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Journal Articles

Lanthanide and actinide ion complexes containing organic ligands investigated by surface-enhanced infrared absorption spectroscopy

Hirata, Sakiko*; Kusaka, Ryoji; Meiji, Shogo*; Tamekuni, Seita*; Okudera, Kosuke*; Hamada, Shoken*; Sakamoto, Chihiro*; Honda, Takumi*; Matsushita, Kosuke*; Muramatsu, Satoru*; et al.

Inorganic Chemistry, 62(1), p.474 - 486, 2023/01

 Times Cited Count:0 Percentile:0.01(Chemistry, Inorganic & Nuclear)

Journal Articles

Modelling concrete degradation by coupled non-linear processes

Oda, Chie; Kawama, Daisuke*; Shimizu, Hiroyuki*; Benbow, S. J.*; Hirano, Fumio; Takayama, Yusuke; Takase, Hiroyasu*; Mihara, Morihiro; Honda, Akira

Journal of Advanced Concrete Technology, 19(10), p.1075 - 1087, 2021/10

 Times Cited Count:0 Percentile:0(Construction & Building Technology)

Concrete in a transuranic (TRU) waste repository is considered a suitable material to ensure safety, provide structural integrity and retard radionuclide migration after the waste containers fail. In the current study, coupling between chemical, mass-transport and mechanical, so-called non-linear processes that control concrete degradation and crack development were investigated by coupled numerical models. Application of such coupled numerical models allows identification of the dominant non-linear processes that will control long-term concrete degradation and crack development in a TRU waste repository.

JAEA Reports

Mesh effect around burnable poison rod of cell model for HTTR fuel block

Fujimoto, Nozomu*; Fukuda, Kodai*; Honda, Yuki*; Tochio, Daisuke; Ho, H. Q.; Nagasumi, Satoru; Ishii, Toshiaki; Hamamoto, Shimpei; Nakano, Yumi*; Ishitsuka, Etsuo

JAEA-Technology 2021-008, 23 Pages, 2021/06

JAEA-Technology-2021-008.pdf:2.62MB

The effect of mesh division around the burnable poison rod on the burnup calculation of the HTTR core was investigated using the SRAC code system. As a result, the mesh division inside the burnable poison rod does not have a large effect on the burnup calculation, and the effective multiplication factor is closer to the measured value than the conventional calculation by dividing the graphite region around the burnable poison rod into a mesh. It became clear that the mesh division of the graphite region around the burnable poison rod is important for more appropriately evaluating the burnup behavior of the HTTR core..

Journal Articles

A Coupled modeling simulator for near-field processes in cement engineered barrier systems for radioactive waste disposal

Benbow, S. J.*; Kawama, Daisuke*; Takase, Hiroyasu*; Shimizu, Hiroyuki*; Oda, Chie; Hirano, Fumio; Takayama, Yusuke; Mihara, Morihiro; Honda, Akira

Crystals (Internet), 10(9), p.767_1 - 767_33, 2020/09

 Times Cited Count:2 Percentile:27.08(Crystallography)

Details are presented of the development of a coupled modeling simulator for assessing the evolution in the near-field of a geological repository for radioactive waste disposal where concrete is used as a backfill. The simulator uses OpenMI, a standard for exchanging data between simulation software programs at run-time, to form a coupled chemical-mechanical-hydrogeological model of the system. The approach combines a tunnel scale stress analysis finite element model, a discrete element model for accurately modeling the patterns of emerging cracks in the concrete, and a finite element and finite volume model of the chemical processes and alteration in the porous matrix and cracks in the concrete, to produce a fully coupled model of the system. Combining existing detailed simulation software in this way with OpenMI has the benefit of not relying on simplifications that might be necessary to combine all of the modeled processes in a single piece of software.

