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Journal Articles

Brightening triplet excitons enable high-performance white-light emission in organic small molecules via integrating n-$$pi^*/pi$$-$$pi^*$$ transitions

Yang, Q.*; Yang, X.*; Wang, Y.*; Fei, Y.*; Li, F.*; Zheng, H.*; Li, K.*; Han, Y.*; Hattori, Takanori; Zhu, P.*; et al.

Nature Communications (Internet), 15, p.7778_1 - 7778_9, 2024/09

 Times Cited Count:47 Percentile:94.53(Multidisciplinary Sciences)

Luminescent materials that simultaneously embody bright singlet and triplet excitons hold great potential in optoelectronics, signage, and information encryption. However, achieving high-performance white-light emission is severely hampered by their inherent unbalanced contribution of fluorescence and phosphorescence. Herein, we address this challenge by pressure treatment engineering via hydrogen bonding cooperativity effect to realize the mixture of n-$$pi^*/pi$$-$$pi^*$$ transitions, where the triplet state emission was boosted from 7% to 40% in isophthalic acid (IPA). A superior white-light emission based on hybrid fluorescence and phosphorescence was harvested in pressure-treated IPA, and the photoluminescence quantum yield was increased to 75% from the initial 19% (blue-light emission). In-situ high-pressure IR spectra, X ray diffraction, and neutron diffraction reveal continuous strengthening of the hydrogen bonds with the increase of pressure. Furthermore, this enhanced hydrogen bond is retained down to the ambient conditions after pressure treatment, awarding the targeted IPA efficient intersystem crossing for balanced singlet/triplet excitons population and resulting in efficient white-light emission. This work not only proposes a route for brightening triplet states in organic small molecule, but also regulates the ratio of singlet and triplet excitons to construct high-performance white-light emission.

Journal Articles

Gradient residual strain measurement procedure in surface impacted railway steel axles by using neutron scattering

Zhou, L.*; Zhang, H.*; Qin, T. Y.*; Hu, F. F.*; Xu, P. G.; Ao, N.*; Su, Y. H.; He, L. H.*; Li, X. H.*; Zhang, J. R.*; et al.

Metallurgical and Materials Transactions A, 55(7), p.2175 - 2185, 2024/07

 Times Cited Count:4 Percentile:36.86(Materials Science, Multidisciplinary)

Journal Articles

Martensitic transformation in CrCoNi medium-entropy alloy at cryogenic temperature

Naeem, M.*; Zhou, H.*; He, H.*; Harjo, S.; Kawasaki, Takuro; Lan, S.*; Wu, Z.*; Zhu, Y.*; Wang, X.-L.*

Applied Physics Letters, 119(13), p.131901_1 - 131901_7, 2021/09

 Times Cited Count:23 Percentile:73.89(Physics, Applied)

Journal Articles

Quasifree neutron knockout reaction reveals a small $$s$$-Orbital component in the Borromean nucleus $$^{17}$$B

Yang, Z. H.*; Kubota, Yuki*; Corsi, A.*; Yoshida, Kazuki; Sun, X.-X.*; Li, J. G.*; Kimura, Masaaki*; Michel, N.*; Ogata, Kazuyuki*; Yuan, C. X.*; et al.

Physical Review Letters, 126(8), p.082501_1 - 082501_8, 2021/02

AA2020-0819.pdf:1.29MB

 Times Cited Count:94 Percentile:97.22(Physics, Multidisciplinary)

A quasifree ($$p$$,$$pn$$) experiment was performed to study the structure of the Borromean nucleus $$^{17}$$B, which had long been considered to have a neutron halo. By analyzing the momentum distributions and exclusive cross sections, we obtained the spectroscopic factors for $$1s_{1/2}$$ and $$0d_{5/2}$$ orbitals, and a surprisingly small percentage of 9(2)% was determined for $$1s_{1/2}$$. Our finding of such a small $$1s_{1/2}$$ component and the halo features reported in prior experiments can be explained by the deformed relativistic Hartree-Bogoliubov theory in continuum, revealing a definite but not dominant neutron halo in $$^{17}$$B. The present work gives the smallest $$s$$- or $$p$$-orbital component among known nuclei exhibiting halo features and implies that the dominant occupation of $$s$$ or $$p$$ orbitals is not a prerequisite for the occurrence of a neutron halo.

