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Sato, Tetsuya; Asai, Masato; Borschevsky, A.*; Stora, T.*; Sato, Nozomi*; Kaneya, Yusuke; Tsukada, Kazuaki; Dllmann, C. E.*; Eberhardt, K.*; Eliav, E.*; et al.
EPJ Web of Conferences, 131, p.05001_1 - 05001_6, 2016/12
Times Cited Count:0 Percentile:0.9(Chemistry, Inorganic & Nuclear)Ionization efficiency in a surface ionization process depends on the first ionization potential of the atom. Based on the dependence, the ionization potential of the atom can be determined. We measured ionization efficiencies of fermium, einsteinium, mendelevium, and lawrencium by using a newly developed gas-jet coupled surface ion-source. The ionization potential of the elements have not been determined so far due to their low production rates and/or their short half-lives. Based on a relationship between the ionization efficiency and the ionization potential obtained via measurements of short-lived lanthanide isotopes, the ionization potentials of these actinide elements have been successfully determined.
Sato, Tetsuya; Asai, Masato; Borschevsky, A.*; Stora, T.*; Sato, Nozomi; Kaneya, Yusuke; Tsukada, Kazuaki; Dllmann, Ch. E.*; Eberhardt, K.*; Eliav, E.*; et al.
Nature, 520(7546), p.209 - 211, 2015/04
Times Cited Count:107 Percentile:97.49(Multidisciplinary Sciences)Ionization efficiency in a surface ionization process depends on the first ionization potential of the atom. Based on the dependence, the ionization potential of the atom can be determined. We successfully measured ionization efficiencies of lawrencium (Lr, =103) using a gas-jet coupled surface ion-source. The ionization potential of Lr has not been determined owing to its low production rate and its short half-life. Based on a relationship between the ionization efficiency and the ionization potential obtained via measurements of short-lived lanthanide isotopes, the ionization potential of Lr was determined.
Sato, Tetsuya; Asai, Masato; Sato, Nozomi; Tsukada, Kazuaki; Toyoshima, Atsushi; Oe, Kazuhiro*; Miyashita, Sunao*; Kaneya, Yusuke; Osa, Akihiko; Schdel, M.; et al.
Journal of Radioanalytical and Nuclear Chemistry, 303(2), p.1253 - 1257, 2015/02
Times Cited Count:8 Percentile:56.13(Chemistry, Analytical)We have developed a surface-ionization ion-source coupled to the He/CdI gas-jet transport system for the Isotope Separator On-Line (ISOL) at the JAEA tandem accelerator for experimental determination of the first ionization potential of lawrencium (Lr, ). We performed to ionize a short-lived Lr isotope and various lanthanide isotopes. We successfully observed mass-separated ions of Lr by using our present system at the first time. The first ionization potential of Lr was evaluated based on a correlation between of effective ionization potential and ionization efficiency of short-lived lanthanide isotopes in our system.
Sato, Nozomi; Sato, Tetsuya; Asai, Masato; Toyoshima, Atsushi; Tsukada, Kazuaki; Li, Z.*; Nishio, Katsuhisa; Nagame, Yuichiro; Schdel, M.; Haba, Hiromitsu*; et al.
Radiochimica Acta, 102(3), p.211 - 219, 2014/03
Times Cited Count:9 Percentile:57.19(Chemistry, Inorganic & Nuclear)Production cross-sections of the isotope Lr in the Cf + B, Am + O, and Cm + N reactions were measured using a He/KCl gas-jet transport system and a rotating wheel -particle detection apparatus. The -particle energy of Lr was distributed from 8.3 to 8.7 MeV and its half-life, , was measured to be s. The maximum cross sections in the Cf(B, 4)Lr and Am(O, 5)Lr reactions were determined to be nb at the beam energy of 63 MeV and nb at 96 MeV, respectively. In the Cm(N, 6)Lr reaction, the cross section was measured to be nb at 91 MeV.
Sato, Tetsuya; Sato, Nozomi; Asai, Masato; Tsukada, Kazuaki; Toyoshima, Atsushi; Oe, Kazuhiro; Miyashita, Sunao; Schdel, M.; Kaneya, Yusuke*; Nagame, Yuichiro; et al.
Review of Scientific Instruments, 84(2), p.023304_1 - 023304_5, 2013/02
Times Cited Count:16 Percentile:58.95(Instruments & Instrumentation)We have developed the surface ion-source coupled to the He/CdI gas-jet transport system to measure the ionization potential of Lr atatom-at-a-time conditions. We successfully ionized and mass-separated for the first time Lr ions by applying the present ion-source and the ISOL technique. The ionization efficiencies of Lr were estimated to be approximately 42% and 24% at 2600 K on Re and Ta surfaces, respectively. These values were higher than those of Lu in all of ionization condition. The results indicate that the ionization potential of Lr would be lower than that of Lu, 5.4 eV. Therefore, it is concluded that the surface ion-source is a promising apparatus tomeasure the first ionization potential of Lr. Using the present system, determination of the ionization potential of Lr is being performed.