Journal Articles

Numerical evaluation on fluctuation absorption characteristics based on nuclear heat supply fluctuation test using HTTR

Takada, Shoji; Honda, Yuki*; Inaba, Yoshitomo; Sekita, Kenji; Nemoto, Takahiro; Tochio, Daisuke; Ishii, Toshiaki; Sato, Hiroyuki; Nakagawa, Shigeaki; Sawa, Kazuhiro*

Proceedings of 9th International Topical Meeting on High Temperature Reactor Technology (HTR 2018) (USB Flash Drive), 7 Pages, 2018/10

Nuclear heat utilization systems connected to HTGRs will be designed on the basis of non-nuclear grade standards for easy entry of chemical plant companies, requiring reactor operations to continue even if abnormal events occur in the systems. The inventory control is considered as one of candidate methods to control reactor power for load following operation for siting close to demand area, in which the primary gas pressure is varied while keeping the reactor inlet and outlet coolant temperatures constant. Numerical investigation was carried out based on the results of nuclear heat supply fluctuation tests using HTTR by non-nuclear heating operation to focus on the temperature transient of the reactor core bottom structure by imposing stepwise fluctuation on the reactor inlet temperature under different primary gas pressures below 120C. As a result, it was emerged that the fluctuation absorption characteristics are not deteriorated by lowering pressure. It was also emerged that the reactor outlet temperature did not reach the scram level by increasing the reactor inlet temperature 10 C stepwise at 80% of the rated power as same with the full power case.

Journal Articles

Measurement of temperature response of intermediate heat exchanger in heat application system abnormal simulating test using HTTR

Ono, Masato; Fujiwara, Yusuke; Honda, Yuki; Sato, Hiroyuki; Shimazaki, Yosuke; Tochio, Daisuke; Homma, Fumitaka; Sawahata, Hiroaki; Iigaki, Kazuhiko; Takada, Shoji

Proceedings of 2017 International Congress on Advances in Nuclear Power Plants (ICAPP 2017) (CD-ROM), 5 Pages, 2017/04

Japan Atomic Energy Agency (JAEA) has carried out research and developments towards nuclear heat utilization of High Temperature Gas-cooled Reactor (HTGR) using High Temperature Engineering Test Reactor (HTTR). The nuclear heat utilization systems connected to HTGR will be designed on the basis of non-nuclear-grade standards in terms of easier entry for the chemical plant companies and the construction economics of the systems. Therefore, it is necessary that the reactor operations continue even if abnormal events occur in the systems. Heat application system abnormal simulating test with HTTR was carried out in non-nuclear heating operation to focus on the thermal effect in order to obtain data of the transient temperature behavior of the metallic components in the Intermediate Heat Exchanger (IHX). The IHX is the key components to connect the HTTR with the heat application system. In the test, the coolant helium gas temperature was heated up to 120$$^{circ}$$C by the compression heat of the gas circulators in the HTTR under the ideal condition to focus on the heat transfer. The tests were conducted by decreasing the helium gas temperature stepwise by increasing the mass flow rate to the air cooler. The temperature responses of the IHX were investigated. For the components such as the heat transfer tubes and heat transfer enhancement plates of IHX, the temperature response was slower in the lower position in comparison with the higher position. The reason is considered that thermal load fluctuation is imposed in the secondary helium gas which flows from the top to the bottom in the heat transfer tubes of the IHX. The test data are useful to verify the numerical model of the safety evaluation code.

Journal Articles

Investigation of absorption characteristics for thermal-load fluctuation using HTTR

Tochio, Daisuke; Honda, Yuki; Sato, Hiroyuki; Sekita, Kenji; Homma, Fumitaka; Sawahata, Hiroaki; Takada, Shoji; Nakagawa, Shigeaki

Journal of Nuclear Science and Technology, 54(1), p.13 - 21, 2017/01

 Times Cited Count:1 Percentile:10.71(Nuclear Science & Technology)

GTHTR300C is designed and developed in JAEA. The reactor system is required to continue a stable and safety operation as well as a stable power supply in the case that thermal-load is fluctuated by the occurrence of abnormal event in the heat utilization system. Then, it is necessary to demonstrate that the thermal-load fluctuation should be absorbed by the reactor system so as to continue the stable and safety operation could be continued. The thermal-load fluctuation absorption tests without nuclear heating were planned and conducted in JAEA to clarify the absorption characteristic of thermal-load fluctuation mainly by the reactor and by the IHX. As the result it was revealed that the reactor has the larger absorption capacity of thermal-load fluctuation than expected one, and the IHX can be contributed to the absorption of the thermal-load fluctuation generated in the heat utilization system in the reactor system. It was confirmed from there result that the reactor and the IHX has effective absorption capacity of the thermal-load fluctuation generated in the heat utilization system. Moreover it was confirmed that the safety estimation code based on RELAP5/MOD3 can represents the thermal-load fluctuation absorption behavior conservatively.

