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Journal Articles

Development of nondestructive elemental analysis system for Hayabusa2 samples using muonic X-rays

Osawa, Takahito; Nagasawa, Shunsaku*; Ninomiya, Kazuhiko*; Takahashi, Tadayuki*; Nakamura, Tomoki*; Wada, Taiga*; Taniguchi, Akihiro*; Umegaki, Izumi*; Kubo, Kenya*; Terada, Kentaro*; et al.

ACS Earth and Space Chemistry (Internet), 7(4), p.699 - 711, 2023/04

 Times Cited Count:4 Percentile:93.95(Chemistry, Multidisciplinary)

The concentrations of carbon and other major elements in asteroid samples provide very important information on the birth of life on the Earth and the solar-system evolution. Elemental analysis using muonic X-rays is one of the best analytical methods to determine the elemental composition of solid materials, and notably, is the only method to determine the concentration of light elements in bulk samples in a non-destructive manner. We developed a new analysis system using muonic X-rays to measure the concentrations of carbon and other major elements in precious and expectedly tiny samples recovered from the asteroid Ryugu by spacecraft Hayabusa2. Here we report the development process of the system in 4 stages and their system configurations, The analysis system is composed of a stainless-steel analysis chamber, an acrylic glove box for manipulating asteroid samples in a clean environment, and Ge semiconductor detectors arranged to surround the analysis chamber. The performance of the analysis system, including the background level, which is crucial for the measurement, was greatly improved from the first stage to the later ones. Our feasibility study showed that the latest model of our muonic X-ray analysis system is capable of determining the carbon concentration in Hayabusa2's sample model with an uncertainty of less than 10 percent in a 6-day measurement.

Journal Articles

Density and X-ray emission profile relationships in highly ionized high-Z laser-produced plasmas

Yoshida, Kensuke*; Fujioka, Shinsuke*; Higashiguchi, Takeshi*; Ugomori, Teruyuki*; Tanaka, Nozomi*; Kawasaki, Masato*; Suzuki, Yuhei*; Suzuki, Chihiro*; Tomita, Kentaro*; Hirose, Ryoichi*; et al.

Applied Physics Letters, 106(12), p.121109_1 - 121109_5, 2015/03

 Times Cited Count:10 Percentile:38.07(Physics, Applied)

Journal Articles

Dynamics of low-energy electrons in liquid water with consideration of Coulomb interaction with positively charged water molecules induced by electron collision

Kai, Takeshi; Yokoya, Akinari; Ukai, Masatoshi*; Fujii, Kentaro; Higuchi, Mariko; Watanabe, Ritsuko

Radiation Physics and Chemistry, 102, p.16 - 22, 2014/09

 Times Cited Count:24 Percentile:86.35(Chemistry, Physical)

no abstracts in English

Journal Articles

Efficient extreme ultraviolet emission from one-dimensional spherical plasmas produced by multiple lasers

Yoshida, Kensuke*; Fujioka, Shinsuke*; Higashiguchi, Takeshi*; Ugomori, Teruyuki*; Tanaka, Nozomi*; Ohashi, Hayato*; Kawasaki, Masato*; Suzuki, Yuhei*; Suzuki, Chihiro*; Tomita, Kentaro*; et al.

Applied Physics Express, 7(8), p.086202_1 - 086202_4, 2014/08

 Times Cited Count:29 Percentile:73.72(Physics, Applied)

We demonstrate high conversion efficiency for extreme ultraviolet (EUV) emission at 6.5-6.7 nm from multiple laser beam-produced one-dimensional spherical plasmas. Multiply charged-state ions produce strong resonance emission lines, which combine to yield intense unresolved transition arrays in Gd, Tb, and Mo. The maximum in-band EUV conversion efficiency was observed to be 0.8%, which is one of the highest values ever reported due to the reduction of plasma expansion loss.

Journal Articles

Development of a simulation method for dynamics of electrons ejected from DNA molecules irradiated with X-rays

Kai, Takeshi; Higuchi, Mariko; Fujii, Kentaro; Watanabe, Ritsuko; Yokoya, Akinari

International Journal of Radiation Biology, 88(12), p.928 - 932, 2012/12

 Times Cited Count:1 Percentile:12.53(Biology)

Journal Articles

Cement based encapsulation trials for low-level radioactive effluent containing nitrate salts

Sugaya, Atsushi; Horiguchi, Kenichi; Tanaka, Kenji; Kobayashi, Kentaro

Materials Research Society Symposium Proceedings, Vol.1107, p.173 - 179, 2008/00

In Nuclear Fuel Reprocessing Plant, it is necessary to dispose of a large amount of low level radioactive effluent containing nitrate as a major ingredient, safely and economically. Therefore, engineering developments concerning a cement based encapsulation process have been carried out in JAEA. From the viewpoint of disposal cost decrease, a low level radioactive effluent is passed through the nuclide separation process before cementation to concentrate the radioactivity into the minimum volume for conditioning and disposal. Two kinds of effluents are generated as a result of the nuclide separation; Non-radioactive simulants were prepared for each of these waste streams, and used in encapsulation trials to investigate a special slag cement, on a beaker scale and at full scale (200-litres). The results have confirmed that the nitrate effluent, evaporated up to a predetermined density, can be successfully encapsulated at a salt filling rate of 50wt%, to produce a wasteform which satisfies the required conditions. In the slurry effluent, the strength of the product decreased when carbonate concentration was high. However, it was confirmed that the product made at salt filling rate 50wt% satisfied the required conditions, if the carbonate concentration in the effluent was decreased to 10 g/L or less.

