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Shimizu, Kazuyuki*; Toda, Hiroyuki*; Hirayama, Kyosuke*; Fujihara, Hiro*; Tsuru, Tomohito; Yamaguchi, Masatake; Sasaki, Taisuke*; Uesugi, Masayuki*; Takeuchi, Akihisa*
International Journal of Hydrogen Energy, 109, p.1421 - 1436, 2025/03
Times Cited Count：0Our preceding investigation revealed that multiple hydrogen traps at coherent interfaces of MgZn
precipitates initiated spontaneous interface decohesion, causing hydrogen-induced quasicleavage cracking in Al-Zn-Mg alloys. Herein, we performed a quantitative and systematic investigation to discern the mechanisms by which hydrogen trapped at coherent/semi-coherent interfaces of precipitates could influence macroscopic hydrogen embrittlement by modulating the coherent interface of MgZn through aging. To explore this hydrogen embrittlement phenomenon based on hydrogen trapping at the precipitate interface, we determined the hydrogen trapping energy of the semi-coherent MgZn interface via first-principles calculations (0.56 eV/atom). Hydrogen partitioning of all hydrogen trapping sites, including vacancies, grain boundaries, and coherent and semi-coherent MgZn interfaces, revealed that in overaged alloys, over 90% of the hydrogen was sequestered at semi-coherent interfaces. Owing to the inherent characteristics of the MgZn interface, the hydrogen sequestered at the semi-coherent interface decreased the interfacial cohesive energy, causing semispontaneous decohesion of the interface and quasicleavage fracture in the Al-Zn-Mg alloys. These results implied that intergranular fracture was not directly induced by hydrogen trapped at grain boundaries but rather by the decohesion of precipitate interfaces along grain boundaries.
Nakamura, Satoshi; Ishii, Sho*; Kato, Hitoshi*; Ban, Yasutoshi; Hiruta, Kenta; Yoshida, Takuya; Uehara, Hiroyuki; Obata, Hiroki; Kimura, Yasuhiko; Takano, Masahide
Journal of Nuclear Science and Technology, 62(1), p.56 - 64, 2025/01
Times Cited Count：1 Percentile：68.64(Nuclear Science & Technology)A dissolution method for analyzing the elemental composition of fuel debris using the sodium peroxide (NaO) fusion technique has been developed. Herein, two different types of simulated debris materials (such as solid solution of (Zr,RE)O and molten core-concrete interaction products (MCCI)) were taken. At various temperatures, these debris materials were subsequently fused with NaO in crucibles, which are made of different materials, such as Ni, AlO
, Fe, and Zr. Then, the fused samples are dissolved in nitric acid. Furthermore, the effects of the experimental conditions on the elemental composition analysis were evaluated using inductively coupled plasma-atomic emission spectroscopy (ICP-AES), which suggested the use of a Ni crucible at 923 K as an optimum testing condition. The optimum testing condition was then applied to the demonstration tests with Three Mile Island unit-2 (TMI-2) debris in a shielded concrete cell, thereby achieving complete dissolution of the debris. The elemental composition of TMI-2 debris revealed by the proposed dissolution method has good reproducibility and has an insignificant contradiction in the mass balance of the sample. Therefore, this newly developed reproducible dissolution method can be effectively utilized in practical applications by dissolving fuel debris and estimating its elemental composition.
Higa, Ryota*; Fujihara, Hiro*; Toda, Hiroyuki*; Kobayashi, Masakazu*; Ebihara, Kenichi; Takeuchi, Akihisa*
Materials Transactions, 65(8), p.899 - 906, 2024/08
Times Cited Count：0 Percentile：0.00(Materials Science, Multidisciplinary)It is indispensable to suppress hydrogen embrittlement (HE) to develop the strength of the Al-Zn-Mg alloy. Because intergranular fracture (IGF) is mainly observed when HE occurs in the alloy, we need to understand the IGF initiation to suppress HE. In the present study, we investigated the stress, strain, and H concentration, which influence the IGF initiation, in actual fractured regions by simulation of a crystal plasticity finite element method and H diffusion analysis in a 3D image-based model, which was created based on 3D polycrystalline microstructure data obtained from X-ray imaging technique. Combining the simulation and in-situ observation of the tensile test sample by X-ray CT, we examined the stress, strain, and H concentration, and discussed the IG crack initiation condition. As a result, it is revealed that stress normal to grain boundary induced by crystal plasticity dominates IG crack initiation while the accumulation of H due to stress has little impact on it.
