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Journal Articles

Ion-induced irradiation hardening of the weld heat-affected zone in low alloy steel

Ha, Yoosung; Takamizawa, Hisashi; Katsuyama, Jinya; Hanawa, Satoshi; Nishiyama, Yutaka

Nuclear Instruments and Methods in Physics Research B, 461, p.276 - 282, 2019/12

 Times Cited Count:0 Percentile:100(Instruments & Instrumentation)

Journal Articles

Preliminary verification of water radiolysis and ECP calculation models by in-pile ECP measurements

Hanawa, Satoshi; Hata, Kuniki; Chimi, Yasuhiro; Kasahara, Shigeki

Proceedings of 21st International Conference on Water Chemistry in Nuclear Reactor Systems (Internet), 12 Pages, 2019/09

Journal Articles

Influence of applied load on oxidation in the vicinity of crack tips of stainless steel under high temperature water

Kasahara, Shigeki; Chimi, Yasuhiro; Hata, Kuniki; Hanawa, Satoshi

Zairyo To Kankyo, 68(9), p.240 - 247, 2019/09

In order to study environment assisted cracking mechanism of stainless steel under BWR primary coolant condition, effects of applied load on oxidation in the vicinity of crack tips of CT specimens were evaluated. Loaded CT specimens were immersed in an aqueous condition at 290$$^{circ}$$C as a simulated BWR coolant condition, and microstructural observation on oxide near the tips of pre-cracks was carried out. Oxide inner layers, which consisted of fine grain magnetite containing Fe and Cr were formed, and oxide outer layers consisting of large grains of Fe$$_{3}$$O$$_{4}$$ were observed to cover the inner layers. FEM analysis of stress and strain in the loaded CT specimen suggests that both of dislocations due to localized plastic deformation and elastic strain could play important roles to accelerate inner oxide formation in the vicinity of the crack tip of the specimens.

Journal Articles

Improvement of plant reliability based on combining of prediction and inspection of crack growth due to intergranular stress corrosion cracking

Uchida, Shunsuke; Chimi, Yasuhiro; Kasahara, Shigeki; Hanawa, Satoshi; Okada, Hidetoshi*; Naito, Masanori*; Kojima, Masayoshi*; Kikura, Hiroshige*; Lister, D. H.*

Nuclear Engineering and Design, 341, p.112 - 123, 2019/01

 Times Cited Count:1 Percentile:53.3(Nuclear Science & Technology)

Improvement of plant reliability based on reliability-centered-maintenance (RCM) is going to be undertaken in NPPs. RCM is supported by risk-based maintenance (RBM). The combination of prediction and inspection is one of the key issues to promote RBM. Early prediction of IGSCC occurrence and its propagation should be confirmed throughout the entire plant systems which should be accomplished by inspections at the target locations followed by timely application of suitable countermeasures. From the inspections, accumulated data will be applied to confirm the accuracy of the code, to tune some uncertainties of the key data for prediction, and then, to increase their accuracy. The synergetic effects of prediction and inspection on application of effective and suitable countermeasures are expected. In the paper, the procedures for the combination of prediction and inspection are introduced.

Journal Articles

Influence of Zn injection on PWSCC crack growth rates and oxide film properties of Alloy 600

Chimi, Yasuhiro; Sato, Kenji*; Kasahara, Shigeki; Umehara, Ryuji*; Hanawa, Satoshi

Proceedings of Contribution of Materials Investigations and Operating Experience to Light Water NPPs' Safety, Performance and Reliability (FONTEVRAUD-9) (Internet), 10 Pages, 2018/09

To investigate the influence of Zinc (Zn) injection on primary water stress corrosion cracking (PWSCC) growth behavior, crack growth tests of 10% cold-worked Alloy 600 were performed in simulated primary water environment of pressurized water reactor (PWR) at 320$$^{circ}$$C with a low-concentration (5-10 ppb) Zn injection under dissolved hydrogen (DH) conditions of 5, 30, and 50 cc/kgH$$_{2}$$O. As a result of the crack growth tests, DH-dependence of crack growth rate (CGR) showed a similar tendency to the predicted CGR based on the CGR data without Zn injection, indicating almost no effect of a low-concentration Zn injection on the crack growth behavior. Moreover, the microstructural analyses of oxide films formed inside the crack and on the specimen surface were conducted, and the intake of Zn in the oxides was detected on the specimen surface, but not detected inside the crack. This result was considered to be the cause of no Zn injection effect on the crack growth behavior.

