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Journal Articles

A Spectrometer for rayleigh scattering of M${"o}$ssbauer radiation using synchrotron radiation

Masuda, Ryo; Mitsui, Takaya; Kobayashi, Yasuhiro*; Higashitaniguchi, Satoshi*; Seto, Makoto

Japanese Journal of Applied Physics, 48(12), p.120221_1 - 120221_3, 2009/12

 Times Cited Count:9 Percentile:36.02(Physics, Applied)

A neV-resolution spectrometer using 14.4 keV synchrotron-based $$^{57}$$Fe M${"o}$ssbauer radiation has been developed to observe the quasi-elastic scattering by condensed matter. It consists of a $$^{57}$$Fe$$_2$$O$$_3$$ nuclear resonant Bragg monochromator and a $$^{57}$$Fe stainless steel nuclear analyzer. As a feasibility study, the quasi-elastic scattering by supercooled glycerol near its melting point has been observed. The instrumental function of the spectrometer was 42.2 neV. The energy broadening of 11 neV due to the quasi-elastic scattering was observed.

Journal Articles

Synchrotron-radiation-based M$"o$ssbauer spectroscopy

Seto, Makoto; Masuda, Ryo; Higashitaniguchi, Satoshi*; Kitao, Shinji*; Kobayashi, Yasuhiro*; Inaba, Chika*; Mitsui, Takaya; Yoda, Yoshitaka*

Physical Review Letters, 102(21), p.217602_1 - 217602_4, 2009/05

 Times Cited Count:58 Percentile:87.91(Physics, Multidisciplinary)

We have developed a new method that yields M$"o$ssbauer absorption spectra using synchrotron radiation (SR); this method is applicable for almost all M$"o$ssbauer nuclides including those that cannot be measured by previous methods using radioisotope (RI) sources. The M$"o$ssbauer spectrum of the 68.752 keV excited state of $$^{73}$$Ge, which cannot be measured using a RI source, was measured using SR. Our results show that this method can be used to perform advanced M$"o$ssbauer spectroscopy measurements owing to the excellent features of SR.

Journal Articles

Development of neV-resolution spectroscopy using synchrotron-based $$^{57}$$Fe M$"o$ssbauer radiation

Masuda, Ryo; Mitsui, Takaya; Kitao, Shinji*; Higashitaniguchi, Satoshi*; Yoda, Yoshitaka*; Seto, Makoto

Japanese Journal of Applied Physics, 47(10), p.8087 - 8090, 2008/10

 Times Cited Count:13 Percentile:46.42(Physics, Applied)

A synchrotron-radiation-based neV-resolution spectrometer has been developed using single-line pure nuclear Bragg reflection. The developed optical system consists of two components: a $$^{57}$$FeBO$$_{3}$$ single crystal near the N$'e$el temperature for producing $$^{57}$$Fe M$"o$ssbauer radiation from synchrotron radiation, and a single-line M$"o$ssbauer absorber ($$^{57}$$Fe-enriched stainless steel foil) for analyzing the energy distribution. As a feasibility study, we have performed the measurement of the M$"o$ssbauer radiation diffracted by a Si crystal under ultrasound vibration with the optical system and have successfully observed the neV-range energy modulation due to the ultrasound vibration.

Journal Articles

Ultrahigh-pressure measurement in the multimegabar range by energy-domain synchrotron radiation $$^{57}$$Fe-M$"o$ssbauer spectroscopy using focused X-rays

Mitsui, Takaya; Seto, Makoto; Hirao, Naohisa*; Oishi, Yasuo*; Kobayashi, Yasuhiro*; Higashitaniguchi, Satoshi*; Masuda, Ryo*

Japanese Journal of Applied Physics, Part 2, 46(16), p.L382 - L384, 2007/04

 Times Cited Count:12 Percentile:44.00(Physics, Applied)

Energy-domain synchrotron radiation M$"o$ssbauer spectroscopy was performed by a single-line M$"o$ssbauer filtering technique and focusing X-ray optics. Pure nuclear Bragg reflection from a heated $$^{57}$$FeBO$$_{3}$$ single crystal was used for a neV order bandwidth ultrahigh energy resolution X-ray analyzer. As an example of small target research, the M$"o$ssbauer transmission spectrum of polycrystalline iron metal was observed using a diamond anvil cell at multimegabar pressures (252 GPa) for the first time.

