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Zhang, M. M.*; Tian, Y. L.*; Wang, Y. S.*; Zhang, Z. Y.*; Gan, Z. G.*; Yang, H. B.*; Huang, M. H.*; Ma, L.*; Yang, C. L.*; Wang, J. G.*; et al.
Physical Review C, 106(2), p.024305_1 - 024305_6, 2022/08
Times Cited Count:1 Percentile:47.37(Physics, Nuclear)Tanaka, Junki*; Yang, Z.*; Typel, S.*; Adachi, Satoshi*; Bai, S.*; Van Beek, P.*; Beaumel, D.*; Fujikawa, Yuki*; Han, J.*; Heil, S.*; et al.
Science, 371(6526), p.260 - 264, 2021/01
Times Cited Count:30 Percentile:98.69(Multidisciplinary Sciences)By employing quasi-free -cluster-knockout reactions, we obtained direct experimental evidence for the formation of
clusters at the surface of neutron-rich tin isotopes. The observed monotonous decrease of the reaction cross sections with increasing mass number, in excellent agreement with the theoretical prediction, implies a tight interplay between
-cluster formation and the neutron skin.
Lam, T.-N.*; Lee, S. Y.*; Tsou, N.-T.*; Chou, H.-S.*; Lai, B.-H.*; Chang, Y.-J.*; Feng, R.*; Kawasaki, Takuro; Harjo, S.; Liaw, P. K.*; et al.
Acta Materialia, 201, p.412 - 424, 2020/12
Times Cited Count:31 Percentile:93.34(Materials Science, Multidisciplinary)Sato, Yusuke*; Fukaya, Yuki; Cameau, M.*; Kundu, A. K.*; Shiga, Daisuke*; Yukawa, Ryu*; Horiba, Koji*; Chen, C.-H.*; Huang, A.*; Jeng, H.-T.*; et al.
Physical Review Materials (Internet), 4(6), p.064005_1 - 064005_6, 2020/06
Times Cited Count:6 Percentile:36.6(Materials Science, Multidisciplinary)no abstracts in English
Naeem, M.*; He, H.*; Zhang, F.*; Huang, H.*; Harjo, S.; Kawasaki, Takuro; Wang, B.*; Lan, S.*; Wu, Z.*; Wang, F.*; et al.
Science Advances (Internet), 6(13), p.eaax4002_1 - eaax4002_8, 2020/03
Times Cited Count:123 Percentile:99.1(Multidisciplinary Sciences)Sun, M. D.*; Liu, Z.*; Huang, T. H.*; Zhang, W. Q.*; Andreyev, A. N.; Ding, B.*; Wang, J. G.*; Liu, X. Y.*; Lu, H. Y.*; Hou, D. S.*; et al.
Physics Letters B, 800, p.135096_1 - 135096_5, 2020/01
Times Cited Count:10 Percentile:81.53(Astronomy & Astrophysics)Tanaka, Taiki*; Narikiyo, Yoshihiro*; Morita, Kosuke*; Fujita, Kunihiro*; Kaji, Daiya*; Morimoto, Koji*; Yamaki, Sayaka*; Wakabayashi, Yasuo*; Tanaka, Kengo*; Takeyama, Mirei*; et al.
Journal of the Physical Society of Japan, 87(1), p.014201_1 - 014201_9, 2018/01
Times Cited Count:16 Percentile:73.87(Physics, Multidisciplinary)Excitation functions of quasielastic scattering cross sections for the Ca +
Pb,
Ti +
Pb, and
Ca +
Cm reactions were successfully measured by using the gas-filled recoil-ion separator GARIS. Fusion barrier distributions were extracted from these data, and compared with the coupled-channels calculations. It was found that the peak energies of the barrier distributions for the
Ca +
Pb and
Ti +
Pb systems coincide with those of the 2n evaporation channel cross sections for the systems, while that of the
Ca +
Cm is located slightly below the 4n evaporation ones. This results provide us helpful information to predict the optimum beam energy to synthesize superheavy nuclei.
