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Journal Articles

Neutron imaging of generated water inside polymer electrolyte fuel cell using newly-developed gas diffusion layer with gas flow channels during power generation

Nasu, Mitsunori*; Yanai, Hiroshi*; Hirayama, Naoki*; Adachi, Hironori*; Kakizawa, Yu*; Shirase, Yuto*; Nishiyama, Hiromichi*; Kawamoto, Teppei*; Inukai, Junji*; Shinohara, Takenao; et al.

Journal of Power Sources, 530, p.231251_1 - 231251_11, 2022/05

 Times Cited Count:9 Percentile:88.61(Chemistry, Physical)

Journal Articles

Estimation of I-131 concentration using time history of pulse height distribution at monitoring post and detector response for radionuclide in plume

Hirayama, Hideo*; Kawasaki, Masatsugu; Matsumura, Hiroshi*; Okura, Takehisa; Namito, Yoshihito*; Sanami, Toshiya*; Taki, Mitsumasa; Oishi, Tetsuya; Yoshizawa, Michio

Insights Concerning the Fukushima Daiichi Nuclear Accident, Vol.4; Endeavors by Scientists, p.295 - 307, 2021/10

Journal Articles

Beta decay of the axially asymmetric ground state of $$^{192}$$Re

Watanabe, Hiroshi*; Watanabe, Yutaka*; Hirayama, Yoshikazu*; Andreyev, A. N.; Hashimoto, Takashi*; Kondev, F. G.*; Lane, G. J.*; Litvinov, Yu. A.*; Liu, J. J.*; Miyatake, Hiroari*; et al.

Physics Letters B, 814, p.136088_1 - 136088_6, 2021/03

 Times Cited Count:1 Percentile:48.27(Astronomy & Astrophysics)

Journal Articles

Enhancement of element production by incomplete fusion reaction with weakly bound deuteron

Wang, H.*; Otsu, Hideaki*; Chiga, Nobuyuki*; Kawase, Shoichiro*; Takeuchi, Satoshi*; Sumikama, Toshiyuki*; Koyama, Shumpei*; Sakurai, Hiroyoshi*; Watanabe, Yukinobu*; Nakayama, Shinsuke; et al.

Communications Physics (Internet), 2(1), p.78_1 - 78_6, 2019/07

 Times Cited Count:7 Percentile:56.64(Physics, Multidisciplinary)

Searching for effective pathways for the production of proton- and neutron-rich isotopes through an optimal combination of reaction mechanism and energy is one of the main driving forces behind experimental and theoretical nuclear reaction studies as well as for practical applications in nuclear transmutation of radioactive waste. We report on a study on incomplete fusion induced by deuteron, which contains one proton and one neutron with a weak binding energy and is easily broken up. This reaction study was achieved by measuring directly the cross sections for both proton and deuteron for $$^{107}$$Pd at 50 MeV/u via inverse kinematics technique. The results provide direct experimental evidence for the onset of a cross-section enhancement at high energy, indicating the potential of incomplete fusion induced by loosely-bound nuclei for creating proton-rich isotopes and nuclear transmutation of radioactive waste.

Journal Articles

Investigation of main radiation source above shield plug of Unit 3 at Fukushima Daiichi Nuclear Power Station

Hirayama, Hideo*; Kondo, Kenjiro*; Suzuki, Seishiro*; Tanimura, Yoshihiko; Iwanaga, Kohei*; Nagata, Hiroshi*

EPJ Web of Conferences, 153, p.08010_1 - 08010_3, 2017/09

 Times Cited Count:1 Percentile:61.28

Pulse height distributions were measured using a CdZnTe detector inside a lead collimator to investigate main source producing high dose rates above the shield plugs of Unit 3 at Fukushima Daiichi Nuclear Power Station. It was confirmed that low energy photons are dominant. Concentrations of Cs-137 under 60 cm concrete of the shield plug were estimated to be between 8.1$$times$$10$$^9$$ and 5.7$$times$$10$$^{10}$$ Bq/cm$$^2$$ from the measured peak count rate of 0.662 MeV photons. If Cs-137 was distributed on the surfaces of the gaps of the shied plugs with radius 6 m and with the averaged concentration of 5 points, 2.6$$times$$10$$^{10}$$ Bq/cm$$^2$$, total amount of Cs-137 is estimated to be 30 PBq.

Journal Articles

New measurement of the $$^{8}$$Li($$alpha$$,n)$$^{11}$$B reaction in a lower-energy region below the Coulomb barrier

Das, S. K.*; Fukuda, Tomokazu*; Mizoi, Yutaka*; Ishiyama, Hironobu*; Miyatake, Hiroari*; Watanabe, Yutaka*; Hirayama, Yoshikazu*; Jeong, S. C.*; Ikezoe, Hiroshi*; Matsuda, Makoto; et al.

