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Journal Articles

Intrinsic factors responsible for brittle versus ductile nature of refractory high-entropy alloys

Tsuru, Tomohito; Han, S.*; Matsuura, Shutaro*; Chen, Z.*; Kishida, Kyosuke; Lobzenko, I.; Rao, S.*; Woodward, C.*; George, E.*; Inui, Haruyuki*

Nature Communications (Internet), 15, p.1706_1 - 1706_10, 2024/02

 Times Cited Count:0

Refractory high-entropy alloys (RHEAs) have attracted attention because of their potential for use in ultrahigh-temperature applications. Unfortunately, their body-centered-cubic (BCC) crystal structures make them more brittle than the ductile and fracture-resistant face-centered-cubic (FCC) HEAs. RHEAs also display significantly lower creep strengths than a leading Ni-base superalloy and its FCC matrix. To overcome these drawbacks and develop RHEAs into viable structural materials, improved fundamental understanding is needed of factors that control strength and ductility. Here we investigate two model RHEAs, TiZrHfNbTa and VNbMoTaW, and show that the former is plastically compressible down to 77 K, whereas the latter is not below 298 K. We find that hexagonal close-packed (HCP) elements in TiZrHfNbTa lower its dislocation core energy, increase its lattice distortion, and lower its shear modulus relative to VNbMoTaW whose elements are all BCC, leading to the formers higher ductility and modulus-normalized yield strength. Consistent with our yield strength models, primarily screw dislocations are present in TiZrHfNbTa after deformation, but equal numbers of edge and screw segments in VNbTaMoW. Dislocation cores are compact in VNbTaMoW and extended in TiZrHfNbTa, and different macroscopic slip planes are activated in the two RHEAs, which we attribute to the concentration of HCP elements. Our findings demonstrate how electronic structure changes related to the ratio of HCP to BCC elements can be used to control strength, ductility, and slip behavior to develop the next generation of high-temperature materials for more efficient power plants and transportation.

Journal Articles

Recrystallization of bulk nanostructured magnesium alloy AZ31 after severe plastic deformation; An in situ diffraction study

Liss, K.-D.*; Han, J.-K.*; Blankenburg, M.*; Lienert, U.*; Harjo, S.; Kawasaki, Takuro; Xu, P. G.; Yukutake, Eitaro*; Kawasaki, M.*

Journal of Materials Science, 23 Pages, 2024/00

 Times Cited Count:0 Percentile:0.01(Materials Science, Multidisciplinary)

Journal Articles

Tetrahedral triple-Q magnetic ordering and large spontaneous Hall conductivity in the metallic triangular antiferromagnet Co$$_{1/3}$$TaS$$_{2}$$

Park, P.*; Cho, W.*; Kim, C.*; An, Y.*; Kang, Y.-G.*; Avdeev, M.*; Sibille, R.*; Iida, Kazuki*; Kajimoto, Ryoichi; Lee, K. H.*; et al.

Nature Communications (Internet), 14, p.8346_1 - 8346_9, 2023/12

 Times Cited Count:0 Percentile:0(Multidisciplinary Sciences)

Journal Articles

PANDORA Project for the study of photonuclear reactions below $$A=60$$

Tamii, Atsushi*; Pellegri, L.*; S$"o$derstr$"o$m, P.-A.*; Allard, D.*; Goriely, S.*; Inakura, Tsunenori*; Khan, E.*; Kido, Eiji*; Kimura, Masaaki*; Litvinova, E.*; et al.

European Physical Journal A, 59(9), p.208_1 - 208_21, 2023/09

 Times Cited Count:1 Percentile:0.02(Physics, Nuclear)

no abstracts in English

Journal Articles

Superfluid signatures in a dissipative quantum point contact

Huang, M.-Z.*; Mohan, J.*; Visuri, A.-M.*; Fabritius, P.*; Talebi, M.*; Wili, S.*; Uchino, Shun; Giamarchi, T.*; Esslinger, T.*

Physical Review Letters, 130(20), p.200404_1 - 200404_8, 2023/05

 Times Cited Count:4 Percentile:88.42(Physics, Multidisciplinary)

We measure superfluid transport of strongly-interacting fermionic lithium atoms through a quantum point contact with local, spin-dependent particle loss. We observe that the characteristic non-Ohmic superfluid transport enabled by high-order multiple Andreev reflections transitions into an excess Ohmic current as the dissipation strength exceeds the superfluid gap. We develop a model with mean-field reservoirs connected via tunneling to a dissipative site. Our calculations in the Keldysh formalism reproduce the observed non-equilibrium particle current, yet do not fully explain the observed loss rate or spin current.