Journal Articles

Nuclear heat supply fluctuation tests by non-nuclear heating with HTTR

Inaba, Yoshitomo; Sekita, Kenji; Nemoto, Takahiro; Honda, Yuki; Tochio, Daisuke; Sato, Hiroyuki; Nakagawa, Shigeaki; Takada, Shoji; Sawa, Kazuhiro

Journal of Nuclear Engineering and Radiation Science, 2(4), p.041001_1 - 041001_7, 2016/10

The nuclear heat utilization systems connected to High Temperature Gas-cooled Reactors (HTGRs) will be designed on the basis of non-nuclear grade standards in terms of the easier entry of chemical plant companies and the construction economics of the systems. Therefore, it is necessary that the reactor operations can be continued even if abnormal events occur in the systems. The Japan Atomic Energy Agency has developed a calculation code to evaluate the absorption of thermal load fluctuations by the reactors when the reactor operations are continued after such events, and has improved the code based on the High Temperature engineering Test Reactor (HTTR) operating data. However, there were insufficient data on the transient temperature behavior of the metallic core side components and the graphite core support structures corresponding to the fluctuation of the reactor inlet coolant temperature for further improvement of the code. Thus, nuclear heat supply fluctuation tests with the HTTR were carried out in non-nuclear heating operation to focus on thermal effect. In the tests, the coolant helium gas temperature was heated up to 120$$^{circ}$$C by the compression heat of the gas circulators in the HTTR, and a sufficiently high fluctuation of 17$$^{circ}$$C by devising a new test procedure was imposed on the reactor inlet coolant under the ideal condition without the effect of the nuclear power. Then, the temperature responses of the metallic core side components and the graphite core support structures were investigated. The test results adequately showed as predicted that the temperature responses of the metallic components are faster than those of the graphite structures, and the mechanism of the thermal load fluctuation absorption by the metallic components was clarified.

JAEA Reports

HTTR thermal load fluctuation test (non-nuclear heating test); Confirmation of HTGR system response against temperature transient

Honda, Yuki; Tochio, Daisuke; Nakagawa, Shigeaki; Sekita, Kenji; Homma, Fumitaka; Sawahata, Hiroaki; Sato, Hiroyuki; Sakaba, Nariaki; Takada, Shoji

JAEA-Technology 2016-016, 16 Pages, 2016/08

JAEA-Technology-2016-016.pdf:2.84MB

A system analysis code is validated with the thermal-load fluctuation absorption test with nun-nuclear heating by using the High Temperature Engineering test Reactor (HTTR) to clarify the High Temperature Gas-cooled Reactor (HTGR) system response against temperature transient. The thermal-load fluctuation absorption test consists on the thermal load fluctuation tests (non-nuclear heating) and heat application system abnormal simulating test (non-nuclear heating). The HTGR reactor response against temperature transient is clarified in the thermal load fluctuation test (non-nuclear heating). The Intermediate Heat Exchanger (IHX) reactor response against temperature transient is clarified in the heat application system abnormal simulating test (non-nuclear heating). With the two HTTR non-nuclear heating test, HTGR system response against temperature transient is obtained.

