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Journal Articles

Quantum proton entanglement on a nanocrystalline silicon surface

Matsumoto, Takahiro*; Sugimoto, Hidehiko*; Ohara, Takashi; Tokumitsu, Akio*; Tomita, Makoto*; Ikeda, Susumu*

Physical Review B, 103(24), p.245401_1 - 245401_9, 2021/06

 Times Cited Count:0 Percentile:0(Materials Science, Multidisciplinary)

Journal Articles

Optimization of a slab geometry type cold neutron moderator for RIKEN accelerator-driven compact neutron source

Ma, B.*; Teshigawara, Makoto; Wakabayashi, Yasuo*; Yan, M.*; Hashiguchi, Takao*; Yamagata, Yutaka*; Wang, S.*; Ikeda, Yujiro*; Otake, Yoshie*

Nuclear Instruments and Methods in Physics Research A, 995, p.165079_1 - 165079_7, 2021/04

We have optimized a cold neutron moderator to be operated at the RIKEN accelerator-driven compact neutron source. We selected a safe and easy to manage material, mesitylene, as the RANS cold moderator. An efficient moderator system was designed by studying and optimizing a coupled cold neutron moderator of mesitylene at 20 K with a polyethylene (PE) pre-moderator at room temperature in the slab geometry with Particle and Heavy Ion Transport code System (PHITS) simulations. The parameters of mesitylene and PE thickness, the reflector, and the shielding configuration were studied to increase cold neutron intensities. Consequently, an integrated cold neutron intensity of 1.15$$times$$10$$^{3}$$n/cm$$^{2}$$/$$mu$$A at 2 m from the neutron-producing target was finally achieved, which was 12 times higher than that of the current PE moderator. The results showed attractive application prospect of mesitylene as cold neutron moderator material.

Journal Articles

Study on B$$_{4}$$C decoupler with burn-up reduction aiming at 1-MW pulsed neutron source

Oi, Motoki; Teshigawara, Makoto; Harada, Masahide; Ikeda, Yujiro

Journal of Nuclear Science and Technology, 56(7), p.573 - 579, 2019/07

 Times Cited Count:0 Percentile:0.01(Nuclear Science & Technology)

In pulsed neutron sources, a neutron absorber called decoupler is attached to the moderator to sharpen the neutron pulses for achieving good neutron energy resolutions. Cadmium and boron carbide (B$$_{4}$$C) are widely used as the decoupler materials. However, it is difficult to use B$$_{4}$$C in MW-class spallation neutron sources owing to high burn-up, which decreases cut-off energy and increase of helium gas swelling. To solve these issues, we introduce the concept of pre-decoupler to reduce neutron absorption in the B$$_{4}$$C decoupler, which is sandwiched by appropriate neutron absorption materials. Then, we study impacts of the pre-decouplers on B$$_{4}$$C decoupler in terms of burn-up by performing simplified model calculations. It is shown that neutron absorption in B$$_{4}$$C is reduced by 60% by using a Cd pre-decoupler without neutron intensity penalty. Moreover, helium gas swelling in B$$_{4}$$C is restrained to be one-third of the value when not using the pre-decoupler.

Journal Articles

Measurement of neutron scattering cross section of nano-diamond with particle diameter of approximately 5 nm in energy range of 0.2 meV to 100 meV

Teshigawara, Makoto; Tsuchikawa, Yusuke*; Ichikawa, Go*; Takata, Shinichi; Mishima, Kenji*; Harada, Masahide; Oi, Motoki; Kawamura, Yukihiko*; Kai, Tetsuya; Kawamura, Seiko; et al.

