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Journal Articles

Revising the 4${it f}$ symmetry in CeCu$$_{2}$$Ge$$_{2}$$; Soft X-ray absorption and hard X-ray photoemission spectroscopy

Aratani, Hidekazu*; Nakatani, Yasuhiro*; Fujiwara, Hidenori*; Kawada, Moeki*; Kanai, Yuina*; Yamagami, Kohei*; Fujioka, Shuhei*; Hamamoto, Satoru*; Kuga, Kentaro*; Kiss, Takayuki*; et al.

Physical Review B, 98(12), p.121113_1 - 121113_6, 2018/09

AA2018-0352.pdf:1.16MB

 Times Cited Count:3 Percentile:24.8(Materials Science, Multidisciplinary)

Journal Articles

Probing strongly correlated 4$$f$$-orbital symmetry of the ground state in Yb compounds by linear dichroism in core-level photoemission

Mori, Takeo*; Kitayama, Satoshi*; Kanai, Yuina*; Naimen, Sho*; Fujiwara, Hidenori*; Higashiya, Atsushi*; Tamasaku, Kenji*; Tanaka, Arata*; Terashima, Kensei*; Imada, Shin*; et al.

Journal of the Physical Society of Japan, 83(12), p.123702_1 - 123702_5, 2014/12

 Times Cited Count:15 Percentile:71.43(Physics, Multidisciplinary)

We show that the strongly correlated 4$$f$$-orbital symmetry of the ground state is revealed by linear dichroism in core-level photoemission spectra, as we have discovered for YbRh$$_{2}$$Si$$_{2}$$ and YbCu$$_{2}$$Si$$_{2}$$. Theoretical analysis shows us that the linear dichroism reflects the anisotropic charge distributions resulting from a crystalline electric field. We have successfully determined the ground-state 4$$f$$ symmetry for both compounds from the polarization-dependent angle resolved core-level spectra at a temperature well below the first excitation energy. The excited-state symmetry is also probed by temperature dependence of the linear dichroism where the high measurement temperatures are on the order of the crystal-field-splitting energies.

Journal Articles

XUV-FEL spectroscopy; He two-photon ionization cross-sections

Sato, Takahiro*; Iwasaki, Atsushi*; Ishibashi, Kazuki*; Okino, Tomoya*; Yamanouchi, Kaoru*; Adachi, Junichi*; Yagishita, Akira*; Yazawa, Hiroki*; Kannari, Fumihiko*; Aoyama, Makoto; et al.

Europhysics News, 42(5), P. 10, 2011/09

The resonant and non-resonant two-photon single ionization processes of He were investigated using intense free electron laser light in the extreme ultraviolet (XUV) region (53.4-61.4 nm) covering the 1s-2p and 1s-3p resonant transitions of He. On the basis of the dependences of the yield of He$$^{+}$$ on the XUV light-field intensity at 53.4, 58.4, 56.0 and 61.4 nm, the absolute values of the two-photon ionization cross sections of He at the four different wavelengths and their dependence on the light-field intensity were determined for the first time.

Journal Articles

Determination of the absolute two-photon ionization cross section of He by an XUV free electron laser

Sato, Takahiro*; Iwasaki, Atsushi*; Ishibashi, Kazuki*; Okino, Tomoya*; Yamanouchi, Kaoru*; Adachi, Junichi*; Yagishita, Akira*; Yazawa, Hiroki*; Kannari, Fumihiko*; Aoyama, Makoto; et al.

Journal of Physics B; Atomic, Molecular and Optical Physics, 44(16), p.161001_1 - 161001_5, 2011/08

 Times Cited Count:33 Percentile:84.31(Optics)

The resonant and non-resonant two-photon single ionization processes of He were investigated using intense free electron laser light in the extreme ultraviolet (XUV) region (53.4-61.4 nm) covering the 1s-2p and 1s-3p resonant transitions of He. On the basis of the dependences of the yield of He$$^{+}$$ on the XUV light-field intensity at 53.4, 58.4, 56.0 and 61.4 nm, the absolute values of the two-photon ionization cross sections of He at the four different wavelengths and their dependence on the light-field intensity were determined for the first time.

Journal Articles

Photoemission spectroscopy and X-ray absorption spectroscopy studies of the superconducting pyrochlore oxide Cd$$_{2}$$Re$$_{2}$$O$$_{7}$$

Irizawa, Akinori*; Higashiya, Atsushi*; Kasai, Shuichi*; Sasabayashi, Takehisa*; Shigemoto, Akihiko*; Sekiyama, Akira*; Imada, Shin*; Suga, Shigemasa*; Sakai, Hironori; Ono, Hiroyuki*; et al.

Journal of the Physical Society of Japan, 75(9), p.094701_1 - 094701_5, 2006/09

 Times Cited Count:6 Percentile:43.33(Physics, Multidisciplinary)

Photoemission spectroscopy (PES) and O $$1s$$ X-ray absorption spectroscopy (XAS) measurements have been performed for Cd$$_2$$ Re$$_2$$ O$$_7$$ single crystals. Temperature variations of their spectra reveal that the phase transition at 120 K directly changes the band structure near the Fermi level compared with another transition near 200 K. The roles of the transitions are discussed in terms of the changes in the Re-O orbital hybridization.

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