Journal Articles

General synthesis of single-atom catalysts for hydrogen evolution reactions and room-temperature Na-S batteries

Lai, W.-H.*; Wang, H.*; Zheng, L.*; Jiang, Q.*; Yan, Z.-C.*; Wang, L.*; Yoshikawa, Hirofumi*; Matsumura, Daiju; Sun, Q.*; Wang, Y.-X.*; et al.

Angewandte Chemie; International Edition, 59(49), p.22171 - 22178, 2020/12

 Times Cited Count:134 Percentile:96.06(Chemistry, Multidisciplinary)

Journal Articles

Clades of huge phages from across Earth's ecosystems

Al-Shayeb, B.*; Sachdeva, R.*; Chen, L.-X.*; Ward, F.*; Munk, P.*; Devoto, A.*; Castelle, C. J.*; Olm, M. R.*; Bouma-Gregson, K.*; Amano, Yuki; et al.

Nature, 578(7795), p.425 - 431, 2020/02

 Times Cited Count:361 Percentile:99.46(Multidisciplinary Sciences)

Journal Articles

Fine structure in the $$alpha$$ decay of $$^{223}$$U

Sun, M. D.*; Liu, Z.*; Huang, T. H.*; Zhang, W. Q.*; Andreyev, A. N.; Ding, B.*; Wang, J. G.*; Liu, X. Y.*; Lu, H. Y.*; Hou, D. S.*; et al.

Physics Letters B, 800, p.135096_1 - 135096_5, 2020/01

 Times Cited Count:15 Percentile:74.21(Astronomy & Astrophysics)

Journal Articles

Spin Hall effect by surface roughness

Zhou, L.*; Grigoryan, V. L.*; Maekawa, Sadamichi; Wang, X.*; Xiao, J.*

Physical Review B, 91(4), p.045407_1 - 045407_6, 2015/01

 Times Cited Count:43 Percentile:79.89(Materials Science, Multidisciplinary)

Journal Articles

Overview of plasma-material interaction experiments on EAST employing MAPES

Ding, F.*; Luo, G.-N.*; Pitts, R.*; Litnovsky, A.*; Gong, X.*; Ding, R.*; Mao, H.*; Zhou, H.*; Wampler, W. R.*; Stangeby, P. C.*; et al.

Journal of Nuclear Materials, 455(1-3), p.710 - 716, 2014/12

 Times Cited Count:31 Percentile:88.59(Materials Science, Multidisciplinary)

Journal Articles

In-beam $$gamma$$ spectroscopy of the even-even nucleus $$^{190}$$Pt

Li, G. S.*; Liu, M. L.*; Zhou, X. H.*; Zhang, Y. H.*; Liu, Y. X.*; Zhang, N. T.*; Hua, W.*; Zheng, Y. D.*; Fang, Y. D.*; Guo, S.*; et al.

Physical Review C, 89(5), p.054303_1 - 054303_9, 2014/05

 Times Cited Count:6 Percentile:39.58(Physics, Nuclear)

High-spin states of $$^{190}$$Pt have been reinvestigated using the $$^{176}$$Yb($$^{18}$$O, 4$$n$$) reaction at a beam energy of 88 MeV. The previously known positive parity band associated with the $$nu$$ $$i^{-2}_{13/2}$$ $$nu$$ $$h^{-1}_{9/2}$$ $$nu$$ $$j^{-1}$$ ($$nu j$$ being $$nu p_{3/2}$$ or $$nu f_{5/2}$$) configuration has been revised and extended significantly. A new negative parity band has been established and proposed to be based on the $$nu$$ $$i^{-3}_{13/2}$$ $$nu$$ $$j^{-1}$$ configuration. Possible structure evolution of the yrast line from predominantly vibrational to rotational with increasing spin is discussed with the help of E$$_gamma$$ over spin curves. Additionally, calculations of Total Routhian surfaces have been performed to investigate the band properties.

