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Cu and 
Cu with accelerator neutrons by deuterons and their separation from zincNagai, Yasuki*; Kawabata, Masako*; Saeki, Hideya*; Motoishi, Shoji*; Hashimoto, Kazuyuki; Tsukada, Kazuaki; Motomura, Arata*; Ota, Akio*; Takashima, Naoki*; Hashimoto, Shintaro; et al.
Frontiers in Nuclear Medicine (Internet), 5, p.1657125_1 - 1657125_11, 2025/10
In recent years, the radionuclide pair of Cu and Cu has attracted attention as an ideal theranostic agent. We proposed a novel production method utilizing a neutron source generated by deuteron beams at an accelerator facility. By irradiating enriched 
Zn samples with this neutron source, we measured the absolute activity and radionuclidic purity of the produced Cu. The results were consistent with calculations performed using PHITS and JENDL-5 developed by the Japan Atomic Energy Agency, confirming the reliability of the calculation method and demonstrating its capability to estimate the yields of trace radionuclides that are difficult to measure experimentally. Furthermore, we successfully separated Cu from the irradiated Zn sample using our developed sublimation and column separation techniques. These findings suggest that the production of Cu and Cu can be achieved in an economically sustainable manner at multiple sites.
lattice QCD with chiral fermionsAoki, Shinya*; Aoki, Yasumichi*; Fukaya, Hidenori*; Hashimoto, Shoji*; Kanamori, Issaku*; Kaneko, Takashi*; Nakamura, Yoshifumi*; Rohrhofer, C.*; Suzuki, Kei
Proceedings of Science (Internet), 396, p.332_1 - 332_7, 2022/07
The axial U(1) anomaly in high-temperature QCD plays an important role to understand the phase diagram of QCD. The previous works by JLQCD Collaboration studied high-temperature QCD using 2-flavor dynamical chiral fermions such as the domain-wall fermion and reweighted overlap fermion. We extend our simulations to QCD with 2+1-flavor dynamical quarks, where the masses of the up, down, and strange quarks are near the physical point, and the temperatures are close to or higher than the pseudocritical temperature. In this talk, we will present the results for the Dirac spectrum, topological susceptibility, axial U(1) susceptibility, and hadronic collelators.
Aoki, Shinya*; Aoki, Yasumichi*; Fukaya, Hidenori*; Hashimoto, Shoji*; Rohrhofer, C.*; Suzuki, Kei
Proceedings of Science (Internet), 396, p.050_1 - 050_9, 2022/07
In the early days of QCD, the axial 
anomaly was considered as a trigger for the breaking of the 
symmetry through topological excitations of gluon fields. However, it has been a challenge for lattice QCD to quantify the effect. In this work, we simulate QCD at high temperatures with chiral fermions. The exact chiral symmetry enables us to separate the contribution from the axial breaking from others among the susceptibilities in the scalar and pseudoscalar channels. Our result in two-flavor QCD indicates that the chiral susceptibility, which is conventionally used as a probe for breaking, is actually dominated by the axial breaking at temperatures 
MeV.
plantationAbe, Yukiko*; Liang, N.*; Teramoto, Munemasa*; Koarashi, Jun; Atarashi-Andoh, Mariko; Hashimoto, Shoji*; Tange, Takeshi*
Geoderma Regional (Internet), 29, p.e00529_1 - e00529_11, 2022/06
Times Cited Count：5 Percentile：24.99(Soil Science)This study aimed to clarify the causes of spatial variation in soil respiration rate on volcanic ash soil. From January 2013 to August 2019, soil respiration rates were measured at 40 measuring points periodically at a 35-year-old plantation in Tokyo, Japan. In August 2019, the carbon content of the litter layer, total carbon content of soil organic matter (SOM), carbon content of the low-density fraction (LF-C) of SOM, fine root biomass, and bulk density of soil were measured at all measuring points. Results of the multiple regression analysis showed that the model with only the LF-C as an explanatory variable had the highest capability for predicting the respiration rate at a soil temperature of 20
C, indicating that LF-C, which is considered to be readily available to soil microorganisms, can be the main factor responsible for the spatial variation in soil respiration rate.