Physical Review C, 95(5), p.055805_1 - 055805_4, 2017/05

 Times Cited Count:1 Percentile:27.8(Physics, Nuclear)

Journal Articles

Overview of JENDL-4.0/HE and benchmark calculations

Kunieda, Satoshi; Iwamoto, Osamu; Iwamoto, Nobuyuki; Minato, Futoshi; Okamoto, Tsutomu; Sato, Tatsuhiko; Nakashima, Hiroshi; Iwamoto, Yosuke; Iwamoto, Hiroki; Kitatani, Fumito; et al.

JAEA-Conf 2016-004, p.41 - 46, 2016/09

Neutron- and proton-induced cross-section data are required in a wide energy range beyond 20 MeV, for the design of accelerator applications. New evaluations are performed with recent knowledge in the optical and pre-equilibrium model calculations. We also evaluated cross-sections for p+$$^{6,7}$$Li and p+$$^{9}$$Be which have been highly requested from a medical field. The present high-energy nuclear data library, JENDL-4.0/HE, includes evaluated cross-sections for incident neutrons and protons up to 200 MeV (for about 130 nuclei). We overview substantial features of the library, i.e., (1) systematic evaluation with CCONE code, (2) challenges for evaluations of light nuclei and (3) inheritance of JENDL-4.0 and JENDL/HE-2007. In this talk, we also focus on the results of benchmark calculation for neutronics to show performance of the present library.

Journal Articles

Progress and prospects of calculation methods for radiation shielding

Hirayama, Hideo*; Nakashima, Hiroshi; Morishima, Makoto*; Uematsu, Mikio*; Sato, Osamu*

Journal of Nuclear Science and Technology, 52(11), p.1339 - 1361, 2015/11

AA2014-0681.pdf:1.15MB

 Times Cited Count:6 Percentile:20.83(Nuclear Science & Technology)

Progress in calculation methods for radiation shielding are reviewed based on basis of the activities of research committees related to radiation shielding fields established in the Atomic Energy Society of Japan. A technological roadmap for the field of radiation shielding, progress and prospects for specific shielding calculation methods such as the Monte Carlo, discrete ordinate Sn transport, and simplified methods, and shielding experiments used to validate calculation methods are presented in this paper.

Journal Articles

Interaction of double-stranded DNA with polymerized PprA protein from ${it Deinococcus radiodurans}$

Adachi, Motoyasu; Hirayama, Hiroshi; Shimizu, Rumi; Sato, Katsuya; Narumi, Issey*; Kuroki, Ryota

Protein Science, 23(10), p.1349 - 1358, 2014/10

 Times Cited Count:9 Percentile:25.73(Biochemistry & Molecular Biology)

Pleiotropic protein promoting DNA repair A (PprA) is a key protein that facilitates the extreme radioresistance of ${it Deinococcus radiodurans}$. To clarify the role of PprA in the radioresistance mechanism, the interaction between recombinant PprA expressed in Escherichia coli with several double-stranded DNAs was investigated. In a gel-shift assay, the band shift of supercoiled pUC19 DNA caused by the binding of PprA showed a bimodal distribution, which was promoted by the addition of 1 mM Mg, Ca, or Sr ions. The dissociation constant of the PprA-supercoiled pUC19 DNA complex, calculated from the relative portions of shifted bands, was 0.6 $$mu$$M with a Hill coefficient of 3.3 in the presence of 1 mM Mg acetate. This indicates that at least 281 PprA molecules are required to saturate a supercoiled pUC19 DNA, which is consistent with the number of bound PprA molecules estimated by the UV absorption of the PprA-pUC19 complex purified by gel filtration. This saturation also suggests linear polymerization of PprA along the dsDNA. On the other hand, the bands of linear dsDNA and nicked circular dsDNA that eventually formed PprA complexes did not saturate, but created larger molecular complexes when the PprA concentration was greater than 1.3 $$mu$$M. This result implies that DNA-bound PprA aids association of the termini of damaged DNAs, which is regulated by the concentration of PprA.