Nuclear Instruments and Methods in Physics Research A, 929, p.113 - 120, 2019/06

 Times Cited Count:7 Percentile:75.46(Instruments & Instrumentation)

A nano-diamond is an attractive neutron reflection material below cold neutron energy. The total neutron cross section of a nano-diamond was derived from a neutron transmission measurement over the neutron energy range of 0.2 meV to 100 meV because total neutron cross section data were not available. The total cross section of a nano-diamond with particle size of approximately 5 nm increased with a decrease in neutron energy to 0.2 meV. It was approximately two orders of magnitude larger than that of graphite at 0.2 meV. The contribution of inelastic scattering to the total cross section was to be shown negligible small at neutron energies of 1.2, 1.5, 1.9, 2.6, and 5.9 meV in the inelastic neutron scattering measurement. Moreover, small-angle neutron scattering measurements of the nano-diamond showed a large scattering cross section in the forward direction for low neutron energies.

Journal Articles

Experimental validation of the brightness distribution on the surfaces of coupled and decoupled moderators composed of 99.8% parahydrogen at the J-PARC pulsed spallation neutron source

Harada, Masahide; Teshigawara, Makoto; Oi, Motoki; Klinkby, E.*; Zanini, L.*; Batkov, K.*; Oikawa, Kenichi; Toh, Yosuke; Kimura, Atsushi; Ikeda, Yujiro

Nuclear Instruments and Methods in Physics Research A, 903, p.38 - 45, 2018/09

 Times Cited Count:5 Percentile:64.98(Instruments & Instrumentation)

Journal Articles

Evaluation of combined pre- and post-excavation grouting for reducing water inflow under high water pressure condition

Mikake, Shinichiro; Ikeda, Koki; Matsui, Hiroya; Tsuji, Masakuni*; Nishigaki, Makoto*

Doboku Gakkai Rombunshu, C (Chiken Kogaku) (Internet), 74(1), p.76 - 91, 2018/03

Pre-grouting of shafts and galleries had been conducted during the construction of MIU in the aspect of reducing water inflow. After excavating GL.-500m gallery, a post-grouting was performed on section of the pre-excavation grouting area under high water pressure condition (max: 4MPa). The post-grouting experiment was performed outside of the pre-grouting zone with designs, applying colloidal silica grouting material and complex dynamic grouting. It was estimated that the inflow after post-grouting was reduced by 1/100 of the case that pre- and post-grouting were not performed. These results indicate that the applied combined pre- and post-grouting methodology is effective in reducing water inflow and it can be applicable under high water pressure condition. Then, this paper states the theoretical evaluation of relationship between reduction of hydraulic conductivity and the grouting zone is very convenient and useful for grouting design and estimate of water inflow.

Journal Articles

Implementation of a low-activation Au-In-Cd decoupler into the J-PARC 1 MW short pulsed spallation neutron source

Teshigawara, Makoto; Ikeda, Yujiro; Oi, Motoki; Harada, Masahide; Takada, Hiroshi; Kakishiro, Masanori*; Noguchi, Gaku*; Shimada, Tsubasa*; Seita, Kyoichi*; Murashima, Daisuke*; et al.

Nuclear Materials and Energy (Internet), 14, p.14 - 21, 2018/01

 Times Cited Count:0 Percentile:0.01(Nuclear Science & Technology)

We developed an Au-In-Cd (AuIC) decoupler material to reduce induced radioactivity instead of Ag-In-Cd one, which has a cut off energy of 1eV. In order to implement it into an actual moderator-reflector assembly, a number of critical engineering issues need to be resolved with regard to large-sized bonding between AuIC and A5083 alloys by the hot isostatic pressing process. We investigated this process in terms of the surface conditions, sizes, and heat capacities of large AuIC alloys. We also show a successful implementation of an AuIC decoupler into a reflector assembly, resulting in a remarkable reduction of radioactivity by AuIC compared to AIC without sacrificing neutronic performance.