Kaji, Daiya*; Morita, Kosuke*; Morimoto, Koji*; Haba, Hiromitsu*; Asai, Masato; Fujita, Kunihiro*; Gan, Z.*; Geissel, H.*; Hasebe, Hiroo*; Hofmann, S.*; et al.
Journal of the Physical Society of Japan, 86(3), p.034201_1 - 034201_7, 2017/03
Times Cited Count:24 Percentile:81.31(Physics, Multidisciplinary)The fusion reaction of Ca +
Cm
Lv
was studied using the gas-filled recoil-ion separator GARIS at RIKEN. A total of seven
and spontaneous-fission decay chains were observed, which would originate from the reaction products of the element 116,
Lv and
Lv. Decay properties observed in the chains are in good agreement with the previously published ones. However, one of the chains showed a discrepancy, indicating the new spontaneous-fission branch in
Cn or the production of the new isotope
Lv.
Usoltsev, I.*; Eichler, R.*; Wang, Y.*; Even, J.*; Yakushev, A.*; Haba, Hiromitsu*; Asai, Masato; Brand, H.*; Di Nitto, A.*; Dllmann, Ch. E.*; et al.
Radiochimica Acta, 104(3), p.141 - 151, 2016/03
Times Cited Count:30 Percentile:95.47(Chemistry, Inorganic & Nuclear)Conditions of the production and decomposition of hexacarbonyl complexes of short-lived Mo and W isotopes were investigated to study thermal stability of the heaviest group 6 hexacarbonyl complex Sg(CO). A tubular flow reactor was tested to decompose the hexacarbonyl complexes and to extract the first bond dissociation energies. A silver was found to be the most appropriate reaction surface to study the decomposition of the group 6 hexacarbonyl. It was found that the surface temperature at which the decomposition occurred was correlated to the first bond dissociation energy of Mo(CO)
and W(CO)
, indicating that the first bond dissociation energy of Sg(CO)
could be determined with this technique.
Even, J.*; Ackermann, D.*; Asai, Masato; Block, M.*; Brand, H.*; Di Nitto, A.*; Dllmann, Ch. E.*; Eichler, R.*; Fan, F.*; Haba, Hiromitsu*; et al.
Journal of Radioanalytical and Nuclear Chemistry, 303(3), p.2457 - 2466, 2015/03
Times Cited Count:14 Percentile:77.04(Chemistry, Analytical)Rapid In situ synthesis of metal carbonyl complexes has been demonstrated using short-lived isotopes produced in nuclear fission and fusion reactions. The short-lived isotopes with high recoil energy directly react with carbon-monoxides and form carbonyl complexes. Only highly volatile complexes were fast transported in a gas stream to counting and chemistry devices. Short-lived Mo, Tc, Ru, Rh, W, Re, Os, and Ir were found to form volatile carbonyl complexes, while no volataile complex of Hf and Ta were detected. This technique has been applied to a chemical investigation of the superheavy element Sg (atomic number 106), and will be applicable to various fields of nuclear science with short-lived transition metal isotopes.
Oe, Kazuhiro*; Attallah, M. F.*; Asai, Masato; Goto, Naoya*; Gupta, N. S.*; Haba, Hiromitsu*; Huang, M.*; Kanaya, Jumpei*; Kaneya, Yusuke*; Kasamatsu, Yoshitaka*; et al.
Journal of Radioanalytical and Nuclear Chemistry, 303(2), p.1317 - 1320, 2015/02
Times Cited Count:8 Percentile:58.17(Chemistry, Analytical)A new technique for continuous dissolution of nuclear reaction products transported by a gas-jet system was developed for superheavy element (SHE) chemistry. In this technique, a hydrophobic membrane is utilized to separate an aqueous phase from the gas phase. With this technique, the dissolution efficiencies of short-lived radionuclides of Mo and
W were measured. Yields of more than 80% were observed for short-lived radionuclides at aqueous-phase flow rates of 0.1-0.4 mL/s. The gas flow-rate had no influence on the dissolution efficiency within the studied flow range of 1.0-2.0 L/min. These results show that this technique is applicable for on-line chemical studies of SHEs in the liquid phase.