Murase, Kiyoka*; Kataoka, Ryuho*; Nishiyama, Takanori*; Nishimura, Koji*; Hashimoto, Taishi*; Tanaka, Yoshimasa*; Kadokura, Akira*; Tomikawa, Yoshihiro*; Tsutsumi, Masaki*; Ogawa, Yasunobu*; et al.
Journal of Space Weather and Space Climate (Internet), 12, p.18_1 - 18_16, 2022/06
Times Cited Count：4 Percentile：28.31(Astronomy & Astrophysics)We identified two energetic electron precipitation (EEP) events during the growth phase of moderate substorms and estimated the mesospheric ionization rate for an EEP event for which the most comprehensive dataset from ground-based and space-born instruments was available. The mesospheric ionization signature reached below 70 km altitude and continued for ~15 min until the substorm onset, as observed by the PANSY radar and imaging riometer at Syowa Station in the Antarctic region. We also used energetic electron flux observed by the Arase and POES 15 satellites as the input for the air-shower simulation code PHITS to quantitatively estimate the mesospheric ionization rate. Combining the cutting-edge observations and simulations, we shed new light on the space weather impact of the EEP events during geomagnetically quiet times, which is important to understand the possible link between the space environment and climate.
Yb for producing 
Lu with high radionuclide purity by Yb(
)LuNagai, Yasuki*; Kawabata, Masako*; Hashimoto, Shintaro; Tsukada, Kazuaki; Hashimoto, Kazuyuki*; Motoishi, Shoji*; Saeki, Hideya*; Motomura, Arata*; Minato, Futoshi; Ito, Masatoshi*
Journal of the Physical Society of Japan, 91(4), p.044201_1 - 044201_10, 2022/04
Times Cited Count：6 Percentile：51.58(Physics, Multidisciplinary)Recently, Lu is considered as one of the most important medical RIs for treating neuroendocrine tumors. A plan to produce Lu with high purity by using enriched Yb samples with irradiation of deuteron beams in accelerators has been discussed. However, since the other Yb isotopes contained in the Yb sample interacts with deuterons, Lu isotopes other than Lu are produced as impurities. Since the purity of Lu is important for medical use, a method to evaluate the impurity of Lu has been required. In this study, we proposed a new method to estimate production yields of each Lu isotopes in Yb samples with arbitrary isotopic compositions by using excitation functions of Yb()Lu reactions and the particle transport calculation code PHITS. The method plays an important role in discussing the isotopic composition of enriched samples to produce high-purity Lu using accelerators.
anomaly in the chiral susceptibility of QCD at high temperatureAoki, Shinya*; Aoki, Yasumichi*; Fukaya, Hidenori*; Hashimoto, Shoji*; Rohrhofer, C.*; Suzuki, Kei
Progress of Theoretical and Experimental Physics (Internet), 2022(2), p.023B05_1 - 023B05_12, 2022/02
Times Cited Count：17 Percentile：78.29(Physics, Multidisciplinary)The chiral susceptibility, or the first derivative of the chiral condensate with respect to the quark mass, is often used as a probe for the QCD phase transition since the chiral condensate is an order parameter of 
symmetry breaking. However, the chiral condensate also breaks the axial symmetry, which is usually not studied as it is already broken by the anomaly and apparently has little impact on the transition. We investigate the susceptibilities in the scalar and pseudoscalar channels in order to quantify how much the axial breaking contributes to the chiral phase transition. Employing a chirally symmetric lattice Dirac operator and its eigenmode decomposition, we separate the axial breaking effects from others. Our result in two-flavor QCD indicates that both of the connected and disconnected chiral susceptibilities are dominated by axial breaking at temperatures 
MeV after the quadratically divergent constant is subtracted.