Journal Articles

Fracture toughness evaluation of heat-affected zone under weld overlay cladding in reactor pressure vessel steel

Ha, Yoosung; Tobita, Toru; Takamizawa, Hisashi; Hanawa, Satoshi; Nishiyama, Yutaka

Proceedings of 2018 ASME Pressure Vessels and Piping Conference (PVP 2018), 6 Pages, 2018/07

JAEA Reports

Confirmation tests for Warm Pre-stress (WPS) effect in reactor pressure vessel steel (Contract research)

Chimi, Yasuhiro; Iwata, Keiko; Tobita, Toru; Otsu, Takuyo; Takamizawa, Hisashi; Yoshimoto, Kentaro*; Murakami, Takeshi*; Hanawa, Satoshi; Nishiyama, Yutaka

JAEA-Research 2017-018, 122 Pages, 2018/03


Warm pre-stress (WPS) effect is a phenomenon that after applying a load at a high temperature fracture does not occur in unloading during cooling, and then the fracture toughness in reloading at a lower temperature increases effectively. Engineering evaluation models to predict an apparent fracture toughness in reloading are established using experimental data with linear elasticity. However, there is a lack of data on the WPS effect for the effects of specimen size and surface crack in elastic-plastic regime. In this study, fracture toughness tests were performed after applying load-temperature histories which simulate pressurized thermal shock transients to confirm the WPS effect. The experimental results of an apparent fracture toughness tend to be lower than the predictive results using the engineering evaluation models in the case of a high degree of plastic deformation in preloading. Considering the plastic component of preloading can refine the engineering evaluation models.

Journal Articles

Microstructure analysis using X-ray absorption on heat-affected zone of reactor pressure vessel steel

Iwata, Keiko; Takamizawa, Hisashi; Ha, Yoosung; Okamoto, Yoshihiro; Shimoyama, Iwao; Honda, Mitsunori; Hanawa, Satoshi; Nishiyama, Yutaka

Photon Factory Activity Report 2017, 2 Pages, 2018/00

no abstracts in English

Journal Articles

An Empirical model for the corrosion of stainless steel in BWR primary coolant

Uchida, Shunsuke*; Hanawa, Satoshi; Naito, Masanori*; Okada, Hidetoshi*; Lister, D. H.*

Corrosion Engineering, Science and Technology, 52(8), p.587 - 595, 2017/10

 Times Cited Count:1 Percentile:86.86(Materials Science, Multidisciplinary)

Based on the relationship among ECP, metal surface conditions, exposure time and other environmental conditions, a model to evaluate the ECP and corrosion rate of steel was developed by coupling a static electrochemical analysis and a dynamic oxide layer growth analysis. Major conclusion obtained on the model are as follows. The effect of H$$_{2}$$O$$_{2}$$ and O$$_{2}$$ concentrations on ECP were successfully explained as the effects of oxide layer growth. Hysteresis of ECP under changes in water chemistry conditions were successfully explained with the model. Decreases in ECP due to neutron exposure were explained well by radiation-induced diffusion in the oxide layers.

Journal Articles

Radiolysis of mixed solutions of Cl$$^{-}$$ and Br$$^{-}$$ and its effect on corrosion of a low-alloy steel

Hata, Kuniki; Inoue, Hiroyuki*; Kojima, Takao*; Kasahara, Shigeki; Hanawa, Satoshi; Ueno, Fumiyoshi; Tsukada, Takashi; Iwase, Akihiro*

Proceedings of Symposium on Water Chemistry and Corrosion in Nuclear Power Plants in Asia 2017 (AWC 2017) (USB Flash Drive), p.304 - 314, 2017/09

A model simulation of $$gamma$$ radiolysis of mixed solutions of NaCl and NaBr was carried out. The simulation result agreed well with the experimental result, and Br$$^{-}$$ played an important role in determining the amounts of products from water radiolysis. The simulation result also showed that, in highly pure NaCl solutions, the steady-state concentration of a radolytic product, H$$_{2}$$O$$_{2}$$, was mainly controlled by three reactions (Cl$$^{-}$$ + $$^{.}$$OH $$rightarrow$$ ClOH$$^{.-}$$, ClOH$$^{.-}$$ $$rightarrow$$ Cl$$^{-}$$ + $$^{.}$$OH, and ClOH$$^{.-}$$ + H$$^{+}$$ $$rightarrow$$ Cl$$^{.}$$ + H$$_{2}$$O), which indicated that accurate evaluation of the rate constants of these reactions was very important in improving the radiolysis simulation of solutions containing Cl$$^{-}$$. An immersion test using a low-alloy steel, SQV2A, in the mixed solutions was also carried out under irradiation. The corrosion rate increased or decreased depending on the pH or the concentrations of the halide ions in a similar way to the change in concentration of H$$_{2}$$O$$_{2}$$ produced from water radiolysis, which is affected by the presence of Cl$$^{-}$$ and Br$$^{-}$$. However, at high pH values ($$>$$12), the corrosion rate was almost zero even though the concentration of H$$_{2}$$O$$_{2}$$ was high. This could be attributed to enhancement of the passivity of test specimens at higher pH values.