Journal Articles

Estimation of I-131 concentration using time history of pulse height distribution at monitoring post and detector response for radionuclide in plume

Hirayama, Hideo*; Kawasaki, Masatsugu; Matsumura, Hiroshi*; Okura, Takehisa; Namito, Yoshihito*; Sanami, Toshiya*; Taki, Mitsumasa; Oishi, Tetsuya; Yoshizawa, Michio

Nihon Genshiryoku Gakkai Wabun Rombunshi, 13(3), p.119 - 126, 2014/09

A method of deducing the I-131 concentration in a radioactive plume from the time history of peak count rates determined from pulse height spectra obtained from an NaI(Tl)scintillation detector employed as a detector of a monitoring post was presented. The concentrations of I-131 in the plumes were estimated from the count rates using the calculated response of the NaI(Tl) detector with egs5 for a model of a plume uniformly containing I-131. This method was applied to the data from the monitoring posts at Nuclear Science Research Institutes of Japan Atomic Energy Agency (JAEA). The estimated time history variation of I-131 concentrations in plumes was in fair agreement with those measured directly by an air sampling method. The difference was less than a factor of 4 for plumes that arrived on March 15 and March 21, indicating relatively high I-131 concentrations among the plumes studied in this work.

JAEA Reports

Annual report of Nuclear Emergency Assistance and Training Center (April 1, 2012 - March 31, 2013)

Sato, Takeshi; Muto, Shigeo; Okuno, Hiroshi; Katagiri, Hiromi; Akiyama, Kiyomitsu; Okamoto, Akiko; Koie, Masahiro; Ikeda, Takeshi; Nemotochi, Toshimasa; Saito, Toru; et al.

JAEA-Review 2013-046, 65 Pages, 2014/02

JAEA-Review-2013-046.pdf:11.18MB

When a nuclear emergency occurs in Japan, the Japan Atomic Energy Agency (JAEA) has the responsibility of providing technical support to the National government, local governments, police, fire stations and nuclear operators etc., because the JAEA has been designated as the Designated Public Institution under the Basic Act on Disaster Control Measures and the Act on Response to Armed Attack Situations, etc.. The Nuclear Emergency Assistance and Training Center (NEAT) of JAEA provides a comprehensive range of technical support activities to an Off-Site Center in case of a nuclear emergency. Specifically, NEAT gives technical advice and information, dispatches specialists as required, and supplies the National Government and local governments with emergency equipments and materials. NEAT provides various exercise and training courses concerning nuclear disaster prevention to those personnel taking an active part in emergency response organizations at normal times. The tasks of NEAT, with its past experiences as a designated public institution including the responses to TEPCO's Fukushima Accident, have been shifted to technical supports to the national government for strengthening its abilities to emergency responses; the NEAT therefore focused on maintenance and operation of its functions, and strengthening its response abilities in cooperation with the national government. This annual report summarized these activities of JAEA/NEAT in the fiscal year 2012.

Journal Articles

The Concept of dose system for radiological protection

Hirayama, Hideo*; Nakashima, Hiroshi; Sanami, Toshiya*; Yamaguchi, Yasuhiro; Sato, Osamu*; Takagi, Shunji*; Suzuki, Toshikazu*; Iwai, Satoshi*

Nihon Genshiryoku Gakkai-Shi ATOMO$$Sigma$$, 55(2), p.83 - 96, 2013/02

Since the accident at the Fukushima Daiichi Power Plant, units of radiation doses such as Sv have been frequently reported by newspapers. However, it is not exactly understood even by experts on nuclear engineering that there are two different concepts which are the protection quantity such as the effective dose related to a radiation health risk and the practical quantity such as ambient dose equivalents related to measurements. In this special issue, Radiological Protection Quantity, and Operational Quantity and Radiological Protection Quantity, explain the radiation protection dose system including the protection and practical quantities established by ICRP and ICRU. Relation between Dosimeters used at Fukushima etc. and Radiological Protection Quantity describes a method and its problems to measure radiations from Cs on surface and underground using survey meters and personal dosimeters, and convert the measured values to effective doses.

Journal Articles

Fitting method for spectrum deduction in high-energy neutron field induced by GeV-protons using experimental reaction-rate data

Kasugai, Yoshimi; Matsuda, Norihiro; Sakamoto, Yukio; Nakashima, Hiroshi; Yashima, Hiroshi*; Matsumura, Hiroshi*; Iwase, Hiroshi*; Hirayama, Hideo*; Mokhov, N.*; Leveling, A.*; et al.

Reactor Dosimetry; 14th International Symposium (ASTM STP 1550), p.675 - 689, 2012/08

Under the collaborative study project of JASMIN, shielding experiments has been carried out using the anti-proton target station (Pbar) of Fermilab. In the experiment, the multi-foil activation technique was utilized, and the neutron spectra in high-energy region between 1 and 100 MeV were deduced by using the "fitting method", which is newly developed. In this method, we made an assumption that neutron energy spectra could be expressed with a simple function. The validity of the fitting method was confirmed by comparison with the results of the unfolding method and the theoretical calculations. Finally, it was found that there are simple correlations between reaction rates and the adjusting parameters in the fitting function. The correlations are useful for estimating the adjusting parameters easily, and a neutron spectrum in the high-energy region can be deduced from a set of reaction-rate data without the complicated calculations of unfolding.