Journal Articles

Mechanical surface treatment studies by Bragg edge neutron imaging

Ramadhan, R. S.*; Glaser, D.*; Soyama, Hitoshi*; Kockelmann, W.*; Shinohara, Takenao; Pirling, T.*; Fitzpatrick, M. E.*; Tremsin, A. S.*

Acta Materialia, 239, p.118259_1 - 118259_12, 2022/10

 Times Cited Count:3 Percentile:45.58(Materials Science, Multidisciplinary)

Journal Articles

Novel graphene-based foam composite as a highly reactive filter medium for the efficient removal of gemfibrozil from (waste)water

Khalil, A. M. E.*; Han, L.*; Maamoun, I.; Tabish, T. A.*; Chen, Y.*; Eljamal, O.*; Zhang, S.*; Butler, D.*; Memon, F. A.*

Advanced Sustainable Systems (Internet), 6(8), p.2200016_1 - 2200016_16, 2022/08

 Times Cited Count:2 Percentile:29.01(Green & Sustainable Science & Technology)

Journal Articles

Assessment of radioactive contamination and effectiveness of remedial measures in urban environments, Report of Working Group 2, Modelling and Data for Radiological Impact Assessments (MODARIA) Programme

Boznar, M. Z.*; Charnock, T. W.*; Chouhan, S. L.*; Grsic, Z.*; Halsall, C.*; Heinrich, G.*; Helebrant, J.*; Hettrich, S.*; Ku$v{c}$a, P.*; Mancini, F.*; et al.

IAEA-TECDOC-2001, 226 Pages, 2022/06

The IAEA organized a programme from 2012 to 2015 entitled Modelling and Data for Radiological Impact Assessments (MODARIA), which aimed to improve capabilities in the field of environmental radiation dose assessment by acquiring improved data, model testing and comparison of model inputs, assumptions and outputs, reaching a consensus on modelling philosophies, aligning approaches and parameter values, developing improved methods and exchanging information. This publication describes the activities of Working Group 2, Exposures in Contaminated Urban Environments and Effect of Remedial Measures.

Journal Articles

Urban Working Groups in the IAEA's model testing programmes; Overview from the MODARIA I and MODARIA II programmes

Thiessen, K. M.*; Boznar, M. Z.*; Charnock, T. W.*; Chouhan, S. L.*; Federspiel, L.; Gra$v{s}$i$v{c}$, B.*; Grsic, Z.*; Helebrant, J.*; Hettrich, S.*; Hulka, J.*; et al.

Journal of Radiological Protection, 42(2), p.020502_1 - 020502_8, 2022/06

 Times Cited Count:5 Percentile:78.52(Environmental Sciences)

Journal Articles

The $$^{59}$$Fe(n,$$gamma$$)$$^{60}$$Fe cross section from the surrogate ratio method and its effect on the $$^{60}$$Fe nucleosynthesis

Yan, S. Q.*; Li, X. Y.*; Nishio, Katsuhisa; Lugaro, M.*; Li, Z. H.*; Makii, Hiroyuki; Pignatari, M.*; Wang, Y. B.*; Orlandi, R.; Hirose, Kentaro; et al.

Astrophysical Journal, 919(2), p.84_1 - 84_7, 2021/10

 Times Cited Count:1 Percentile:8.87(Astronomy & Astrophysics)

Journal Articles

Half-integer Shapiro steps in strong ferromagnetic Josephson junctions

Yao, Y.*; Cai, R.*; Yang, S.-H.*; Xing, W.*; Ma, Y.*; Mori, Michiyasu; Ji, Y.*; Maekawa, Sadamichi; Xie, X.-C.*; Han, W.*

Physical Review B, 104(10), p.104414_1 - 104414_6, 2021/09

 Times Cited Count:2 Percentile:7.92(Materials Science, Multidisciplinary)

Journal Articles

Evaluation report of Task 9B based on comparisons and analyses of modelling results for the $"A$sp$"o$ HRL LTDE-SD experiments

Soler, J. M.*; Meng, S.*; Moreno, L.*; Neretnieks, I.*; Liu, L.*; Kek$"a$l$"a$inen, P.*; Hokr, M.*; $v{R}$$'i$ha, J.*; Vete$v{s}$n$'i$k, A.*; Reimitz, D.*; et al.