JAEA Reports

Investigation and measures of abnormal events of helium refrigerator for cryogenic hydrogen system at J-PARC

Aso, Tomokazu; Teshigawara, Makoto; Hasegawa, Shoichi; Aoyagi, Katsuhiro*; Muto, Hideki*; Nomura, Kazutaka*; Takada, Hiroshi; Ikeda, Yujiro

JAEA-Technology 2017-021, 75 Pages, 2017/08


Liquid hydrogen is employed as a cold neutron moderator material at the spallation neutron source of Materials and Life science experimental Facility of Japan Proton Accelerator Research Complex (J-PARC). From January 2015, it became observable that the differential pressure between heat exchangers and an 80 K adsorber (ADS) in a helium refrigerator system increased with operating time. In November 2015, the differential pressure rise became more significant, leading to degrade the refrigerating performance in cooling liquid hydrogen. In order to investigate the cause of the abnormal differential pressure rise between the heat exchangers and the ADS, we carried out visual inspection inside the heat exchangers and analyzed the impurities contained in the helium gas. Unfortunately, we could not identify the impurities causing the performance degradation, but observed a trace of oil in the inlet piping of the heat exchanger. Based on investigations of the abnormal events occurred in the refrigerators with similar refrigerating capacity at other facilities, we took measures that cleaning the heat exchangers with Freon and replacing the ADS with new one. As a result, the differential pressure rise phenomenon was removed to recover the performance. We have detected oil from the Freon used for cleaning the heat exchangers and at a felt supporting charcoal packed in the ADS. In particular, oil was accumulated in membranous form onto the felt at the entrance side in the ADS. The amount of oil contained in the helium gas was about 10 ppb or so, less than the design value, in the helium refrigerator. However, the oil accumulated onto the felt in the ADS through long operating period may cause abnormal differential pressure rise, leading to the performance degradation of the helium refrigerator. Further study is needed to specify the cause more clearly.

Journal Articles

Model verification and validation procedure for a neutronics design methodology of next generation fast reactors

Ohgama, Kazuya; Ikeda, Kazumi*; Ishikawa, Makoto; Kan, Taro*; Maruyama, Shuhei; Yokoyama, Kenji; Sugino, Kazuteru; Nagaya, Yasunobu; Oki, Shigeo

Proceedings of 2017 International Congress on Advances in Nuclear Power Plants (ICAPP 2017) (CD-ROM), 10 Pages, 2017/04

JAEA Reports

Work and safety managements for on-site installation, commissioning, tests by EU of quench protection circuits for JT-60SA

Yamauchi, Kunihito; Okano, Jun; Shimada, Katsuhiro; Omori, Yoshikazu; Terakado, Tsunehisa; Matsukawa, Makoto; Koide, Yoshihiko; Kobayashi, Kazuhiro; Ikeda, Yoshitaka; Fukumoto, Masahiro; et al.

JAEA-Technology 2015-053, 36 Pages, 2016/03


The superconducting Satellite Tokamak machine "JT-60SA" under construction in Naka Fusion Institute is an international collaborative project between Japan (JA) and Europe (EU). The contributions for this project are based on the supply of components, and thus European manufacturer shall conduct the installation, commissioning and tests on Naka site. This means that Japan Atomic Energy Agency (JAEA) had a quite difficult issue to manage the works by European workers and their safety although there is no direct contract. This report describes the approaches for the work and safety managements, which were agreed with EU after the tough negotiation, and then the completed on-site works for Quench Protection Circuits (QPC) as the first experience for EU in JT-60SA project. With the help of these approaches by JAEA, the EU works for QPC were successfully completed with no accident, and a great achievement was made for both EU and JA.

Journal Articles

Observation of momentum-resolved charge fluctuations proximate to the charge-order phase using resonant inelastic X-ray scattering

Yoshida, Masahiro*; Ishii, Kenji; Naka, Makoto*; Ishihara, Sumio*; Jarrige, I.*; Ikeuchi, Kazuhiko*; Murakami, Yoichi*; Kudo, Kazutaka*; Koike, Yoji*; Nagata, Tomoko*; et al.

