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筋田 涼太*; 今井 彩帆里*; 大内 誠*; 青木 裕之; 寺島 崇矢*
Macromolecules, 56(23), p.9738 - 9749, 2023/12
被引用回数：0 パーセンタイル：0(Polymer Science)Constructing ordered ionic nanostructures into bulk polymers and thin films is an important technique to create functional materials, such as polyelectrolytes and proton- and ion-conducting materials, for various applications. Herein, we report microphase separation of cationic homopolymers bearing alkyl ammonium bromides to create sub-4 nm lamellar materials, where an ionic phase is alternatingly layered with a hydrophobic alkyl phase and serves as a channel for water intercalation. We prepared cationic homopolymers with linear or branched alkyl pendants (octyl or 2-ethylhexyl group: C8-eicosyl or 2-octyldodecyl group: C20) via the free radical polymerization of 2-(dimethylamino)ethyl acrylate (DMAEA), followed by the quaternization of the polyDMAEA with corresponding alkyl bromides. The homopolymers carrying linear hexadecyl, octadecyl, and eicosyl groups were crystalline at room temperature, whereas the others were amorphous. The homopolymers bearing linear alkyl pendants longer than the decyl group or branched alkyl pendants larger than the 2-butyloctyl group formed lamellar structures by the self-assembly of the side chains. The domain spacing can be controlled between 2.5 and 3.7 nm by tuning the pendant structures and are smaller than that formed by the corresponding random copolymers. A cationic homopolymer bearing crystalline octadecyl groups maintained lamellar structures up to 
210 
C far beyond the melting temperature (50 C). The cationic homopolymer further formed a multilayered lamellar thin film on a silicon substrate, in which the cationic layers absorbed water under humid conditions and reversibly released the water therefrom in a N
gas atmosphere.
埋田 真樹; 中堂 博之; 今井 正樹; 佐藤 奈々; 齊藤 英治
Review of Scientific Instruments, 94(6), p.063906_1 - 063906_8, 2023/06
被引用回数：0 パーセンタイル：0(Instruments & Instrumentation)We have developed experimental equipment for observing the Barnett effect, in which mechanical rotation magnetizes an object, at low temperatures. A sample in a rotor is rotated bidirectionally using a temperature-controlled high-pressure gas. The stray field generated from the sample due to the Barnett effect was detected using a fluxgate magnetic sensor with a sensitivity on the order of several picoteslas, even at low temperatures. By replacing the rotor with a solenoid coil, the magnetic susceptibility of the sample was estimated from the stray field to be of the same order of magnitude as that due to the Barnett effect. The Barnett field was estimated using the dipole model. To assess the performance of the setup at low temperatures, measurements were performed on commercial magnetite (Fe
O
) nanogranules. We confirmed the accordance of the 
factor between the experimental results using the present setup and those of our previous study performed at room temperature.
今井 彩帆里*; 荒川 勝利*; 中西 洋平*; 竹中 幹人*; 青木 裕之; 大内 誠*; 寺島 崇矢*
Macromolecules, 55(20), p.9113 - 9125, 2022/10
被引用回数：2 パーセンタイル：27.19(Polymer Science)Microphase separation of copolymers is a key technique to produce polymer bulk materials or thin films with ordered nanostructures for applications in various research fields including nanotechnologies, electronic devices, among many others. Herein, we report water-assisted microphase separation of amphiphilic random copolymers bearing quaternary ammonium cations and hydrophobic alkyl or oleyl groups in the solid state and the thin films. We investigated the effects of sample preparation protocols and the hydrophobic pendants (a butyl group: C4 - octadecyl or oleyl group: C18), composition, and molecular weight of the copolymers on the microphase separation behavior. By annealing under humid conditions, the copolymers bearing alkyl groups longer than an octyl group (C8) formed sub-5 nm lamellar structures comprising cationic layers and hydrophobic layers. Water hardly remained in the resulting lamellar materials under ambient conditions. The domain spacing was controlled between 3.7 and 5.3 nm by tuning the length of the hydrophobic pendants and composition and was independent of the molecular weight and molecular weight distribution. The cationic random copolymers carrying amorphous hydrophobic pendants provided transparent or translucent polymer materials containing small lamellar structures. The random copolymers further formed multilayered lamellar thin films on silicon substrates by spin-coating the copolymer solutions, followed by a humid annealing process. The layered lamellae were directly observed as terrace structures with about 4-5 nm steps by atomic force microscopy.