SKB TR-20-17, 71 Pages, 2021/07

Task 9B of the SKB Task Force on Modelling of Groundwater Flow and Transport of Solutes in fractured rock focused on the modelling of experimental results from the LTDE-SD in situ tracer test performed at the $"A$sp$"o$ Hard Rock Laboratory in Sweden. Ten different modelling teams provided results for this exercise, using different concepts and codes. Three main types of modelling approaches were used: (1) analytical solutions to the transport-retention equations, (2) continuum-porous-medium numerical models, and (3) microstructure-based models accounting for small-scale heterogeneity (i.e. mineral grains and microfracture distributions). The modelling by the different teams allowed the comparison of many different model concepts, especially in terms of potential zonations of rock properties (porosity, diffusion, sorption), such as the presence of a disturbed zone at the rock and fracture surface, the potential effects of micro- and cm-scale fractures.

Journal Articles

Formation of $$alpha$$ clusters in dilute neutron-rich matter

Tanaka, Junki*; Yang, Z.*; Typel, S.*; Adachi, Satoshi*; Bai, S.*; van Beek, P.*; Beaumel, D.*; Fujikawa, Yuki*; Han, J.*; Heil, S.*; et al.

Science, 371(6526), p.260 - 264, 2021/01

 Times Cited Count:48 Percentile:99.12(Multidisciplinary Sciences)

By employing quasi-free $$alpha$$-cluster-knockout reactions, we obtained direct experimental evidence for the formation of $$alpha$$ clusters at the surface of neutron-rich tin isotopes. The observed monotonous decrease of the reaction cross sections with increasing mass number, in excellent agreement with the theoretical prediction, implies a tight interplay between $$alpha$$-cluster formation and the neutron skin.

Journal Articles

Soft, skin-interfaced microfluidic systems with integrated immunoassays, fluorometric sensors, and impedance measurement capabilities

Kim, S.*; Lee, B.*; Reeder, J. T.*; Seo, S. H.*; Lee, S.-U.*; Hourlier-Fargette, A.*; Shin, J.*; Sekine, Yurina; Jeong, H.*; Oh, Y. S.*; et al.

Proceedings of the National Academy of Sciences of the United States of America, 117(45), p.27906 - 27915, 2020/11

 Times Cited Count:75 Percentile:93.23(Multidisciplinary Sciences)

In this study, we present a wireless, battery-free, skin-interfaced microfluidic system that combines lateral flow immunoassay for sweat cortisol assay, fluorometric imaging of glucose and ascorbic acid (vitamin C) assays, and digital tracking of sweat rate using electrodes that measure skin galvanic response. Systematic benchtop testing and on-body field studies on human subjects exercising in a gym environment highlight the key multifunctional features of this platform in tracking the biochemical correlates of physical stress.

Journal Articles

International network of nuclear structure and decay data evaluators

Dimitriou, P.*; Basunia, S*; Bernstein, L.*; Chen, J.*; Elekes, Z.*; Huang, X.*; Hurst, A.*; Iimura, Hideki; Jain, A. K.*; Kelley, J.*; et al.

EPJ Web of Conferences, 239, p.15004_1 - 15004_4, 2020/09

BB2020-0008.pdf:0.34MB

 Times Cited Count:0 Percentile:0.1(Nuclear Science & Technology)

The Evaluated Nuclear Structure Data File (ENSDF) includes the most extensive and comprehensive set of nuclear structure and decay data evaluations performed by the international network of Nuclear Structure and Decay Data evaluators (NSDD) under the auspices of the IAEA. In this report we describe some of the recent NSDD activities and provide future perspectives.

Journal Articles

Nuclear data sheets for A=218

Singh, B.*; Basunia, M. S.*; Martin, M.*; McCutchan, E. A.*; Bara, I.*; Caballero-Folch, R.*; Canavan, R.*; Chakrabarti, R.*; Chekhovska, A.*; Grinder, M. M.*; et al.

Nuclear Data Sheets, 160, p.405 - 471, 2019/09

 Times Cited Count:10 Percentile:71.88(Physics, Nuclear)

Journal Articles

Computation speeds and memory requirements of mesh-type ICRP reference computational phantoms in Geant4, MCNP6, and PHITS

Yeom, Y. S.*; Han, M. C.*; Choi, C.*; Han, H.*; Shin, B.*; Furuta, Takuya; Kim, C. H.*

Health Physics, 116(5), p.664 - 676, 2019/05

 Times Cited Count:7 Percentile:61.94(Environmental Sciences)

Recently, Task Group 103 of the ICRP developed the mesh-type reference computational phantoms (MCRPs), which are planned for use in future ICRP dose coefficient calculation. Performance of major Monte Carlo particle transport codes (Geant4, MCNP6, and PHITS) were tested with MCRP. External and internal exposure of various particles and energies were calculated and the computational times and required memories were compared. Additionally calculation for voxel-mesh phantom was also conducted so that the influence of different mesh-representation in each code was studied. Memory usage of MRCP was as large as 10 GB with Geant4 and MCNP6 while it is much less with PHITS (1.2 GB). In addition, the computational time required for MRCP tends to increase compared to voxel-mesh phantoms with Geant4 and MCNP6 while it is equal or tends to decrease with PHITS.

