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Journal Articles

Permeability and Forchheimer coefficient of packed beds with different particle sizes

Kawabe, Tomosaburo*; Sano, Yoshihiko*; Kuwahara, Fujio*; Uesawa, Shinichiro; Yoshida, Hiroyuki

Dai-63-Kai Nihon Dennetsu Shimpojiumu Koen Rombunshu (Internet), 1 Pages, 2026/05

To estimate the thermal behavior of fuel debris inside the Primary Containment Vessels (PCVs) of TEPCO's Fukushima Daiichi Nuclear Power Station, a simulation method has been developed using the JUPITER code with porous medium models. However, it has been found that the selection of models and parameters according to the internal structure of the porous media significantly affects the accuracy of simulation results, highlighting the need for appropriate model selection strategies. In this study, we focus on packed beds with particles as one form of porous media and investigate a methodology for determining model parameters that characterize their flow behavior. Systematic knowledge of packed beds with heterogeneous particle size ratios and packing structures remains limited, and comprehensive organization accounting for structural differences has not yet been fully established. Therefore, numerical simulations were employed to evaluate the permeability and Forchheimer coefficient of packed beds with different particle size ratios and packing structures. Based on the obtained results, a method for appropriately determining these parameters according to the structural characteristics of packed beds is proposed, and insights are provided that contribute to improving the accuracy of flow analysis models in porous media.

Journal Articles

Coupled hydro-mechanical simulations of tunnel excavation in the Horonobe Underground Research Laboratory; A Multi-institutional, multi-method approach

Ozaki, Yusuke; Ogata, Sho*; Nakaoka, Kenichi*; Shimizu, Hiroyuki*; Yasuhara, Hideaki*; Akaki, Toshifumi*; Aoyagi, Kazuhei; Fukuda, Daisuke*

Dai-51-Kai Gamban Rikigaku Ni Kansuru Shimpojiumu Koen Rombunshu(Internet), p.125 - 130, 2025/12

The Subcommittee on Research of Coupled Phenomena in Rock, under the Japan Society of Civil Engineers, conducts coupled numerical simulations using various approaches by participating members. The evaluation of the excavation damaged zone (EDZ) in the Horonobe Underground Research Laboratory using hydro-mechanical coupled simulation is one of the tasks of the subcommittee. In this presentation, the problem statement, modeling approaches, and current results from participating organizations are summarized.

Journal Articles

Lyotropic polymer liquid crystal coating; Enabling lamellar ion-conduction pathways for superior C-Rate performance in NCM523 cathodes

Marium, M.*; Aoki, Kentaro*; He, Y.*; Yamamoto, Katsuhiro*; Suwansoontorn, A.*; Ikuta, Seiya*; Hara, Mitsuo*; Nagano, Shusaku*; Nagao, Yuki*; Nishikawa, Kei*; et al.

ACS Applied Energy Materials (Internet), 8(22), p.16589 - 16600, 2025/11

 Times Cited Count:1 Percentile:20.13(Chemistry, Physical)

Journal Articles

Experimental simulation of high-temperature and high-pressure annular two-phase flow using an HFC134a-ethanol system; Characterization of disturbance wave flow

Zhang, H.*; Umehara, Yutaro*; Horiguchi, Naoki; Yoshida, Hiroyuki; Eto, Atsuro*; Mori, Shoji*

Energy, 335, p.138090_1 - 138090_18, 2025/10

 Times Cited Count:0 Percentile:0.00(Thermodynamics)

Nuclear power is a key low-carbon energy source for a carbon-neutral future. In boiling water reactors (BWRs), steam-water annular flow near fuel rods is crucial for reactor safety, but its high-temperature, high-pressure conditions (285$$^{circ}$$C, 7 MPa) make direct measurement challenges. To address this, we used an HFC134a-ethanol system at lower conditions (40$$^{circ}$$C, 0.7 MPa) to simulate BWR annular flow. Using a high-speed camera and the constant electric current method, we analyzed liquid-film characteristics, wave velocity and frequency. We also examined surface tension and interfacial shear stress effects. Furthermore, we proposed a new correlation for base film thickness.

