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論文

Integrated thermal power measurement in the modified STACY for the performance inspections

荒木 祥平; 會澤 栄寿; 村上 貴彦; 新垣 優; 多田 裕太; 神川 豊; 長谷川 健太; 吉川 智輝; 住谷 正人; 関 真和; et al.

Annals of Nuclear Energy, 217, p.111323_1 - 111323_8, 2025/07

 被引用回数:0 パーセンタイル:0.00(Nuclear Science & Technology)

原子力機構では、臨界集合体STACYを均質溶液体系から非均質軽水減速体系へと更新した。STACY更新炉においても最大熱出力は200Wと定められており、熱出力校正は運転を行う上で重要である。熱出力測定においては、溶液系STACYで用いていたFPの分析による熱出力の評価が適応できなかったため、放射化法をベースとする実験データと数値計算を組み合わせて出力を評価する手法をSTACY更新炉の体系に適応し、測定を実施した。測定データを基に出力校正を実施した結果、校正後の指示値は放射化法による測定結果と3%以内で一致した。

論文

Achievements and status of the STRAD project for radioactive liquid waste management

荒井 陽一; 渡部 創; 中原 将海; 船越 智雅; 星野 貴紀; 高畠 容子; 坂本 淳志; 粟飯原 はるか; 長谷川 健太; 吉田 稔生; et al.

Progress in Nuclear Science and Technology (Internet), 7, p.168 - 174, 2025/05

STRADプロジェクトの進捗に係る報告として、CPFホットセルの処理状況とともに、新たなターゲットに係る研究計画と最新のトピックスについて報告する。

論文

Evaluation of the performance of event reconstruction algorithms in the JSNS$$^2$$ experiment using a $$^{252}$$Cf calibration source

Lee, D. H.*; 百々 拓; 羽賀 勝洋; 原田 正英; 長谷川 勝一; 春日井 好己; 木下 秀孝; 増田 志歩; 明午 伸一郎; 酒井 健二; et al.

Nuclear Instruments and Methods in Physics Research A, 1072, p.170216_1 - 170216_6, 2025/03

 被引用回数:2 パーセンタイル:94.02(Instruments & Instrumentation)

JSNS$$^2$$ investigates short-baseline neutrino oscillations using a 24-meter baseline and a 17-tonne Gd-loaded liquid scintillator target. Accurate event-reconstruction algorithms are crucial for analyzing experimental data. The algorithms undergo meticulous validation through calibration with a $$^{252}$$Cf source. This paper outlines the methodology and evaluates the reconstruction performance, focusing on neutrino interactions up to approximately 50 MeV for sterile neutrino searches. Both $$^{252}$$Cf and Michel electron events are studied to evaluate reconstruction accuracy. The analysis concludes that the uncertainty of the fiducial volume, with an appropriate correction, is much less than the requirement of JSNS$$^2$$ requirement (10%). Furthermore, the energy resolution is measured to be 3.3 $$pm$$ 0.1% for the Michel electron endpoint and 4.3 $$pm$$ 0.1% for the n-Gd peak in the central region.

論文

Pulse shape discrimination in JSNS$$^2$$

百々 拓; 羽賀 勝洋; 原田 正英; 長谷川 勝一; 春日井 好己; 木下 秀孝; 増田 志歩; 明午 伸一郎; 酒井 健二; 鈴谷 賢太郎; et al.

Progress of Theoretical and Experimental Physics (Internet), 2025(2), p.023H02_1 - 023H02_8, 2025/02

 被引用回数:0 パーセンタイル:0.00(Physics, Multidisciplinary)

JSNS$$^2$$ (J-PARC Sterile Neutrino Search a t J-PARC Spallation Neutron Source) is an experiment that is searching for sterile neutrinos via the observation of $$bar{nu}_{mu} to bar{nu}_e$$ appearance oscillations using neutrinos from muon decay-at-rest. For this search, rejecting cosmic-ray-induced neutron events by Pulse Shape Discrimination (PSD) is essential because the JSNS$$^2$$ detector is located above ground, on the third floor of the building. We have achieved 94.95$$% pm 0.15%$$ rejection of neutron events while keeping 92.82$$% pm 1.77%$$ of signal, electron-like events using a data-driven likelihood method. This article will report the PSD technique using the full fiducial volume of the JSNS$$^2$$ detector.

論文

First measurement of missing energy due to nuclear effects in monoenergetic neutrino charged-current interactions

Marzec, E.*; 百々 拓; 羽賀 勝洋; 原田 正英; 長谷川 勝一; 春日井 好己; 木下 秀孝; 増田 志歩; 明午 伸一郎; 酒井 健二; et al.

