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Journal Articles

Investigation of snow cover effects and attenuation correction of $$gamma$$ ray in aerial radiation monitoring

Ishizaki, Azusa; Sanada, Yukihisa; Mori, Airi; Imura, Mitsuo; Ishida, Mutsushi; Munakata, Masahiro

Remote Sensing, 8(11), p.892_1 - 892_12, 2016/11

 Times Cited Count:6 Percentile:25.09(Environmental Sciences)

In aerial radiation monitoring (ARM), the air dose rate cannot be appropriately estimated under snowy conditions due to attenuation of $$gamma$$ ray by the snow layer. A technique to address this issue is required for ARM to obtain enough signals for air dose rate. To develop this technique, we investigated the relationship between snow depth and ARM measurement results using ARM, laser imaging detection and ranging, and ground measurement before and after snowfall. From the measured data, the results obtained using three different correction factors were examined and compared. An appropriate correction improved the underestimation of the air dose rate. However, further improvement in the accuracy of the analysis require accurate estimation of the snow water equivalent.

JAEA Reports

Radiation monitoring using manned helicopter around the Nuclear Power Station in the fiscal year 2015 (Contract research)

Sanada, Yukihisa; Munakata, Masahiro; Mori, Airi; Ishizaki, Azusa; Shimada, Kazumasa; Hirouchi, Jun; Nishizawa, Yukiyasu; Urabe, Yoshimi; Nakanishi, Chika*; Yamada, Tsutomu*; et al.

JAEA-Research 2016-016, 131 Pages, 2016/10

JAEA-Research-2016-016.pdf:20.59MB

By the nuclear disaster of Fukushima Daiichi Nuclear Power Station (FDNPS), Tokyo Electric Power Company (TEPCO), caused by the East Japan earthquake and the following tsunami occurred on March 11, 2011, a large amount of radioactive materials was released from the NPS. After the nuclear disaster, airborne radiation monitoring using manned helicopter was conducted around FDNPS. In addition, background dose rate monitoring was conducted around Sendai Nuclear Power Station. These results of the aerial radiation monitoring using the manned helicopter in the fiscal 2015 were summarized in the report.

JAEA Reports

Radiation monitoring using manned helicopter around the Fukushima Daiichi Nuclear Power Station in the fiscal year 2014 (Contract research)

Sanada, Yukihisa; Mori, Airi; Ishizaki, Azusa; Munakata, Masahiro; Nakayama, Shinichi; Nishizawa, Yukiyasu; Urabe, Yoshimi; Nakanishi, Chika; Yamada, Tsutomu; Ishida, Mutsushi; et al.

JAEA-Research 2015-006, 81 Pages, 2015/07

JAEA-Research-2015-006.pdf:22.96MB

By the nuclear disaster of Fukushima Daiichi Nuclear Power Station (NPS), Tokyo Electric Power Company (TEPCO), caused by the East Japan earthquake and the following tsunami occurred on March 11, 2011, a large amount of radioactive materials was released from the NPP. These results of the aerial radiation monitoring using the manned helicopter in the fiscal 2014 were summarized in the report.

JAEA Reports

Radiation monitoring using manned helicopter around the Fukushima Daiichi Nuclear Power Station in the fiscal year 2013 (Contract research)

Sanada, Yukihisa; Nishizawa, Yukiyasu; Urabe, Yoshimi; Yamada, Tsutomu; Ishida, Mutsushi; Sato, Yoshiharu; Hirayama, Hirokatsu; Takamura, Yoshihide; Nishihara, Katsuya; Imura, Mitsuo; et al.

JAEA-Research 2014-012, 110 Pages, 2014/08

JAEA-Research-2014-012.pdf:169.17MB
JAEA-Research-2014-012(errata).pdf:0.27MB

By the nuclear disaster of Fukushima Daiichi Nuclear Power Station (NPS), Tokyo Electric Power Company (TEPCO), caused by the East Japan earthquake and the following tsunami occurred on March 11, 2011, a large amount of radioactive materials was released from the NPP. This document was summarized in the results of the aerial radiation monitoring using the manned helicopter in the fiscal 2013.