Journal Articles

Characteristic confirmation test by using HTTR and investigation of absorbing thermal load fluctuation

Honda, Yuki; Tochio, Daisuke; Sato, Hiroyuki; Nakagawa, Shigeaki; Ono, Masato; Fujiwara, Yusuke; Hamamoto, Shimpei; Iigaki, Kazuhiko; Takada, Shoji

Proceedings of 24th International Conference on Nuclear Engineering (ICONE-24) (DVD-ROM), 5 Pages, 2016/06

The characteristic confirmation test has been demonstrating by using the High Temperature engineering Test Reactor (HTTR). The thermal load fluctuation test, which is one of marginal performance test is planned to be carried out after restarting of the HTTR. The preliminary analysis for the thermal load fluctuation test has been investigated. In the analysis, the reactor outlet temperature can continue to be stable against the reactor inlet temperature changing by thermal fluctuation. It means that HTGR have the capability of absorbing thermal fluctuation. This paper focuses on the investigation of mechanism of absorbing thermal fluctuation. With additional analysis, it is cleared that the large negative graphite moderator reactivity enhances the capability of absorbing thermal fluctuation. In addition, in the middle of the core, graphite moderator reactivity insertion trend are inverted. This trend is unique to HTGR because of large temperature difference between core inlet and outlet.

JAEA Reports

Validation of system analysis code with HTTR thermal load fluctuation test data (non-nuclear heating) and evaluation of reactor temperature behavior during upsets in hydrogen production plant

Honda, Yuki; Sato, Hiroyuki; Nakagawa, Shigeaki; Takada, Shoji; Tochio, Daisuke; Sakaba, Nariaki; Sawa, Kazuhiro

JAEA-Technology 2015-012, 17 Pages, 2015/06

JAEA-Technology-2015-012.pdf:11.38MB

Japan Atomic Energy Agency (JAEA) proposed a draft safety requirement, which consists of the requirements for constructing a H$$_{2}$$ plant under conventional chemical plant regulations as well as the requirements for collocation of a nuclear facility and a H$$_{2}$$ plant. One of the key requirements is to maintain reactor normal operation condition during every possible condition in the H$$_{2}$$ plant. In order to show that the requirement can be reasonably achieved, a system analysis code is validated with the HTTR experimental data obtained in January 2015. The validated code is applied for the evaluation of a postulated abnormal event in H$$_{2}$$ plant to be connected to the HTTR. The results showed that the evaluation items such as reactor power and reactor outlet coolant temperature do not exceed evaluation criteria. As a conclusion, a feasibility of H$$_{2}$$ plant construction under non-nuclear regulations is validated by showing that the stable reactor operation can be achieved against temperature transients induced by abnormal conditions in the H$$_{2}$$ plant.

Journal Articles

Nuclear heat supply fluctuation test by non-nuclear heating using HTTR

Takada, Shoji; Sekita, Kenji; Nemoto, Takahiro; Honda, Yuki; Tochio, Daisuke; Inaba, Yoshitomo; Sato, Hiroyuki; Nakagawa, Shigeaki; Sawa, Kazuhiro

Proceedings of 23rd International Conference on Nuclear Engineering (ICONE-23) (DVD-ROM), 7 Pages, 2015/05

To investigate the safety design criteria of heat utilization system for the HTGRs, it is necessary to evaluate the effect of fluctuation of thermal load on the reactor. The nuclear heat supply fluctuation test by non-nuclear heating was carried out to simulate the nuclear heat supply test which is carried out in the nuclear powered operation. The test data is used to verify the numerical code to calculate the temperature of core bottom structure to carry out the safety evaluation of abnormal events in the heat utilization system. In the test, the helium gas temperature was heated up to 120$$^{circ}$$C. A sufficiently high temperature disturbance was imposed on the reactor inlet temperature. It was found that the response of temperatures of metallic components such as side shielding blocks was faster than those of graphite blocks in the core bottom structure, which was significantly affected by the heat capacities of components, the level of imposed disturbance and heat transfer performance.