Physical Review Letters, 134, p.081801_1 - 081801_9, 2025/00

 被引用回数:0

We present the first measurement of the missing energy due to nuclear effects in monoenergetic, muon neutrino charged-current interactions on carbon, originating from $$K^+ to mu^+ nu_{mu}$$ decay at rest ($$E_{nu_{mu}} = 235.5 MeV$$), performed with the J-PARC Sterile Neutrino Search at the J-PARC Spallation Neutron Source liquid scintillator based experiment. Toward characterizing the neutrino interaction, ostensibly $$nu_{mu}n to mu^- p$$ or $$nu_{mu}$$ $$^{12}$$C $$to$$ $$mu^-$$ $$^{12}$$N, we define the missing energy as the energy transferred to the nucleus ($$omega$$) minus the kinetic energy of the outgoing proton(s), $$E_m equiv omega - Sigma T_p$$, and relate this to visible energy in the detector, $$E_m = E_{nu_{mu}} (235.5 MeV) - m_{mu}(105.7 MeV) + [m_n - m_p(1.3 MeV)] - E_{vis}$$. The missing energy, which is naively expected to be zero in the absence of nuclear effects (e.g., nucleon separation energy, Fermi momenta, and final-state interactions), is uniquely sensitive to many aspects of the interaction, and has previously been inaccessible with neutrinos. The shape-only, differential cross section measurement reported, based on a $$(77pm 3%)$$ pure double-coincidence kaon decay-at-rest signal (621 total events), provides detailed insight into neutrino-nucleus interactions, allowing even the nuclear orbital shell of the struck nucleon to be inferred. The measurement provides an important benchmark for models and event generators at hundreds of MeV neutrino energies, characterized by the difficult-to-model transition region between neutrino-nucleus and neutrino-nucleon scattering, and relevant for applications in nuclear physics, neutrino oscillation measurements, and Type-II supernova studies.

論文

Investigation of adsorption mechanism of Mo(VI) by baker's yeast and applicability to the uranium liquid waste treatment process

荒井 陽一; 長谷川 健太; 渡部 創; 渡部 雅之; 箕輪 一希*; 松浦 治明*; 羽倉 尚人*; 勝木 健太*; 新井 剛*; 小西 康裕*

Journal of Radioanalytical and Nuclear Chemistry, 333(7), p.3585 - 3593, 2024/07

 被引用回数:1 パーセンタイル:25.62(Chemistry, Analytical)

Radioactive aqueous and organic liquid wastes contaminated by U are generated by solvent extraction of nuclear fuel materials in experiments of reprocessing technologies. Although incineration and denitrification/conversion processes are promising for treating such liquid waste, the installation of large equipment is essential. To give appropriate treatment procedures for radioactive liquid waste generated in nuclear facilities, STRAD (Systematic Treatments of RAdioactive liquid wastes for Decommissioning) project was started by Japan Atomic Energy Agency (JAEA) with several organizations. We are focusing on baker's yeasts for their excellent metal ions adsorption characteristics, easy handling and low prices. In order to optimize adsorption performance and operation procedures as the liquid waste treatment technology, adsorption performance of U has to be precisely investigated. In this study, adsorption performance of U and anion from nitric acid solution was investigated by batch-wise adsorption experiments.

論文

Study on the accidental background of the JSNS$$^2$$ experiment

Lee, D. H.*; 百々 拓; 羽賀 勝洋; 原田 正英; 長谷川 勝一; 春日井 好己; 木下 秀孝; 増田 志歩; 明午 伸一郎; 酒井 健二; et al.

European Physical Journal C, 84, p.409_1 - 409_6, 2024/04

 被引用回数:1 パーセンタイル:41.24(Physics, Particles & Fields)

JSNS$$^2$$ (J-PARC Sterile Neutrino Search at J-PARC Spallation Neutron Source) is an experiment that searches for sterile neutrinos via the observation of $$bar{nu}_{mu} to bar{nu}_{e}$$ appearance oscillations using muon decay-at-rest neutrinos. The JSNS$$^2$$ experiment performed data taking from 2021. In this manuscript, a study of the accidental background is presented. The rate of the accidental background is (9.29$${pm}$$0.39)$${times}$$10$$^{-8}$$ / spill with 0.75 MW beam power and comparable to the expected number of signal events.