Cu and Cu via the Zn(n, p)Cu and Zn(n, np/d)Cu reactions using accelerator neutronsKawabata, Masako*; Motoishi, Shoji*; Ota, Akio*; Motomura, Arata*; Saeki, Hideya*; Tsukada, Kazuaki; Hashimoto, Shintaro; Iwamoto, Nobuyuki; Nagai, Yasuki*; Hashimoto, Kazuyuki*
Journal of Radioanalytical and Nuclear Chemistry, 330(3), p.913 - 922, 2021/12
Times Cited Count：13 Percentile：76.45(Chemistry, Analytical)Both Cu and Cu are promising radionuclides in nuclear medicine. Production yields of these radionuclides were quantified by irradiating 55.4 g of natural zinc with accelerator neutrons. Clinically suitable Cu and Cu yields were estimated by experimental based numerical simulations using 100 g of enriched Zn and Zn, respectively, and elevated neutron fluxes from 40 MeV, 2 mA deuterons. A combined thermal- and resin-separation method was developed to isolate Cu and Cu from zinc, resulting in 73% separation efficiency and 97% zinc recovery. Such methods can provide large scale production of Cu and Cu for clinical applications.
Hashimoto, Shoji*; Tanaka, Taku*; Komatsu, Masabumi*; Gonze, M.-A.*; Sakashita, Wataru*; Kurikami, Hiroshi; Nishina, Kazuya*; Ota, Masakazu; Ohashi, Shinta*; Calmon, P.*; et al.
Journal of Environmental Radioactivity, 238-239, p.106721_1 - 106721_10, 2021/11
Times Cited Count：21 Percentile：63.26(Environmental Sciences)This study was aimed at analysing performance of models for radiocesium migration mainly in evergreen coniferous forest in Fukushima, by inter-comparison between models of several research teams. The exercise included two scenarios of countermeasures against the contamination, namely removal of soil surface litter and forest renewal, and a specific konara oak forest scenario in addition to the evergreen forest scenario. All the models reproduced trend of time evolution of radiocesium inventories and concentrations in each of the components in forest such as leaf and organic soil layer. However, the variations between models enlarged in long-term predictions over 50 years after the fallout, meaning continuous field monitoring and model verification/validation is necessary.
anomaly at high temperature with lattice chiral fermionsAoki, Shinya*; Aoki, Yasumichi*; Cossu, G.*; Fukaya, Hidenori*; Hashimoto, Shoji*; Kaneko, Takashi*; Rohrhofer, C.*; Suzuki, Kei
Physical Review D, 103(7), p.074506_1 - 074506_18, 2021/04
Times Cited Count：37 Percentile：86.45(Astronomy & Astrophysics)We investigate the axial anomaly of two-flavor QCD at temperatures 190-330 MeV. In order to preserve precise chiral symmetry on the lattice, we employ the M
bius domain-wall fermion action as well as overlap fermion action implemented with a stochastic reweighting technique. Compared to our previous studies, we reduce the lattice spacing to 0.07 fm, simulate larger multiple volumes to estimate finite size effect, and take more than four quark mass points, including one below physical point to investigate the chiral limit. We measure the topological susceptibility, axial susceptibility, and examine the degeneracy of partners in meson/baryon correlators. All the data above the critical temperature indicate that the axial violation is consistent with zero within statistical errors. The quark mass dependence suggests disappearance of the anomaly at a rate comparable to that of the symmetry breaking.
