Nuclear hydrogen demonstration project using the HTTR; Demarcation of nuclear-industrial laws and design standards

Aoki, Takeshi; Shimizu, Atsushi; Ishii, Katsunori; Morita, Keisuke; Mizuta, Naoki; Kurahayashi, Kaoru; Yasuda, Takanori; Noguchi, Hiroki; Nomoto, Yasunobu; Iigaki, Kazuhiko; et al.

Annals of Nuclear Energy, 220, p.111503_1 - 111503_7, 2025/09

https://doi.org/10.1016/j.anucene.2025.111503

Aiming to establish coupling technologies between a high temperature gas cooled reactor and a hydrogen production plant, JAEA has initiated the HTTR Heat Application Test Project and is conducting the safety design and the safety analysis for the licensing of the HTTR Heat Application Test Facility. The present study proposed a relative evaluation methodology for the demarcation of applicable laws and design standards for the nuclear hydrogen production system and applied it to the HTTR Heat Application Test Facility. The evaluation results showed that a candidate applying the High Pressure Gas Safety Act to the Heat Application Test Facility (hydrogen production plant) and design standards established under the High Pressure Gas Safety Act to the steam reformer did not show the lowest category in any of the metrics, and was proposed as the most superior demarcation option for the HTTR Heat Application Test Facility.

Kinetic analysis of mass transfer of Eu(III) in extractant-impregnated polymer-layered silica particle in multiple-ion distribution system

Miyagawa, Akihisa*; Hayashi, Naoki*; Iwamoto, Hibiki*; Arai, Tsuyoshi*; Nagatomo, Shigenori*; Miyazaki, Yasunori; Hasegawa, Kenta; Sano, Yuichi; Nakatani, Kiyoharu*

Analytical Sciences, 40(2), p.347 - 352, 2024/02

https://doi.org/10.1007/s44211-023-00462-x

The Eu(III) distribution mechanism in single extractant-impregnated polymer-layered silica particle in a complex solution containing multiple lanthanide ions was investigated using fluorescence microspectroscopy. The rate-determining step was the reaction of Eu(III) with the two extractant molecules. The obtained mechanism and rate constants agreed with those of the single-ion distribution system, in which Eu(III) was distributed to the particles in the Eu(III) solution.

Development of new data acquisition system for several beam monitors in J-PARC RCS

Yoshimoto, Masahiro; Takahashi, Hiroki; Harada, Hiroyuki; Chimura, Motoki; Fuwa, Yasuhiro; Hayashi, Naoki; Kuriyama, Yasutoshi*; Sawabe, Yuki*; Hatakeyama, Shuichiro*

Proceedings of 20th Annual Meeting of Particle Accelerator Society of Japan (Internet), p.839 - 843, 2023/11

https://www.pasj.jp/web_publish/pasj2023/proceedings/PDF/FRP0/FRP08.pdf

In the J -PARC 3GeV synchrotron accelerator (RCS), a new signal processing system for beam monitors is been developing to replace the existing system for the main beam monitors that monitor the stability of the accelerator: beam loss monitor, beam position monitor and beam current monitor. The new system will consist of a TAG server and an ADC module that can be used commonly for the three main monitors. The main design concepts of the new system are: (1) the TAG server divides various beam J-PARC tag information to each ADC module, (2) the ADC module converts acquisition data from beam monitors to digital signals by ADC and performs high-speed analysis by FPGA with switching analysis methods to suit each monitor, (3) the ADC module periodically outputs the analysis data with tag information by packing the signal processing data of all shots for about 10 seconds, and also outputs any one shot data on-demand, and (4) the raw waveform data, the latest four shots of FFT-related data in the process of analysis and bunch data for each cycle are stored in the internal memory of the ADC module, and the data can be read out as needed. In this presentation, we will report on the progress of the data acquisition test of tag information reading and beam monitor signals using the prototype under development.