JAEA Reports

Research and development of in-situ measurement for radiation distribution of waterbed

Sanada, Yukihisa; Takamura, Yoshihide; Urabe, Yoshimi; Tsuchida, Kiyofumi; Nishizawa, Yukiyasu; Yamada, Tsutomu; Sato, Yoshiharu; Hirayama, Hirokatsu; Nishihara, Katsuya; Imura, Mitsuo; et al.

JAEA-Research 2014-005, 67 Pages, 2014/05

JAEA-Research-2014-005.pdf:52.68MB

Distribution of radiocesium existing on the waterbed such as lake or pond was concerned about at the present that passed for two years by an accident. Here, the direct measurement technique of the radiocesium concentration (in-situ measurement technique) was developed. This method was used an plastic scintillation detector (p-Scanner). This detector carried out quick measurement of a large area. In addition, the count-rate of p-Scanner was converted to the radiocesium concentration (Ba/kg-wet) by comparative measurement of $$gamma$$-ray spectrometer. We applied the technique to the agricultural pond in Fukushima and made a map of distribution of radiocesium concentration.

JAEA Reports

Radiation monitoring using the unmanned helicopter after the accident of the nuclear power plant

Sanada, Yukihisa; Nishizawa, Yukiyasu; Yamada, Tsutomu; Ikeda, Kazutaka*; Matsui, Masashi*; Tsuchida, Kiyofumi; Sato, Yoshiharu; Hirayama, Hirokatsu; Takamura, Yoshihide; Nishihara, Katsuya; et al.

JAEA-Research 2013-049, 129 Pages, 2014/03

JAEA-Research-2013-049.pdf:15.5MB

By the nuclear disaster of Fukushima Daiichi Nuclear Power Plant (NPP), Tokyo Electric Power Company (TEPCO), caused by the East Japan earthquake and the following tsunami occurred on March 11, 2011, a large amount of radioactive materials was released from the NPP. In recent years, technologies for autonomous unmanned helicopters (AUHs) have been developed and applied to natural disasters. In expectation of the application of the AUHs to aerial radiation monitoring, we had developed a remote radiation monitoring system. Then, we measured the radiation level by using unmanned helicopter in soil contaminated areas by radioactive cesium emitted from the NPP to evaluate ambient dose-rate distribution around the areas and to investigate the decontamination effect by the measurements before and after decontamination treatment. Here, we reports on the measurement technique and the result.

JAEA Reports

Measurement performance of the NDA using Q2 system for uranium waste drum

Ohara, Yoshiyuki; Naganuma, Masaki; Nohiro, Tetsuya*; Yoshida, Kimikazu*; Makita, Akinori*; Sakate, Mitsuo*; Irisawa, Takumi*; Murashita, Tatsuya*

JAEA-Technology 2012-048, 39 Pages, 2013/03

JAEA-Technology-2012-048.pdf:5.1MB

In Japan Atomic Energy Agency Ningyo-Toge Environmental Engineering Center, exploration for uranium and technical development of uranium refining, conversion and enrichment which are the front end of a nuclear fuel cycle have been performed since 1955. By these research and development, about 15000 radioactive waste (200 liter drum) has occurred by now. The analytical and measurement technique of the amount of uranium which are included in radioactive waste drum were very an inexperienced in those days. Therefore, measurement strict till 2002 was not able to be started. Such a situation as this, we introduced "Q2 low-level-waste drum measuring system" which is a bulk measuring method of the passive $$gamma$$ ray using a NaI scintillation detector in 2002. As a result, the total amount of uranium in a waste drum was estimated as about 20 tons.

Journal Articles

New result in the production and decay of an isotope, $$^{278}$$113 of the 113th element

Morita, Kosuke*; Morimoto, Koji*; Kaji, Daiya*; Haba, Hiromitsu*; Ozeki, Kazutaka*; Kudo, Yuki*; Sumita, Takayuki*; Wakabayashi, Yasuo*; Yoneda, Akira*; Tanaka, Kengo*; et al.