Journal Articles

Cesium, iodine and tritium in NW Pacific waters; A Comparison of the Fukushima impact with global fallout

Povinec, P. P.*; Aoyama, Michio*; Biddulph, D.*; Breier, R.*; Buesseler, K. O.*; Chang, C. C.*; Golser, R.*; Hou, X. L.*; Je$v{s}$kovsk$'y$, M.*; Jull, A. J. T.*; et al.

Biogeosciences, 10(8), p.5481 - 5496, 2013/08

 Times Cited Count:119 Percentile:93.92(Ecology)

Radionuclide impact of the Fukushima Dai-ichi Nuclear Power Plant accident on the distribution of radionuclides in seawater of the NW Pacific Ocean is compared with global fallout from atmospheric tests of nuclear weapons. Surface and water column seawater samples collected during the international expedition in June 2011 were analyzed for $$^{134}$$Cs, $$^{137}$$Cs, $$^{129}$$I and $$^{3}$$H. The $$^{137}$$Cs, $$^{129}$$I and $$^{3}$$H levels in surface seawater offshore Fukushima varied between 0.002-3.5 Bq/L, 0.01-0.8 $$mu$$Bq/L, and 0.05-0.15 Bq/L, respectively. At the sampling site about 40 km from the coast, where all three radionuclides were analyzed, the Fukushima impact on the levels of these three radionuclides represent an increase above the global fallout background by factors of about 1000, 30 and 3, respectively. The water column data indicate that the transport of Fukushima-derived radionuclides downward to the depth of 300 m has already occurred. The observed $$^{137}$$Cs levels in surface waters and in the water column are in reasonable agreement with predictions obtained from the Ocean General Circulation Model, which indicates that the radionuclides have been transported from the Fukushima coast eastward. Due to a suitable residence time in the ocean, Fukushima-derived radionuclides will provide useful tracers for isotope oceanography studies on the transport of water masses in the NW Pacific Ocean.

Journal Articles

Rotational band properties of $$^{173}$$W

Wang, H. X.*; Zhang, Y. H.*; Zhou, X. H.*; Liu, M. L.*; Ding, B.*; Li, G. S.*; Hua, W.*; Zhou, H. B.*; Guo, S.*; Qiang, Y. H.*; et al.

Physical Review C, 86(4), p.044305_1 - 044305_11, 2012/10

AA2012-0752.pdf:0.78MB

 Times Cited Count:6 Percentile:34.74(Physics, Nuclear)

Journal Articles

High-j proton alignments in $$^{101}$$Pd

Zhou, H. B.*; Zhou, X. H.*; Zhang, Y. H.*; Zheng, Y.*; Liu, M. L.*; Zhang, N. T.*; Chen, L.*; Wang, S. T.*; Li, G. S.*; Wang, H. X.*; et al.

European Physical Journal A, 47(9), p.107_1 - 107_7, 2011/09

 Times Cited Count:7 Percentile:43.67(Physics, Nuclear)

High-spin states in $$^{101}$$Pd have been investigated by means of in-beam $$gamma$$-ray spectroscopic techniques. The previously known $$d$$$$_{5/2}$$ and 1/2$$^-$$[550] bands were extended to higher spins. The band crossings observed experimentally are explained by the alignment of $$g$$$$_{9/2}$$ protons. The band properties in $$^{101}$$Pd are compared with those in the neighboring nuclei and are discussed within the framework of the cranked shell model.