Rohrhofer, C.*; Aoki, Yasumichi*; Cossu, G.*; Fukaya, Hidenori*; Gattringer, C.*; Glozman, L. Ya.*; Hashimoto, Shoji*; Lang, C. B.*; Suzuki, Kei
Proceedings of Science (Internet), 363, p.227_1 - 227_7, 2020/08
Properties of QCD matter change significantly around the chiral crossover temperature, and the effects on 
and topological susceptibilities, as well as the meson spectrum have been studied with much care. Baryons and the effect of parity doubling in this temperature range have been analyzed previously by various other groups employing different setups. Here we construct suitable operators to investigate chiral and axial symmetries in the baryon spectrum. Measurements for different volumes and quark-masses are done with two flavors of chirally symmetric domain-wall fermions at temperatures above the critical one. The possibility of emergent 
and 
symmetries is discussed.
lattice QCDSuzuki, Kei; Aoki, Shinya*; Aoki, Yasumichi*; Cossu, G.*; Fukaya, Hidenori*; Hashimoto, Shoji*; Rohrhofer, C.*
Proceedings of Science (Internet), 363, p.178_1 - 178_7, 2020/08
We investigate the high-temperature phase of QCD using lattice QCD simulations with dynamical Mbius domain-wall fermions. On generated configurations, we study the axial symmetry, overlap-Dirac spectra, screening masses from mesonic correlators, and topological susceptibility. We find that some of the observables are quite sensitive to lattice artifacts due to a small violation of the chiral symmetry. For those observables, we reweight the Mbius domain-wall fermion determinant by that of the overlap fermion. We also check the volume dependence of observables. Our data near the chiral limit indicates a strong suppression of the axial anomaly at temperatures 
220 MeV.
ZnO using polyethylene by accelerator neutronsTsukada, Kazuaki; Nagai, Yasuki*; Hashimoto, Shintaro; Minato, Futoshi; Kawabata, Masako*; Hatsukawa, Yuichi*; Hashimoto, Kazuyuki*; Watanabe, Satoshi*; Saeki, Hideya*; Motoishi, Shoji*
Journal of the Physical Society of Japan, 89(3), p.034201_1 - 034201_7, 2020/03
Times Cited Count：3 Percentile：22.83(Physics, Multidisciplinary)We found anomalously large yields of Ga, 
Ga, 
Zn and Cu by neutron irradiation on a ZnO sample in a polyethylene shield. Neutron beams are generated from the 
Be(
) reaction for 50 MeV deuterons. The yields obtained were more than 20 times larger than those in the unshielded sample. On the other hand, the yields of Ga, Ga, Zn and Cu from a metallic Zn sample and the yields of Cu, 
Ni and Zn from the ZnO and Zn samples were almost insensitive to the shield conditions. This finding would provide us a unique capability of accelerator neutrons to simultaneously produce a large amount of several radioisotopes, including proton induced reaction products, by using a single sample. The experimental data were compared with the yields estimated by using the Particle and Heavy Ion Transport code System and the result was discussed.
Mo yield using large sample mass of MoO
for sustainable production of MoTsukada, Kazuaki; Nagai, Yasuki*; Hashimoto, Kazuyuki*; Kawabata, Masako*; Minato, Futoshi; Saeki, Hideya*; Motoishi, Shoji*; Ito, Masatoshi*
Journal of the Physical Society of Japan, 87(4), p.043201_1 - 043201_5, 2018/04
Times Cited Count：10 Percentile：54.04(Physics, Multidisciplinary)
Tc-radiopharmaceuticals obtained from Mo produced by 
Mo(n,2n)Mo and fission of 
UHashimoto, Kazuyuki; Nagai, Yasuki; Kawabata, Masako; Sato, Nozomi*; Hatsukawa, Yuichi; Saeki, Hideya; Motoishi, Shoji*; Ota, Masayuki; Konno, Chikara; Ochiai, Kentaro; et al.