Oral presentation

Cement based encapsulation experiment for low radioactive effluent that contains nitrate

Sugaya, Atsushi; Horiguchi, Kenichi; Tanaka, Kenji; Kobayashi, Kentaro

no journal, , 

In Nuclear Fuel Reprocessing Plant, it is necessary to dispose of a large amount of low level radioactive effluent containing nitrate as a major ingredient, safely and economically. Therefore, engineering developments concerning a cement based encapsulation process have been carried out in JAEA. From the viewpoint of disposal cost decrease, a low level radioactive effluent is passed through the nuclide separation process before cementation to concentrate the radioactivity into the minimum volume for conditioning and disposal. Two kinds of effluents are generated as a result of the nuclide separation; a nitrate effluent of which the principal ingredient is nitrate with a comparatively low radiation level, and a slurry effluent including several kinds of salts with a comparatively high radiation level. Non-radioactive simulants were prepared for each of these waste streams, and used in encapsulation trials to investigate a special slag cement, on a beaker scale and at full scale (200-litres). The results have confirmed that the nitrate effluent, evaporated up to a predetermined density, can be successfully encapsulated at a salt filling rate of 50wt%, to produce a wasteform which satisfies the required conditions. In the slurry effluent, the strength of the product decreased when carbonate concentration was high. However, it was confirmed that the product made at salt filling rate 50wt% satisfied the required conditions, if the carbonate concentration in the effluent was decreased to 10g/L or less.

Oral presentation

Development on nitric ion decomposition technique at Tokai Reprocessing Plant

Takano, Masato; Horiguchi, Kenichi; Tanaka, Kenji; Kobayashi, Kentaro

no journal, , 

no abstracts in English

Oral presentation

Development of treatment for low radioactive effluent in Tokai Reprocessing Plant, 1; Cement based encapsulation experiment for low radioactive effluent

Horiguchi, Kenichi; Sugaya, Atsushi; Tanaka, Kenji; Kobayashi, Kentaro; Sasaki, Tadashi*

no journal, , 

no abstracts in English

Oral presentation

Development of treatment for low radioactive effluent in Tokai Reprocessing Plant, 1; Cement solidification process

Horiguchi, Kenichi; Sugaya, Atsushi; Tanaka, Kenji; Kobayashi, Kentaro; Sasaki, Tadashi*

no journal, , 

In Nuclear Fuel Reprocessing Plant, it is necessary to dispose of a large amount of low level radioactive effluent containing nitrate as a major ingredient, safely and economically. Therefore, engineering developments concerning a cement based encapsulation process have been carried out in JAEA. From the view point of disposal cost decrease, a low level radioactive effluent is passed through the nuclide separation process before cementation to concentrate the radioactivity into the minimum volume for conditioning and disposal. Two kinds of effluents are generated as a result of the nuclide separation; A nitrate effluent of which the principal ingredient is nitrate with a comparatively low radiation level, and; A slurry effluent including several kinds of salts with a comparatively high radiation level. Non-radioactive stimulants were prepared for each of these waste streams, and used in encapsulation trials to investigate special slag cement, on a beaker scale and full scale(200-litres). Furthermore, JAEA has carried out hazardous material judgment for cement products and leaching test of the cement products which encapsulated actual effluent. I will report that result of there development trials.

Oral presentation

Development of treatment for low radioactive effluent in Tokai Reprocessing Plant, 3; Cement solidification experiment for phosphate effluent

Horiguchi, Kenichi; Sugaya, Atsushi; Tanaka, Kenji; Kobayashi, Kentaro; Sasaki, Tadashi*

no journal, , 

In Nuclear Fuel Reprocessing Plant, it is necessary to dispose of a large amount of low level radioactive effluent safely and economically. In JAEA engineering developments concerning a cement solidification process have been carried out. The phosphate effluent occurring from solvent waste treatment facility is based on sodium dihydrogen phosphate. The acidity of this effluent (pH 4) requires a pre-treatment process before cement solidification. Phosphate effluent interfere with cementing reactions by retard of reaction rate and loss of strength, because it is combined with calcium that is element of cement material. It reports on the result of Non-radioactive simulant was prepared for the phosphate effluent, and used in cementation trials to investigate a special slag cement, on a beaker scale and at full scale (200-litres).