Scientific Reports (Internet), 6, p.23611_1 - 23611_8, 2016/03

 Times Cited Count:0 Percentile:0(Multidisciplinary Sciences)

Journal Articles

Probing carbon edge exposure of iron phthalocyanine-based oxygen reduction catalysts by soft X-ray absorption spectroscopy

Niwa, Hideharu*; Saito, Makoto*; Kobayashi, Masaki*; Harada, Yoshihisa*; Oshima, Masaharu*; Moriya, Shogo*; Matsubayashi, Katsuyuki*; Nabae, Yuta*; Kuroki, Shigeki*; Ikeda, Takashi; et al.

Journal of Power Sources, 223, p.30 - 35, 2013/02

 Times Cited Count:17 Percentile:54.86(Chemistry, Physical)

To design non-platinum, inexpensive, but high performance carbon-based cathode catalysts for polymer electrolyte fuel cells, it is important to elucidate the active site for oxygen reduction reaction (ORR). However, it is difficult to directly identify the active site by applying conventional structural or electronic probes to such complex systems. Here, we used C 1${it s}$ X-ray absorption spectroscopy (XAS) to observe electronic structure of carbon in iron phthalocyanine-based catalysts, and found a signature of edge exposure below the $$pi^{ast}$$ edge, whose intensity is well correlated with the ORR activity. These results demonstrate that C 1${it s}$ XAS can be used to characterize the ORR activity of carbon-based cathode catalysts in terms of the edge exposure.

Journal Articles

Indirect contribution of transition metal towards oxygen reduction reaction activity in iron phthalocyanine-based carbon catalysts for polymer electrolyte fuel cells

Kobayashi, Masaki*; Niwa, Hideharu*; Saito, Makoto*; Harada, Yoshihisa*; Oshima, Masaharu*; Ofuchi, Hironori*; Terakura, Kiyoyuki*; Ikeda, Takashi; Koshigoe, Yuka*; Ozaki, Junichi*; et al.

Electrochimica Acta, 74, p.254 - 259, 2012/07

 Times Cited Count:48 Percentile:82.87(Electrochemistry)

The electronic structure of the residual metal atoms in FePc-based carbon catalysts, prepared by pyrolyzing a mixture of FePc and phenolic resin polymer at 800$$^{circ}$$C, before and after acid washing have been investigated using XAFS spectroscopy to clarify the role of Fe in the ORR activity. The decomposition analyses for the XAFS spectra reveal that the composition ratio of each Fe component is unaltered by the acid washing, indicating that the residual Fe components were removed by the acid washing irrespective of their chemical states. Because the oxygen reduction potential was approximately unchanged by the acid washing, the residual Fe itself does not seem to contribute directly to the ORR activity. The residual Fe can act as a catalyst to accelerate the growth of the sp$$^{2}$$ carbon network during pyrolysis. The results imply that light elements are components of the ORR active sites in the FePc-based carbon catalysts.

Journal Articles

Real-time structural analysis of compositionally graded InGaAs/GaAs(001) layers

Sasaki, Takuo*; Suzuki, Hidetoshi*; Inagaki, Makoto*; Ikeda, Kazuma*; Shimomura, Kenichi*; Takahashi, Masamitsu; Kozu, Miwa*; Hu, W.; Kamiya, Itaru*; Oshita, Yoshio*; et al.

IEEE Journal of Photovoltaics, 2(1), p.35 - 40, 2012/01

 Times Cited Count:5 Percentile:25.16(Energy & Fuels)

Journal Articles

Construction work of Mizunami Underground Research Laboratory

Kubo, Makoto*; Mikake, Shinichiro; Ikeda, Koki; Yamamoto, Masaru

Kisoko, 39(9), p.82 - 85, 2011/09

Japan Atomic Energy Agency (JAEA)'s task is to provide the scientific and technical basis for safe geological disposal of high-level radioactive waste. This involves researches on development and improvement of techniques for characterization of the deep geological environment and a wide range of engineering for deep underground application in crystalline rock at "Mizunami Underground Research Laboratory". This report describes the summary of construction.