elastic scattering in the momentum range 0.44-0.80 GeV/c七村 拓野; 藤田 真奈美; 長谷川 勝一; 市川 真也; 市川 裕大; 今井 憲一*; 成木 恵; 佐藤 進; 佐甲 博之; 田村 裕和; et al.
Progress of Theoretical and Experimental Physics (Internet), 2022(9), p.093D01_1 - 093D01_35, 2022/09
被引用回数：5 パーセンタイル：67.44(Physics, Multidisciplinary)We performed a novel 
scattering experiment at the J-PARC Hadron Experimental Facility. Approximately 2400 elastic scattering events were identified from 
tagged 
particles in the momentum range 0.44 - 0.80 GeV/c. The differential cross sections of the elastic scattering were derived with much better precision than in previous experiments. The obtained differential cross sections were approximately 2 mb/sr or less, which were not as large as those predicted by the fss2 and FSS models based on the quark cluster model in the short-range region. By performing phase-shift analyses for the obtained differential cross sections, we experimentally derived the phase shifts of the 
and 
channels for the first time. The phase shift of the 3S1 channel, where a large repulsive core was predicted owing to the Pauli effect between quarks, was evaluated to be 
. If the sign of 
is assumed to be negative, the interaction in this channel is moderately repulsive, as the Nijmegen extended-sort-core models predicted.
elastic scattering in momentum range 470 to 850 MeV/
三輪 浩司*; 藤田 真奈美; 長谷川 勝一; 細見 健二; 市川 裕大; 今井 憲一*; 七村 拓野; 成木 恵; 佐甲 博之; 佐藤 進; et al.
Physical Review C, 104(4), p.045204_1 - 045204_20, 2021/10
被引用回数：12 パーセンタイル：89.15(Physics, Nuclear)A high statistics 
scattering experiment is performed at the J-PARC Hadron Experimental Facility. Momentum-tagged 
s running in a liquid hydrogen target are accumulated by detecting the reaction with a high intensity 
beam of 20 M/spill. The differential cross sections of the elastic scattering were derived with a drastically improved accuracy by identifying approximately 4,500 events from 1.72 
10
. The derived differential cross section shows a clear forward-peaking angular distribution for a momentum range from 470 to 850 MeV/. The accurate data will impose a strong constraint on the theoretical models of the baryon-baryon interactions.
collisions at 
=200 GeVAcharya, U. A.*; 長谷川 勝一; 今井 憲一*; 佐甲 博之; 佐藤 進; 谷田 聖; PHENIX Collaboration*; 他306名*
Physical Review Letters, 127(16), p.162001_1 - 162001_8, 2021/10
被引用回数：9 パーセンタイル：72.45(Physics, Multidisciplinary)Studying spin-momentum correlations in hadronic collisions offers a glimpse into a three-dimensional picture of proton structure. The transverse single-spin asymmetry for midrapidity isolated direct photons in collisions at =200 GeV is measured with the PHENIX detector at the Relativistic Heavy Ion Collider (RHIC). Because direct photons in particular are produced from the hard scattering and do not interact via the strong force, this measurement is a clean probe of initial-state spin-momentum correlations inside the proton and is in particular sensitive to gluon interference effects within the proton. This is the first time direct photons have been used as a probe of spin-momentum correlations at RHIC. The uncertainties on the results are a fifty-fold improvement with respect to those of the one prior measurement for the same observable, from the Fermilab E704 experiment. These results constrain gluon spin-momentum correlations in transversely polarized protons.
