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Journal Articles

Distinct variation of electronic states due to annealing in $$T'$$-type La$$_{1.8}$$Eu$$_{0.2}$$CuO$$_{4}$$ and Nd$$_{2}$$CuO$$_{4}$$

Asano, Shun*; Ishii, Kenji*; Matsumura, Daiju; Tsuji, Takuya; Kudo, Kota*; Taniguchi, Takanori*; Saito, Shin*; Sunohara, Toshiki*; Kawamata, Takayuki*; Koike, Yoji*; et al.

Physical Review B, 104(21), p.214504_1 - 214504_7, 2021/12

JAEA Reports

Re-examinations of MA fuel composition for accelerator-driven system and its heat removal

Sugawara, Takanori; Moriguchi, Daisuke*; Ban, Yasutoshi; Tsubata, Yasuhiro; Takano, Masahide; Nishihara, Kenji

JAEA-Research 2021-008, 63 Pages, 2021/10

JAEA-Research-2021-008.pdf:4.43MB

This study aims to perform the neutronics calculations for accelerator-driven system (ADS) with a new fuel composition based on the SELECT process developed by Japan Atomic Energy Agency because the previous studies had used the ideal MA (minor actinide) fuel composition without uranium and rare earth elements. Through the neutronics calculations, it is shown that two calculation cases, with/without neptunium, satisfy the design criteria. Although the new fuel composition includes uranium and rare earth elements, the ADS core with the new fuel composition is feasible and consistent with the partitioning and transmutation (P&T) cycle. Based on the new fuel composition, the heat removal during fuel powder storage and fuel assembly assembling is evaluated. For the fuel powder storage, it is found that a cylindrical tube container with a length of 500 [mm] and a diameter of 11 - 21 [mm] should be stored under water. For the fuel assembly assembling, CFD analysis indicates that the cladding tube temperature would satisfy the criterion if the inlet velocity of air is larger than 0.5 [m/s]. Through these studies, the new fuel composition which is consistent with the P&T cycle is obtained and the heat removal with the latest conditions is investigated. It is also shown that the new fuel composition can be practically handled with respect to heat generation, which is one of the most difficult points in handling MA fuel.

Journal Articles

Development of a radiation survey device for a multipurpose unmanned surface vehicle

Sanada, Yukihisa; Miyamoto, Kenji*; Momma, Hiroyasu*; Miyazaki, Nobuyuki*; Nakasone, Takamasa*; Tahara, Junichiro*; Baba, Shoichiro*; Furuyama, Hiroki*

Marine Technology Society Journal, 55(5), p.222 - 230, 2021/09

Large quantities of volatile radionuclides were released into the atmosphere following the Fukushima Daiichi Nuclear Power Station (FDNPS) accident in March 2011. To evaluate their effect on aquatic organisms and radiocesium behavior in the environment, the monitoring of radioactive cesium in the waterbed soil is important. We developed a dedicated radiation survey device that can both directly measure and collect some sediment samples. A comprehensive test was conducted using this device, which was installed in an unmanned surface vehicle at Fukushima offshore contaminated by radiocesium that resulted from the FDNPS accident. Consequently, the effectiveness of this device was confirmed because the measurement results of the sediment-core sample and in-situ radiation survey results show a good correlation. A successful application of this device in the time of post-nuclear facility accident is expected.

Journal Articles

Observation of adsorbed hydrogen species on supported metal catalysts by inelastic neutron scattering

Yoshida, Hisao*; Yamamoto, Akira*; Hosokawa, Saburo*; Yamazoe, Seiji*; Kikkawa, Soichi*; Hara, Kenji*; Nakamura, Mitsutaka; Kamazawa, Kazuya*; Tanaka, Tsunehiro*

Topics in Catalysis, 64(9-12), p.660 - 671, 2021/08

 Times Cited Count:0 Percentile:0.01(Chemistry, Applied)

Journal Articles

Mechanistic study on the removal of Cs from contaminated soil by rapid ion exchange in subcritical water