Even, J.*; Yakushev, A.*; Dllmann, Ch. E.*; Haba, Hiromitsu*; Asai, Masato; Sato, Tetsuya; Brand, H.*; Di Nitto, A.*; Eichler, R.*; Fan, F. L.*; et al.
Science, 345(6203), p.1491 - 1493, 2014/09
Times Cited Count:60 Percentile:83.11(Multidisciplinary Sciences)A new superheavy element complex, a seaborgium carbonyl, has been successfully synthesized, and its adsorption property has been studied using a cryo-thermochromatography and -detection apparatus COMPACT. Nuclear reaction products of short-lived
Sg preseparated with a gas-filled recoil ion separator GARIS at RIKEN were directly injected into a gas cell filled with He/CO mixture gas, and chemical reaction products of volatile carbonyl complexes were trasported to COMPACT. The Sg carbonyl complex detected with COMPACT was found to be very volatile with adsorption enthalpy of
50 kJ/mol, from which we have concluded that this complex should be a Sg hexacarbonyl Sg(CO)
. This is the first synthesis of organometallic compounds of transactinide elements for which only simple inorganic comounds have been synthesized so far.
Johnson, B. E.*; Santschi, P. H.*; Chuang, C.-Y.*; Otosaka, Shigeyoshi; Addleman, R. S.*; Douglas, M.*; Rutledge, R. D.*; Chouyyok, W.*; Davidson, J. D.*; Fryxell, G. E.*; et al.
Environmental Science & Technology, 46(20), p.11251 - 11258, 2012/11
Times Cited Count:81 Percentile:88.84(Engineering, Environmental)Effective collection of trace-level lanthanides and actinides is advantageous for recovery and recycling of valuable resources, environmental remediation, chemical separations, and in situ monitoring. Using isotopic tracers, we have evaluated a number of conventional and nanoporous sorbent materials for their ability to capture and remove selected lanthanides (Ce and Eu) and actinides (Th, Pa, U, and Np) from fresh and salt water systems. In general, the nanostructured materials demonstrated a higher level of performance and consistency. Nanoporous silica surface modified with 3,4-hydroxypyridinone provided excellent collection and consistency in both river water and seawater.
Adare, A.*; Afanasiev, S.*; Aidala, C.*; Ajitanand, N. N.*; Akiba, Yasuyuki*; Al-Bataineh, H.*; Alexander, J.*; Aoki, Kazuya*; Aphecetche, L.*; Armendariz, R.*; et al.
Physical Review C, 83(6), p.064903_1 - 064903_29, 2011/06
Times Cited Count:176 Percentile:99.44(Physics, Nuclear)Transverse momentum distributions and yields for , and
in
collisions at
= 200 and 62.4 GeV at midrapidity are measured by the PHENIX experiment at the RHIC. We present the inverse slope parameter, mean transverse momentum, and yield per unit rapidity at each energy, and compare them to other measurements at different
collisions. We also present the scaling properties such as
and
scaling and discuss the mechanism of the particle production in
collisions. The measured spectra are compared to next-to-leading order perturbative QCD calculations.
Adare, A.*; Afanasiev, S.*; Aidala, C.*; Ajitanand, N. N.*; Akiba, Yasuyuki*; Al-Bataineh, H.*; Alexander, J.*; Aoki, Kazuya*; Aphecetche, L.*; Aramaki, Y.*; et al.
Physical Review C, 83(4), p.044912_1 - 044912_16, 2011/04
Times Cited Count:7 Percentile:46.61(Physics, Nuclear)Measurements of electrons from the decay of open-heavy-flavor mesons have shown that the yields are suppressed in Au+Au collisions compared to expectations from binary-scaled collisions. Here we extend these studies to two particle correlations where one particle is an electron from the decay of a heavy flavor meson and the other is a charged hadron from either the decay of the heavy meson or from jet fragmentation. These measurements provide more detailed information about the interaction between heavy quarks and the quark-gluon matter. We find the away-side-jet shape and yield to be modified in Au+Au collisions compared to
collisions.