Journal Articles

Battery-free, skin-interfaced microfluidic/electronic systems for simultaneous electrochemical, colorimetric, and volumetric analysis of sweat

Bandodkar, A. J.*; Gutruf, P.*; Choi, J.*; Lee, K.-H.*; Sekine, Yurina; Reeder, J. T.*; Jeang, W. J.*; Aranyosi, A. J.*; Lee, S. P.*; Model, J. B.*; et al.

Science Advances (Internet), 5(1), p.eaav3294_1 - eaav3294_15, 2019/01

 Times Cited Count:446 Percentile:99.88(Multidisciplinary Sciences)

Interest in advanced wearable technologies increasingly extends beyond systems for biophysical measurements to those that enable continuous, non-invasive monitoring of biochemical markers in biofluids. Here, we introduce battery-free, wireless microelectronic platforms that perform sensing via schemes inspired by the operation of biofuel cells. Combining these systems in a magnetically releasable manner with chrono-sampling microfluidic networks that incorporate assays based on colorimetric sensing yields thin, flexible, lightweight, skin-interfaced technologies with broad functionality in sweat analysis. A demonstration device allows simultaneous monitoring of sweat rate/loss, along with quantitative measurements of pH and of lactate, glucose and chloride concentrations using biofuel cell and colorimetric approaches.

Journal Articles

Conceptual uncertainties in modelling the interaction between engineered and natural barriers of nuclear waste repositories in crystalline rocks

Finsterle, S.*; Lanyon, B.*; ${AA}$kesson, M.*; Baxter, S.*; Bergstr$"o$m, M.*; Bockg${aa}$rd, N.*; Dershowitz, W.*; Dessirier, B.*; Frampton, A.*; Fransson, ${AA}$.*; et al.

Geological Society, London, Special Publications, No.482, p.261 - 283, 2019/00

 Times Cited Count:9 Percentile:70.92(Geology)

Nuclear waste disposal in geological formations relies on a multi-barrier concept that includes engineered components which in many cases includes a bentonite buffer surrounding waste packages and the host rock. An SKB's (Swedish Nuclear Fuel and Waste Management Co.) Modelling Task Force project facilitated to improve the overall understanding of rock - bentonite interactions, as 11 teams used different conceptualisations and modelling tools to analyse the in-situ experiment at the $"A$ps$"o$ Hard Rock Laboratory. The exercise helped identify conceptual uncertainties that led to different assessments of the relative importance of the engineered and natural barrier subsystems and of aspects that need to be better understood to arrive at reliable predictions of bentonite wetting.

Journal Articles

Numerical simulation on self-leveling behavior of mixed particle beds using multi-fluid model coupled with DEM

Phan, L. H. S.*; Ohara, Yohei*; Kawata, Ryo*; Liu, X.*; Liu, W.*; Morita, Koji*; Guo, L.*; Kamiyama, Kenji; Tagami, Hirotaka

Proceedings of 12th International Topical Meeting on Nuclear Reactor Thermal-Hydraulics, Operation and Safety (NUTHOS-12) (USB Flash Drive), 12 Pages, 2018/10

Self-leveling behavior of core fuel debris beds is one of the key phenomena for the safety assessment of core disruptive accidents (CDAs) in sodium-cooled fast reactors (SFRs). The SIMMER code has been developed for CDA analysis of SFRs, and the code has been successfully applied to numerical simulations for key thermal-hydraulic phenomena involved in CDAs as well as reactor safety assessment. However, in SIMMER's fluid-dynamics model, it is always difficult to represent the strong interactions between solid particles as well as the discrete particle characteristics. To solve this problem, a new method has been developed by combining the multi-fluid model of the SIMMER code with the discrete element method (DEM) for the solid phase to reasonably simulate the particle behaviors as well as the fluid-particle interactions in multi-phase flows. In this study, in order to validate the multi-fluid model of the SIMMER code coupled with DEM, numerical simulations were performed on a series of self-leveling experiments using a gas injection method in cylindrical particle beds. The effects of friction coefficient on the simulation results were investigated by sensitivity analysis. Though more extensive validations are needed, the reasonable agreement between simulation results and corresponding experimental data preliminarily demonstrates the potential ability of the present method in simulating the self-leveling behaviors of debris bed. It is expected that the SIMMER code coupled with DEM is a prospective computational tool for analysis of safety issues related to solid particle debris bed in SFRs.

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