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Journal Articles

First-principles simulation of an ejected electron produced by monochromatic deposition energy to water at the femtosecond order

Kai, Takeshi; Toigawa, Tomohiro; Matsuya, Yusuke; Hirata, Yuho; Tezuka, Tomoya*; Tsuchida, Hidetsugu*; Yokoya, Akinari*

RSC Advances (Internet), 13(46), p.32371 - 32380, 2023/11

 Times Cited Count:0 Percentile:0(Chemistry, Multidisciplinary)

Although scientific knowledge of photolysis and radiolysis of water is widely used in the life sciences and other fields, the formation mechanism of the spatial distribution of hydrated electrons (spur) resulting from energy deposition to water is still not well understood. The chemical reaction times of hydrated electrons, OH radicals, and H$$_{3}$$O$$^{+}$$ in the spur strongly depend on the spur radius. In our previous study, we elucidated the mechanism at a specific given energy (12.4 eV) by first-principles calculations. In the present study, we performed first-principles calculations of the spur radius at the deposition energies of 11-19 eV. The calculated spur radius is 3-10 nm, which is consistent with the experimental prediction (~4 nm) for the energy range of 8-12.4 eV, and the spur radius gradually increases with increasing energy. The spur radius is a new scientific knowledge and is expected to be widely used for estimating radiation DNA damage.

Journal Articles

Initial yield of hydrated electron production from water radiolysis based on first-principles calculation

Kai, Takeshi; Toigawa, Tomohiro; Matsuya, Yusuke*; Hirata, Yuho; Tezuka, Tomoya*; Tsuchida, Hidetsugu*; Yokoya, Akinari*

RSC Advances (Internet), 13(11), p.7076 - 7086, 2023/03

 Times Cited Count:3 Percentile:81.33(Chemistry, Multidisciplinary)

Scientific insights of water radiolysis are widely used in the life sciences and so on, however, the formation mechanism of radicals, a product of water radiolysis, is still not well understood. We are challenging to develop a simulation code to solve this formation mechanism from the viewpoint of radiation physics. Our first-principles calculations have revealed that the behavior of secondary electrons in water is governed not only by collisional effects but also by polarization effects. Furthermore, from the predicted ratio of ionization to electronic excitation, based on the spatial distribution of secondary electrons, we successfully reproduce the initial yield of hydrated electrons predicted in terms of radiation chemistry. The code provides us a reasonable spatiotemporal connection from radiation physics to radiation chemistry. Our findings are expected to provide newly scientific insights for understanding the earliest stages of water radiolysis.

Journal Articles

Progress report of Japanese simulation research projects using the high-performance computer system Helios in the International Fusion Energy Research Centre

Ishizawa, Akihiro*; Idomura, Yasuhiro; Imadera, Kenji*; Kasuya, Naohiro*; Kanno, Ryutaro*; Satake, Shinsuke*; Tatsuno, Tomoya*; Nakata, Motoki*; Nunami, Masanori*; Maeyama, Shinya*; et al.

Purazuma, Kaku Yugo Gakkai-Shi, 92(3), p.157 - 210, 2016/03

The high-performance computer system Helios which is located at The Computational Simulation Centre (CSC) in The International Fusion Energy Research Centre (IFERC) started its operation in January 2012 under the Broader Approach (BA) agreement between Japan and the EU. The Helios system has been used for magnetised fusion related simulation studies in the EU and Japan and has kept high average usage rate. As a result, the Helios system has contributed to many research products in a wide range of research areas from core plasma physics to reactor material and reactor engineering. This project review gives a short catalogue of domestic simulation research projects. First, we outline the IFERC-CSC project. After that, shown are objectives of the research projects, numerical schemes used in simulation codes, obtained results and necessary computations in future.