Nagatsuka, Kentaro; Noguchi, Hiroki; Nagasumi, Satoru; Nomoto, Yasunobu; Shimizu, Atsushi; Sato, Hiroyuki; Nishihara, Tetsuo; Sakaba, Nariaki
Nuclear Engineering and Design, 425, p.113338_1 - 113338_11, 2024/08
Times Cited Count：2 Percentile：68.64(Nuclear Science & Technology)HTGR has a potential to contribute to decarbonization of hard-to-abate industries by supplying a large amount of hydrogen and high temperature heat or steam without carbon dioxide emission. JAEA has been conducting R&Ds for HTGR technologies with High Temperature Engineering Test Reactor (HTTR). This paper shows that HTTR's tests including the loss of core cooing test as a joint the OECD/NEA international research project and a HTTR heat application test plan which demonstrate hydrogen production by coupling the HTTR with a hydrogen production test facility. Additionally, aiming for operation start from the latter half of 2030s, the basic design of the HTGR demonstration reactor has been shown. The Japan's HTGR technology capabilities established by the HTTR project will be fully utilized for the construction of HTGR demonstration reactor.
Uchida, Kazuto*; Masuda, Tsukuru*; Hara, Shintaro*; Matsuo, Yoichi*; Liu, Y.*; Aoki, Hiroyuki; Asano, Yoshihiko*; Miyata, Kazuki*; Fukuma, Takeshi*; Ono, Toshiya*; et al.
ACS Applied Materials & Interfaces, 16(30), p.39104 - 39116, 2024/07
Times Cited Count：1 Percentile：0.00(Nanoscience & Nanotechnology)Inaba, Yoshitomo; Sato, Hiroyuki; Sumita, Junya; Ohashi, Hirofumi; Nishihara, Tetsuo; Sakaba, Nariaki
Nihon Kikai Gakkai-Shi, 127(1267), p.25 - 28, 2024/06
Aiming to contribute to net-zero emissions through early social implementation of HTGRs, JAEA promote five projects: HTTR-Heat Application Test, HTGR Domestic Demonstration Reactor, UK HTGR Demonstration Program, UK HTGR Fuel Development Program, and Poland HTGR Research Reactor Basic Design. In addition to these five projects, this article provides an overview of the safety demonstration tests using HTTR.
Miyazaki, Kanako*; Takehara, Masato*; Minomo, Kenta*; Horie, Kenji*; Takehara, Mami*; Yamasaki, Shinya*; Saito, Takumi*; Onuki, Toshihiko*; Takano, Masahide; Shiotsu, Hiroyuki; et al.
Journal of Hazardous Materials, 470(15), p.134104_1 - 134104_11, 2024/05
Times Cited Count：0 Percentile：0.00(Engineering, Environmental)Noguchi, Hiroki; Sato, Hiroyuki; Nishihara, Tetsuo; Sakaba, Nariaki
Kagaku Kogaku, 88(5), p.211 - 214, 2024/05
High temperature gas-cooled reactor (HTGR), one of the next-generation innovative reactors, has an inherent safety and can generate very high-temperature heat which can be used for various heat application including hydrogen production. In Japan, Green Growth Strategy for Carbon Neutrality in 2050 and Basic Policy for the Realization of GX state the promotion of technology development necessary for mass and low-cost carbon-free hydrogen production and development and construction of next-generation innovative reactors including the HTGR for the decarbonization of industrial sectors. Based on these policies, JAEA has been conducted the world's first hydrogen production test using nuclear heat from an HTGR, in addition to verifying the excellent safety features of HTGR, and has also started to study the construction of an HTGR demonstration reactor in cooperation with the industrial community. This paper shows the current status of R&D of HTGR in Japan.
Holm-Janas, S.*; Akaki, Mitsuru*; Fogh, E.*; Kihara, Takumi*; Le, M. D.*; Forino, P. C.*; Nikitin, S. E.*; Fennell, T.*; Painganoor, A.*; Vaknin, D.*; et al.