Journal Articles

Signature inversion in the 7/2$$^-$$[503] band of $$^{185}$$Pt

Li, G. S.*; Zhou, X. H.*; Zhang, Y. H.*; Zheng, Y.*; Liu, M. L.*; Hua, W.*; Zhou, H. B.*; Ding, B.*; Wang, H. X.*; Lei, X. G.*; et al.

Journal of Physics G; Nuclear and Particle Physics, 38(9), p.095105_1 - 095105_9, 2011/09

 Times Cited Count:1 Percentile:11.09(Physics, Nuclear)

High-spin states in $$^{185}$$Pt have been investigated by means of in beam $$gamma$$-ray spectroscopic method at the JAEA tandem facility. Low-spin signature inversion is revealed in the 7/2$$^-$$[503] band. The inversion can be interpreted as a configuration change from the 7/2$$^-$$[503] orbital to the 7/2$$^-$$[514] orbital with increasing spin, which is supported by a theoretical calculation of the semi-classical Donau and Frauendorf approach.

Journal Articles

Event structure and double helicity asymmetry in jet production from polarized $$p + p$$ collisions at $$sqrt{s}$$ = 200 GeV

Adare, A.*; Afanasiev, S.*; Aidala, C.*; Ajitanand, N. N.*; Akiba, Y.*; Al-Bataineh, H.*; Alexander, J.*; Aoki, K.*; Aphecetche, L.*; Armendariz, R.*; et al.

Physical Review D, 84(1), p.012006_1 - 012006_18, 2011/07

 Times Cited Count:36 Percentile:74.69(Astronomy & Astrophysics)

We report on the event structure and double helicity asymmetry ($$A_{LL}$$) of jet production in longitudinally polarized $$p + p$$ collisions at $$sqrt{s}$$ = 200 GeV. Photons and charged particles were measured by the PHENIX experiment. Event structure was compared with the results from PYTHIA event generator. The production rate of reconstructed jets is satisfactorily reproduced with the next-to-leading-order perturbative QCD calculation. We measured $$A_{LL}$$ = -0.0014 $$pm$$ 0.0037 at the lowest $$P_T$$ bin and -0.0181 $$pm$$ 0.0282 at the highest $$P_T$$ bin. The measured $$A_{LL}$$ is compared with the predictions that assume various $$Delta G(x)$$ distributions.

Journal Articles

Identified charged hadron production in $$p + p$$ collisions at $$sqrt{s}$$ = 200 and 62.4 GeV

Adare, A.*; Afanasiev, S.*; Aidala, C.*; Ajitanand, N. N.*; Akiba, Yasuyuki*; Al-Bataineh, H.*; Alexander, J.*; Aoki, Kazuya*; Aphecetche, L.*; Armendariz, R.*; et al.

Physical Review C, 83(6), p.064903_1 - 064903_29, 2011/06

 Times Cited Count:200 Percentile:99.33(Physics, Nuclear)

Transverse momentum distributions and yields for $$pi^{pm}, K^{pm}, p$$, and $$bar{p}$$ in $$p + p$$ collisions at $$sqrt{s}$$ = 200 and 62.4 GeV at midrapidity are measured by the PHENIX experiment at the RHIC. We present the inverse slope parameter, mean transverse momentum, and yield per unit rapidity at each energy, and compare them to other measurements at different $$sqrt{s}$$ collisions. We also present the scaling properties such as $$m_T$$ and $$x_T$$ scaling and discuss the mechanism of the particle production in $$p + p$$ collisions. The measured spectra are compared to next-to-leading order perturbative QCD calculations.

Journal Articles

Azimuthal correlations of electrons from heavy-flavor decay with hadrons in $$p+p$$ and Au+Au collisions at $$sqrt{s_{NN}}$$ = 200 GeV

Adare, A.*; Afanasiev, S.*; Aidala, C.*; Ajitanand, N. N.*; Akiba, Yasuyuki*; Al-Bataineh, H.*; Alexander, J.*; Aoki, Kazuya*; Aphecetche, L.*; Aramaki, Y.*; et al.

