 107292_9, 2020/06
Times Cited Count:0 Percentile:0.00(Nuclear Science & Technology)Atmospheric dispersion simulations can provide crucial information to assess radioactive plumes in the environment for nuclear emergency preparedness. However, it is a difficult and time-consuming task to make simulations assuming many possible scenarios and to derive data from a vast number of results. Therefore, an interface was developed to assist users in conveying characteristics of plumes from simulation results. The interface uses a large database that contains WSPEEDI-II simulations for the first 20-days of radioactive release from the Fukushima Daiichi Nuclear Power Plant, and it displays essential quantitative data to the user from the database. The user may conduct sensitivity analysis with the help of the interface by changing release condition to generate many different case scenarios.
Yeom, Y. S.*; Han, M. C.*; Choi, C.*; Han, H.*; Shin, B.*; Furuta, Takuya; Kim, C. H.*
Health Physics, 116(5), p.664 - 676, 2019/05
Times Cited Count:15 Percentile:79.66(Environmental Sciences)Recently, Task Group 103 of the ICRP developed the mesh-type reference computational phantoms (MCRPs), which are planned for use in future ICRP dose coefficient calculation. Performance of major Monte Carlo particle transport codes (Geant4, MCNP6, and PHITS) were tested with MCRP. External and internal exposure of various particles and energies were calculated and the computational times and required memories were compared. Additionally calculation for voxel-mesh phantom was also conducted so that the influence of different mesh-representation in each code was studied. Memory usage of MRCP was as large as 10 GB with Geant4 and MCNP6 while it is much less with PHITS (1.2 GB). In addition, the computational time required for MRCP tends to increase compared to voxel-mesh phantoms with Geant4 and MCNP6 while it is equal or tends to decrease with PHITS.
Yang, P.-J.*; Li, Q.-J.*; Tsuru, Tomohito; Ogata, Shigenobu*; Zhang, J.-W.*; Sheng, H.-W.*; Shan, Z.-W.*; Sha, G.*; Han, W.-Z.*; Li, J.*; et al.
Acta Materialia, 168, p.331 - 342, 2019/04
Times Cited Count:83 Percentile:96.81(Materials Science, Multidisciplinary)Body-centred-cubic metallic materials, such as niobium (Nb) and other refractory metals, are prone to embrittlement due to low levels of oxygen solutes. The mechanisms responsible for the oxygen-induced rampant hardening and damage are unclear. Here we illustrate that screw dislocations moving through a random repulsive force field imposed by impurity oxygen interstitials readily form cross-kinks and emit excess vacancies in Nb. The vacancies bind strongly with oxygen and screw dislocation in a three-body fashion, rendering dislocation motion difficult and hence pronounced dislocation storage and hardening. This leads to unusually high strain hardening rates and fast breeding of nano-cavities that underlie damage and failure.
Bandodkar, A. J.*; Gutruf, P.*; Choi, J.*; Lee, K.-H.*; Sekine, Yurina; Reeder, J. T.*; Jeang, W. J.*; Aranyosi, A. J.*; Lee, S. P.*; Model, J. B.*; et al.
Science Advances (Internet), 5(1), p.eaav3294_1 - eaav3294_15, 2019/01
Times Cited Count:566 Percentile:99.88(Multidisciplinary Sciences)Interest in advanced wearable technologies increasingly extends beyond systems for biophysical measurements to those that enable continuous, non-invasive monitoring of biochemical markers in biofluids. Here, we introduce battery-free, wireless microelectronic platforms that perform sensing via schemes inspired by the operation of biofuel cells. Combining these systems in a magnetically releasable manner with chrono-sampling microfluidic networks that incorporate assays based on colorimetric sensing yields thin, flexible, lightweight, skin-interfaced technologies with broad functionality in sweat analysis. A demonstration device allows simultaneous monitoring of sweat rate/loss, along with quantitative measurements of pH and of lactate, glucose and chloride concentrations using biofuel cell and colorimetric approaches.