Giant barocaloric effects in sodium hexafluorophosphate and hexafluoroarsenate

Zhang, Z.*; Hattori, Takanori; Song, R.*; Yu, D.*; Mole, R.*; Chen, J.*; He, L.*; Zhang, Z.*; Li, B.*

Journal of Applied Physics, 136(3), p.035105_1 - 035105_8, 2024/07

https://doi.org/10.1063/5.0211085

Solid-state refrigeration using barocaloric materials is environmentally friendly and highly efficient, making it a subject of global interest over the past decade. Here, we report giant barocaloric effects in sodium hexafluorophosphate (NaPF) and sodium hexafluoroarsenate (NaAsF) that both undergo a cubic-to-rhombohedral phase transition near room temperature. We have determined that the low-temperature phase structure of NaPF is a rhombohedral structure with space group R and NaAsF, i.e., F, E, and A. The phase transition temperature varies with pressure at a rate of dT/dP = 250 and 310 K/GPa for NaPF and NaAsF. The pressure-induced entropy changes of NaPF and NaAsF are determined to be around 45.2 and 35.6J kgK, respectively. The saturation driving pressure is about 40 MPa. The pressure-dependent neutron powder diffraction suggests that the barocaloric effects are related to the pressure-induced cubic-to-rhombohedral phase transitions.

Patterns of gene content and co-occurrence constrain the evolutionary path toward animal association in Candidate Phyla Radiation bacteria

Jaffe, A. L.*; Thomas, A. D.*; He, C.*; Keren, R.*; Valentin-Alvarado, L. E.*; Munk, P.*; Bouma-Gregson, K.*; Farag, I. F.*; Amano, Yuki; Sachdeva, R.*; et al.

mBio, 12(4), p.e00521-21_1 - e00521-21_21, 2021/08

https://doi.org/10.1128/mBio.00521-21

Simultaneous determination of neutron-induced fission and radiative capture cross sections from decay probabilities obtained with a surrogate reaction

Prez Snchez, R.*; Jurado, B.*; Mot, V.*; Roig, O.*; Dupuis, M.*; Bouland, O.*; Denis-Petit, D.*; Marini, P.*; Mathieu, L.*; Tsekhanovich, I.*; et al.

Physical Review Letters, 125(12), p.122502_1 - 122502_5, 2020/09

https://doi.org/10.1103/PhysRevLett.125.122502

In-source laser spectroscopy of dysprosium isotopes at the ISOLDE-RILIS

Chrysalidis, K.*; Barzakh, A. E.*; Ahmed, R.*; Andreyev, A. N.; Ballof, J.*; Cubiss, J. G.*; Fedorov, D. V.*; Fedosseev, V. N.*; Fraile, L. M.*; Harding, R. D.*; et al.

Nuclear Instruments and Methods in Physics Research B, 463, p.472 - 475, 2020/01

https://doi.org/10.1016/j.nimb.2019.04.021

A number of radiogenically produced dysprosium isotopes have been studied by in-source laser spectroscopy at ISOLDE using the Resonance Ionization Laser Ion Source (RILIS). Isotope shifts were measured relative to Dy in the (gs) (418.8 nm )resonance transition. The electronic factor, , and mass shift factor, M, were extracted and used for determining the changes in mean-squared charge radii for Dy and Dy for the first time.

-decay branching ratio of Pt

Cubiss, J. G.*; Harding, R. D.*; Andreyev, A. N.; Althubiti, N.*; Andel, B.*; Antalic, S.*; Barzakh, A. E.*; Cocolios, T. E.*; Day Goodacre, T.*; Farooq-Smith, G. J.*; et al.

Physical Review C, 101(1), p.014314_1 - 014314_4, 2020/01

https://doi.org/10.1103/PhysRevC.101.014314

The -decay branching ratio of 0.52(5)% from the ground state of Pt to the ground state of the daughter nucleus Os has been determined more precisely than before. The Pt was produced as the -decay granddaughter of Hg which was produced and separated with the CERN-ISOLDE facility. The reduced -decay width calculated with the present result has provided a new picture of the systematics for the -decay width of neutron-deficient Pt isotopes.