Journal Articles

Estimation of permeability and Forchheimer coefficient for non-uniform packed beds

Sano, Yoshihiko*; Ota, Kensuke*; Kuwahara, Fujio*; Uesawa, Shinichiro; Yoshida, Hiroyuki

Nihon Kikai Gakkai Netsu Kogaku Konfuarensu 2025 Koen Rombunshu, 1 Pages, 2025/10

To estimate the thermal behavior of fuel debris inside the Primary Containment Vessels (PCVs) of TEPCO's Fukushima Daiichi nuclear power station, a simulation method has been developed using the JUPITER code with porous medium models. However, it has been found that the selection of models and parameters according to the internal structure of the porous media significantly affects the accuracy of simulation results, highlighting the need for appropriate model selection strategies. In this study, we investigated methods for calculating macroscopic model constants that characterize flow behavior in porous media. These properties are influenced not only by the volume ratio of solid and gas phases but also by the structural features of the porous media. Focusing on packed beds composed of particles with varying diameters, we conducted numerical simulations to evaluate permeability and Forchheimer coefficient across diverse structural configurations. Based on the results, we propose a method for appropriately determining these parameters according to the structure of the packed bed, thereby contributing to the improvement of the porous media heat transfer and flow model.

Journal Articles

Estimation of H$$_{2}$$ demand and HTGR development potential in the industrial complex in Japan

Noguchi, Hiroki; Ishii, Katsunori; Ono, Masato; Kasahara, Seiji; Sato, Hiroyuki; Sakaba, Nariaki

Proceedings of World Hydrogen Technologies Convention 2025 (WHTC 2025) (Internet), p.50 - 52, 2025/10

Achieving carbon neutrality in Japan in 2050, hydrogen is expected to be used as an alternative to fossil fuels in the hard-to-abate sectors. In steelmaking, hydrogen-based reduction process has been developed as a substitute for the conventional blast furnace steelmaking process, which involves the reduction of iron ore by coke. In chemical industry, a novel olefin production process has been developed using hydrogen and CO$$_{2}$$, through methanol as an intermediate chemical. A large amount of hydrogen is required for these novel processes. Nuclear energy is well-suited to large-scale low-carbon hydrogen production. High temperature gas cooled reactor (HTGR) is a type of nuclear reactor featuring extraction of high temperature heat. The heat can be applicable to hydrogen production. This study predicts hydrogen demand in five industrial complexes in Japan in 2050 and estimates the potential for introducing HTGR to meet the demand. The introduction of HTGR could be a promising solution for decarbonizing industrial complexes due to their large-scale hydrogen supply capacity.

Journal Articles

Effect of surface tension and gas-liquid density ratio on the wave height and interfacial shear stress in annular flows

Zhang, H.*; Umehara, Yutaro*; Horiguchi, Naoki; Yoshida, Hiroyuki; Mori, Shoji*

Proceedings of 12th International Conference of Fluid Flow, Heat and Mass Transfer (FFHMT 2025), P. 222_1, 2025/07

In the past decades, the liquid film characteristics of annular flow, such as film thickness and wave height, have been studied extensively. However, most of experimental data and analyses available in previous studies are limited to the air-water annular flows under near-atmospheric conditions. Thus, the variation in surface tension and gas-liquid density ratio is also limited, and their effects on the characteristics of annular flow are not well-understood. The objective of this study is to clarify the effect of surface tension and gas-liquid density ratio on the wave height and interfacial shear stress in annular flows. We conducted experiments for gas-liquid annular flows and measured the time-varying liquid film thickness. Using water and ethanol as working liquids, whereas nitrogen and HFC134a gas as working gases, we varied the surface tension range from 30.7 to 67.4 mN/m and density ratio range from 27 to 434. The accuracy of sensors for the measurement using the conductance probe method is $$pm$$ 5%. By post-processing for the measurement data, liquid film thicknesses (base, average, and maximum film thickness) and wave height were estimated. As the experimental results, the data of both the maximum film thickness and the height of disturbance wave converged on a single curve when they plotted for the interfacial shear stress. The reason was considered that the shape of the disturbance wave is decided by the balance between the surface tension and the interfacial shear stress. With additional analysis based on a potential method, a direct relationship between the height of disturbance wave and interfacial shear stress was clarified. These findings enhance the understanding of annular flow dynamics and contribute to improving the two-phase flow modelling.