Fukuda, Tatsuya*; Takahashi, Ryo*; Hara, Takuhi*; Ohara, Koji*; Kato, Kazuo*; Matsumura, Daiju; Inaba, Yusuke*; Nakase, Masahiko*; Takeshita, Kenji*

Journal of Nuclear Science and Technology, 58(4), p.399 - 404, 2021/04

 Times Cited Count:1 Percentile:0.01(Nuclear Science & Technology)

JAEA Reports

Manufacturing miniature beam window for accelerator-driven system by cutting T91 steel

Watanabe, Nao; Sugawara, Takanori; Okubo, Nariaki; Nishihara, Kenji

JAEA-Technology 2020-026, 59 Pages, 2021/03

JAEA-Technology-2020-026.pdf:3.95MB

As a part of partitioning and transmutation technology development to reduce the burden of radioactive disposal, an investigation of Accelerator-Driven System (ADS) has been performed by Japan Atomic Energy Agency. A beam window, which is an inherent structure of the ADS, is planned to be made from T91 steel and its shape is a thin hemisphere shell. However, it had never been tried to manufacture it out of T91 steel. In this investigation, we tried to manufacture miniature beam windows by cutting T91 steel, and to discuss the process, manufacturing accuracy and geometry measurement methods. As a result, considering a real scale ADS beam window, a figure error between designing and machining ones is estimated to be about 5%. Its effect would be very small to the structural strength.

JAEA Reports

Selection of nuclides for mass-balance analysis of fission products

Okamura, Tomohiro*; Oizumi, Akito; Nishihara, Kenji; Nakase, Masahiko*; Takeshita, Kenji*

JAEA-Data/Code 2020-023, 32 Pages, 2021/03

JAEA-Data-Code-2020-023.pdf:1.67MB

Nuclear Material Balance code (NMB code) have been developed in Japan Atomic Energy Agency. The NMB code will be updated with the function of mass balance analysis at the backend process such as reprocessing, vitrification and geological disposal. In order to perform its analysis with high accuracy, it is necessary to expand the number of FP nuclides calculated in the NMB code. In this study, depletion calculation by ORIGEN code was performed under 3 different burn-up conditions such as spent uranium fuel from light water reactor, and nuclides were selected from 5 evaluation indexes such as mass and heat generation. In addition, the FP nuclides required to configure a simple burnup chain with the same calculation accuracy as ORIGEN in the NMB code was selected. As the result, two lists with different number of nuclides, such as "Detailed list" and a "Simplified list", were created.

Journal Articles

Mode distribution analysis for superionic melt of CuI by coherent quasielastic neutron scattering

Kawakita, Yukinobu; Kikuchi, Tatsuya*; Tahara, Shuta*; Nakamura, Mitsutaka; Inamura, Yasuhiro; Maruyama, Kenji*; Yamauchi, Yasuhiro*; Kawamura, Seiko; Nakajima, Kenji

JPS Conference Proceedings (Internet), 33, p.011071_1 - 011071_6, 2021/03

CuI is a well-known superionic conductor in a high temperature solid phase where the mobile cations migrate between interstitial sites in the f.c.c. sublattice formed by iodine ions. Even in the molten state, it shows several features suggesting collective or cooperative ionic motion. MD results show that Cu diffuses much faster than I. The Cu-Cu partial structure factor have a FSDP which indicates a medium-range ordering of Cu ions. Moreover the Cu-Cu partial pair distribution deeply penetrates into the nearest neighboring Cu-I shell. To reveal origin such anomalous behaviors of molten CuI, we performed quaiselastic neutron scattering (QENS) by the disk-chopper spectrometer AMATERAS at MLF, J-PARC. To interpret the total dynamic structure factor obtained from coherent QENS, the mode distribution analysis was applied. It is found that the motion of iodine is a kind of fluctuating within an almost local area while Cu ions diffuse much faster than iodine ions.