論文

Optimization in granulation conditions for adsorbent of extraction chromatography

長谷川 健太; 後藤 一郎*; 宮崎 康典; 安倍 弘; 渡部 創; 渡部 雅之; 佐野 雄一; 竹内 正行

Mechanical Engineering Journal (Internet), 11(2), p.23-00407_1 - 23-00407_8, 2024/04

JAEA has been working on development of extraction chromatography technology for recovery of trivalent minor actinides (MA(III)) from high-level radioactive waste generated in reprocessing of spent fuel. The technology utilizes porous silica particles with about 50 micrometre diameter for support of adsorbents. Pressure drop of the packed column depends on characteristics of the particle. Large pressure drop of the column is not favorable for safety assessment of the technology although a certain level of the pressure drop is indispensable for excellent separation performance. In this study, we applied a granulation technique using a spray dryer that is widely used in industry, and conducted experiments to find the optimal specifications for silica support particles and conditions for the granulation operation. A basic characterization of the adsorbent prepared from the produced particles was carried out by an adsorption test of simulated high level liquid waste.

論文

Overview of development program for engineering scale extraction chromatography MA(III) recovery system

渡部 創; 高畠 容子; 長谷川 健太; 後藤 一郎*; 宮崎 康典; 渡部 雅之; 佐野 雄一; 竹内 正行

Mechanical Engineering Journal (Internet), 11(2), p.23-00461_1 - 23-00461_10, 2024/04

Japan Atomic Energy Agency is developing extraction chromatography technology to recover MA(III) from spent nuclear fuel. Developments in the extraction chromatography system especially focusing on safety and stable operation are required for practical application of the technology. This paper discusses the main tasks that have to be challenged preferentially based on achievements obtained by previous studies and potential MA(III) recovery process flow.

論文

Kinetic analysis of mass transfer of Eu(III) in extractant-impregnated polymer-layered silica particle in multiple-ion distribution system

宮川 晃尚*; 林 直輝*; 岩本 響*; 新井 剛*; 長友 重紀*; 宮崎 康典; 長谷川 健太; 佐野 雄一; 中谷 清治*

Analytical Sciences, 40(2), p.347 - 352, 2024/02

 被引用回数:2 パーセンタイル:11.65(Chemistry, Analytical)

複数のランタノイドイオンを含む錯体溶液中における単一抽出剤含浸高分子被覆シリカ粒子中のEu(III)分配機構を蛍光顕微分光法を用いて調べた。律速段階はEu(III)と2つの抽出剤分子との反応であった。得られた機構と速度定数は、Eu(III)溶液中でEu(III)が粒子に分配される単元素系の機構と一致した。

論文

The Acrylic vessel for JSNS$$^2$$-II neutrino target

Shin, C. D.*; 百々 拓; 羽賀 勝洋; 原田 正英; 長谷川 勝一; 春日井 好己; 木下 秀孝; 増田 志歩; 明午 伸一郎; 酒井 健二; et al.

Journal of Instrumentation (Internet), 18(12), p.T12001_1 - T12001_9, 2023/12

 被引用回数:0 パーセンタイル:0.00(Instruments & Instrumentation)

The JSNS$$^2$$ (J-PARC Sterile Neutrino Search at J-PARC Spallation Neutron Source) is an experiment designed for the search for sterile neutrinos. The experiment is currently at the stage of the second phase named JSNS$$^2$$-II with two detectors at near and far locations from the neutrino source. One of the key components of the experiment is an acrylic vessel, that is used for the target volume for the detection of the anti-neutrinos. The specifications, design, and measured properties of the acrylic vessel are described.

論文

Validation of integrated thermal power measurement using solution fuel STACY experimental data for modified STACY performance test

荒木 祥平; 郡司 智; 新垣 優; 村上 貴彦; 吉川 智輝; 長谷川 健太; 多田 裕太; 井澤 一彦; 須山 賢也

Proceedings of 4th Reactor Physics Asia Conference (RPHA2023) (Internet), 4 Pages, 2023/10

STACY更新炉における熱出力校正試験に向けて、放射化箔を用いた積算出力の評価方法の妥当性を検証するため、溶液系STACYで測定された放射化実験データを用いて、積算出力を評価した。放射化法による評価結果と溶液系STACYにおいて出力評価に用いられていた核分裂生成物の測定による評価結果とを比較し両者がよく一致することを確認した。

論文

Competitive distribution of europium and samarium based on reaction rate-limiting process in nitrilotriacetamide extractant-impregnated polymer-coated silica particles

宮川 晃尚*; 林 直輝*; 岩本 響*; 新井 剛*; 長友 重紀*; 宮崎 康典; 長谷川 健太; 佐野 雄一; 中谷 清治*

Bulletin of the Chemical Society of Japan, 96(9), p.1019 - 1025, 2023/09

 被引用回数:4 パーセンタイル:34.10(Chemistry, Multidisciplinary)

