Band gap formation in graphene by hybridization with Hex-Au(001) reconstructed surface

Terasawa, Tomoo; Matsunaga, Kazuya*; Hayashi, Naoki*; Ito, Takahiro*; Tanaka, Shinichiro*; Yasuda, Satoshi; Asaoka, Hidehito

Vacuum and Surface Science, 66(9), p.525 - 530, 2023/09

https://doi.org/10.1380/vss.66.525

As Au (001) surfaces exhibit a quasi-one-dimensional corrugated structure, Hex-Au(001), its periodicity was predicted to change the electronic structure of graphene when graphene was grown on this surface. Furthermore, the hybridization between graphene and Au is known to introduce bandgap and spin polarization into graphene. Here, we report angle-resolved photoemission spectroscopy and density functional theory calculation of graphene on a Hex-Au(001) surface. A bandgap of 0.2 eV in the graphene Dirac cone was observed at the crossing point of the graphene Dirac cone and Au 6sp bands, indicating that the origin of the bandgap formation was the hybridization between the graphene Dirac cone and Au 6sp band. We discussed the hybridization mechanism and anticipated spin injection into the graphene Dirac cone.

Physical property investigation of gloves for glove boxes in nuclear fuel reprocessing plants; Physical properties of used gloves and estimation of its life-time

Yamamoto, Masahiko; Nishida, Naoki; Kobayashi, Daisuke; Nemoto, Ryo*; Hayashi, Hiroyuki*; Kitao, Takahiko; Kuno, Takehiko

JAEA-Technology 2023-004, 30 Pages, 2023/06

JAEA-Technology-2023-004.pdf:1.94MB

Glove-box gloves, that are used for handling nuclear fuel materials at the Tokai Reprocessing Plant (TRP) of the Japan Atomic Energy Agency, have an expiration date by internal rules. All gloves are replaced at a maximum of every 4-year. However, degrees of glove deterioration varies depending on its usage environment such as frequency, chemicals, and radiation dose. Therefore, physical properties such as tensile strength, elongation, hardness of gloves are measured and technical evaluation method for the glove life-time is established. It was found that gloves without any defects in its appearance have enough physical properties and satisfies the acceptance criteria values of new gloves. Thus, it was considered that the expired gloves could be used for total of 8-year, by adding 4-year of new glove life-time. In addition, the results of extrapolation by plotting the glove's physical properties versus the used years showed that the physical properties at 8-year is on the safer side than the reported physical properties of broken glove. Also, the data are not significantly different from the physical properties of the long-term storage glove (8 and 23 years). Based on these results, life-time of gloves at TRP is set to be 8-year. The frequency of glove inspections are not changed, and if any defects is found, the glove is promptly replaced. Thus, the risk related to glove usage is not increased. The cost of purchasing gloves, labor for glove replacement, and the amount of generated waste can be reduced by approximately 40%, respectively, resulting in more efficient and rationalized glove management.

Development plan for coupling technology between high temperature gas-cooled reactor HTTR and Hydrogen Production Facility, 2; Development plan for coupling equipment between HTTR and Hydrogen Production Facility

Mizuta, Naoki; Morita, Keisuke; Aoki, Takeshi; Okita, Shoichiro; Ishii, Katsunori; Kurahayashi, Kaoru; Yasuda, Takanori; Tanaka, Masato; Isaka, Kazuyoshi; Noguchi, Hiroki; et al.

Proceedings of 30th International Conference on Nuclear Engineering (ICONE30) (Internet), 6 Pages, 2023/05

Band gap opening in graphene by hybridization with Au (001) reconstructed surfaces

Terasawa, Tomoo; Matsunaga, Kazuya*; Hayashi, Naoki*; Ito, Takahiro*; Tanaka, Shinichiro*; Yasuda, Satoshi; Asaoka, Hidehito

Physical Review Materials (Internet), 7(1), p.014002_1 - 014002_10, 2023/01

https://doi.org/10.1103/PhysRevMaterials.7.014002

Au(001) surfaces exhibit a complex reconstructed structure [Hex-Au(001)] comprising a hexagonal surface and square bulk lattices, yielding a quasi-one-dimensional corrugated surface. When graphene was grown on this surface, the periodicity of the corrugated surface was predicted to change the electronic structure of graphene, forming bandgaps and new Dirac points. Furthermore, the graphene-Au interface is promising for bandgap generation and spin injection due to band hybridization. Here, we report the angle-resolved photoemission spectroscopy and density functional calculation of graphene on a Hex-Au(001) surface. The crossing point of the original and replica graphene bands showed no bandgap, suggesting that the one-dimensional potential was too small to modify the electronic structure. A bandgap of 0.2 eV was observed at the crossing point of the graphene and Au bands, indicating that the bandgap is generated using hybridization of the graphene and Au bands. We discussed the hybridization mechanism and concluded that the R30 configuration between graphene and Au and an isolated electronic structure of Au are essential for effective hybridization between graphene and Au. We anticipate that hybridization between graphene and Au would result in spin injection into graphene.

Longitudinal measurement of high-intensity beam with bunch-shape monitor in front-end

Kitamura, Ryo; Hayashi, Naoki; Hirano, Koichiro; Miyao, Tomoaki*; Miura, Akihiko; Morishita, Takatoshi

Proceedings of 19th Annual Meeting of Particle Accelerator Society of Japan (Internet), p.212 - 214, 2023/01

In the J-PARC linac, the bunch-shape monitor (BSM) is developed to precisely and rapidly measure the longitudinal beam profile at the front-end, towards the improvement of the beam matching. The graphite target having the good strength to the high-power beam, has been introduced in order to resist the heat loading of the high-intensity beam. The resolution and other uncertainties were evaluated for the BSM. The longitudinal Twiss parameters and emittance were measured using the BSM and the IMPACT, which was the 3D particle-in-cell simulation code. The precision of the longitudinal emittance measurement was improved, by implementing uncertainties related to the BSM into the calculation. In this presentation, we will report a series of the measurement result, the method of the beam diagnostics with the BSM at the front-end, and the comparison between the measurement and the beam simulation.