Sato, Nozomi; Sato, Tetsuya; Asai, Masato; Toyoshima, Atsushi; Tsukada, Kazuaki; Li, Z.*; Nishio, Katsuhisa; Nagame, Yuichiro; Schdel, M.; Haba, Hiromitsu*; et al.
RIKEN Accelerator Progress Report, Vol.46, P. 237, 2013/00
Due to the strong relativistic effects, the weakly-bound outermost electron results in a significantly low first ionization potential (IP) of Lr as compared with its neighboring heavy actinides. The isotope Lr, with a relatively long half-life of 27 s, is the suitable candidates for the IP measurement of Lr through the surface ionization method. In the present study, we measured the cross section of the Cm(N, 6)Lr reaction to evaluate the production rate of Lr. A Cm target with 960 60 g/cm thickness was bombarded with a N beam from the RIKEN AVF Cyclotron. The beam energy was 91 MeV in the middle of the target. The average beam intensity was 1.2 particle-A. Reaction products were transported to the rotating wheel -particle detection system with a He/KCl gas-jet system. The Lr cross section of 271 nb was calculated based on the -particle events between 8.3 and 8.7 MeV.
Sato, Nozomi; Haba, Hiromitsu*; Ichikawa, Takatoshi*; Kaji, Daiya*; Kudo, Yuki*; Morimoto, Koji*; Morita, Kosuke*; Ozeki, Kazutaka*; Sumita, Takayuki*; Yoneda, Akira*; et al.
Journal of the Physical Society of Japan, 80(9), p.094201_1 - 094201_7, 2011/09
Times Cited Count:15 Percentile:65.33(Physics, Multidisciplinary)Decay properties of Hs and Hs produced in the Pb(Fe, ) [=1, 2] reactions were studied using a gas-filled recoil ion separator at the linear accelerator facility of RIKEN. A total of 6 decay chains were assigned to Hs. Cross sections for the Hs production in the Pb(Fe,) and Pb(Fe,) reactions were measured to be pb and pb, respectively. The isotope Hs decayed with a half-life of ms by -particle emission and spontaneous fission. The -particle energy of Hs was observed at 10.610.04 and 10.800.08 MeV. The spontaneous fission branch of Hs was found to be .
Morita, Kosuke*; Morimoto, Koji*; Kaji, Daiya*; Haba, Hiromitsu*; Ozeki, Kazutaka*; Kudo, Yuki*; Sato, Nozomi*; Sumita, Takayuki*; Yoneda, Akira*; Ichikawa, Takatoshi*; et al.
Journal of the Physical Society of Japan, 78(6), p.064201_1 - 064201_6, 2009/06
Times Cited Count:30 Percentile:78.34(Physics, Multidisciplinary)Decay properties of an isotope Bh and its daughter nucleus Db produced by the Cm(Na,5) reaction were studied by using a gas-filled recoil separator coupled with a position-sensitive semiconductor detector. Bh was clearly identified from the correlation of the known nuclide, Db. The obtained decay properties of Bh and Db are consistent with those observed in the 113 chain, which provided further confirmation of the discovery of 113.
Kaji, Daiya*; Morimoto, Koji*; Sato, Nozomi*; Ichikawa, Takatoshi*; Ideguchi, Eiji*; Ozeki, Kazutaka*; Haba, Hiromitsu*; Koura, Hiroyuki; Kudo, Yuki*; Ozawa, Akira*; et al.
Journal of the Physical Society of Japan, 78(3), p.035003_1 - 035003_2, 2009/03
A new hassium isotopes Hs is directly produced for the first time. The experiment was performed at the linear accelerator (RILAC) facility in RIKEN (the Institute of Physical and Chemical Research) from Jun. 19 to 25. In the 25-h irradiation of Fe on Pb and 46-h irradiation of Fe on Pb, 8 decay chains and 1 decay chain, respectively, were observed. All decay chains were assigned to subsequent decays from Hs. The half-life of Hs is 0.60 ms. In this experiment, the total beam dose was ions for Fe and ions for Fe. The production cross section corresponding to 8 decay events and 1 decay chain was deduced to be 21 pb and 1.6 pb by assuming that the transmission of the system is 80%.