Journal Articles

Establishment of control technology of the HTTR and future test plan

Honda, Yuki; Saito, Kenji; Tochio, Daisuke; Aono, Tetsuya; Hirato, Yoji; Kozawa, Takayuki; Nakagawa, Shigeaki

Journal of Nuclear Science and Technology, 51(11-12), p.1387 - 1397, 2014/11

 Times Cited Count:1 Percentile:8.95(Nuclear Science & Technology)

The operational experiments of the HTTR would be useful for future high-temperature gas-cooled reactors (HTGRs). Main PID control constants of the HTTR are selected with reasonably damped characteristics and without undershoot or overshoot. For utilization the HTGR as a commercial reactor, it should be demonstrated that the HTGR system can supply stable heat to a heat utilization system for the long-term operation. The control characteristics in the long-term high-temperature operation are evaluated by the result of operation performed in 2010. In addition, from a viewpoint of HTGRs with heat utilization system, a future possibility of the experiments for heat utilization design is examined.

Journal Articles

Na-montmorillonite dissolution rate determined by varying the Gibbs free energy of reaction in a dispersed system and its application to a coagulated system in 0.3M NaOH solution at 70$$^{circ}$$C

Oda, Chie; Walker, C.; Chino, Daisuke*; Ichige, Satoru; Honda, Akira; Sato, Tsutomu*; Yoneda, Tetsuro*

Applied Clay Science, 93-94, p.62 - 71, 2014/05

 Times Cited Count:7 Percentile:24.7(Chemistry, Physical)

Na-montmorillonite dissolution in a 0.3M NaOH solution has been investigated at pH12 and 70$$^{circ}$$C. The flow-through dissolution experiments were conducted in a dispersed system with varying concentrations of Si and Al to derive a Na-montmorillonite dissolution rate, as a non-linear function of the Gibbs free energy of reaction, dGr. This rate equation was used to simulate the batch-type Na-montmorillonite reaction experiments conducted in a coagulated system. The model simulation of the batch-type experiment adopting the empirical rate equations of Na-montmorillonite dissolution and secondary mineral analcime precipitation were able to reproduce the measured changes in the amount of dissolved Na-montmorillonite and concentrations of Si and Al in solution. The results showed that the empirical rate equation of Na-montmorillonite dissolution determined in the dispersed system was applicable to the coagulated system over a higher dGr range and that the concentrations of Si and Al in the batch experiment were controlled by the precipitation of analcime.

Journal Articles

Basic vacuum test of 500-kV photocathode DC gun components at KEK

Yamamoto, Masahiro*; Uchiyama, Takashi*; Miyajima, Tsukasa*; Honda, Yosuke*; Sato, Kotaro*; Matsuba, Shunya*; Saito, Yoshio*; Kobayashi, Masanori*; Kurisu, Hiriki*; Hajima, Ryoichi; et al.

Proceedings of 7th Annual Meeting of Particle Accelerator Society of Japan (DVD-ROM), p.717 - 720, 2010/08

A 500-kV photocathode DC electron gun which can supply the beam of a low emittance and a high average current has been developed in collaboration with KEK, JAEA, Hiroshima Univ., Nagoya Univ. and Yamaguchi Univ. The vacuum of the gun chamber has to be lower Extreme High Vacuum for maintain cathode-life time. A titanium chamber and new material of ceramic were employed to reduce outgassing rate. The result of outgassing rate of the gun chamber is described in this report.

Journal Articles

Design of a 500kV electron gun for ERL light source at KEK

Yamamoto, Masahiro*; Honda, Yosuke*; Miyajima, Tsukasa*; Uchiyama, Takashi*; Kobayashi, Masanori*; Muto, Toshiya*; Matsuba, Shunya*; Sakanaka, Shogo*; Sato, Kotaro*; Saito, Yoshio*; et al.

Proceedings of 6th Annual Meeting of Particle Accelerator Society of Japan (CD-ROM), p.860 - 862, 2009/08

A newly 500 kV electron gun (2nd - 500 kV gun) for an ERL light source is designed at KEK. A new concept and state of-the-art technologies of vacuum system, ceramic insulators, high voltage power supply, photocathode and preparation system will be employed. The details are described in this report.

Journal Articles

Change of the Fermi surface across the critical pressure in CeIn$$_3$$; The de Haas-van Alphen study under pressure

Settai, Rikio*; Kubo, Tetsuo*; Shiromoto, Tomoyuki*; Honda, Daisuke*; Shishido, Hiroaki*; Sugiyama, Kiyohiro*; Haga, Yoshinori; Matsuda, Tatsuma; Betsuyaku, Kiyoshi*; Harima, Hisatomo*; et al.