Journal Articles

Generation and application of ultrahigh monochromatic X-ray using high-quality $$^{57}$$FeBO$$_{3}$$ single crystal

Mitsui, Takaya; Seto, Makoto; Kikuta, Seishi*; Hirao, Naohisa*; Oishi, Yasuo*; Takei, Fumihiko*; Kobayashi, Yasuhiro*; Kitao, Shinji*; Higashitaniguchi, Satoshi*; Masuda, Ryo*

Japanese Journal of Applied Physics, Part 1, 46(2), p.821 - 825, 2007/02

 Times Cited Count:34 Percentile:74.61(Physics, Applied)

Ultrahigh monochromatic 14.4 keV X-rays with a narrow bandwidth of 15.4 neV were generated successfully with a high counting rate of 12,000 counts/s at the undulator beamline (BL11XU) of SPring-8. It was achieved by combining an intense X-ray from the third generation synchrotron radiation facility SPring-8 and pure nuclear Bragg scattering of a very highquality $$^{57}$$FeBO$$_{3}$$ perfect single crystal at the N$'e$el temperature. We describe the detailed study of the beam characteristics and some performance test experiments of energy-domain synchrotron radiation M$"o$ssbauer spectroscopy, including a highpressure experiment using a diamond anvil cel.

Journal Articles

High-energy-resolution monochromator for nuclear resonant scattering of synchrotron radiation by Te-125 at 35.49 keV

Imai, Yasuhiko*; Yoda, Yoshitaka*; Kitao, Shinji*; Masuda, Ryo; Higashitaniguchi, Satoshi*; Inaba, Chika*; Seto, Makoto

Advances in X-ray/EUV Optics and Components II (Proceedings of SPIE Vol.6705), p.670512_1 - 670512_7, 2007/00

We have developed a high-resolution monochromator (HRM) for the measurement of nuclear resonant scattering of synchrotron radiation by $$^{125}$$Te at 35.49 keV using the backscattering of sapphire (9 1 -10 68). The relative energy resolution of $$2.1times10^{-7}$$ is achieved, that is 7.5 meV in energy bandwidth. A new HRM has been desired at this energy region because of the low efficiency of usual Si HRMs. This HRM opens studies on element-specific dynamics and electronic state of substances containing $$^{125}$$Te.

Journal Articles

Nuclear resonant scattering of synchrotron radiation by Yb nuclides

Masuda, Ryo*; Higashitaniguchi, Satoshi*; Kitao, Shinji*; Kobayashi, Yasuhiro*; Seto, Makoto*; Mitsui, Takaya; Yoda, Yoshitaka*; Haruki, Rie*; Kishimoto, Shunji*

Journal of the Physical Society of Japan, 75(9), p.094716_1 - 094716_4, 2006/09

 Times Cited Count:2 Percentile:19.25(Physics, Multidisciplinary)

no abstracts in English

Oral presentation

Development of energy variable nuclear monochromator

Mitsui, Takaya; Seto, Makoto; Higashitaniguchi, Satoshi*

no journal, , 

no abstracts in English

Oral presentation

neV-Range inelastic scattering spectroscopy using single-line pure nuclear bragg reflection of synchrotron radiation

Masuda, Ryo; Mitsui, Takaya; Kitao, Shinji*; Higashitaniguchi, Satoshi*; Yoda, Yoshitaka*; Seto, Makoto

no journal, , 

no abstracts in English

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