JAEA Reports

Annual report on the environmental radiation monitoring around the Tokai Reprocessing Plant FY2019

Nakano, Masanao; Fujii, Tomoko; Nemoto, Masashi; Tobita, Keiji; Seya, Natsumi; Nishimura, Shusaku; Hosomi, Kenji; Nagaoka, Mika; Yokoyama, Hiroya; Matsubara, Natsumi; et al.

JAEA-Review 2020-069, 163 Pages, 2021/02

JAEA-Review-2020-069.pdf:4.78MB

Environmental radiation monitoring around the Tokai Reprocessing Plant has been performed by the Nuclear Fuel Cycle Engineering Laboratories, based on "Safety Regulations for the Reprocessing Plant of Japan Atomic Energy Agency, Chapter IV - Environmental Monitoring". This annual report presents the results of the environmental monitoring and the dose estimation to the hypothetical inhabitant due to the radioactivity discharged from the plant to the atmosphere and the sea during April 2019 to March 2020. In this report, some data include the influence of the accidental release from the Fukushima Daiichi Nuclear Power Station of Tokyo Electric Power Co., Inc. (the trade name was changed to Tokyo Electric Power Company Holdings, Inc. on April 1, 2016) in March 2011. Appendices present comprehensive information, such as monitoring programs, monitoring methods, monitoring results and their trends, meteorological data and discharged radioactive wastes. In addition, the data which were influenced by the accidental release and exceeded the normal range of fluctuation in the monitoring, were evaluated.

Journal Articles

Identification of hydrogen species on Pt/Al$$_{2}$$O$$_{3}$$ by ${it in situ}$ inelastic neutron scattering and their reactivity with ethylene

Yamazoe, Seiji*; Yamamoto, Akira*; Hosokawa, Saburo*; Fukuda, Ryoichi*; Hara, Kenji*; Nakamura, Mitsutaka; Kamazawa, Kazuya*; Tsukuda, Tatsuya*; Yoshida, Hisao*; Tanaka, Tsunehiro*

Catalysis Science & Technology, 11(1), p.116 - 123, 2021/01

 Times Cited Count:3 Percentile:81.22(Chemistry, Physical)

JAEA Reports

Hydrochemical investigation at the Mizunami Underground Research Laboratory; Compilation of groundwater chemistry data in the Mizunami Group and the Toki Granite (fiscal year 2019)

Fukuda, Kenji; Watanabe, Yusuke; Murakami, Hiroaki; Amano, Yuki; Aosai, Daisuke*; Hara, Naohiro*

JAEA-Data/Code 2020-012, 80 Pages, 2020/10

JAEA-Data-Code-2020-012.pdf:3.55MB

Japan Atomic Energy Agency has been investigating groundwater chemistry to understand the influence of excavation and maintenance of underground facilities as part of the Mizunami Underground Research Laboratory (MIU) Project in Mizunami, Gifu, Japan. In this report, we compiled data of groundwater chemistry and microbiology obtained at the MIU in the fiscal year 2019. In terms of ensuring traceability of data, basic information (e.g. sampling location, sampling time, sampling method and analytical method) and methodology for quality control are described.

Journal Articles

Hydrogen trapping in Mg$$_2$$Si and Al$$_7$$FeCu$$_2$$ intermetallic compounds in aluminum alloy; First-principles calculations

Yamaguchi, Masatake; Tsuru, Tomohito; Ebihara, Kenichi; Itakura, Mitsuhiro; Matsuda, Kenji*; Shimizu, Kazuyuki*; Toda, Hiroyuki*

Materials Transactions, 61(10), p.1907 - 1911, 2020/10

 Times Cited Count:2 Percentile:26.63(Materials Science, Multidisciplinary)

no abstracts in English

Journal Articles

Development and application of a $$^3$$He neutron spin filter at J-PARC

Okudaira, Takuya; Oku, Takayuki; Ino, Takashi*; Hayashida, Hirotoshi*; Kira, Hiroshi*; Sakai, Kenji; Hiroi, Kosuke; Takahashi, Shingo*; Aizawa, Kazuya; Endo, Hitoshi*; et al.