Journal Articles

A Modelling study on water radiolysis for primary coolant in PWR

Mukai, Satoru*; Umehara, Ryuji*; Hanawa, Satoshi; Kasahara, Shigeki; Nishiyama, Yutaka

Proceedings of 20th International Conference on Water Chemistry of Nuclear Reactor Systems (NPC 2016) (USB Flash Drive), 9 Pages, 2016/10

In Japanese PWR, the concentration of dissolved hydrogen in the primary coolant is controlled in the range from 25 cc/kg-H$$_{2}$$O to 35 cc/kg-H$$_{2}$$O for suppression of water decomposition. However this concentration is desired to reduce for the purpose of radiation source reduction in Japan. So, the concentration due to water radiolysis in primary coolant was evaluated at lower hydrogen concentration by the water radiolysis model in consideration of $$gamma$$ ray, fast neutron and alpha ray due to the reaction $$^{10}$$B(n,$$alpha$$)$$^{7}$$Li. The results of evaluation showed that the water radiolysis was suppressed even if the hydrogen concentration was decreased to 5 cc/kg-H$$_{2}$$O. The effects of the different G-value and the rate constants of major reaction on the concentration of H$$_{2}$$O$$_{2}$$ and O$$_{2}$$ were studied under hydrogen addition. We also focused on the effect of the alpha radiolysis in boron acid water.

Journal Articles

Evaluation of ECP measured in in-pile environment

Hanawa, Satoshi; Uchida, Shunsuke; Hata, Kuniki; Chimi, Yasuhiro; Kasahara, Shigeki*; Nishiyama, Yutaka

Proceedings of 20th Nuclear Plant Chemistry International Conference (NPC 2016) (USB Flash Drive), 11 Pages, 2016/10

ECP is the exclusive index to evaluate corrosion condition directly at the points of interest in the mixing of neutron and $$gamma$$-ray environment. ECP can be calculated through the combination of water radiolysis and ECP model. A water radiolysis model have been applied to experiments performed in in-pile loops in the experimental reactors and applicability was confirmed. An ECP model based on the Butler-Volmer equation was also prepared. ECP of stainless steel was measured under well controlled water chemistry condition in in-pile loop in the Halden reactor, and the model was applied to evaluate ECP measured in the Halden reactor. The measured data were well explained by the water radiolysis calculation and ECP model. Accumulation of in-pile ECP data are expected for further validation of the models.

Journal Articles

Study of irradiation effect on ECP using in-pile loops in the JMTR

Hanawa, Satoshi; Uchida, Shunsuke; Hata, Kuniki; Chimi, Yasuhiro; Kasahara, Shigeki*; Nishiyama, Yutaka

Proceedings of 20th Nuclear Plant Chemistry International Conference (NPC 2016) (USB Flash Drive), 10 Pages, 2016/10

The authors proposed and ECP evaluation model introducing irradiation-induced diffusion in the oxide layer to simulate neutron irradiation effect, and predicted with this model that ECP is started to depress from the neutron flux of about ten to the fourteenth per square meter. As the JMTR has in-pile loops applicable to water chemistry experiments, degree of irradiation effect on ECP appears in the in-pile loop was estimated by the model. Under oxygen injected condition, ECP in a capsule becomes constant along the vertical direction due to the presence of high amount of oxygen and hydrogen peroxide in a capsule. However, if neutron irradiation depress ECP, ECP in a capsule along vertical direction wouldn't become constant, and the degree to the decrement is detectable by experiments.

Journal Articles

Simulation for radiolytic products of seawater; Effects of seawater constituents, dilution rate, and dose rate

Hata, Kuniki; Sato, Tomonori; Motooka, Takafumi; Ueno, Fumiyoshi; Hanawa, Satoshi; Kasahara, Shigeki; Tsukada, Takashi

Journal of Nuclear Science and Technology, 53(8), p.1183 - 1191, 2016/08

 Times Cited Count:4 Percentile:55.86(Nuclear Science & Technology)

Journal Articles

Hydrogen peroxide production by $$gamma$$ radiolysis of sodium chloride solutions containing a small amount of bromide ion

Hata, Kuniki; Inoue, Hiroyuki*; Kojima, Takao*; Iwase, Akihiro*; Kasahara, Shigeki; Hanawa, Satoshi; Ueno, Fumiyoshi; Tsukada, Takashi

Nuclear Technology, 193(3), p.434 - 443, 2016/03

 Times Cited Count:4 Percentile:45.52(Nuclear Science & Technology)

Journal Articles

Corrosion of structural materials and electrochemistry in high-temperature water; Relationships among water chemistry, corrosion, oxide film and electrochemical corrosion potential