Journal of the Physical Society of Japan, 81(10), p.103201_1 - 103201_4, 2012/10

 Times Cited Count:179 Percentile:97.24(Physics, Multidisciplinary)

An isotope of the 113th element, $$^{278}$$113, was produced in a nuclear reaction with a $$^{70}$$Zn beam on a $$^{209}$$Bi target. We observed six consecutive $$alpha$$ decays following the implantation of a heavy particle in nearly the same position in the semiconductor detector, in extremely low background condition. The fifth and sixth decays are fully consistent with the sequential decays of $$^{262}$$Db and $$^{258}$$Lr both in decay energies and decay times. This indicates that the present decay chain consisted of $$^{278}$$113, $$^{274}$$Rg (Z = 111), $$^{270}$$Mt (Z = 109), $$^{266}$$Bh (Z = 107), $$^{262}$$Db (Z = 105), and $$^{258}$$Lr (Z = 103) with firm connections. This result, together with previously reported results from 2004 and 2007, conclusively leads the unambiguous production and identification of the isotope $$^{278}$$113, of the 113th element.

Journal Articles

Recent progress in the energy recovery linac project in Japan

Sakanaka, Shogo*; Akemoto, Mitsuo*; Aoto, Tomohiro*; Arakawa, Dai*; Asaoka, Seiji*; Enomoto, Atsushi*; Fukuda, Shigeki*; Furukawa, Kazuro*; Furuya, Takaaki*; Haga, Kaiichi*; et al.

Proceedings of 1st International Particle Accelerator Conference (IPAC '10) (Internet), p.2338 - 2340, 2010/05

Future synchrotron light source using a 5-GeV energy recovery linac (ERL) is under proposal by our Japanese collaboration team, and we are conducting R&D efforts for that. We are developing high-brightness DC photocathode guns, two types of cryomodules for both injector and main superconducting (SC) linacs, and 1.3 GHz high CW-power RF sources. We are also constructing the Compact ERL (cERL) for demonstrating the recirculation of low-emittance, high-current beams using above-mentioned critical technologies.

JAEA Reports

Recent progress of analytical methods of spent nuclear fuel, Review

Yoshida, Zenko; Watanabe, Kazuo; Ito, Mitsuo; Ueno, Takashi; Takeshita, Hidefumi

JAEA-Review 2008-062, 34 Pages, 2009/01

JAEA-Review-2008-062.pdf:4.07MB

Analytical methods for the spent nuclear fuel (SF) have been greatly innovated recently. This methodological innovation is mainly caused by rapid and remarkable progress of induced coupled plasma-mass spectrometry (ICP-MS) which is utilized for the isotopic analysis of actinoid elements (U, Np, Pu, Am, Cm) and fission product elements in the SF samples. The quantity of the objective element as well as the volume of the sample solution needed for the ICP-MS measurement are, in principle, much less than those required for the measurement by other analytical methods. ICP-MS makes it possible to reduce the radiation dose of the operator and to minimize the amount of the radioactive wastes generated from the analytical work. For the precise and accurate isotopic analysis of the objective element in the SF sample by mass spectrometry, the interfering element having isobars needs to be separated prior to the measurement. This review highlights the development of the separation methods and isotopic analysis methods for the analysis of the SF based on more than 50 recent publications and the future problems to be solved and prospects are discussed.

Journal Articles

Multiple $$gamma$$-ray detection method and its application to nuclear chemistry

Oshima, Masumi; Toh, Yosuke; Hatsukawa, Yuichi; Koizumi, Mitsuo; Kimura, Atsushi; Haraga, Tomoko; Ebihara, Mitsuru*; Sushida, Kazuyoshi*

Journal of Radioanalytical and Nuclear Chemistry, 278(2), p.257 - 262, 2008/11

 Times Cited Count:25 Percentile:81.22(Chemistry, Analytical)

It is well known that most radioactive nuclides emit coincident multiple $$gamma$$-rays. The multiple $$gamma$$-ray detection method takes advantage of this feature and the $$gamma$$-rays are detected in coincidence with a $$gamma$$-ray detector array. From the correlated data we can create a $$gamma$$-$$gamma$$ two-dimensional matrix or $$gamma$$-$$gamma$$-$$gamma$$ three-dimensional cube. On this matrix or cube an energy resolution much better than the ordinary one-dimensional spectrum can be achieved. Furthermore signal-to-noise ratio is considerably improved. Hence this method can be applied widely to radioactive nuclide analysis. In the talk I will present its typical application to the analysis of nuclear waste, neutron activation analysis (NAAMG), and prompt $$gamma$$-ray analysis (MPGA).