Adare, A.*; Afanasiev, S.*; Aidala, C.*; Ajitanand, N. N.*; Akiba, Y.*; Al-Bataineh, H.*; Alexander, J.*; Aoki, K.*; Aphecetche, L.*; Armendariz, R.*; et al.
Physical Review D, 83(5), p.052004_1 - 052004_26, 2011/03
Times Cited Count:169 Percentile:98.48(Astronomy & Astrophysics)The PHENIX experiment at RHIC has measured the invariant differential cross section for production of ,
,
and
mesons in
collisions at
= 200 GeV. The spectral shapes of all hadron transverse momentum distributions are well described by a Tsallis distribution functional form with only two parameters,
and
, determining the high
and characterizing the low
regions for the spectra, respectively. The integrated invariant cross sections calculated from the fitted distributions are found to be consistent with existing measurements and with statistical model predictions.
Chen, L.-M.; Kotaki, Hideyuki; Nakajima, Kazuhisa*; Koga, J. K.; Bulanov, S. V.; Tajima, Toshiki; Gu, Y. Q.*; Peng, H. S.*; Wang, X. X.*; Wen, T. S.*; et al.
Physics of Plasmas, 14(4), p.040703_1 - 040703_4, 2007/04
Times Cited Count:36 Percentile:76.18(Physics, Fluids & Plasmas)An experiment for the laser self-guiding studies has been carried out with 100 TW laser pulse interaction with the long underdense plasma. Formation of extremely long plasma channel with its length, about 10 mm, 20 times above the Rayleigh length is observed. The self-focusing channel features such as the laser pulse significant bending and the electron cavity formation are demonstrated experimentally for the first time.
Miyashita, Sunao; Toyoshima, Atsushi; Oe, Kazuhiro*; Asai, Masato; Sato, Tetsuya; Tsukada, Kazuaki; Nagame, Yuichiro; Schdel, M.; Kaneya, Yusuke; Haba, Hiromitsu*; et al.
no journal, ,
Solvent extraction of Mo and
W using 4-isopropyltropolone (Hinokitiol, HT) was investigated. Extraction mechanism of Mo and W with HT was examined by slope analysis. The slopse of the distribution ratio of Mo and W vs. [HT] in logarithmic scale are 1.88 and 1.54, respectively.
Miyashita, Sunao; Toyoshima, Atsushi; Oe, Kazuhiro*; Sato, Tetsuya; Asai, Masato; Tsukada, Kazuaki; Nagame, Yuichiro; Schdel, M.; Kaneya, Yusuke; Haba, Hiromitsu*; et al.
no journal, ,
The extraction behavior of hexavalent and reduced Mo and W were investigated when aqueous phase was 0.1 M HCl/0.9 M LiCl solution. The D value of Mo was changed from 10 to 1 when applied potential was near 0 to -0.2 V. On the other hand, the D value of W was not changed at all applied potentials in this experimental condition. Those results indicated that Mo was reduced by FEC, and the extraction behavior of reduced Mo was different from hexavalent Mo. In the case of W, W was not reduced or the D values of reduced W was same as hexavalent W.
Toyoshima, Atsushi; Miyashita, Sunao*; Asai, Masato; Sato, Tetsuya; Kaneya, Yusuke; Tsukada, Kazuaki; Kitatsuji, Yoshihiro; Nagame, Yuichiro; Schdel, M.; Lerum, H. V.*; et al.
no journal, ,
To carry out a continuous reduction experiment of Sg with the low production rates and the short half-life, we are developing a new chemistry assembly consisting of a membrane degasser (MDG), a flow electrolytic column (FEC), the continuous liquid-liquid extraction apparatus, and the liquid scintillation counting system (SISAK). Recently, we have begun preparatory studies with Mo and W isotopes. Aqueous solution dissolving Mo and W was successfully separated from a carrier gas. Redox couples of Mo(VI)/Mo(V) and W(VI)/W(V) in HCl have been characterized for their macro amounts. Extraction behavior of Mo(VI) and W(VI) between toluene containing hinokitiol (HT) and HCl was successfully observed by a batch method. On-line extractions of short-lived Mo and W were also carried out using SISAK and MDG. In the symposium, our present status of the preparation with Mo and W will be presented.