本研究では、ニトリロトリアセトアミド(NTA)抽出液を含浸させたポリマーコートシリカ単粒子において、Eu(III)とSm(III)のこれらのイオンを含む溶液中での物質移動機構を明らかにした。質量移動の律速過程は、NO$$_{3}$$$$^{-}$$イオンが関与しないイオンとNTA分子の反応過程であり、これは単一イオン分配系で得られたものと一致した。

論文

高温ガス炉と水素製造施設の接続技術開発; HTTR-熱利用試験計画

石井 克典; 守田 圭介; 野口 弘喜; 青木 健; 水田 直紀; 長谷川 武史; 永塚 健太郎; 野本 恭信; 清水 厚志; 飯垣 和彦; et al.

第27回動力・エネルギー技術シンポジウム講演論文集(インターネット), 4 Pages, 2023/09

JAEA initiated the HTTR heat application test project coupling a hydrogen production facility to the HTTR (high temperature engineering test reactor). The project aims to establish "coupling technologies" between HTGR and hydrogen production achieving large-scale, stable and economically competitive carbon-free hydrogen production using the HTGR heat. Important considerations towards establishment of coupling technologies are development of system technologies for HTGR hydrogen production systems and components required for coupling between two facilities. This paper explains a system concept of the HTTR heat application system which can maintain safe and stable operation of the HTTR against temperature transients induced by abnormal events in a hydrogen production plant with the results of operational scheme as well as heat and mass balance of the system. Development plans for hot gas duct, high temperature isolation valves and helium gas circulators are also presented.

論文

Evaluation of the remaining spent extraction solvent in vermiculite after leaching tests via PIXE analysis

荒井 陽一; 渡部 創; 長谷川 健太; 岡村 信生; 渡部 雅之; 武田 啓佑*; 福元 博基*; 吾郷 友宏*; 羽倉 尚人*; 塚原 剛彦*

Nuclear Instruments and Methods in Physics Research B, 542, p.206 - 213, 2023/09

 被引用回数:1 パーセンタイル:26.66(Instruments & Instrumentation)

Spent PUREX solvent, which mainly consists of tributyl phosphate (TBP) and normal dodecane, is generated by solvent extraction of Plutonium and Uranium in the spent nuclear fuel reprocessing. One of the treatment options for storage of the spent solvent is adsorption of the liquid into vermiculite. The organic liquid is considered to be trapped between layers of the vermiculite. Our previous experiments on the adsorption of spent solvent into the vermiculite have shown that some parts of loaded solvent gradually leaked out from the vermiculite. In order to investigate the adsorption mechanism and capacity, elution behavior of the loaded solvent into organic diluents were evaluated. A part of the loaded solvent was easily leaked into the diluent, while some solvent remained inside the particle even after the leaching test. In this study, the adsorption capacity of the vermiculite was evaluated through amount of remaining solvent after washing with diluents. The amount of the remaining solvent was analyzed by Particle Induced X-ray Emission (PIXE) on P contained in TBP. Peak intensity of P-K$$alpha$$ line depended on the washing condition, and the behavior of the amount of change in adsorbed P atom qualitatively agreed with the results of the leaching test.

論文

Kinetic mass transfer behavior of Eu(III) in nitrilotriacetamide-impregnated polymer-coated silica particles

宮川 晃尚*; 林 直輝*; 崩 愛昌*; 高橋 拓海*; 岩本 響*; 新井 剛*; 長友 重紀*; 宮崎 康典; 長谷川 健太; 佐野 雄一; et al.

Bulletin of the Chemical Society of Japan, 96(7), p.671 - 676, 2023/07

 被引用回数:7 パーセンタイル:58.25(Chemistry, Multidisciplinary)

HONTAおよびTOD2EHNTAとして知られるニトリロトリアセトアミド(NTA)抽出剤を含む単一ポリマー被覆シリカ粒子におけるEu(III)の分配機構を検討した。本研究は、「単一の抽出剤を含浸したポリマー被覆シリカ粒子」の機能性を評価・向上させるための貴重なアプローチを提供するものである。

論文

Development of engineering scale extraction chromatography separation system, 1; Overview of developments in engineering scale system

渡部 創; 高畠 容子; 長谷川 健太; 後藤 一郎*; 宮崎 康典; 渡部 雅之; 佐野 雄一; 竹内 正行

Proceedings of 30th International Conference on Nuclear Engineering (ICONE30) (Internet), 6 Pages, 2023/05

Japan Atomic Energy Agency is developing extraction chromatography technology for MA(III) recovery from spent nuclear fuel. Developments in the extraction chromatography system especially focusing on safety and stable operation are required for practical application of the technology. In this paper, main tasks which have to be challenged preferentially are discussed based on achievements obtained by previous studies and potential MA(III) recovery process flow.