JAEA Reports

Estimation of runoff volume by geomorphometry and statistics analysis using digital elevation model in Tono area

Takeuchi, Ryuji; Kosaka, Hiroshi; Sato, Atsuya*; Tomiyama, Shingo*; Kageyama, Soichiro*; Ikeda, Makoto*

JAEA-Research 2011-008, 77 Pages, 2011/06


Subsurface water balance observation is a kind of methods in order to estimate a recharge rate. Results of the observation are affected by the various factors such as the scale, the topography, a geological feature, the climate. Therefore, the observation in the regional scale is necessary at many basins. The purpose of this study is to confirm the applicability of the method for the evaluation of runoff volume, which is one of parameters to evaluate the recharge rate by surface water balance observation, by geomorphometry and statistical analyses using digital elevation model (DEM). The runoff index which is the original indicator to evaluate the degree of flow rate on a catchment was calculated by the comparison between the result of geomorphometry and statistics analyses, and the observed data of river flow rate in the monitoring stations. Using this index, the flow rate of the Hiyoshi River was evaluated. The evaluated flow rate was about 60% against the observed flow rate.

Journal Articles

Recharge evaluation of northern area in Hokkaido, Japan

Ikeda, Makoto; Munakata, Masahiro; Sakai, Ryutaro; Kimura, Hideo; Jia, H.*; Matsuba, Hisashi*

Nihon Chikasui Gakkai 2011-Nen Shunki Koenkai Koen Yoshi, p.86 - 91, 2011/05

no abstracts in English

Journal Articles

Recharge evaluation using distributed tank model

Ikeda, Makoto; Munakata, Masahiro; Sakai, Ryutaro; Fuchiwaki, Hirotaka; Kimura, Hideo; Matsuba, Hisashi*

Nihon Chikasui Gakkai 2010-Nen Shuki Koenkai Koen Yoshi, p.282 - 287, 2010/11

no abstracts in English

Journal Articles

First neutron production utilizing J-PARC pulsed spallation neutron source JSNS and neutronic performance demonstrated

Maekawa, Fujio; Harada, Masahide; Oikawa, Kenichi; Teshigawara, Makoto; Kai, Tetsuya; Meigo, Shinichiro; Oi, Motoki; Sakamoto, Shinichi; Takada, Hiroshi; Futakawa, Masatoshi; et al.

Nuclear Instruments and Methods in Physics Research A, 620(2-3), p.159 - 165, 2010/08

 Times Cited Count:63 Percentile:97.68(Instruments & Instrumentation)

The J-PARC 1-MW pulsed spallation neutron source JSNS was successfully launched on 30th of May 2008. To demonstrate the unique features of the moderator design and the neutronic performance of JSNS the neutron spectral intensity, absolute neutron flux, and time structure of the neutron pulse shapes etc have been measured using several neutron instruments since then. The measured energy spectra clearly revealed the feature of the para-hydrogen, as expected when designing the moderator. The measured neutron flux below 0.4 eV agreed with the corresponding design value within $$pm$$20%, thus suggesting that the JSNS design calculations to have been reliable. World-class high-resolution diffraction data could be recorded due to the suitability of design of the moderators and the instruments. Another world-class high-intensity neutron flux was also capable of being demonstrated due to the unique design of the large cylindrical coupled moderator.

Journal Articles

Applicability of countermeasure for reduction of groundwater inflow and construction of the Mizunami Underground Research Laboratory

Mikake, Shinichiro; Yamamoto, Masaru; Ikeda, Koki; Ishida, Hideaki; Nishigaki, Makoto*

Dai-54-Kai Jiban Kogaku Shimpojiumu Rombunshu, p.39 - 46, 2009/11

The Mizunami Underground Research Laboratory (MIU) is currently being constructed. During its construction, water inflow into the shafts of the MIU has been increasing and affecting the project progress. In order to reduce the water inflow into the shafts, borehole investigations and pre-excavation grouting have been conducted. The pre-excavation grouting has been undertaken at the predicted inflow area with existing method.

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