Journal Articles

Production of $$^{186 rm m}$$Re by proton bombardment of enriched $$^{186}$$W

Iimura, Hideki; Horiguchi, Takayoshi*; Ishida, Yoshihisa*; Ito, Mitsuo; Koizumi, Mitsuo; Miyabe, Masabumi; Oba, Masaki

Journal of the Physical Society of Japan, 77(2), p.025004_1 - 025004_2, 2008/02

 Times Cited Count:2 Percentile:19.78(Physics, Multidisciplinary)

The nucleus $$^{186 rm m}$$Re is of interest from the astrophysical point of view, since production of this nucleus in stars could change an accuracy of nucleo-cosmochronometer. In order to calculate the neutron capture cross section theoretically, it is necessary to know the spin of nucleus. However, the spin of $$^{186 rm m}$$Re has not been established so far. In order to clarify the nuclear structure of this nucleus, we plan laser spectroscopy of $$^{186 rm m}$$Re, and first, we measured the production yield of the ($$p,n$$) reaction. The experiment was carried out by irradiating a $$^{186}$$W target with a proton beam from the JAEA tandem accelerator. Rhenium was chemically separated from the irradiated sample, and then $$gamma$$-ray measurements were performed. As a result, we determined the production yield of the $$^{186}$$W($$p,n$$)$$^{186 rm m}$$Re reaction for the first time and suggested the same spin for $$^{186 rm m}$$Re as the known spin of $$I$$=8 for $$^{184 rm m}$$Re.

Journal Articles

Separation of americium from plutonium-solvent extraction raffinate and conversion to americium oxide

Sugikawa, Susumu; Nakazaki, Masato; Kimura, Akihiro; Kida, Takashi*; Kihara, Takehiro*; Akabori, Mitsuo; Minato, Kazuo; Suda, Kazuhiro*; Chikazawa, Takahiro*

Nihon Genshiryoku Gakkai Wabun Rombunshi, 6(4), p.476 - 483, 2007/12

A one-step simple extraction chromatography method using TODGA (${it N,N,N,N'}$-tetraoctyl-diglycolamide) adsorbent column has been developed to separate the americium from plutonium-solvent extraction raffinate. The raffinate contained Am($$sim$$620 mg/$$l$$), Np($$sim$$107 mg/$$l$$), Ag($$sim$$2000 mg/$$l$$), Fe($$sim$$290 mg/$$l$$), Cr($$sim$$38 mg/$$l$$), Ni($$sim$$52 mg/$$l$$) and trace of TBP. Small-scale and scale-up tests for separation of americium and conversion to americium oxide were carried out in NUCEF. Efforts were made to increase yield and purity of americium. The americium was separated with 83-92% yields and 97-98% purities by small-scale tests and 85-95% yields and 98-99% purities by scale-up tests. The yields for conversion of americium nitrate solution to americium oxide were 89-100% by small-scale tests and 85-96 % by scale-up tests. Approximately 1.8 gram americium oxide was recovered from 6 litres of the raffinate and supplied for the research on the high-temperature chemistry of TRU.

JAEA Reports

Development of module for TRU high temperature chemistry (Joint research)

Minato, Kazuo; Akabori, Mitsuo; Tsuboi, Takashi; Kurobane, Shiro; Hayashi, Hirokazu; Takano, Masahide; Otobe, Haruyoshi; Misumi, Masahiro*; Sakamoto, Takuya*; Kato, Isao*; et al.

JAERI-Tech 2005-059, 61 Pages, 2005/09

JAERI-Tech-2005-059.pdf:20.67MB

An experimental facility called the Module for TRU High Temperature Chemistry (TRU-HITEC) was installed in the Back-end Cycle Key Elements Research Facility (BECKY) of the Nuclear Fuel Cycle Safety Engineering Research Facility (NUCEF) for the basic studies of the behavior of the transuranium elements (TRU) in pyrochemical reprocessing and oxide fuels. TRU-HITEC consists of three alpha/gamma cells shielded by steel and polyethylene and a glove box shielded by leaded acrylic resin, where experimental apparatuses have been equipped and a high purity argon gas atmosphere is maintained. In the facility 10 g of $$^{241}$$Am as well as the other TRU of Np, Pu and Cm can be handled. This report summarizes the outline, structure, performance and interior apparatuses of the facility, and is the result of the joint research between the Japan Atomic Energy Research Institute and three electric power companies of Tokyo Electric Power Co., Tohoku Electric Power Co. and the Japan Atomic Power Co.