Nuclear Instruments and Methods in Physics Research A, 977, p.164301_1 - 164301_8, 2020/10

 Times Cited Count:4 Percentile:76.41(Instruments & Instrumentation)

Journal Articles

Nonresonant $$p$$-wave direct capture and interference effect observed in the $$^{16}$$O$$(n,gamma)^{17}$$O reaction

Nagai, Yasuki*; Kinoshita, Mitsutaka*; Igashira, Masayuki*; Nobuhara, Yuriko*; Makii, Hiroyuki; Mishima, Kenji*; Shima, Tatsushi*; Mengoni, A.*

Physical Review C, 102(4), p.044616_1 - 044616_8, 2020/10

 Times Cited Count:0 Percentile:0.02(Physics, Nuclear)

Journal Articles

Strong lattice anharmonicity exhibited by the high-energy optical phonons in thermoelectric material

Wu, P.*; Fan, F.-R.*; Hagihara, Masato*; Kofu, Maiko; Peng, K.*; Ishikawa, Yoshihisa*; Lee, S.*; Honda, Takashi*; Yonemura, Masao*; Ikeda, Kazutaka*; et al.

New Journal of Physics (Internet), 22(8), p.083083_1 - 083083_9, 2020/08

 Times Cited Count:2 Percentile:51.78(Physics, Multidisciplinary)

Thermoelectric material SnSe has aroused world-wide interests in the past years, and its inherent strong lattice anharmonicity is regarded as a crucial factor for its outstanding thermoelectric performance. However, the understanding of lattice anharmonicity in SnSe system remains inadequate, especially regarding how phonon dynamics are affected by this behavior. In this work, we present a comprehensive study of lattice dynamics on Na$$_{0.003}$$Sn$$_{0.997}$$Se$$_{0.9}$$S$$_{0.1}$$ by means of neutron total scattering, inelastic neutron scattering, Raman spectroscopy as well as frozen-phonon calculations. Lattice anharmonicity is evidenced by pair distribution function, inelastic neutron scattering and Raman measurements. By separating the effects of thermal expansion and multi-phonon scattering, we found that the latter is very significant in high-energy optical phonon modes. The strong temperature-dependence of these phonon modes indicate the anharmonicity in this system. Moreover, our data reveals that the linewidths of high-energy optical phonons become broadened with mild doping of sulfur. Our studies suggest that the thermoelectric performance of SnSe could be further enhanced by reducing the contributions of high-energy optical phonon modes to the lattice thermal conductivity via phonon engineering.

JAEA Reports

Material balance analysis for wide range of nuclear power generation scenarios

Nishihara, Kenji

JAEA-Data/Code 2020-005, 48 Pages, 2020/07

JAEA-Data-Code-2020-005.pdf:2.95MB
JAEA-Data-Code-2020-005-appendix(CD-ROM).zip:3.62MB

In order to discuss the technological development and human resource development necessary for the future nuclear fuel cycle, various quantitative analyzes were conducted assuming a wide range of future nuclear power generation scenarios. In the evaluation of quantities, the future power generation of LWR and fast reactor, the amount of spent fuel reprocessing, etc. were assumed, and the amount of uranium demand, the accumulation of spent fuel, plutonium, vitrified waste etc. were estimated.

Journal Articles

Gapless spin liquid in a square-kagome lattice antiferromagnet

Fujihara, Masayoshi*; Morita, Katsuhiro*; Mole, R.*; Mitsuda, Setsuo*; Toyama, Takami*; Yano, Shinichiro*; Yu, D.*; Sota, Shigetoshi*; Kuwai, Tomohiko*; Koda, Akihiro*; et al.