Kaji, Daiya*; Morimoto, Koji*; Sato, Nozomi*; Ichikawa, Takatoshi*; Ideguchi, Eiji*; Ozeki, Kazutaka*; Haba, Hiromitsu*; Koura, Hiroyuki; Kudo, Yuki*; Ozawa, Akira*; et al.
Journal of the Physical Society of Japan, 78(3), p.035003_1 - 035003_2, 2009/03
Times Cited Count:3 Percentile:26.3(Physics, Multidisciplinary)A new neutron deficient hassium (=108) isotope of Hs was identified via two different reactions of Pb(Fe,n) and Pb(Fe,n) by using a gas-filled recoil separator GARIS at June 2008. During the 25-h irradiation of Pb with the Fe beam and 46-h irradiation of Pb with the Fe beam, 8 decay chains and 1 decay chain, respectively, have been observed. The half-life of Hs is 0.60 ms. In this experiment, the total beam doses of the Fe and Fe was 4.110 ions and 6.210 ions, respectively. The production cross sections corresponding to the 8 decay chains and 1 decay chain have been deduced to be 21 pb and 1.6 pb by assuming the transmission of the system to be 80%.
Sato, Nozomi*; Haba, Hiromitsu*; Ichikawa, Takatoshi*; Ideguchi, Eiji*; Kaji, Daiya*; Koura, Hiroyuki; Kudo, Yuki*; Morimoto, Koji*; Morita, Kosuke*; Ozawa, Akira*; et al.
RIKEN Accelerator Progress Report, Vol.42, P. 16, 2009/00
New Decay Properties of Hs and its -decay daughter nuclei were studied by using reactions of Pb(Fe,2n) and Pb(Fe,n) by using a gas-filled recoil ion separator, GARIS at RIKEN. We observed three correlated events in irradiation of Fe on Pb, and eight events in irradiation of Fe on Pb. A half-life was deduced to be 0.90. We assigned these eleven events to be the decays of Hs. We found different decay-chain events of Hs from a previous report. One is a long-lived -decay of Sg with 180ms of half-life. Another is a long-lived -decay of Rf with 10.4s of half-life. For Sg and Rf, the decay of such a long-lived state have not been reported. These are the first observations of isomerism in Sg and Rf.
Sato, Nozomi; Kaji, Daiya*; Morimoto, Koji*; Haba, Hiromitsu*; Ichikawa, Takatoshi*; Ideguchi, Eiji*; Koura, Hiroyuki; Kudo, Yuki*; Ozawa, Akira*; Ozeki, Kazutaka*; et al.
no journal, ,
In this work, the production and decay properties of Hs produced in the Pb(Fe, ) [] and Pb(Fe, ) reactions were investigated. The experiment was performed at the RILAC facility in RIKEN. The evaporation residues (ERs) were separated from the primary beam with the gas-filled recoil ion separator, GARIS. In the focal plane of GARIS the products were implanted into a position-sensitive Si detector for measuring the arrival of ERs and subsequent -decays or spontaneous fission from ERs. We have measured production cross-sections of Hs in the Fe + Pb reaction at several bombarding energies. For the Pb(Fe, )Hs reaction, the cross-section maximum of () pb was obtained at the bombarding energy of 220.5 MeV at the middle of the target. For even-even nucleus Hs, we have also observed accurate decay data with good statistics.
Kaji, Daiya*; Morimoto, Koji*; Sato, Nozomi; Haba, Hiromitsu*; Ichikawa, Takatoshi*; Ideguchi, Eiji*; Koura, Hiroyuki; Kudo, Yuki*; Ozawa, Akira*; Ozeki, Kazutaka*; et al.
no journal, ,
A new neutron deficient hassium () isotope of Hs was identified via two different reactions of Pb(Fe,) and Pb(Fe,) by using the gas-filled recoil separator GARIS. During irradiation of Pb with the Fe beam and irradiation of Pb with the Fe beam, 8 decay chains and 1 decay chain, respectively, were observed. The properties of decay events obtained by irradiation of Fe on Pb match well with those by irradiation of Fe on Pb. The mean -decay energies for the 3 groups are 10.82, 10.55, and 10.37 MeV, respectively. The half-life of Hs is determined to be 0.60 ms.
Morimoto, Koji*; Morita, Kosuke*; Kaji, Daiya*; Haba, Hiromitsu*; Ozeki, Kazutaka*; Kudo, Yuki*; Sato, Nozomi; Sumita, Takayuki*; Yoneda, Akira*; Ichikawa, Takatoshi*; et al.
no journal, ,
A nuclide, Bh, is the great-grand-daughter of 113 that is produced in the Bi + Zn reaction. The identification was based on a genetic link to the known daughter nucleus Db by alpha-decays. The main purpose of this work is to provide further confirmation of the production and identification of the isotope 113. As a present result, a state in Bh, which decays by an alpha emission with the energies ranging from 9.05 to 9.23 MeV, feeds a state in Db, which decays by alpha emission and by SF with a previously known half-life. The result provided a further confirmation of the production and identification of the isotope of the 113th element, 113, studied by a research group at RIKEN.