Physical Review B, 109(17), p.174413_1 - 174413_11, 2024/05
Times Cited Count：0 Percentile：0.00(Materials Science, Multidisciplinary)
-odd/
-odd interactions on the 0.75 eV 
-wave resonance in 
+
forward transmission determined using a pulsed neutron beamNakabe, Rintaro*; Auton, C. J.*; Endo, Shunsuke; Fujioka, Hiroyuki*; Gudkov, V.*; Hirota, Katsuya*; Ide, Ikuo*; Ino, Takashi*; Ishikado, Motoyuki*; Kambara, Wataru*; et al.
Physical Review C, 109(4), p.L041602_1 - L041602_4, 2024/04
Times Cited Count：0 Percentile：0.00(Physics, Nuclear)-wave resonance of 
+
Okudaira, Takuya*; Nakabe, Rintaro*; Auton, C. J.*; Endo, Shunsuke; Fujioka, Hiroyuki*; Gudkov, V.*; Ide, Ikuo*; Ino, Takashi*; Ishikado, Motoyuki*; Kambara, Wataru*; et al.
Physical Review C, 109(4), p.044606_1 - 044606_9, 2024/04
Times Cited Count：0 Percentile：0.00(Physics, Nuclear)Fujihara, Hiro*; Toda, Hiroyuki*; Ebihara, Kenichi; Kobayashi, Masakazu*; Mayama, Tsuyoshi*; Hirayama, Kyosuke*; Shimizu, Kazuyuki*; Takeuchi, Akihisa*; Uesugi, Masayuki*
International Journal of Plasticity, 174, p.103897_1 - 103897_22, 2024/03
Times Cited Count：8 Percentile：96.89(Engineering, Mechanical)Hydrogen(H) embrittlement in high-strength aluminum(Al) alloys is a crucial problem. H accumulation at the interface of precipitates in Al alloy is considered to cause embrittlement. However, there is no quantitative knowledge regarding the interaction between H distribution and stress field near cracks. In this study, using a multi-modal three-dimensional image-based simulation combining the crystal plasticity finite element method and H diffusion analysis, we tried to capture the stress distribution near the crack, its influence on the H distribution, and the probability of crack initiation in the experimental condition. As a result, it was found that grain boundary cracks transition to quasi-cleavage cracks in the region where the cohesive energy of the semi-coherent interface of MgZn
precipitates decreases due to H accumulation near the tip. We believe the present simulation method successfully bridges nanoscale delamination and macroscale brittle fracture.
CoSiYamauchi, Hiroki; Sari, D. P.*; Yasui, Yukio*; Sakakura, Terutoshi*; Kimura, Hiroyuki*; Nakao, Akiko*; Ohara, Takashi; Honda, Takashi*; Kodama, Katsuaki; Igawa, Naoki; et al.
Physical Review Research (Internet), 6(1), p.013144_1 - 013144_9, 2024/02
Zhang, H.*; Umehara, Yutaro*; Yoshida, Hiroyuki; Mori, Shoji*
International Journal of Heat and Mass Transfer, 218, p.124750_1 - 124750_11, 2024/01
Times Cited Count：6 Percentile：63.68(Thermodynamics)Tang, J.*; Wang, Y.*; Fujihara, Hiro*; Shimizu, Kazuyuki*; Hirayama, Kyosuke*; Ebihara, Kenichi; Takeuchi, Akihisa*; Uesugi, Masayuki*; Toda, Hiroyuki*
Scripta Materialia, 239, p.115804_1 - 115804_5, 2024/01
Times Cited Count：11 Percentile：80.15(Nanoscience & Nanotechnology)Stress corrosion cracking (SCC) behaviors induced by the combination of external and internal hydrogen (H) in an Al-Zn-Mg-Cu alloy were systematically investigated via in situ 3D characterization techniques. SCC of the Al-Zn-Mg-Cu alloy could initiate and propagate in the potential crack region where the H concentration exceeded a critical value, in which the nanoscopic H-induced decohesion of 
-MgZn precipitates resulted in macroscopic cracking. External H that penetrated the alloy from the environment played a crucial role during the SCC of the Al-Zn-Mg-Cu alloy by generating gradient-distributed H-affected zones near the crack tips, which made Al alloys in water environment more sensitive to SCC. Additionally, the pre-existing internal H was driven toward the crack tips during plastic deformation. It was involved in the SCC and made contributions to both the cracks initiation and propagation.