Journal Articles

Mechanism of synthesis of metallic oxide powder from aqueous metallic nitrate solution by microwave denitration method

Fukui, Kunihiro*; Igawa, Yusuke*; Arimitsu, Naoki*; Suzuki, Masahiro; Segawa, Tomoomi; Fujii, Kanichi*; Yamamoto, Tetsuya*; Yoshida, Hideto*

Chemical Engineering Journal, 211-212, p.1 - 8, 2012/11

 Times Cited Count:13 Percentile:41.13(Engineering, Environmental)

The process for synthesizing metallic oxide powders by the microwave denitration method was investigated using hexahydrated nickel nitrate and trihydrated copper nitrate aqueous solutions, and the electrical field and the temperature distributions in the reactor were numerically simulated. Although CuO powder can be obtained from a trihydrated copper nitrate aqueous solution by the microwave denitration method, a hexahydrated nickel nitrate aqueous solution cannot be heated up to over 270 $$^{circ}$$C by microwave irradiation. It was also found that the reaction routes for microwave heating are the same as those for conventional external heating. This finding indicates that the success of producing oxide particles by microwave denitration depends not only on the microwave absorptivity of the intermediate and the metallic oxide, but also on the temperature difference.

JAEA Reports

Conceptual design of the SlimCS fusion DEMO reactor

Tobita, Kenji; Nishio, Satoshi*; Enoeda, Mikio; Nakamura, Hirofumi; Hayashi, Takumi; Asakura, Nobuyuki; Uto, Hiroyasu; Tanigawa, Hiroyasu; Nishitani, Takeo; Isono, Takaaki; et al.

JAEA-Research 2010-019, 194 Pages, 2010/08

JAEA-Research-2010-019-01.pdf:48.47MB
JAEA-Research-2010-019-02.pdf:19.4MB

This report describes the results of the conceptual design study of the SlimCS fusion DEMO reactor aiming at demonstrating fusion power production in a plant scale and allowing to assess the economic prospects of a fusion power plant. The design study has focused on a compact and low aspect ratio tokamak reactor concept with a reduced-sized central solenoid, which is novel compared with previous tokamak reactor concept such as SSTR (Steady State Tokamak Reactor). The reactor has the main parameters of a major radius of 5.5 m, aspect ratio of 2.6, elongation of 2.0, normalized beta of 4.3, fusion out put of 2.95 GW and average neutron wall load of 3 MW/m$$^{2}$$. This report covers various aspects of design study including systemic design, physics design, torus configuration, blanket, superconducting magnet, maintenance and building, which were carried out increase the engineering feasibility of the concept.

Journal Articles

Compact DEMO, SlimCS; Design progress and issues

Tobita, Kenji; Nishio, Satoshi; Enoeda, Mikio; Kawashima, Hisato; Kurita, Genichi; Tanigawa, Hiroyasu; Nakamura, Hirofumi; Honda, Mitsuru; Saito, Ai*; Sato, Satoshi; et al.

Nuclear Fusion, 49(7), p.075029_1 - 075029_10, 2009/07

 Times Cited Count:137 Percentile:97.72(Physics, Fluids & Plasmas)

Recent design study on SlimCS focused mainly on the torus configuration including blanket, divertor, materials and maintenance scheme. For vertical stability of elongated plasma and high beta access, a sector-wide conducting shell is arranged in between replaceable and permanent blanket. The reactor adopts pressurized-water-cooled solid breeding blanket. Compared with the previous advanced concept with supercritical water, the design options satisfying tritium self-sufficiency are relatively scarce. Considered divertor technology and materials, an allowable heat load to the divertor plate should be 8 MW/m$$^{2}$$ or lower, which can be a critical constraint for determining a handling power of DEMO (a combination of alpha heating power and external input power for current drive).

Journal Articles

SlimCS; Compact low aspect ratio DEMO reactor with reduced-size central solenoid

Tobita, Kenji; Nishio, Satoshi; Sato, Masayasu; Sakurai, Shinji; Hayashi, Takao; Shibama, Yusuke; Isono, Takaaki; Enoeda, Mikio; Nakamura, Hirofumi; Sato, Satoshi; et al.

Nuclear Fusion, 47(8), p.892 - 899, 2007/08

 Times Cited Count:57 Percentile:86.6(Physics, Fluids & Plasmas)

The concept for a compact DEMO reactor named "SlimCS" is presented. Distinctive features of the concept is low aspect ratio ($$A$$ = 2.6) and use of a reduced-size center solenoid (CS) which has a function of plasma shaping rather than poloidal flux supply. The reduced-size CS enables us to introduce a thin toroidal field (TF) coil system which contributes to reducing the weight and construction cost of the reactor. SlimCS is as compact as advanced commercial reactor designs such as ARIES-RS and produces 1 GWe in spite of moderate requirements for plasma parameters. Merits of low-$$A$$, i.e. vertical stability for high elongation and high beta limit are responsible for such reasonable physics requirements.