Study of medium-spin states of neutron-rich Rb isotopes

Torres, D. A.*; Chapman, R.*; Kumar, V.*; Hadinia, B.*; Hodsdon, A.*; Labiche, M.*; Liang, X.*; O'Donnell, D.*; Ollier, J.*; Orlandi, R.; et al.

European Physical Journal A, 55(9), p.158_1 - 158_21, 2019/09

https://doi.org/10.1140/epja/i2019-12839-6

Fine structure in the decay of At

Cubiss, J. G.*; Andreyev, A. N.; Barzakh, A. E.*; Andel, B.*; Antalic, S.*; Cocolios, T. E.*; Day Goodacre, T.*; Fedorov, D. V.*; Fedosseev, V. N.*; Ferrer, R.*; et al.

Physical Review C, 99(6), p.064317_1 - 064317_6, 2019/06

https://doi.org/10.1103/PhysRevC.99.064317

An decay of At was studied at the CERN-ISOLDE facility using a laser-ionization technique. Coincidence - data were collected for the first time and a more precise half-life value of T = 1.27(6) s was measured. A new -decay scheme was deduced based on the fine-structure of the decay. The results lead to a preferred spin and parity assignment of J = (3) for the ground state of At; however, J = (2) cannot be fully excluded.

Study of fission using multi-nucleon transfer reactions

Nishio, Katsuhisa; Hirose, Kentaro; Vermeulen, M. J.; Makii, Hiroyuki; Orlandi, R.; Tsukada, Kazuaki; Asai, Masato; Toyoshima, Atsushi; Sato, Tetsuya; Nagame, Yuichiro; et al.

EPJ Web of Conferences, 163, p.00041_1 - 00041_6, 2017/11

https://doi.org/10.1051/epjconf/201716300041

Study of fission using multi-nucleon transfer reactions

Nishio, Katsuhisa; Hirose, Kentaro; Lguillon, R.*; Makii, Hiroyuki; Orlandi, R.; Tsukada, Kazuaki; Smallcombe, J.*; Chiba, Satoshi*; Aritomo, Yoshihiro*; Tanaka, Shoya*; et al.

Proceedings of 6th International Conference on Fission and Properties of Neutron-rich Nuclei (ICFN-6), p.590 - 597, 2017/11

https://doi.org/10.1142/9789813229426_0101

Measurement of high-energy prompt -rays from neutron induced fission of U-235

Makii, Hiroyuki; Nishio, Katsuhisa; Hirose, Kentaro; Orlandi, R.; Lguillon, R.; Ogawa, Tatsuhiko; Soldner, T.*; Hambsch, F.-J.*; Astier, A.*; Pollitt, A.*; et al.

EPJ Web of Conferences, 146, p.04036_1 - 04036_4, 2017/09

https://doi.org/10.1051/epjconf/201714604036

The measurement of the prompt fission -ray spectrum (PFGS) is quite important to study the de-excitation process of neutron-rich fission fragments as well as to generate data required to design a generation-IV reactors. The PFGS measured for spontaneous fission of Cf shows a broad hump at energies more than 8 MeV. This is interpreted as a giant dipole resonance (GDR) of the fragments centered around 15 MeV. To understand how the GDR is populated in the fission process, one needs to measure the PFGS for the reactions with the mass yields different from the spontaneous fission of Cf, such as (n,f). The measurements of the PFGS for (n,f), however, are limited less than 9 MeV even in the recent experiment. This prompts us to make a new measurement to extend the know PFGS up to 20 MeV. The measurement has been carried out at the PF1B beam line of Institut Laue-Langevin. In this contribution we will present the results obtained the measurement.