Band gap formation in graphene by hybridization with Hex-Au(001) reconstructed surface

Terasawa, Tomoo; Matsunaga, Kazuya*; Hayashi, Naoki*; Ito, Takahiro*; Tanaka, Shinichiro*; Yasuda, Satoshi; Asaoka, Hidehito

Vacuum and Surface Science, 66(9), p.525 - 530, 2023/09

https://doi.org/10.1380/vss.66.525

As Au (001) surfaces exhibit a quasi-one-dimensional corrugated structure, Hex-Au(001), its periodicity was predicted to change the electronic structure of graphene when graphene was grown on this surface. Furthermore, the hybridization between graphene and Au is known to introduce bandgap and spin polarization into graphene. Here, we report angle-resolved photoemission spectroscopy and density functional theory calculation of graphene on a Hex-Au(001) surface. A bandgap of 0.2 eV in the graphene Dirac cone was observed at the crossing point of the graphene Dirac cone and Au 6sp bands, indicating that the origin of the bandgap formation was the hybridization between the graphene Dirac cone and Au 6sp band. We discussed the hybridization mechanism and anticipated spin injection into the graphene Dirac cone.

Physical property investigation of gloves for glove boxes in nuclear fuel reprocessing plants; Physical properties of used gloves and estimation of its life-time

Yamamoto, Masahiko; Nishida, Naoki; Kobayashi, Daisuke; Nemoto, Ryo*; Hayashi, Hiroyuki*; Kitao, Takahiko; Kuno, Takehiko

JAEA-Technology 2023-004, 30 Pages, 2023/06

JAEA-Technology-2023-004.pdf:1.94MB

Glove-box gloves, that are used for handling nuclear fuel materials at the Tokai Reprocessing Plant (TRP) of the Japan Atomic Energy Agency, have an expiration date by internal rules. All gloves are replaced at a maximum of every 4-year. However, degrees of glove deterioration varies depending on its usage environment such as frequency, chemicals, and radiation dose. Therefore, physical properties such as tensile strength, elongation, hardness of gloves are measured and technical evaluation method for the glove life-time is established. It was found that gloves without any defects in its appearance have enough physical properties and satisfies the acceptance criteria values of new gloves. Thus, it was considered that the expired gloves could be used for total of 8-year, by adding 4-year of new glove life-time. In addition, the results of extrapolation by plotting the glove's physical properties versus the used years showed that the physical properties at 8-year is on the safer side than the reported physical properties of broken glove. Also, the data are not significantly different from the physical properties of the long-term storage glove (8 and 23 years). Based on these results, life-time of gloves at TRP is set to be 8-year. The frequency of glove inspections are not changed, and if any defects is found, the glove is promptly replaced. Thus, the risk related to glove usage is not increased. The cost of purchasing gloves, labor for glove replacement, and the amount of generated waste can be reduced by approximately 40%, respectively, resulting in more efficient and rationalized glove management.

Development plan for coupling technology between high temperature gas-cooled reactor HTTR and Hydrogen Production Facility, 2; Development plan for coupling equipment between HTTR and Hydrogen Production Facility

Mizuta, Naoki; Morita, Keisuke; Aoki, Takeshi; Okita, Shoichiro; Ishii, Katsunori; Kurahayashi, Kaoru; Yasuda, Takanori; Tanaka, Masato; Isaka, Kazuyoshi; Noguchi, Hiroki; et al.

Proceedings of 30th International Conference on Nuclear Engineering (ICONE30) (Internet), 6 Pages, 2023/05

Band gap opening in graphene by hybridization with Au (001) reconstructed surfaces

Terasawa, Tomoo; Matsunaga, Kazuya*; Hayashi, Naoki*; Ito, Takahiro*; Tanaka, Shinichiro*; Yasuda, Satoshi; Asaoka, Hidehito

