Experimental study on transport behavior of cesium iodide in the reactor coolant system under LWR severe accident conditions

Miyahara, Naoya; Miwa, Shuhei; Goullo, M.*; Imoto, Jumpei; Horiguchi, Naoki; Sato, Isamu*; Osaka, Masahiko

Journal of Nuclear Science and Technology, 57(12), p.1287 - 1296, 2020/12

https://doi.org/10.1080/00223131.2020.1782281

In order to clarify the cesium iodide (CsI) transport behavior with a focus on the mechanisms of gaseous iodine formation in the reactor coolant system of LWR under a severe accident condition, a reproductive experiment of CsI transport behavior was conducted using a facility equipped with a thermal gradient tube. Various analyses on deposits and airborne materials during transportation could elucidate two mechanisms for the gaseous iodine formation. One was the gaseous phase chemical reaction in Cs-I-O-H system at relatively high-temperature region, which led to gaseous iodine transport to the lower temperature region without any further changes in gas species due to the kinetics limitation effects. The other one was the chemical reactions related to condensed phase of CsI, namely those of CsI deposits on walls with surface of stainless steel to form CsCrO compound and CsI aerosol particles with steam, which were newly found in this study.

Development of fission product chemistry database ECUME for the LWR severe accident

Miwa, Shuhei; Nakajima, Kunihisa; Miyahara, Naoya; Nishioka, Shunichiro; Suzuki, Eriko; Horiguchi, Naoki; Liu, J.; Miradji, F.; Imoto, Jumpei; Mohamad, B. A.; et al.

Mechanical Engineering Journal (Internet), 7(3), p.19-00537_1 - 19-00537_11, 2020/06

https://doi.org/10.1299/mej.19-00537

We constructed the fission product (FP) chemistry database named ECUME for LWR severe accident. This version of ECUME is equipped with dataset of the chemical reactions and their kinetics constants for the reactions of cesium(Cs)-iodine(I)-boron(B)-molybdenum(Mo)-oxygen(O)-hydrogen(H) system in gas phase, the elemental model for the high temperature chemical reaction of Cs with stainless steel applied as the structural material in a reactor, and thermodynamic data for CsBO vapor species and solids of CsSiO and CsFeSiO for these chemical reactions. The ECUME will provide estimation of Cs distribution due to the evaluation of effects of interaction with BWR control material B and stainless steel on Cs behavior in the Fukushima Daiichi Nuclear Power Station.

Development of evaluation method for aerosol particle deposition in a reactor building based on CFD

Horiguchi, Naoki; Miyahara, Naoya; Uesawa, Shinichiro; Yoshida, Hiroyuki; Osaka, Masahiko

Proceedings of 27th International Conference on Nuclear Engineering (ICONE-27) (Internet), 8 Pages, 2019/05

For source term evaluation from reactor buildings (RBs) in LWR severe accidents, we have launched to develop an evaluation method of FP aerosol particle deposition onto surfaces of internal structures in an RB based on computational fluid dynamics (CFD). This paper describes development of a CFD simulation tool as the base part of the evaluation method. A preliminary simulation for a representative RB under a representative flow condition was conducted to confirm the tool performance by roughly grasping the deposition behaviors of FP aerosol particle and decontamination factor (DF) in the RB. Calculation results showed that most of aerosol particles were deposited along with gas flow formed by the internal structures in the RB, demonstrating the advantageous feature of the present CFD tool. The DFs from 4 to 14 were obtained with increase of the particle diameters from 0.1 to 10 m as expected in terms of the particle movement equation.

Visualized measurement of extremely high-speed droplets in Venturi scrubber

Horiguchi, Naoki; Yoshida, Hiroyuki; Abe, Yutaka*

Journal of Nuclear Science and Technology, 56(3), p.278 - 290, 2019/03

https://doi.org/10.1080/00223131.2018.1564707

Venturi scrubber (VS) has been installed in NPPs as one of the components of filtered venting systems. It can eliminate fine aerosol particles including fission products from polluted gas. Under extremely high-velocity conditions during severe accident, the data related to the droplet in the VS, which affects decontamination performance, is insufficient. This objective is to obtain the diameter of the extremely high-speed droplets and clarify an applicability of the existing correlations for the diameter. To visualize the extremely high-velocity droplet, an optical system with high frame rate and high resolution was developed. Visualization experiment using the VS under air-water condition was conducted, and droplet diameter distributions and Sauter mean diameter (SMD) were obtained. By comparing experimental data with values evaluated by existing correlations, it was clarified that the Nukiyama-Tanasawa equation can evaluate the SMD with good accuracy in the gas velocity range 82-250 m/s.