Journal Articles

Characterization of extreme ultraviolet emission from laser-produced spherical tin plasma generated with multiple laser beams

Shimada, Yoshinori*; Nishimura, Hiroaki*; Nakai, Mitsuo*; Hashimoto, Kazuhisa*; Yamaura, Michiteru*; Tao, Y.*; Shigemori, Keisuke*; Okuno, Tomoharu*; Nishihara, Katsunobu*; Kawamura, Toru*; et al.

Applied Physics Letters, 86(5), p.051501_1 - 051501_3, 2005/01

 Times Cited Count:115 Percentile:94.17(Physics, Applied)

no abstracts in English

Journal Articles

Determination of detection efficiency curves of HPGe detectors on radioactivity measurement of volume samples

Saegusa, Jun; Kawasaki, Katsuya; Mihara, Akira; Ito, Mitsuo; Yoshida, Makoto

Applied Radiation and Isotopes, 61(6), p.1383 - 1390, 2004/12

 Times Cited Count:29 Percentile:84.31(Chemistry, Inorganic & Nuclear)

no abstracts in English

Journal Articles

Characterizations of heavy ion irradiated PET membranes

Takahashi, Shuichi*; Yoshida, Masaru; Asano, Masaharu; Notomi, Mitsuo*; Nakagawa,Tsutomu*

Nuclear Instruments and Methods in Physics Research B, 217(3), p.435 - 441, 2004/05

 Times Cited Count:15 Percentile:67.04(Instruments & Instrumentation)

Various characterization were used to study the effect of heavy ion irradiation on a poly(ethylen terephthalate)(PET) membrane. My study was followed using some dynamic and thermal measurements with the aim to undestand the chemical change in the material by heavy ion irradiation. The anyalyese included DMA, tensile measurement, DSC and micro-FT-IR. The overall structure change in the PET polymer was investigated as a function of the Xe ion fluence in the range from 3$$times$$10$$^{3}$$ to 3$$times$$10$$^{9}$$ions/cm$$^{2}$$. Based on some mechanical measurements such as the tensile analysis and dynamic test, the heavy ion irradiated PET membranes exhibited a significant change in cross-linking. I believe that the secondary electron induced by collision between the irradiated ion and the constituent atoms of the membrane material form the cross-linking. The polymer chain scission and structure degradations are expected to result at higher ion fluence. Also, a slight change in the structure such as amorphization has been shown by DSC and the micro-FT-IR test.

JAEA Reports

Annual report on the services for chemical analysis and scientific glassblowing in the fiscal year 2001 and 2002

Ito, Mitsuo; Obara, Kazuhiro; Toida, Yukio*; Suzuki, Daisuke; Gunji, Katsubumi*; Watanabe, Kazuo

JAERI-Review 2004-007, 65 Pages, 2004/03

JAERI-Review-2004-007.pdf:5.53MB

no abstracts in English

Journal Articles

Nuclear moments and isotope shifts of $$^{135}$$La, $$^{137}$$La and $$^{138}$$La by collinear laser spectroscopy

Iimura, Hideki; Koizumi, Mitsuo; Miyabe, Masabumi; Oba, Masaki; Shibata, Takemasa; Shinohara, Nobuo; Ishida, Yoshihisa*; Horiguchi, Takayoshi*; Schuessler, H. A.*

Physical Review C, 68(5), p.054328_1 - 054328_7, 2003/11

 Times Cited Count:11 Percentile:57.41(Physics, Nuclear)

no abstracts in English

Journal Articles

A Laser ion source with a thin ohmic-heating ionizer for the TIARA-ISOL

Koizumi, Mitsuo; Osa, Akihiko; Oshima, Masumi; Sekine, Toshiaki; Wakui, Takashi*; Jin, W.*; Katsuragawa, H.*; Miyatake, Hiroari*; Ishida, Yoshihisa*

Nuclear Instruments and Methods in Physics Research B, 204(1-4), p.359 - 362, 2003/05

 Times Cited Count:7 Percentile:46.32(Instruments & Instrumentation)

no abstracts in English

42 (Records 1-20 displayed on this page)