Nature Communications (Internet), 11(1), p.3429_1 - 3429_7, 2020/07

 Times Cited Count:8 Percentile:81.73(Multidisciplinary Sciences)

Journal Articles

Hydrogen-accelerated spontaneous microcracking in high-strength aluminium alloys

Tsuru, Tomohito; Shimizu, Kazuyuki*; Yamaguchi, Masatake; Itakura, Mitsuhiro; Ebihara, Kenichi; Bendo, A.*; Matsuda, Kenji*; Toda, Hiroyuki*

Scientific Reports (Internet), 10, p.1998_1 - 1998_8, 2020/04

 Times Cited Count:5 Percentile:69.45(Multidisciplinary Sciences)

Age-hardening has been one and only process to achieve high strength aluminum alloys since unlike iron and titanium, pure aluminum does not have other solid phases during heat treatment. Highly-concentrated precipitations play therefore dominant role in mechanical properties and hydrogen embrittlement of aluminium alloys. It has been considered that the coherent interface between matrix and precipitation does not contribute to the crack initiation and embrittlement due to its coherency. Here, we discovered the origin of unprecedented quasi-cleavage fracture mode. Hydrogen partitioning at various defect sites is investigated comprehensively combined with experiment, theory and first-principles calculations. We demonstrate that despite low excess free volume, the aluminum-precipitation interface is more preferable trap site than void and grain boundary. The cohesivity of the interface deteriorates significantly with increasing occupancy while hydrogen atoms are trapped stably up to extremely high occupancy equivalent to spontaneous cleavage.

JAEA Reports

Annual report on the environmental radiation monitoring around the Tokai Reprocessing Plant FY2018

Nakano, Masanao; Fujii, Tomoko; Nemoto, Masashi; Tobita, Keiji; Kono, Takahiko; Hosomi, Kenji; Nishimura, Shusaku; Matsubara, Natsumi; Maehara, Yushi; Narita, Ryosuke; et al.

JAEA-Review 2019-048, 165 Pages, 2020/03

JAEA-Review-2019-048.pdf:2.69MB

Environmental radiation monitoring around the Tokai Reprocessing Plant has been performed by the Nuclear Fuel Cycle Engineering Laboratories, based on "Safety Regulations for the Reprocessing Plant of Japan Atomic Energy Agency, Chapter IV - Environmental Monitoring". This annual report presents the results of the environmental monitoring and the dose estimation to the hypothetical inhabitant due to the radioactivity discharged from the plant to the atmosphere and the sea during April 2018 to March 2019. In this report, some data include the influence of the accidental release from the Fukushima Daiichi Nuclear Power Station of Tokyo Electric Power Co., Inc. (the trade name was changed to Tokyo Electric Power Company Holdings, Inc. on April 1, 2016) in March 2011. Appendices present comprehensive information, such as monitoring programs, monitoring methods, monitoring results and their trends, meteorological data and discharged radioactive wastes. In addition, the data which were influenced by the accidental release and exceeded the normal range of fluctuation in the monitoring, were evaluated.

Journal Articles

JENDL/ImPACT-2018; A New nuclear data library for innovative studies on transmutation of long-lived fission products

Kunieda, Satoshi; Furutachi, Naoya; Minato, Futoshi; Iwamoto, Nobuyuki; Iwamoto, Osamu; Nakayama, Shinsuke; Ebata, Shuichiro*; Yoshida, Toru*; Nishihara, Kenji; Watanabe, Yukinobu*; et al.

Journal of Nuclear Science and Technology, 56(12), p.1073 - 1091, 2019/12

 Times Cited Count:3 Percentile:57.07(Nuclear Science & Technology)

A new nuclear data library, JENDL/ImPACT-2018, is developed for an innovative study on the transmutation of long-lived fission products. Nuclear reaction cross- sections are newly evaluated for incident neutrons and protons up to 200 MeV for 163 nuclides including long-lived nuclei such as $$^{79}$$Se, $$^{93}$$Zr, $$^{107}$$Pd and $$^{135}$$Cs. Our challenge is an evaluation of cross-sections for a number of unstable nuclei over a wide energy range where the experimental data are very scarce. We estimated cross- sections based on a nuclear model code CCONE that incorporates an advanced knowledge on the nuclear structure theory and a model-parameterization based on a new experimental cross-sections measured by the inverse kinematics. Through comparisons with available experimental data on the stable isotopes, it is found that the present data give predictions of cross-sections better than those in the existing libraries.

698 (Records 1-20 displayed on this page)