Morimoto, Koji*; Morita, Kosuke*; Kaji, Daiya*; Haba, Hiromitsu*; Ozeki, Kazutaka*; Kudo, Yuki*; Sato, Nozomi; Sumita, Takayuki*; Yoneda, Akira*; Ichikawa, Takatoshi*; et al.
no journal, ,
no abstracts in English
Kaji, Daiya*; Morimoto, Koji*; Sato, Nozomi; Haba, Hiromitsu*; Ichikawa, Takatoshi*; Ideguchi, Eiji*; Koura, Hiroyuki; Kudo, Yuki*; Ozawa, Akira*; Ozeki, Kazutaka*; et al.
no journal, ,
no abstracts in English
Sato, Nozomi; Kaji, Daiya*; Morimoto, Koji*; Haba, Hiromitsu*; Ichikawa, Takatoshi*; Ideguchi, Eiji*; Koura, Hiroyuki; Kudo, Yuki*; Ozawa, Akira*; Ozeki, Kazutaka*; et al.
no journal, ,
In the superheavy nuclei region, the deformed proton shell at and neutron shells at and 162 have been found. Hs with and is expected to be the doubly deformed magic nuclei, however, decay properties of Hs and its neighboring nuclei is not well known. In order to approach Hs, we synthesized Hs by Pb(Fe,xn) [], Pb(Fe,n), Pb(Fe,n), Pb(Fe,n) reactions. The experiment was performed with the gas-filled recoil ion separator GARIS at the linear accelerator facility in RIKEN. In this work, 9 -decay events of Hs were observed with half-life ms and -decay energy MeV. For Hs, we have also observed new -particle energy, 10.65 MeV. values of Hs isotopes increase with decreasing neutron number.
Sato, Nozomi; Asai, Masato; Tsukada, Kazuaki; Sato, Tetsuya; Toyoshima, Atsushi; Li, Z.; Nagame, Yuichiro; Schdel, M.; Ichikawa, Shinichi
no journal, ,
First ionization potentials (IPs) of heavy elements with atomic numbers Z 100 have not been determined up to now. Recently we have been developing a surface ionization type ion source to measure the IP of the heaviest actinide, lawrencium (Lr, Z = 103). The surface ionization comparison technique is a promising approach to measure the IP of Lr on an atom-at-a-time scale. We will present the status of our development for an apparatus for this measurement.
Sato, Nozomi; Asai, Masato; Tsukada, Kazuaki; Sato, Tetsuya; Toyoshima, Atsushi; Li, Z.; Kikuchi, Takahiro; Kaneya, Yusuke*; Ichikawa, Shinichi; Nagame, Yuichiro; et al.
no journal, ,
It is important to determine the first ionization potentials (IPs) of the heaviest elements with atomic number Z 100 to understand their valence electronic structure affected by relativistic effects. Due to low production rates and short half-lives of the heaviest nuclides, IPs of these elements have not been so far determined. We are developing a surface-ionization-type ion source coupled to a gas-jet transport system in the Isotope Separator On-Line (ISOL) at the JAEA tandem accelerator facility to measure the IP of the heaviest actinide, lawrencium (Lr, Z = 103). In the symposium, we report the present status of the development of the apparatus. Production yield measurements of Lr (half-life 27 s), that is suitable for this study, will be also presented.
Morimoto, Koji*; Morita, Kosuke*; Kaji, Daiya*; Haba, Hiromitsu*; Ozeki, Kazutaka*; Kudo, Yuki*; Sato, Nozomi; Sumita, Takayuki*; Yoneda, Akira*; Ichikawa, Takatoshi*; et al.
no journal, ,
We performed the experiment to synthesize an isotope of the element 113 produced by a Bi(Zn,n)113 reaction using a gas-filled recoil ion separator (GARIS) at RIKEN. Two decay chains were observed, and assigned to those originating from an isotope 113. Both chains were connected into the previously known decays of Bh and Db via previously unknown decays of 113, Rg, and Mt. Although the Bh was known nuclide, a number of atoms reported so far was limited. In order to study more precise decay property of the Bh, we performed the direct production of Bh by the Cm(Na,5n)Bh reaction. In this experiment, the Bh was clearly identified from the correlation of the nuclide, Db. The obtained decay properties of Bh and Db are consistent with those observed in the 113 chain, which provided further confirmation of the discovery of 113.