Journal Articles

Numerical verification for the effect of suppressing hydrogen embrittlement by Sn doping in the Al-Zn-Mg alloy

Ebihara, Kenichi; Fujihara, Hiro*; Shimizu, Kazuyuki*; Yamaguchi, Masatake; Toda, Hiroyuki*

International Journal of Hydrogen Energy, 136, p.751 - 756, 2025/06

 Times Cited Count:1 Percentile:16.37(Chemistry, Physical)

It has been experimentally reported that adding tin (Sn) to high-strength aluminum-zinc-magnesium (Al-Zn-Mg) alloys effectively suppresses hydrogen (H) embrittlement, which may be attributed to H absorption by the second-phase particles of Sn. To verify this fact, a simulation of H entry into the Sn phase in Al was performed using a model based on the reaction-diffusion equation that incorporates the solid solution energy of H evaluated by first-principles calculations. The results showed that the H solid solution site concentration of the second-phase particles must be at least five times higher than that of the Al phase for H absorption by the Sn second-phase particles to suppress H embrittlement. Therefore, the actual H embrittlement suppression effect of Sn second-phase particles is limited, and other factors may influence the suppression of H embrittlement in the experiment.

Journal Articles

Depositional age of the Lower-Middle Miocene Tanabe Group constrained by detrital zircon U-Pb ages and its implications for stress field

Abe, Noriaki; Hoshi, Hiroyuki*; Haji, Toshiki*; Sato, Katsushi*; Niki, Sota*; Hirata, Takafumi*; Iwano, Hideki*; Danhara, Toru*

Chishitsugaku Zasshi (Internet), 131(1), p.59 - 70, 2025/04

To constrain the upper limit of the depositional age of the Tanabe Group, Early-Middle Miocene forearc basin deposit, this study obtained the detrital zircon U-Pb ages separated from eight sedimentary rock samples. We obtained 221 concordant ages from 330 zircon grains. The youngest grain age was 19.4 Ma, suggesting the upper limit of the depositional age is younger than 19.4 Ma, and no grain showed the depositional age indicated by foraminifera (16.3-15.1 Ma). Large-scale volcanic activities occurred in the Middle Miocene around Kii Peninsula, mainly after 15 Ma. The lack of grain younger than 15 Ma suggests that the Tanabe Group was deposited before 15 Ma. Sluggish volcanic activities in the provenance areas before 15 Ma may have caused the lack of zircons having ages close to the depositional period inferred from foraminifera.

Journal Articles

Competition between mass-symmetric and asymmetric fission modes in $$^{258}$$Md produced in the $$^{4}$$He + $$^{254}$$Es reaction

Nishio, Katsuhisa; Hirose, Kentaro; Makii, Hiroyuki; Orlandi, R.; Kean, K. R.*; Tsukada, Kazuaki; Toyoshima, Atsushi*; Asai, Masato; Sato, Tetsuya; Chiera, N. M.*; et al.

Physical Review C, 111(4), p.044609_1 - 044609_12, 2025/04

 Times Cited Count:1 Percentile:43.93(Physics, Nuclear)

Journal Articles

Hydrogen embrittlement in Al-Zn-Mg alloys; Semispontaneous decohesion of precipitates

Shimizu, Kazuyuki*; Toda, Hiroyuki*; Hirayama, Kyosuke*; Fujihara, Hiro*; Tsuru, Tomohito; Yamaguchi, Masatake; Sasaki, Taisuke*; Uesugi, Masayuki*; Takeuchi, Akihisa*

International Journal of Hydrogen Energy, 109, p.1421 - 1436, 2025/03

 Times Cited Count:14 Percentile:90.29(Chemistry, Physical)

Our preceding investigation revealed that multiple hydrogen traps at coherent interfaces of MgZn$$_{2}$$ precipitates initiated spontaneous interface decohesion, causing hydrogen-induced quasicleavage cracking in Al-Zn-Mg alloys. Herein, we performed a quantitative and systematic investigation to discern the mechanisms by which hydrogen trapped at coherent/semi-coherent interfaces of precipitates could influence macroscopic hydrogen embrittlement by modulating the coherent interface of MgZn$$_{2}$$ through aging. To explore this hydrogen embrittlement phenomenon based on hydrogen trapping at the precipitate interface, we determined the hydrogen trapping energy of the semi-coherent MgZn$$_{2}$$ interface via first-principles calculations (0.56 eV/atom). Hydrogen partitioning of all hydrogen trapping sites, including vacancies, grain boundaries, and coherent and semi-coherent MgZn$$_{2}$$ interfaces, revealed that in overaged alloys, over 90% of the hydrogen was sequestered at semi-coherent interfaces. Owing to the inherent characteristics of the MgZn$$_{2}$$ interface, the hydrogen sequestered at the semi-coherent interface decreased the interfacial cohesive energy, causing semispontaneous decohesion of the interface and quasicleavage fracture in the Al-Zn-Mg alloys. These results implied that intergranular fracture was not directly induced by hydrogen trapped at grain boundaries but rather by the decohesion of precipitate interfaces along grain boundaries.

