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Development and application of a $$^3$$He neutron spin filter at J-PARC

奥平 琢也; 奥 隆之; 猪野 隆*; 林田 洋寿*; 吉良 弘*; 酒井 健二; 廣井 孝介; 高橋 慎吾*; 相澤 一也; 遠藤 仁*; et al.

Nuclear Instruments and Methods in Physics Research A, 977, p.164301_1 - 164301_8, 2020/10

 被引用回数:0 パーセンタイル:100(Instruments & Instrumentation)

We are developing a neutron polarizer with polarized $$^3$$He gas, referred to as a $$^3$$He spin filter, based on the Spin Exchange Optical Pumping (SEOP) for polarized neutron scattering experiments at Materials and Life Science Experimental Facility (MLF) of Japan Proton Accelerator Research Complex (J-PARC). A $$^3$$He gas-filling station was constructed at J-PARC, and several $$^3$$He cells with long spin relaxation times have been fabricated using the gas-filling station. A laboratory has been prepared in the MLF beam hall for polarizing $$^3$$He cells, and compact pumping systems with laser powers of 30 W and 110 W, which can be installed onto a neutron beamline, have been developed. A $$^3$$He polarization of 85% was achieved at a neutron beamline by using the pumping system with the 110 W laser. Recently, the first user experiment utilizing the $$^3$$He spin filter was conducted, and there have been several more since then. The development and utilization of $$^3$$He spin filters at MLF of J-PARC are reported.


Research on activation assessment of a reactor structural materials for decommissioning, 2

関 美沙紀; 石川 幸治*; 佐野 忠史*; 永田 寛; 大塚 薫; 大森 崇純; 花川 裕規; 井手 広史; 土谷 邦彦; 藤原 靖幸*; et al.

KURNS Progress Report 2019, P. 279, 2020/08

JMTR施設の廃止措置を進めるにあたり、多くの放射性廃棄物が発生するが、これらはドラム缶等に格納し、コンクリートを充填して、廃棄体とする計画である。しかし、アルミニウムは、コンクリートと反応し水素ガスが発生し、廃棄体を破損することが懸念されている。本研究は、これまで行ってきた湿式法によるアルミニウムの安定化処理法の溶液pHの最適条件を求めることを目的とした。JMTRで多く使用されている2種類のアルミニウム試料を準備し、KURで照射した後、強塩基であるNaOHに溶解した。溶解液をろ過した後、中和処理をしてpH=5$$sim$$11にてAl(OH)$$_{3}$$を生成した。それぞれの工程で得た残差及び溶液は放射化分析を行った。この結果、pH=7, 9にてAl全量の固体としての回収が可能であることが分かった。また、廃液中にはCr-51及びNa-24が含まれることが分かった。Cr-51は全ての条件にて同等の回収率であった。一方でNa-24は中和の際に生成されるNaCl量が相対的に多いことから、溶液中のNa-24が増加したと考えられる。


Preventing nuclear fuel material adhesion on glove box components using nanoparticle coating

瀬川 智臣; 川口 浩一; 石井 克典; 鈴木 政浩; 立原 丈二; 高藤 清人; 沖田 高敏; 佐藤根 大士*; 鈴木 道隆*

Proceedings of 2020 International Conference on Nuclear Engineering (ICONE 2020) (Internet), 6 Pages, 2020/08



Analytical study on removal mechanisms of cesium aerosol from a noble gas bubble rising through liquid sodium pool

宮原 信哉*; 河口 宗道; 清野 裕

Proceedings of 2020 International Conference on Nuclear Engineering (ICONE 2020) (Internet), 6 Pages, 2020/08



How different is the core of $$^{25}$$F from $$^{24}$$O$$_{g.s.}$$ ?

Tang, T. L.*; 上坂 友洋*; 川瀬 頌一郎; Beaumel, D.*; 堂園 昌伯*; 藤井 俊彦*; 福田 直樹*; 福永 拓*; Galindo-Uribarri. A.*; Hwang, S. H.*; et al.