Investigation of physical properties of glove for glove-box and estimation of its life-time

Kobayashi, Daisuke; Yamamoto, Masahiko; Nishida, Naoki; Miyoshi, Ryuta; Nemoto, Ryo*; Hayashi, Hiroyuki*; Kato, Keisuke; Nishino, Saki; Kuno, Takehiko; Kitao, Takahiko; et al.

Nihon Hozen Gakkai Dai-18-Kai Gakujutsu Koenkai Yoshishu, p.237 - 240, 2022/07

All gloves attached to glove-box in Tokai Reprocessing Plant have a fixed expiration date and have to be replaced every 4-year. However, degrees of glove deterioration are different depending on its usage environment (frequency, chemicals, radiation, etc.), because of rubber products. Therefore, physical properties such as tensile strength, elongation, hardness of gloves are measured, and the life-time of gloves are estimated. As a result, gloves without any defects in its appearance have enough physical property for acceptance criteria of new glove. The extrapolated physical property of glove is sufficiently larger than the reported values of damaged glove. No deterioration in physical properties of gloves, that are periodically replaced without any defects in its appearance, is observed and the usable life-time of the glove is estimated to be 8 years.

Analysis of machine protection system events in the J-PARC Linac/RCS

Hayashi, Naoki; Hatakeyama, Shuichiro; Fukuta, Shimpei*

Proceedings of 18th Annual Meeting of Particle Accelerator Society of Japan (Internet), p.679 - 682, 2021/10

https://www.pasj.jp/web_publish/pasj2021/proceedings/PDF/WEP0/WEP025.pdf

In order to achieve a high availability in a user facility accelerator complex, it is necessary to understand in detail not only the simple failure cause of the magnet or the acceleration cavity power supply, but also complex interlocked events. At J-PARC, not only the primary interlock information but also the data recorded by the beam diagnostic system before the interlocked event is used to carefully reconstruct the event and clarify the cause more accurately. This time, we proceeded with the analysis based on more detailed waveform of the RCS Beam Loss Monitor and the events during simultaneous operation of MLF and MR. We present various events of the beam destination switching problem, the influence of the ion source discharged, and the events related to the RCS extraction kicker.

Reliability of J-PARC accelerator system over the past decade

Yamamoto, Kazami; Hasegawa, Kazuo; Kinsho, Michikazu; Oguri, Hidetomo; Hayashi, Naoki; Yamazaki, Yoshio; Naito, Fujio*; Yoshii, Masahito*; Toyama, Takeshi*

JPS Conference Proceedings (Internet), 33, p.011016_1 - 011016_7, 2021/03

https://doi.org/10.7566/JPSCP.33.011016

The Japan Proton Accelerator Research Complex (J-PARC) is a multipurpose facility for scientific experiments. The accelerator complex consists of a 400-MeV Linac, a 3-GeV Rapid-Cycling Synchrotron (RCS) and a 30-GeV Main Ring synchrotron (MR). The RCS delivers a proton beam to the neutron target and MR, and the MR delivers the beams to the neutrino target and the Hadron Experimental Facility. The first operation of the neutron experiments began in December 2008. Following this, the user operation has been continued with some accidental suspensions. These suspensions include the recovery work due to the Great East Japan Earthquake in March 2011 and the radiation leak incident at the Hadron Experimental Facility. In this report, we summarize the major causes of suspension, and the statistics of the reliability of J-PARC accelerator system is analyzed. Owing to our efforts to achieve higher reliability, the Mean Time Between Failure (MTBF) has been improved.

1.2-MW-equivalent high-intensity beam tests in J-PARC RCS

Hotchi, Hideaki; Harada, Hiroyuki; Hayashi, Naoki; Kinsho, Michikazu; Okabe, Kota; Saha, P. K.; Shobuda, Yoshihiro; Tamura, Fumihiko; Yamamoto, Kazami; Yamamoto, Masanobu; et al.

JPS Conference Proceedings (Internet), 33, p.011018_1 - 011018_6, 2021/03

https://doi.org/10.7566/JPSCP.33.011018

no abstracts in English

Bunch-size measurement of the high-intensity H beam with 3 MeV by the bunch-shape monitor

Kitamura, Ryo; Futatsukawa, Kenta*; Hayashi, Naoki; Hirano, Koichiro; Kondo, Yasuhiro; Kosaka, Satoshi*; Miyao, Tomoaki*; Nemoto, Yasuo*; Morishita, Takatoshi; Oguri, Hidetomo

JPS Conference Proceedings (Internet), 33, p.011012_1 - 011012_6, 2021/03

https://doi.org/10.7566/JPSCP.33.011012

The new bunch shape monitor (BSM) is required to measure the bunch size of the high-intensity H beam with 3 MeV at the front-end section in the J-PARC linac. The carbon-nano tube wire and the graphene stick are good candidates for the target wire of the BSM, because these materials have the enough strength to detect the high-intensity beam. However, since the negative high voltage of more than a few kV should be applied to the wire in the BSM, the suppression of the discharge is the challenge to realize the new BSM. After the high-voltage test to investigate the effect of the discharge from the wire, the detection of the signal from the BSM was successful at the beam core with the peak current of 55 mA using the graphene stick. The preliminary result of the bunch-size measurement is reported in this presentation.