Journal Articles

Shielding experiments under JASMIN collaboration at Fermilab, 4; Measurement and analyses of high-energy neutron spectra in the anti-proton target station

Matsuda, Norihiro; Kasugai, Yoshimi; Sakamoto, Yukio; Nakashima, Hiroshi; Matsumura, Hiroshi*; Iwase, Hiroshi*; Kinoshita, Norikazu*; Hirayama, Hideo*; Yashima, Hiroshi*; Mokhov, N.*; et al.

Journal of the Korean Physical Society, 59(2), p.2055 - 2058, 2011/08

 Times Cited Count:0 Percentile:0(Physics, Multidisciplinary)

It is important to obtain neutron spectra and its intensity on shielding experiment. Deduction of high-energy neutron spectra were done using fitting and unfolding methods based on the shielding data obtained at the anti-proton (pbar) target station in Fermilab. The neutron spectra for fitting method is useful to be easily obtained and the values gave reasonable results compared with nuclear data. Therefore, that for unfolding methods included inconsistency. Furthermore, the deduced neutron spectra were verified through the calculation analyses by PHITS code.

Journal Articles

Shielding experiments at high energy accelerators of Fermilab, 2; Spatial distribution measurement of reaction rate behind the shield and its application for Moyer model

Yashima, Hiroshi*; Kasugai, Yoshimi; Matsuda, Norihiro; Matsumura, Hiroshi*; Iwase, Hiroshi*; Kinoshita, Norikazu*; Mokhov, N.*; Leveling, A.*; Boehnlein, D.*; Vaziri, K.*; et al.

Progress in Nuclear Science and Technology (Internet), 1, p.48 - 51, 2011/02

The shielding experiment was performed at the anti-proton production target station in Fermi National Accelerator Laboratory. Aluminum, Bismath, Niobium, Copper and Indium samples were placed behind the shields. After irradiation, induced activities of samples were measured by using HPGe detector. The spatial distribution of reaction rate of samples which were placed behind the iron and concrete shields were obtained. The measured data shows that the reaction rates on the outer surfaces of the iron and concrete shields increases toward the downstream of the target. The obtained reaction rates were also fitted to Moyer's formula, and the attenuation lengths for iron and concrete shields were obtained.

Journal Articles

Shielding experiments at high energy accelerators of Fermilab, 3; Neutron spectrum measurements in intense pulsed neutron fields of the 120-GeV proton facility using a current Bonner sphere technique

Hagiwara, Masayuki*; Sanami, Toshiya*; Iwamoto, Yosuke; Arakawa, Hiroyuki*; Shigyo, Nobuhiro*; Mokhov, N.*; Leveling, A.*; Boehnlein, D.*; Vaziri, K.*; Nakamura, Takashi*; et al.

Progress in Nuclear Science and Technology (Internet), 1, p.52 - 56, 2011/02

In pbar target station, the pulsed proton beam with the power of around 75 kW and the time structure of 1.6 $$mu$$s pulse width and 2.2 s cycle time bombards the pbar production target and produces high instantaneous intensity neutron (burst neutron) fields. The duration of the burst neutrons, which is less than $$mu$$s, is very severe condition to measure neutron spectra with a conventional Bonner sphere technique with pulse readout electronics because of signal pile-up problem. In this study, we have developed a current readout Bonner sphere technique to measure neutron spectra in a burst neutron field. We have measured the neutron spectra on the pbar target and graphite dump. The neutron spectra obtained with the present technique show generally good agreements with the calculation results using MARS code except difference of the thermal neutron flux due to the geometrical problem.

Journal Articles

Shielding experiments at high energy accelerators of Fermilab, 4; Calculation analyses

Matsuda, Norihiro; Kasugai, Yoshimi; Matsumura, Hiroshi*; Yashima, Hiroshi*; Iwase, Hiroshi*; Kinoshita, Norikazu*; Sanami, Toshiya*; Mokhov, N.*; Leveling, A.*; Boehnlein, D.*; et al.