Development of numerical simulation method for small particles behavior in two-phase flow by combining interface and Lagrangian particle tracking methods

Yoshida, Hiroyuki; Uesawa, Shinichiro; Horiguchi, Naoki; Miyahara, Naoya; Ose, Yasuo*

Proceedings of 11th Korea-Japan Symposium on Nuclear Thermal Hydraulics and Safety (NTHAS-11) (Internet), 6 Pages, 2018/11

Development of numerical simulation method for capturing behavior of aerosol particles on gas-liquid interface based on interface tracking method

Yoshida, Hiroyuki; Uesawa, Shinichiro; Horiguchi, Naoki; Miyahara, Naoya; Ose, Yasuo*

Dai-23-Kai Doryoku, Enerugi Gijutsu Shimpojiumu Koen Rombunshu (USB Flash Drive), 5 Pages, 2018/06

no abstracts in English

Study on water-vapor two-phase flow behavior in venturi tube

Uesawa, Shinichiro; Horiguchi, Naoki; Shibata, Mitsuhiko; Yoshida, Hiroyuki

Nihon Kikai Gakkai Rombunshu (Internet), 84(859), p.17-00392_1 - 17-00392_10, 2018/03

https://doi.org/10.1299/transjsme.17-00392

no abstracts in English

Prediction and evaluation of decontamination performance of venturi scrubber in actual environments

Horiguchi, Naoki; Yoshida, Hiroyuki; Uesawa, Shinichiro; Abe, Yutaka*

Dai-22-Kai Doryoku, Enerugi Gijutsu Shimpojiumu Koen Rombunshu (USB Flash Drive), 4 Pages, 2017/06

Venturi scrubber is installed in nuclear power plant as a component of filtered venting system and used to remove small aerosols with fission products. There is, however, no method to estimate its decontamination performance in the assumed operating pressure range. In this study, we establish a method to estimate the decontamination performance based on mechanistic thermal hydrodynamic simulation code and report simulated results of the thermal hydrodynamics and decontamination performance in the pressure range in the pressure range in actual environments. With decrease in inlet pressure of the Venturi scrubber, gas flow velocity at the throat of it is suppressed, liquid flow velocity in a hole of it by self-priming changes and the decontamination factor changes were obtained. Also, with larger the aerosol diameter, the decontamination factor become larger was obtained.

Development of evaluation method for hydraulic behavior in venturi scrubber for filtered venting

Horiguchi, Naoki; Yoshida, Hiroyuki; Nakao, Yasuhiro*; Kaneko, Akiko*; Abe, Yutaka*

Proceedings of 10th Japan-Korea Symposium on Nuclear Thermal Hydraulics and Safety (NTHAS-10) (USB Flash Drive), 7 Pages, 2016/11

Numerical simulation of self-priming phenomena in venturi scrubber by two-phase flow simulation code TPFIT

Horiguchi, Naoki; Yoshida, Hiroyuki; Kanagawa, Tetsuya*; Kaneko, Akiko*; Abe, Yutaka*

Proceedings of 23rd International Conference on Nuclear Engineering (ICONE-23) (DVD-ROM), 6 Pages, 2015/05

From the viewpoint of protecting containment and suppressing diffusion of the radioactive materials at severe accidents of nuclear power plant, it is important to install filtered venting devices to permit release of high pressure pollutant gas to the atmosphere by eliminating radioactive materials in the gas. A Multi Venturi Scrubber System (MVSS) is one of the devices for the filtered venting, and is used to realize filtered venting without any power supply. The MVSS is composed of a "Venturi Scrubbers" part and a "bubble column" part. In the Venturi Scrubbers part of the MVSS, there are hundreds of the Venturi scrubbers (VS). In an operation mode of the MVSS, the radioactive materials are eliminated through the gas-liquid interface from the pollutant gas to the liquid phase of a dispersed flow in the VS and a bubbly flow in the bubble column part. In the VS, the dispersed flow is formed from the liquid, which is suctioned through the hole for suction (called self-priming). In previous studies, an evaluation method to evaluate the liquid flow rate by the self-priming was developed. However, to develop evaluation methods of performance of the VSs, the two-phase flow behavior must be investigated, including droplet size and velocity difference of liquid and gas phases. Two-phase flow behavior in the VS is complicated, and it is difficult to estimate two-phase flow behavior of the VS by only experimental procedures. In this study, to investigate the hydraulic behavior of the VS, we tried to apply a detailed numerical simulation method of two-phase flow to the numerical simulation of the VS. In the simulation, TPFIT developed in JAEA was used as the detailed numerical simulation method. In this paper, we performed the numerical simulation air-water two-phase flow in the of the lab scale VS by the TPFIT, and numerical results were compared with experimental results.