Physical Review Letters, 124(21), p.212502_1 - 212502_6, 2020/05

 被引用回数:1 パーセンタイル:30.13(Physics, Multidisciplinary)

中性子過剰核$$^{25}$$Fの構造が($$p,2p$$)反応で調査した。$$pi 0d_{5/2}$$軌道の分光学的因子は1.0$$pm$$0.3と大きいが、一方で残留核である$$^{24}$$Oが基底状態である割合は約35%,励起状態は約0.65%であることが明らかになった。この結果は、$$^{25}$$Fのコア核$$^{24}$$Oは基底状態とは大きく異なり、$$^{24}$$Oの$$0d_{5/2}$$軌道に陽子がひとつ加わることで$$^{24}$$Oと$$^{25}$$Fの中性子軌道が相当に変化していると推測される。これは酸素同位体ドリップライン異常のメカニズムである可能性がある。


Neutron emission spectrum from gold excited with 16.6 MeV linearly polarized monoenergetic photons

桐原 陽一; 中島 宏; 佐波 俊哉*; 波戸 芳仁*; 糸賀 俊朗*; 宮本 修治*; 武元 亮頼*; 山口 将志*; 浅野 芳裕*

Journal of Nuclear Science and Technology, 57(4), p.444 - 456, 2020/04

 被引用回数:0 パーセンタイル:100(Nuclear Science & Technology)



The Energy-resolved neutron imaging system, RADEN

篠原 武尚; 甲斐 哲也; 及川 健一; 中谷 健; 瀬川 麻里子; 廣井 孝介; Su, Y.; 大井 元貴; 原田 正英; 飯倉 寛; et al.

Review of Scientific Instruments, 91(4), p.043302_1 - 043302_20, 2020/04

 被引用回数:1 パーセンタイル:30.41(Instruments & Instrumentation)

The energy-resolved neutron imaging system, RADEN, has been installed at the pulsed neutron source in the Materials and Life Science Experimental Facility of the Japan Proton Accelerator Research Complex. In addition to conventional neutron radiography and tomography, RADEN, the world's first imaging beam-line at a pulsed neutron source, provides three main options for new, quantitative neutron imaging techniques: Bragg-edge imaging to visualize the spatial distribution of crystallographic information, resonance absorption imaging for elemental composition and temperature information, and polarized neutron imaging for magnetic field information. This paper describes the results of characterization studies of the neutronic performance and installed devices at RADEN and shows the results of several demonstration studies for pulsed neutron imaging.



生島 一樹*; 柴原 正和*; 河尻 義貴*; 沖見 優衣*; 内田 友樹*; 秋田 貢一*; 鈴木 裕士; 諸岡 聡

日本船舶海洋工学会論文集, (30), p.123 - 130, 2019/12



Investigation on the influence of additional protective measures on sheltering effectiveness for internal exposure

廣内 淳; 高原 省五; 駒ヶ峯 弘志*; 宗像 雅広

Proceedings of Asian Symposium on Risk Assessment and Management 2019 (ASRAM 2019) (USB Flash Drive), 7 Pages, 2019/09



Research on activation assessment of a reactor structural materials for decommissioning

関 美沙紀; 石川 幸治*; 永田 寛; 大塚 薫; 大森 崇純; 花川 裕規; 井手 広史; 土谷 邦彦; 佐野 忠史*; 藤原 靖幸*; et al.

KURNS Progress Report 2018, P. 257, 2019/08

JMTR施設の廃止措置を進めるにあたり、多くの放射性廃棄物が発生するが、これらはドラム缶等に格納し、コンクリートを充填して、廃棄体とする計画である。しかし、アルミニウムは、コンクリートと反応し水素ガスが発生し、廃棄体を破損することが懸念されている。本研究は、湿式法によるアルミニウムの安定化処理法の開発を行った。JMTRで多く使用されている2種類のアルミニウム試料を準備し、KURで照射した後、強塩基であるNaOHに溶解した。溶解液をろ過した後、中和処理をしてAl(OH)$$_{3}$$を生成した。それぞれの工程で得た残差及び溶液は、放射化分析を行った。この結果、Al合金内に含まれる不純物$$^{51}$$Crおよび$$^{59}$$FeはAl成分と分離することができ、低レベルのAl(OH) $$_{3}$$の抽出が可能であることが示唆された。今後、Al(OH)$$_{3}$$の焼成温度の最適化を図り、安定なAl$$_{2}$$O $$_{3}$$を製作する条件を決定する。


Visualizing an ignition process of hydrogen jets containing sodium mist by high-speed imaging