Journal Articles

Development of a dissolution method for analyzing the elemental composition of fuel debris using sodium peroxide fusion technique

Nakamura, Satoshi; Ishii, Sho*; Kato, Hitoshi*; Ban, Yasutoshi; Hiruta, Kenta; Yoshida, Takuya; Uehara, Hiroyuki; Obata, Hiroki; Kimura, Yasuhiko; Takano, Masahide

Journal of Nuclear Science and Technology, 62(1), p.56 - 64, 2025/01

 Times Cited Count:1 Percentile:18.09(Nuclear Science & Technology)

A dissolution method for analyzing the elemental composition of fuel debris using the sodium peroxide (Na$$_{2}$$O$$_{2}$$) fusion technique has been developed. Herein, two different types of simulated debris materials (such as solid solution of (Zr,RE)O$$_{2}$$ and molten core-concrete interaction products (MCCI)) were taken. At various temperatures, these debris materials were subsequently fused with Na$$_{2}$$O$$_{2}$$ in crucibles, which are made of different materials, such as Ni, Al$$_{2}$$O$$_{3}$$, Fe, and Zr. Then, the fused samples are dissolved in nitric acid. Furthermore, the effects of the experimental conditions on the elemental composition analysis were evaluated using inductively coupled plasma-atomic emission spectroscopy (ICP-AES), which suggested the use of a Ni crucible at 923 K as an optimum testing condition. The optimum testing condition was then applied to the demonstration tests with Three Mile Island unit-2 (TMI-2) debris in a shielded concrete cell, thereby achieving complete dissolution of the debris. The elemental composition of TMI-2 debris revealed by the proposed dissolution method has good reproducibility and has an insignificant contradiction in the mass balance of the sample. Therefore, this newly developed reproducible dissolution method can be effectively utilized in practical applications by dissolving fuel debris and estimating its elemental composition.

Journal Articles

Multi-modal 3D image-based simulation of hydrogen embrittlement crack initiation in Al-Zn-Mg alloy

Higa, Ryota*; Fujihara, Hiro*; Toda, Hiroyuki*; Kobayashi, Masakazu*; Ebihara, Kenichi; Takeuchi, Akihisa*

Materials Transactions, 65(8), p.899 - 906, 2024/08

 Times Cited Count:3 Percentile:28.20(Materials Science, Multidisciplinary)

It is indispensable to suppress hydrogen embrittlement (HE) to develop the strength of the Al-Zn-Mg alloy. Because intergranular fracture (IGF) is mainly observed when HE occurs in the alloy, we need to understand the IGF initiation to suppress HE. In the present study, we investigated the stress, strain, and H concentration, which influence the IGF initiation, in actual fractured regions by simulation of a crystal plasticity finite element method and H diffusion analysis in a 3D image-based model, which was created based on 3D polycrystalline microstructure data obtained from X-ray imaging technique. Combining the simulation and in-situ observation of the tensile test sample by X-ray CT, we examined the stress, strain, and H concentration, and discussed the IG crack initiation condition. As a result, it is revealed that stress normal to grain boundary induced by crystal plasticity dominates IG crack initiation while the accumulation of H due to stress has little impact on it.

Journal Articles

Current status of high temperature gas-cooled reactor development in Japan

Nagatsuka, Kentaro; Noguchi, Hiroki; Nagasumi, Satoru; Nomoto, Yasunobu; Shimizu, Atsushi; Sato, Hiroyuki; Nishihara, Tetsuo; Sakaba, Nariaki

Nuclear Engineering and Design, 425, p.113338_1 - 113338_11, 2024/08

 Times Cited Count:22 Percentile:98.08(Nuclear Science & Technology)

HTGR has a potential to contribute to decarbonization of hard-to-abate industries by supplying a large amount of hydrogen and high temperature heat or steam without carbon dioxide emission. JAEA has been conducting R&Ds for HTGR technologies with High Temperature Engineering Test Reactor (HTTR). This paper shows that HTTR's tests including the loss of core cooing test as a joint the OECD/NEA international research project and a HTTR heat application test plan which demonstrate hydrogen production by coupling the HTTR with a hydrogen production test facility. Additionally, aiming for operation start from the latter half of 2030s, the basic design of the HTGR demonstration reactor has been shown. The Japan's HTGR technology capabilities established by the HTTR project will be fully utilized for the construction of HTGR demonstration reactor.