Physical Review Materials (Internet), 7(1), p.014002_1 - 014002_10, 2023/01

https://doi.org/10.1103/PhysRevMaterials.7.014002

Au(001) surfaces exhibit a complex reconstructed structure [Hex-Au(001)] comprising a hexagonal surface and square bulk lattices, yielding a quasi-one-dimensional corrugated surface. When graphene was grown on this surface, the periodicity of the corrugated surface was predicted to change the electronic structure of graphene, forming bandgaps and new Dirac points. Furthermore, the graphene-Au interface is promising for bandgap generation and spin injection due to band hybridization. Here, we report the angle-resolved photoemission spectroscopy and density functional calculation of graphene on a Hex-Au(001) surface. The crossing point of the original and replica graphene bands showed no bandgap, suggesting that the one-dimensional potential was too small to modify the electronic structure. A bandgap of 0.2 eV was observed at the crossing point of the graphene and Au bands, indicating that the bandgap is generated using hybridization of the graphene and Au bands. We discussed the hybridization mechanism and concluded that the R30 configuration between graphene and Au and an isolated electronic structure of Au are essential for effective hybridization between graphene and Au. We anticipate that hybridization between graphene and Au would result in spin injection into graphene.

Longitudinal measurement of high-intensity beam with bunch-shape monitor in front-end

Kitamura, Ryo; Hayashi, Naoki; Hirano, Koichiro; Miyao, Tomoaki*; Miura, Akihiko; Morishita, Takatoshi

Proceedings of 19th Annual Meeting of Particle Accelerator Society of Japan (Internet), p.212 - 214, 2023/01

In the J-PARC linac, the bunch-shape monitor (BSM) is developed to precisely and rapidly measure the longitudinal beam profile at the front-end, towards the improvement of the beam matching. The graphite target having the good strength to the high-power beam, has been introduced in order to resist the heat loading of the high-intensity beam. The resolution and other uncertainties were evaluated for the BSM. The longitudinal Twiss parameters and emittance were measured using the BSM and the IMPACT, which was the 3D particle-in-cell simulation code. The precision of the longitudinal emittance measurement was improved, by implementing uncertainties related to the BSM into the calculation. In this presentation, we will report a series of the measurement result, the method of the beam diagnostics with the BSM at the front-end, and the comparison between the measurement and the beam simulation.

Investigation of physical properties of glove for glove-box and estimation of its life-time

Kobayashi, Daisuke; Yamamoto, Masahiko; Nishida, Naoki; Miyoshi, Ryuta; Nemoto, Ryo*; Hayashi, Hiroyuki*; Kato, Keisuke; Nishino, Saki; Kuno, Takehiko; Kitao, Takahiko; et al.

Nihon Hozen Gakkai Dai-18-Kai Gakujutsu Koenkai Yoshishu, p.237 - 240, 2022/07

All gloves attached to glove-box in Tokai Reprocessing Plant have a fixed expiration date and have to be replaced every 4-year. However, degrees of glove deterioration are different depending on its usage environment (frequency, chemicals, radiation, etc.), because of rubber products. Therefore, physical properties such as tensile strength, elongation, hardness of gloves are measured, and the life-time of gloves are estimated. As a result, gloves without any defects in its appearance have enough physical property for acceptance criteria of new glove. The extrapolated physical property of glove is sufficiently larger than the reported values of damaged glove. No deterioration in physical properties of gloves, that are periodically replaced without any defects in its appearance, is observed and the usable life-time of the glove is estimated to be 8 years.

Synchronization system of ion source RF and cavity RF in J-PARC linac

Shibata, Takanori*; Hirano, Koichiro; Hirane, Tatsuya*; Shinto, Katsuhiro; Hayashi, Naoki; Oguri, Hidetomo

Proceedings of 18th Annual Meeting of Particle Accelerator Society of Japan (Internet), p.417 - 421, 2021/10

https://www.pasj.jp/web_publish/pasj2021/proceedings/PDF/TUP0/TUP006.pdf

In J-PARC linac, the operation of an rf-driven high-intensity H ion source was initiated in 2014. For plasma ignition, the 2-MHz rf amplifier outputs the power of several tens kW. However the rf amplifier for the ion source and those for the accelerating cavities have not been synchronized. As a result, the wave hights in the beam waveforms were different in shot by shot. Therefore, we have developed an synchronization system between the rf system for the ion source and those for the cavity systems and succeeded the same wave hights in the waveforms.