Journal Articles

Concept of compact low aspect ratio Demo reactor, SlimCS

Tobita, Kenji; Nishio, Satoshi; Sato, Masayasu; Sakurai, Shinji; Hayashi, Takao; Shibama, Yusuke; Isono, Takaaki; Enoeda, Mikio; Nakamura, Hirofumi; Sato, Satoshi; et al.

Proceedings of 21st IAEA Fusion Energy Conference (FEC 2006) (CD-ROM), 8 Pages, 2006/10

no abstracts in English

Journal Articles

Design study of fusion DEMO plant at JAERI

Tobita, Kenji; Nishio, Satoshi; Enoeda, Mikio; Sato, Masayasu; Isono, Takaaki; Sakurai, Shinji; Nakamura, Hirofumi; Sato, Satoshi; Suzuki, Satoshi; Ando, Masami; et al.

Fusion Engineering and Design, 81(8-14), p.1151 - 1158, 2006/02

 Times Cited Count:123 Percentile:99.01(Nuclear Science & Technology)

no abstracts in English

Oral presentation

Successive magnetic transitions and ${it H-T}$ phase diagrams of Kagom$'e$ staircase compound Co$$_{3}$$V$$_{2}$$O$$_{8}$$

Yasui, Yukio*; Kobayashi, Yusuke*; Moyoshi, Taketo*; Soda, Minoru*; Sato, Masatoshi*; Igawa, Naoki; Kakurai, Kazuhisa

no journal, , 

no abstracts in English

Oral presentation

Development of synthesis process of nikel oxide powder by microwave

Segawa, Tomoomi; Suzuki, Masahiro; Fujii, Kanichi; Igawa, Yusuke*; Arimitsu, Naoki*; Yamamoto, Tetsuya*; Fukui, Kunihiro*; Yoshida, Hideto*

no journal, , 

The synthesis process of the denitration reaction by the microwave heating method was investigated using a nickel nitrate (Ni(NO$$_{3}$$)$$_{2}$$) aqueous solution. NiO powder cannot be obtained from Ni(NO$$_{3}$$)$$_{2}$$ aqueous solution by the microwave heating method because of low microwave absorption of the intermediate obtained from nitrate aqueous solution. In the present work, it was showed that Ni(NO$$_{3}$$)$$_{2}$$ aqueous solution with 6.0 g of NiO powder as a microwave absorber can be completely converted to NiO powder by microwave heating. NiO powder promotes the denitration reaction, and reduces the required reaction time with increasing the amount of NiO powder. Furthermore the adiabator was set around the reactor in order to equalize the temperature distribution in the reactor. It was also found that the denitration efficiency of Ni(NO$$_{3}$$)$$_{2}$$ aqueous solution to NiO powder can be improved by using the adiabator when the center of the reactor has the same temperature.

Oral presentation

Computer simulation of the earliest processes of radiation biological effects of; Direct and indirect effects of DNA damage

Kai, Takeshi; Toigawa, Tomohiro; Matsuya, Yusuke; Hirata, Yuho; Tezuka, Tomoya*; Tsuchida, Hidetsugu*; Ito, Yuma*; Yokoya, Akinari*

no journal, , 

Irradiation of living systems forms complex DNA damage that induces biological effects in very rare cases. This complex DNA damage is called cluster damage and is very difficult to detect experimentally. In this study, we have developed physical and chemical codes for analyzing DNA damage, and are working to elucidate the formation mechanism of cluster damage. In this study, we analyzed the results of calculations in a simple system in which energy is deposited to DNA and secondary electrons are emitted, and showed that the formation mechanism of cluster damage strongly depends on the deposition energy to DNA. This scientific insight is expected to contribute to the elucidation of the repair mechanism of DNA damage and lead to the elucidation of radiation biological effects.

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