Oral presentation

Development of treatment for low radioactive effluent in Tokai Reprocessing Plant, 4; Calcium hydroxide based pretreatment experiment for phosphate effluent

Sugaya, Atsushi; Horiguchi, Kenichi; Tanaka, Kenji; Kobayashi, Kentaro

no journal, , 

Tokai Reprocessing Center is developing a cement based encapsulation method to immobilize low level radioactive effluent. Phosphate effluent arising from Solvent Waste Treatment Facility interfere with cementing reactions by retard of reaction rate and loss of strength, because it is combined with calcium that is element of cement material. It reports on the result of pretreatment trials at small scale executed to ease adverse effect of phosphate.

Oral presentation

Analysis of DNA damage by soft X-rays irradiation using a molecular dynamics method

Kai, Takeshi; Higuchi, Mariko; Fujii, Kentaro; Watanabe, Ritsuko; Yokoya, Akinari

no journal, , 

no abstracts in English

Oral presentation

Time evolutionary calculations of collisional events and trajectories of free electrons in water

Kai, Takeshi; Yokoya, Akinari; Ukai, Masatoshi*; Fujii, Kentaro; Higuchi, Mariko; Watanabe, Ritsuko

no journal, , 

no abstracts in English

Oral presentation

Time evolutionary calculations of collisional events and trajectories of primary and secondary electrons in water

Kai, Takeshi; Yokoya, Akinari; Ukai, Masatoshi*; Fujii, Kentaro; Higuchi, Mariko; Watanabe, Ritsuko

no journal, , 

no abstracts in English

Oral presentation

Development of automatic readout and recognition of nuclear emulsion for fast neutron measurement

Sakai, Yosuke*; Minato, Haruna*; Ishihara, Kohei*; Tomita, Hideki*; Kawarabayashi, Jun*; Iguchi, Tetsuo*; Naka, Tatsuhiro*; Asada, Takashi*; Morishima, Kunihiro*; Nakano, Toshiyuki*; et al.

no journal, , 

In order to measure a neutron-spectrum under high $$gamma$$ ray environment, a new nuclear emulsion and its data-processing method are developed. In fast neutron measurement using the nuclear emulsion which can record the three-dimensional track of a charged particle, incidence neutron energy spectrum can be obtained by analyzing the track of the recoil proton generated by the elastic scattering of a neutron. The high-speed automatic analytic method of the recoil proton track in a nuclear plate is developed. It checked that the recoil proton track length distribution obtained by viewing and automatic analysis was in agreement with a model calculation result about by the basic experiment using 14 MeV neutron.

Oral presentation

Development of automatic readout and recognition of recoiled proton track in nuclear emulsion for fast neutron measurement

Sakai, Yosuke*; Minato, Haruna*; Ishihara, Kohei*; Tomita, Hideki*; Kawarabayashi, Jun*; Iguchi, Tetsuo*; Naka, Tatsuhiro*; Asada, Takashi*; Morishima, Kunihiro*; Nakano, Toshiyuki*; et al.

no journal, , 

In order to measure a neutron-spectrum under high $$gamma$$ ray environment, a new nuclear emulsion and its data-processing method are developed. In fast neutron measurement using the nuclear emulsion which can record the three-dimensional track of a charged particle, incidence neutron energy spectrum can be obtained by analyzing the track of the recoil proton generated by the elastic scattering of a neutron. The high-speed automatic analytic method of the recoil proton track in a nuclear plate is developed. It checked that the recoil proton track length distribution obtained by viewing and automatic analysis was in agreement with a model calculation result about by the basic experiment using 14 MeV neutron.

Oral presentation

Dynamics of electrons in water produced by electron impact in the order of femtosecond

Kai, Takeshi; Yokoya, Akinari; Ukai, Masatoshi*; Fujii, Kentaro; Higuchi, Mariko; Watanabe, Ritsuko

no journal, , 

no abstracts in English

Oral presentation

Laser plasma interaction and the ion acceleration experiments by high contrast high intensity laser J-KAREN-P system

Nishiuchi, Mamiko; Sakaki, Hironao; Pirozhkov, A. S.; Sagisaka, Akito; Kon, Akira; Fukuda, Yuji; Kiriyama, Hiromitsu; Dover, N.*; Sekiguchi, Kentaro; Ogura, Koichi; et al.

no journal, , 

Petawatt class laser systems are in nowadays almost ready to work in all over the world. High energy particles accelerated by the interaction between laser pulses from high intensity laser system and the material shows interesting and particular parameters. Therefore those attract many fields of applications. High contrast and ultra high intensity laser system J-KAREN at KPSI is now under upgrading for achieving highest energy ion beams. No laser system with pulse duration less than 100 fs has demonstrated 100 MeV class proton acceleration in the world. To achieve high energy ions requires higher intensity laser on the target. We report on this presentation the status of the upgrading and the experimental results obtained at the first light experiment.

25 (Records 1-20 displayed on this page)