Journal of the Physical Society of Japan, 84(4), p.043202_1 - 043202_4, 2015/04
Times Cited Count：8 Percentile：49.49(Physics, Multidisciplinary)Tc from molten MoOKawabata, Masako; Nagai, Yasuki; Hashimoto, Kazuyuki; Saeki, Hideya; Motoishi, Shoji*; Sato, Nozomi*; Ota, Akio*; Shiina, Takayuki*; Kawauchi, Yukimasa*
Journal of the Physical Society of Japan, 84(2), p.023201_1 - 023201_4, 2015/02
Times Cited Count：6 Percentile：41.97(Physics, Multidisciplinary)Tc for medical use can be separated by thermochromatography from a molten MoO sample. Effect of moist oxygen gas on the Tc release from molten MoO samples was investigated using a Mo/Tc generator. Mo was produced with Mo(n,2n)Mo. A new phenomenon has been observed: release rate, separation- and recovery-efficiencies of Tc were higher in the moist oxygen gas than those in the dry oxygen gas. The present result is a significant progress towards the stable production of a high quality Tc from a molten MoO sample with high separation efficiency. The result would also give us a new insight into the interaction between the moist oxygen gas and the molten MoO.
Tc from molten MoO samples by repeated milking testsNagai, Yasuki; Kawabata, Masako; Sato, Nozomi; Hashimoto, Kazuyuki; Saeki, Hideya; Motoishi, Shoji*
Journal of the Physical Society of Japan, 83(8), p.083201_1 - 083201_4, 2014/07
Times Cited Count：12 Percentile：59.38(Physics, Multidisciplinary)Nagai, Yasuki; Hashimoto, Kazuyuki; Hatsukawa, Yuichi; Saeki, Hideya; Motoishi, Shoji; Sonoda, Nozomi; Kawabata, Masako; Harada, Hideo; Kin, Tadahiro*; Tsukada, Kazuaki; et al.
Journal of the Physical Society of Japan, 82(6), p.064201_1 - 064201_7, 2013/06
Times Cited Count：47 Percentile：84.80(Physics, Multidisciplinary)
Tc-MDP using Tc separated from Mo produced by Mo(
,2)MoNagai, Yasuki; Hatsukawa, Yuichi; Kin, Tadahiro; Hashimoto, Kazuyuki; Motoishi, Shoji; Konno, Chikara; Ochiai, Kentaro; Takakura, Kosuke; Sato, Yuichi*; Kawauchi, Yukimasa*; et al.
Journal of the Physical Society of Japan, 80(8), p.083201_1 - 083201_4, 2011/08
Times Cited Count：15 Percentile：63.55(Physics, Multidisciplinary)We have for the first time succeeded to separate Tc from a Mo oxide sample irradiated by accelerator neutrons, and to formulate Tc-methylene diphosphonate (Tc-MDP). Mo, the mother nuclide of Tc, was produced by the Mo(,2)Mo reaction using about 14 MeV neutrons provided at the Fusion Neutronics Source of Japan Atomic Energy Agency. The Tc was separated from Mo by the sublimation method, and its radionuclide purity was confirmed to be higher than 99.99%. The labeling efficiency of Tc-MDP was shown to be higher than 99%. These values exceed the United States Pharmacopeia requirements for a fission product, Mo. Consequently, a Tc radiopharmaceutical preparation formed by using the mentioned Mo can be a promising substitute for the fission product Mo. A longstanding problem to ensure a reliable and constant supply of Mo in Japan can be partially mitigated.
W/Re generatorsMatsuoka, Hiromitsu; Hashimoto, Kazuyuki; Hishinuma, Yukio*; Ishikawa, Koji*; Terunuma, Hitoshi*; Tatenuma, Katsuyoshi*; Uchida, Shoji*
Journal of Nuclear and Radiochemical Sciences, 6(3), p.189 - 191, 2005/12
Applicability of Mo adsorbent PZC(Poly Zirconium Compound) for W/Re generator was investigated. Long term stability of adsorption of W to the PZC column, elution of Re from PZC column, desorption of 
from PZC column, and labeling of Hydroxyethylidene Diphosphonic Acid(HEDP) and Mercaptoacetyltriglycine(MAG3) with Re eluted from PZC column were tested. The PZC generator gave reproducible Re elution yields with low W parent breakthrough for a long period of time(about 5 months), that is the W/Re generator using PZC has a potential for practical use.