Higa, Ryota*; Fujihara, Hiro*; Toda, Hiroyuki*; Kobayashi, Masakazu*; Ebihara, Kenichi; Takeuchi, Akihisa*
Keikinzoku, 73(11), p.530 - 536, 2023/11
In Al-Zn-Mg alloys, suppression of hydrogen embrittlement is necessary to improve their strength. In this study, the distribution of stress, strain, and hydrogen concentration in the actual fracture region was investigated using the crystal plasticity finite element method and hydrogen diffusion analysis based on a model derived from three-dimensional polycrystalline microstructural data obtained by X-ray CT. In addition, the distributions of stress, strain, and hydrogen concentration were compared with the actual crack initiation behavior by combining in-situ observation of tensile tests using X-ray CT and simulation. The results show that stress loading perpendicular to the grain boundary due to crystal plasticity dominates grain boundary crack initiation. It was also found that internal hydrogen accumulation due to crystal plasticity has little effect on crack initiation.
Katsumura, Kosuke*; Takagi, Junichi*; Hosomi, Kenji*; Miyahara, Naoya*; Koma, Yoshikazu; Imoto, Jumpei; Karasawa, Hidetoshi; Miwa, Shuhei; Shiotsu, Hiroyuki; Hidaka, Akihide*; et al.
Nihon Genshiryoku Gakkai-Shi ATOMO
, 65(11), p.674 - 679, 2023/11
no abstracts in English
Uchibori, Akihiro; Doda, Norihiro; Aoyagi, Mitsuhiro; Sonehara, Masateru; Sogabe, Joji; Okano, Yasushi; Takata, Takashi*; Tanaka, Masaaki; Enuma, Yasuhiro; Wakai, Takashi; et al.
Nuclear Engineering and Design, 413, p.112492_1 - 112492_10, 2023/11
Times Cited Count：2 Percentile：51.90(Nuclear Science & Technology)The ARKAIDA has been developed to realize automatic optimization of plant design from safety evaluation for the advanced reactors represented by a sodium-cooled fast reactor. ARKADIA-Design offers functions to support design optimization both in normal operating conditions and design basis events. The multi-level simulation approach by the coupled analysis such as neutronics, core deformation, core thermal hydraulics was developed as one of the main technologies. On the other hand, ARKAIDA-Safety aims for safety evaluation considering severe accidents. As a key technology, the numerical methods for in- and ex-vessel coupled phenomena during severe accidents in sodium-cooled fast reactors were tested through a hypothetical severe accident event. Improvement of the ex-vessel model and development of the AI technology to find best design solution have been started.
Yamashita, Keishiro*; Nakayama, Kazuya*; Komatsu, Kazuki*; Ohara, Takashi; Munakata, Koji*; Hattori, Takanori; Sano, Asami; Kagi, Hiroyuki*
Acta Crystallographica Section B; Structural Science, Crystal Engineering and Materials (Internet), 79(5), p.414 - 426, 2023/10
Times Cited Count：2 Percentile：47.77(Chemistry, Multidisciplinary)The structure of a recently-found hyperhydrated form of sodium chloride, NaCl
13H(D)O, has been determined by 
single-crystal neutron diffraction at 1.7 GPa and 298 K. It has large hydrogen-bond networks and some water molecules have distorted bonding features such as bifurcated hydrogen bonds and five-coordinated water molecules. The hydrogen-bond network has similarities to ice VI in terms of network topology and disordered hydrogen bonds. Assuming the equivalence of network components connected by pseudo symmetries, the overall network structure of this hydrate can be expressed by breaking it down into smaller structural units which correspond to the ice VI network structure. This hydrogen-bond network contains orientational disorder of water molecules in contrast to the known salt hydrates. Here, we present an example for further insights into a hydrogen-bond network containing ionic species.
Oikawa, Kenichi; Sato, Hirotaka*; Watanabe, Kenichi*; Su, Y. H.; Shinohara, Takenao; Kai, Tetsuya; Kiyanagi, Yoshiaki*; Hasemi, Hiroyuki
Journal of Physics; Conference Series, 2605, p.012013_1 - 012013_6, 2023/10