Journal of the Physical Society of Japan, 74(11), p.3016 - 3026, 2005/11

 Times Cited Count:50 Percentile:12.02(Physics, Multidisciplinary)

We have studied a change of the Fermi surface in an antiferromagnet CeIn$$_3$$ via the de Haas-van Alphen experiment under pressure up to 3 GPa. With increasing pressure P, the Neel temperature $$T_N$$=10 K decreases and becomes zero at a critical pressure Pc $$simeq$$2.6 GPa. In the pressure region $$P > P_c$$, we have observed a large main Fermi surface named a, which indicates that the electronic state of 4 f electron in CeIn$$_3$$ changes from localized to itinerant at Pc, as observed in the similar antiferromagnets CeRh$$_2$$Si$$_2$$ and CeRhIn$$_5$$. The cyclotron effective mass $$m_c^*$$ of this main Fermi surface is extremely enhanced around Pc: $$m_c^*$$ $$simeq$$60 $$m_0$$ at 2.7 GPa for the magnetic field along the $$<$$100$$>$$ direction.

Journal Articles

Magnetic property and pressure effect of a single crystal CeRhGe

Ueda, Taiki*; Honda, Daisuke*; Shiromoto, Tomoyuki*; Metoki, Naoto; Honda, Fuminori*; Kaneko, Koji; Haga, Yoshinori; Matsuda, Tatsuma; Takeuchi, Tetsuya*; Thamizhavel, A.*; et al.

Journal of the Physical Society of Japan, 74(10), p.2836 - 2842, 2005/10

 Times Cited Count:14 Percentile:61.04(Physics, Multidisciplinary)

Oral presentation

Preliminary study of thermal load fluctuation test in normal operation state using the HTTR

Honda, Yuki; Tochio, Daisuke; Aono, Tetsuya; Hirato, Yoji; Kozawa, Takayuki; Saito, Kenji

no journal, , 

The HTGR system with helium turbine and hydrogen production system have been designed based on the HTTR experiments. For the future HTGR control system design, the thermal-load fluctuation and lost test for heat utilization system design is planned. The tests would be important for demonstration of the reactor stability despite thermal load fluctuation, detailed design of the HTGRs with heat utilization system and validation of plant dynamic codes for future HTGR system. Preliminary studies with all main control system are carried out to study on the control characteristics with the thermal-load fluctuation test and determine test condition on normal operation state such as the amount of decrease in the flow rate of the ACL.

Oral presentation

Characteristic confirmation test by using HTTR

Honda, Yuki; Aono, Tetsuya; Sekita, Kenji; Tochio, Daisuke; Takada, Shoji

no journal, , 

The Characteristic confirmation test has been demonstrating by using the High Temperature engineering Test Reactor (HTTR) to confirm the High Temperature Gas Reactor (HTGR) characteristics, which are safety characteristics and various heat utilization. The characteristic confirmation test by using the HTTR consists of the limit performance test and nuclear heat supply fluctuation test. The nuclear heat supply fluctuation testis planned to be carried out after restarting of the HTTR. Towards the realization of industrial utilization of a HTGR cogeneration system as an extension of a nuclear plant, it is important to ensure reactor safety in the case that thermal-load of the facility is fluctuated or lost. The HTTR is under long-term shutdown. However, two nuclear heat supply fluctuation tests were demonstrated without nuclear heating. This report shows outline, progress and results of characteristic confirmation test.

Oral presentation

Effect of BP cell model for HTTR burnup characteristics

Fujimoto, Nozomu*; Honda, Yuki; Fukuda, Kodai*; Goto, Minoru; Tochio, Daisuke; Takada, Shoji

no journal, , 

In the HTTR, BP has been used for keeping excess reactivity change small by burn-up. We will present the analytical results of critical control rod position changing in order to estimate excess reactivity changing at zero power. The effect of mesh division around BP for critical control rod position is cleared by sensitivity analysis.

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