土井 大輔; 清野 裕; 宮原 信哉*; 宇埜 正美*

Journal of Nuclear Science and Technology, 56(6), p.521 - 532, 2019/06

 被引用回数:0 パーセンタイル:100(Nuclear Science & Technology)

In severe accident scenarios for sodium-cooled fast reactors, it is desirable to gradually consume hydrogen generated by various ex-vessel phenomena without posting a challenge to containment integrity. An effective means is combustion of hydrogen jets containing sodium vapor and mist, but previous studies have been limited to determining ignition thresholds experimentally. The aim of this study was to visualize the ignition process in detail to investigate the ignition mechanism of hydrogen-sodium mixed jets. The ignition experiments of the hydrogen jet containing sodium mist were carried out under a condition of little turbulence. The ignition process was measured with an optical measurement system comprised of a high-speed camera and an image intensifier, and a spatial distribution of luminance was analyzed by image processing. Detail observation revealed that sodium mist particles burned as scattering sparks inside the jet and that hydrogen ignited around the mist particles. Additionally, the experimental results and a simple heat balance calculation indicated that the combustion heat of sodium mist particles could ignite the hydrogen as the heterogeneous ignition source in the fuel temperature range where the mist particle formation was promoted.


Improvement of plant reliability based on combining of prediction and inspection of crack growth due to intergranular stress corrosion cracking

内田 俊介; 知見 康弘; 笠原 茂樹; 塙 悟史; 岡田 英俊*; 内藤 正則*; 小嶋 正義*; 木倉 宏成*; Lister, D. H.*

Nuclear Engineering and Design, 341, p.112 - 123, 2019/01

 被引用回数:1 パーセンタイル:58.8(Nuclear Science & Technology)



Investigation of reduction factor of internal exposure for sheltering in Japan

廣内 淳; 高原 省五; 駒ヶ峯 弘志*; 宗像 雅広

Proceedings of Asian Symposium on Risk Assessment and Management 2018 (ASRAM 2018) (USB Flash Drive), 8 Pages, 2018/10



Atmospheric modeling of $$^{137}$$Cs plumes from the Fukushima Daiichi Nuclear Power Plant; Evaluation of the model intercomparison data of the Science Council of Japan

北山 響*; 森野 悠*; 滝川 雅之*; 中島 映至*; 速水 洋*; 永井 晴康; 寺田 宏明; 斉藤 和雄*; 新堀 敏基*; 梶野 瑞王*; et al.

Journal of Geophysical Research; Atmospheres, 123(14), p.7754 - 7770, 2018/07

 被引用回数:10 パーセンタイル:23.43(Meteorology & Atmospheric Sciences)



Mechanical properties of cubic (U,Zr)O$$_{2}$$

北垣 徹; 星野 貴紀; 矢野 公彦; 岡村 信生; 小原 宏*; 深澤 哲生*; 小泉 健治

Journal of Nuclear Engineering and Radiation Science, 4(3), p.031011_1 - 031011_7, 2018/07

Evaluation of fuel debris properties is required to develop fuel debris removal tools for the decommissioning of Fukushima Daiichi Nuclear Power Plant (1F). In this research, the mechanical properties of cubic (U,Zr)O$$_{2}$$ samples containing 10-65% ZrO$$_{2}$$ are evaluated. In case of the (U,Zr)O$$_{2}$$ samples containing less than 50% ZrO$$_{2}$$, Vickers hardness and fracture toughness increased, and the elastic modulus decreased slightly with increasing ZrO$$_{2}$$ content. Moreover, all of those values of the (U,Zr)O$$_{2}$$ samples containing 65% ZrO$$_{2}$$ increased slightly compared to (U,Zr)O$$_{2}$$ samples containing 55% ZrO$$_{2}$$. However, higher Zr content (exceeding 50%) has little effect on the mechanical properties. This result indicates that the wear of core-boring bits in the 1F drilling operation will accelerate slightly compared to that in the TMI-2 drilling operation.