Physical Review C, 83(4), p.044912_1 - 044912_16, 2011/04

 Times Cited Count:10 Percentile:53.47(Physics, Nuclear)

Measurements of electrons from the decay of open-heavy-flavor mesons have shown that the yields are suppressed in Au+Au collisions compared to expectations from binary-scaled $$p+p$$ collisions. Here we extend these studies to two particle correlations where one particle is an electron from the decay of a heavy flavor meson and the other is a charged hadron from either the decay of the heavy meson or from jet fragmentation. These measurements provide more detailed information about the interaction between heavy quarks and the quark-gluon matter. We find the away-side-jet shape and yield to be modified in Au+Au collisions compared to $$p+p$$ collisions.

Journal Articles

Measurement of neutral mesons in $$p$$ + $$p$$ collisions at $$sqrt{s}$$ = 200 GeV and scaling properties of hadron production

Adare, A.*; Afanasiev, S.*; Aidala, C.*; Ajitanand, N. N.*; Akiba, Y.*; Al-Bataineh, H.*; Alexander, J.*; Aoki, K.*; Aphecetche, L.*; Armendariz, R.*; et al.

Physical Review D, 83(5), p.052004_1 - 052004_26, 2011/03

 Times Cited Count:190 Percentile:98.26(Astronomy & Astrophysics)

The PHENIX experiment at RHIC has measured the invariant differential cross section for production of $$K^0_s$$, $$omega$$, $$eta'$$ and $$phi$$ mesons in $$p + p$$ collisions at $$sqrt{s}$$ = 200 GeV. The spectral shapes of all hadron transverse momentum distributions are well described by a Tsallis distribution functional form with only two parameters, $$n$$ and $$T$$, determining the high $$p_T$$ and characterizing the low $$p_T$$ regions for the spectra, respectively. The integrated invariant cross sections calculated from the fitted distributions are found to be consistent with existing measurements and with statistical model predictions.

Journal Articles

Identification of a new band and its signature inversion in $$^{174}$$Re

Zhang, Y. H.*; Guo, S.*; Zhou, X. H.*; Ma, L.*; Guo, W. T.*; Oshima, Masumi; Toh, Yosuke; Koizumi, Mitsuo; Osa, Akihiko; Kimura, Atsushi; et al.

Chinese Physics Letters, 24(5), p.1203 - 1206, 2007/05

High-spin states in $$^{174}$$Re are investigated via in-beam $$gamma$$-ray spectroscopic method and $$gamma - gamma$$ coincidence relationships are analysed. A new band is identified due to its spectroscopic connection with the known $$pi 1/2^-[541] bigotimes nu 1/2^-[521]$$ band. This band is proposed to be the ground-state band built on the $$pi 1/2^-[541] bigotimes nu 5/2^-[512]$$ configuration in view of the low-lying intrinsic states in neighbouring odd-mass nuclei. It is in particular interesting that the new band exhibits a phenomenon of low-spin signature inversion, providing a new situation for theoretical investigations.

Journal Articles

Self-guiding of 100 TW femtosecond laser pulses in centimeter-scale underdense plasma

Chen, L.-M.; Kotaki, Hideyuki; Nakajima, Kazuhisa*; Koga, J. K.; Bulanov, S. V.; Tajima, Toshiki; Gu, Y. Q.*; Peng, H. S.*; Wang, X. X.*; Wen, T. S.*; et al.

Physics of Plasmas, 14(4), p.040703_1 - 040703_4, 2007/04

 Times Cited Count:39 Percentile:75.17(Physics, Fluids & Plasmas)

An experiment for the laser self-guiding studies has been carried out with 100 TW laser pulse interaction with the long underdense plasma. Formation of extremely long plasma channel with its length, about 10 mm, 20 times above the Rayleigh length is observed. The self-focusing channel features such as the laser pulse significant bending and the electron cavity formation are demonstrated experimentally for the first time.

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