Progress in Nuclear Science and Technology (Internet), 1, p.57 - 60, 2011/02

The anti-proton (pbar) production target in Fermi National Accelerator Laboratory can be produced a wide variety of secondary particles including of anti-protons, by bombarding with protons accelerated to 120 GeV. The shielding experimental data, which was obtained around the pbar target, make possible to validate the accuracies of the general-purpose Monte Carlo simulation codes. In this paper, spatial distribution of reaction rates were calculated with two-dimensional (r-z) geometry simplified the real pbar target station using the PHITS, MARS and MCNPX code. These experimental data in iron shield were compared with the calculated data. The comparison for attenuation length of iron were good agreement between the experiments and calculations.

Journal Articles

Barrier distribution of quasi-elastic backward scattering in very heavy reaction systems

Mitsuoka, Shinichi; Ikezoe, Hiroshi; Nishio, Katsuhisa; Watanabe, Yutaka*; Jeong, S. C.*; Ishiyama, Hironobu*; Hirayama, Yoshikazu*; Imai, Nobuaki*; Miyatake, Hiroari

International Journal of Modern Physics E, 19(5&6), p.989 - 996, 2010/07

 Times Cited Count:0 Percentile:0.01(Physics, Nuclear)

We have measured quasi-elastic scattering cross sections in reactions of $$^{48}$$Ti, $$^{54}$$Cr, $$^{56}$$Fe, $$^{64}$$Ni and $$^{70}$$Zn + $$^{208}$$Pb, relating to Pb-based cold fusion reactions for super-heavy elements 104, 106, 108, 110 and 112, respectively. A thin target of $$^{208}$$Pb was bombarded by heavy-ion beams supplied from the JAEA tandem-booster accelerator with changing the beam energy in steps of 1.5 MeV. The barrier distributions were derived from the first derivative of the excitation functions measured at backward angles of 172$$^{circ}$$, 168$$^{circ}$$ and 162$$^{circ}$$. The centroid of the barrier distributions showed a deviation from several predicted barrier heights toward the low energy side. The shape of the barrier distributions was well reproduced by the results of a coupled-channel calculation taking account of the coupling effects of the collective vibrational excitations in the projectile and target nuclei. We have recently obtained similar results in heavier reactions of $$^{76}$$Ge and $$^{86}$$Kr + $$^{208}$$Pb.

Journal Articles

Experimental studies of shielding and irradiation effects at high energy accelerator facilities

Nakashima, Hiroshi; Sakamoto, Yukio; Iwamoto, Yosuke; Matsuda, Norihiro; Kasugai, Yoshimi; Nakane, Yoshihiro; Masukawa, Fumihiro; Mokhov, N.*; Leveling, A.*; Boehnlein, D.*; et al.

Nuclear Technology, 168(2), p.482 - 486, 2009/11

BB2007-3640.pdf:0.22MB

 Times Cited Count:7 Percentile:45.39(Nuclear Science & Technology)

Experimental studies of shielding and radiation effects have been started using 120-GeV proton synchrotron at Fermi National Accelerator Laboratory (FNAL) under collaboration between FNAL and Japan. The first campaign of the experiment was carried out at the Pbar target station and Numi experimental station at FNAL, using antiproton and neutrino production targets irradiated by 120-GeV protons. The generated secondary particles passing through steel, concrete and rock were measured by activation methods as well as by other detectors such as scintillator with a veto counter, phoswich detector and a Bonner ball counter on trial. Preliminary experimental results are presented.

Journal Articles

A New measurement of the astrophysical $$^8$$Li(d,t)$$^7$$Li reaction

Hashimoto, Takashi; Ishiyama, Hironobu*; Watanabe, Yutaka*; Hirayama, Yoshikazu*; Imai, Nobuaki*; Miyatake, Hiroari; Jeong, S.-C.*; Tanaka, Masahiko*; Yoshikawa, Nobuharu*; Nomura, Toru*; et al.

Physics Letters B, 674(4-5), p.276 - 280, 2009/04

 Times Cited Count:6 Percentile:43.52(Astronomy & Astrophysics)

The excitation function of the $$^8$$Li(d,t)$$^7$$Li reaction was directly measured using $$^8$$Li beams at E$$_{mathrm{cm}}$$ = 0.3, 0.4, 0.5, 0.7, 0.8, 1.0, 1.1, and 1.2 MeV with CD$$_2$$ targets. The beam energies covered the Gamow peaks for 1$$sim$$3$$times$$10$$^9$$ K. Large cross sections were observed at around E$$_{mathrm{cm}}$$ = 0.8 MeV, implying a resonance state located at 22.4 MeV in $$^{10}$$Be. The present astrophysical reaction rate is higher in one order magnitude than the presently adopted rate at around 1$$times$$10$$^9$$ K.

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