Deformation analysis of reinforced concrete using neutron imaging technique

小山 拓*; 上野 一貴*; 関根 麻里子*; 松本 吉弘*; 甲斐 哲也; 篠原 武尚; 飯倉 寛; 鈴木 裕士; 兼松 学*

Materials Research Proceedings, Vol.4, p.155 - 160, 2018/05

 被引用回数:0 パーセンタイル:100

We developed, in this study, a novel method to observe internal deformation of concrete by the neutron transmission imaging technique. In order to visualize the internal deformation of concrete, the cement paste markers containing Gd$$_{2}$$O$$_{3}$$ powder were two-dimensionally dispersed around the ferritic deformed rebar in the reinforced concrete. This experiment was conducted using BL22, RADEN, in the Material and Life Science Experimental Facility of the Japan Proton Accelerator Research Complex. The transmission images of the reinforced concrete sample were taken at several positions on the vertical sample stage, and the displacement of the marker from the initial position was successfully evaluated within approximately $$pm$$0.1 mm accuracy by image analysis for selected markers with higher contrast and circularity. Furthermore, concrete deformation under pull-out loading to the embedded rebar was evaluated by the same way, and its reaction compressive deformation was successfully observed by analyzing the displacement of the markers. The results obtained in this study bring beneficial knowledge that the measurement accuracy of the marker displacement can be improved more by choosing a spherical shape of the marker and by increasing the contrast of the marker.


Evidence for momentum-dependent heavy fermionic electronic structures; Soft X-ray ARPES for the superconductor CeNi$$_{2}$$Ge$$_{2}$$ in the normal state

中谷 泰博*; 荒谷 秀和*; 藤原 秀紀*; 森 健雄*; 鶴田 篤史*; 橘 祥一*; 山口 貴司*; 木須 孝幸*; 山崎 篤志*; 保井 晃*; et al.

Physical Review B, 97(11), p.115160_1 - 115160_7, 2018/03


 被引用回数:1 パーセンタイル:87.78(Materials Science, Multidisciplinary)

We present clear experimental evidence for the momentum-dependent heavy fermionic electronic structures of the 4${it f}$-based strongly correlated system CeNi$$_{2}$$Ge$$_{2}$$ by soft X-ray angle-resolved photoemission spectroscopy. A comparison between the experimental three-dimensional quasiparticle dispersion of LaNi$$_{2}$$Ge$$_{2}$$ and CeNi$$_{2}$$Ge$$_{2}$$ has revealed that heavy fermionic electronic structures are seen in the region surrounding at a specific momentum. Furthermore, the wave vectors between the observed "heavy spots" are consistent with a result of neutron scattering reflecting magnetic correlations, which could be a trigger of the superconductivity in CeNi$$_{2}$$Ge$$_{2}$$.



武内 伴照; 柴田 裕司; 花川 裕規; 上原 聡明*; 上野 俊二*; 土谷 邦彦; 熊原 肇*; 柴垣 太郎*; 駒野目 裕久*

JAEA-Technology 2017-026, 26 Pages, 2018/02





桜井 弘*; 篠原 厚*; 小浦 寛之; 上垣外 修一*; 森本 幸司*; 羽場 宏光*; 延輿 秀人*

Isotope News, (特別号2), p.2 - 14, 2018/01

日本アイソトープ協会発行の協会誌「Isotope News」における新春座談会(2018年1月1日誌上掲載)に登壇する。「ニホニウムとその次の元素へ・・・」という座談会のタイトルで、ニホニウム(超重元素)の発見の歴史や今後の超重元素発見にむけての展望など、(1)理論、(2)加速器、(3)実験、(4)周期表を話題の中心として夢のある内容を紹介する。特に原子核物理・理論の観点から座談を展開する。


Prediction method of improved residual stress distribution by shot peening using large scale analysis method

生島 一樹*; 柴原 正和*; 西川 聡*; 古川 敬*; 秋田 貢一; 鈴木 裕士; 諸岡 聡

E-Journal of Advanced Maintenance (Internet), 9(3), p.NT87_1 - NT87_5, 2017/11

In this work, an analysis system that can analyze the modification of the residual stress distribution by peening is proposed based on IEFEM. In the proposed analysis system, IEFEM is extended to consider the dynamic effect to analyze the dynamic phenomenon with an impulsive load. The impulsive load due to the collision of shots is modeled as an equivalent load model. The equivalent load model is integrated with IEFEM considering the dynamic effect to calculate spatially and temporally random load in dynamic analyses. Using the proposed analysis system, the residual stress distribution modification by shot peening in a multi-pass welded pipe joint is predicted. The residual stress distributions obtained by the analysis are compared with those measured by X-ray diffraction (XRD), and the effect of the number of shot collisions on the change in residual stress distribution is discussed.

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