Uchida, Shunsuke; Hanawa, Satoshi; Kysela, J.*; Lister, D. H.*

Power Plant Chemistry, 18(1), p.6 - 17, 2016/01

In order to establish reliable NPP operation, each plant requires its own unique optimal water chemistry control based on careful consideration of its system, materials and operational history. Electrochemistry is one of key issues that determine corrosion related problems, e.g., FAC. Based on the relationships among ECP, metal surface conditions and exposure time, a model to evaluate ECP and corrosion rate of steel was developed by coupling an electrochemical model and an oxide layer growth model. Major conclusions are as follows. (1) The effects of water chemistry improvement and mass transfer coefficients due to local flow velocity on FAC wall thinning rate and ECP could be evaluated with the proposed model. (2) The effects of H$$_{2}$$O$$_{2}$$ and O$$_{2}$$ concentrations on ECP were evaluated with the model. Exposure time dependent ECPs were also explained as the effects of oxide film growth on the specimens. (3) Decreases in ECP due to neutron exposure were explained by radiation-induced diffusion in the oxide layers.

Journal Articles

Advanced water chemistry control based on parameters determined with plant simulation models

Uchida, Shunsuke; Hanawa, Satoshi; Lister, D. H.*

Power Plant Chemistry, 17(6), p.328 - 339, 2015/12

In nuclear power plants, radiation makes the relationship between structural materials and water chemistry much more complex than that in fossil fueled power plants. It is difficult to maintain safer and more reliable plant operation by controlling water chemistry based on only a restricted number of measured data. It is often required to control water chemistry with suitable assistance from computer models, which can extrapolate measured water chemistry parameters to those at the required locations and predict future trends of the interactions between structural materials and water chemistry. In the paper, water chemistry control based on parameters determined with plant simulation models and major computational models to be applied for water chemistry control are discussed.

Journal Articles

Effect of chloride and bromide ion on the concentration of hydrogen peroxide produced from seawater radiolysis

Hata, Kuniki; Hanawa, Satoshi; Motooka, Takafumi; Tsukada, Takashi

JAEA-Review 2014-050, JAEA Takasaki Annual Report 2013, P. 22, 2015/03

Fukushima Daiichi Nuclear Power Plants experienced seawater injection into the cores and spent fuel pools as an emergent measure for a short period after the accident. The injected seawater was exposed to radiation, and radiolytic species were produced. Especially, hydrogen peroxide (H$$_{2}$$O$$_{2}$$) is known as an oxidant which affects corrosion of materials. In order to identify the important factor which results in the high concentration of H$$_{2}$$O$$_{2}$$ in seawater radiolysis, the concentrations of H$$_{2}$$O$$_{2}$$ in $$gamma$$-irradiated artificial seawater was measured and compared with the result of radiolysis calculation. Solutions containing some constituents of seawater were also measured to identify which ion affects H$$_{2}$$O$$_{2}$$ production of seawater radiolysis. The experimental results showed that the H$$_{2}$$O$$_{2}$$ production from seawater radiolysis is mainly attributed to reactions of Cl$$^{-}$$ and Br$$^{-}$$ in water radiolysis, though many kinds of ions are dissolved in seawater.

Journal Articles

Zirconia membrane ECP electrode for water chemistry experiments in the JMTR

Hanawa, Satoshi; Hata, Kuniki; Shibata, Akira; Chimi, Yasuhiro; Kasahara, Shigeki; Tsutsui, Nobuyuki*; Iwase, Akihiro*; Nishiyama, Yutaka

Proceedings of 2014 Nuclear Plant Chemistry Conference (NPC 2014) (USB Flash Drive), 9 Pages, 2014/10

no abstracts in English

Journal Articles

Water chemistry experiment using in-pile loop in the JMTR

Hanawa, Satoshi; Hata, Kuniki; Chimi, Yasuhiro; Nishiyama, Yutaka

Proceedings of Symposium on Water Chemistry and Corrosion in Nuclear Power Plants in Asia 2013 (USB Flash Drive), 7 Pages, 2013/10

Water chemistry experiments will be carried out by using an in-pile loop newly installed in the JMTR. Concentrations of chemical species of O$$_{2}$$, H$$_{2}$$ and H$$_{2}$$O$$_{2}$$ are measured at the inlet and the outlet of the irradiation field. Electrochemical corrosion potential (ECP) at the irradiation field is also monitored. These experimental data will be obtained under wide range of experimental conditions such as absorption dose rate, H$$_{2}$$ or O$$_{2}$$ concentration in the feeding water and water temperature. As a result of preliminary calculations, it became clear that the in-pile loop in the JMTR is capable for water chemistry experiment. Although the operation of the JMTR is being delayed because of the Tohoku district off the Pacific Ocean earthquake, construction of the loops and installation of the instrumentation for the loops have been carried out almost on schedule. The experiments will be started after JMTR restart.

126 (Records 1-20 displayed on this page)