Journal Articles

Stability enhancement by hydrophobic anchoring and a cross-linked structure of a phospholipid copolymer film for medical devices

Uchida, Kazuto*; Masuda, Tsukuru*; Hara, Shintaro*; Matsuo, Yoichi*; Liu, Y.*; Aoki, Hiroyuki; Asano, Yoshihiko*; Miyata, Kazuki*; Fukuma, Takeshi*; Ono, Toshiya*; et al.

ACS Applied Materials & Interfaces, 16(30), p.39104 - 39116, 2024/07

 Times Cited Count:11 Percentile:67.77(Nanoscience & Nanotechnology)

Journal Articles

JAEA's efforts to demonstrate high temperature gas-cooled reactors for carbon-neutral

Inaba, Yoshitomo; Sato, Hiroyuki; Sumita, Junya; Ohashi, Hirofumi; Nishihara, Tetsuo; Sakaba, Nariaki

Nihon Kikai Gakkai-Shi, 127(1267), p.25 - 28, 2024/06

Aiming to contribute to net-zero emissions through early social implementation of HTGRs, JAEA promote five projects: HTTR-Heat Application Test, HTGR Domestic Demonstration Reactor, UK HTGR Demonstration Program, UK HTGR Fuel Development Program, and Poland HTGR Research Reactor Basic Design. In addition to these five projects, this article provides an overview of the safety demonstration tests using HTTR.

Journal Articles

"Invisible" radioactive cesium atoms revealed; Pollucite inclusion in cesium-rich microparticles (CsMPs) from the Fukushima Daiichi Nuclear Power Plant

Miyazaki, Kanako*; Takehara, Masato*; Minomo, Kenta*; Horie, Kenji*; Takehara, Mami*; Yamasaki, Shinya*; Saito, Takumi*; Onuki, Toshihiko*; Takano, Masahide; Shiotsu, Hiroyuki; et al.

Journal of Hazardous Materials, 470(15), p.134104_1 - 134104_11, 2024/05

 Times Cited Count:4 Percentile:32.54(Engineering, Environmental)

Journal Articles

High Temperature Gas-cooled Reactor (HTGR)

Noguchi, Hiroki; Sato, Hiroyuki; Nishihara, Tetsuo; Sakaba, Nariaki

Kagaku Kogaku, 88(5), p.211 - 214, 2024/05

High temperature gas-cooled reactor (HTGR), one of the next-generation innovative reactors, has an inherent safety and can generate very high-temperature heat which can be used for various heat application including hydrogen production. In Japan, Green Growth Strategy for Carbon Neutrality in 2050 and Basic Policy for the Realization of GX state the promotion of technology development necessary for mass and low-cost carbon-free hydrogen production and development and construction of next-generation innovative reactors including the HTGR for the decarbonization of industrial sectors. Based on these policies, JAEA has been conducted the world's first hydrogen production test using nuclear heat from an HTGR, in addition to verifying the excellent safety features of HTGR, and has also started to study the construction of an HTGR demonstration reactor in cooperation with the industrial community. This paper shows the current status of R&D of HTGR in Japan.

Journal Articles

Magnetic structure and magnetoelectric properties of the spin-flop phase in LiFePO$$_{4}$$

Holm-Janas, S.*; Akaki, Mitsuru*; Fogh, E.*; Kihara, Takumi*; Le, M. D.*; Forino, P. C.*; Nikitin, S. E.*; Fennell, T.*; Painganoor, A.*; Vaknin, D.*; et al.

Physical Review B, 109(17), p.174413_1 - 174413_11, 2024/05

 Times Cited Count:6 Percentile:54.38(Materials Science, Multidisciplinary)

Journal Articles

Spin dependence in the $$p$$-wave resonance of $$^{139}$$$overrightarrow{textrm{La}}$+$overrightarrow{n}$

Okudaira, Takuya*; Nakabe, Rintaro*; Auton, C. J.*; Endo, Shunsuke; Fujioka, Hiroyuki*; Gudkov, V.*; Ide, Ikuo*; Ino, Takashi*; Ishikado, Motoyuki*; Kambara, Wataru*; et al.

Physical Review C, 109(4), p.044606_1 - 044606_9, 2024/04

 Times Cited Count:3 Percentile:52.63(Physics, Nuclear)

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