論文

Development of engineering scale extraction chromatography separation system, 2; Spray drying granulation of silica support for adsorbent

長谷川 健太; 後藤 一郎*; 宮崎 康典; 安倍 弘; 渡部 創; 渡部 雅之; 佐野 雄一; 竹内 正行

Proceedings of 30th International Conference on Nuclear Engineering (ICONE30) (Internet), 5 Pages, 2023/05

JAEA has been working on development of extraction chromatography technology for recovery of trivalent minor actinides (MA(III): Am, Cm) from high-level radioactive waste generated in reprocessing of spent fuel. The technology utilizes porous silica particles with about 50 micrometre diameter for support of adsorbents. The particles are coated by styrene-divinylbenzene copolymer, and an extractant for MA recovery is impregnated into the polymer. Pressure drop of the packed column depends on characteristics of the particle (diameter, uniformity and pore size). Large pressure drop of the column is not favorable for safety assessment of the technology although a certain level of the pressure drop is indispensable for excellent separation performance. In this study, spray drying granulation experiments and fundamental characterization of the product particle were carried out to find optimal specs of the particle and conditions of the granulation operation.

論文

The Muon linac project at J-PARC

近藤 恭弘; 北村 遼; 不破 康裕; 森下 卓俊; 守屋 克洋; 高柳 智弘; 大谷 将士*; Cicek, E.*; 恵郷 博文*; 深尾 祥紀*; et al.

Proceedings of 31st International Linear Accelerator Conference (LINAC 2022) (Internet), p.636 - 641, 2022/09

J-PARCにおいて、現代の素粒子物理学で最も重要な課題の一つである、ミューオン異常磁気モーメント、電気双極子モーメントを精密測定する実験のためのミューオンリニアック計画が進行中である。J-PARCミューオン施設からのミューオンはいったん室温まで冷却され、212MeVまで加速される。横エミッタンスは1.5$$pi$$mm mradであり、運動量分散は1%である。高速で規格化した粒子の速度で0.01から0.94におよぶ広い範囲で効率よく加速するため、4種類の加速構造が用いられる。計画は建設段階に移行しつつあり、初段の高周波四重極リニアックによるミューオン再加速はすでに2017年に実証済である。次段の交差櫛形Hモードドリフトチューブリニアックのプロトタイプによる大電力試験が完了し、ディスクアンドワッシャ型結合セルリニアックの第一モジュールの製作が進行中である。さらに円盤装荷型加速管の設計もほぼ終了した。本論文ではこれらミューオンリニアックの最近の進捗について述べる。

論文

Phase transition and domain formation in ferroaxial crystals

林田 健志*; 上村 洋平*; 木村 健太*; 松岡 悟志*; 萩原 雅人; 廣瀬 左京*; 盛岡 仁*; 長谷川 達夫*; 木村 剛*

Physical Review Materials (Internet), 5(12), p.124409_1 - 124409_10, 2021/12

 被引用回数:33 パーセンタイル:83.95(Materials Science, Multidisciplinary)

The ferroaxial order, which is characterized by a rotational structural distortion in a crystal, has been recently proposed as one of ferroic orders. Though the domain formation is a characteristic feature in ferroic materials, there has been little study done concerning that for the ferroaxial order. Here, we investigate ferroaxial domains that are formed through a ferroaxial transition in two representative ferroaxial materials, NiTiO$$_{3}$$ and RbFe(MoO$$_{4}$$)$$_{2}$$. We spatially resolve their domain structures using an optical method based on electric-field- induced optical rotation, that is, electrogyration (EG). In NiTiO$$_{3}$$, multi-domains are constructed when crystals undergo a ferroaxial transition and the domain size depends on the cooling rate around the transition temperature. Furthermore, the ferroaxial domain structure obtained by the EG measurement is well matched with that by scanning X-ray diffraction (XRD). RbFe(MoO$$_{4}$$)$$_{2}$$ also exhibits multi-domain states in which domain patterns are different each time a crystal undergoes a ferroaxial transition. In addition, the temperature dependence of the EG signal well obeys that of the order parameter of a first-order phase transition. These results ensure the effectiveness of the EG effect to elucidate the nature of ferroaxial order.

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