中堂 博之; 今井 正樹; 松尾 衛; 前川 禎通; 齊藤 英治
Journal of the Physical Society of Japan, 90(8), p.081003_1 - 081003_11, 2021/08
被引用回数：3 パーセンタイル：41.09(Physics, Multidisciplinary)We demonstrate observation of the angular momentum compensation temperature 
, at which the net angular momentum is quenched in ferrimagnets. Using the Barnett effect, in which an object is magnetized by mechanical rotation owing to spin-rotation coupling, we measure in the Ho
Dy
Fe
O
system. We determine to be 240 K in Ho
FeO (HoIG). We find that increases with Dy content and show that of Ho
DyFeO corresponds with room temperature. We also demonstrate that 
Fe-NMR measurements can be applied to explore domain wall dynamics in HoIG. We find that the NMR intensity exhibits a maximum at in the multi-domain state. We provide a simple model for describing this NMR signal enhancement caused by enhancement of domain-wall mobility at .
-state of a 
hypernucleus, 
吉本 雅浩*; 藤田 真奈美; 橋本 直; 早川 修平; 市川 裕大; 市川 真也; 今井 憲一*; 七村 拓野; 成木 恵; 佐甲 博之; et al.
Progress of Theoretical and Experimental Physics (Internet), 2021(7), p.073D02_1 - 073D02_19, 2021/07
被引用回数：13 パーセンタイル：81.3(Physics, Multidisciplinary)Bound-systems of 
-
are studied via capture at rest followed by emission of a twin single-
hypernucleus in the emulsion detectors. Two events forming extremely deep bound states were obtained by analysis of a hybrid method in the E07 experiment at J-PARC and reanalysis of the E373 experiment at KEK-PS. The decay mode of one event was assigned as 
+
+
+
. Since there are no excited states for daughter particles, the binding energy of the hyperon, 
, in nucleus was uniquely determined to be 6.27 
0.27 MeV. Another - system via the decay 
+ + brings a value, 8.00 0.77 MeV or 4.96 0.77 MeV, where the two possible values of correspond to the ground and the excited states of the daughter nucleus, respectively. Because the values are larger than those of the previously reported events (KISO and IBUKI), which are both interpreted as the nuclear 
state of the - system, these new events give the first indication of the nuclear 
state of the hypernucleus, .
吉田 純也; 赤石 貴也; 藤田 真奈美; 長谷川 勝一; 橋本 直; 細見 健二; 市川 真也; 市川 裕大; 今井 憲一*; Kim, S.; et al.
JPS Conference Proceedings (Internet), 33, p.011112_1 - 011112_8, 2021/03
J-PARC E07 is the most ambitious and complex emulsion experiment to date investigating double hypernuclei with Hybrid emulsion method. The physics run at the K1.8 beam line in the J-PARC hadron experimental facility have been completed in 2017. The emulsion sheets are presently being analyzed with dedicated optical microscopes. Current statistics are estimated to be more 3 times than that of previous experiments. Quantitative data on the 
and 
interaction are being accumulated successfully via analysis of double and hypernuclei. Multiple hypernucleus candidates suggests several features about hypernucleus that the identification efficiency of 
C is significantly higher than other mode, many daughters of C are identified as He or Be, and multiple bound states of exist in the 
N nucleus. An analysis of X-ray spectroscopy of hyperatoms are ongoing.
identification method by the 
reaction for a 
scattering experiment at J-PARC坂尾 珠和*; 藤田 真奈美; 長谷川 勝一; 細見 健二; 市川 真也; 市川 裕大; 今井 憲一*; 七村 拓野; 成木 恵; 佐甲 博之; et al.
JPS Conference Proceedings (Internet), 33, p.011133_1 - 011133_6, 2021/03
The reaction is an important elementary process to produce from a proton target and is a key for a scattering experiment where the momentum of should be tagged from the missing momentum of the 
reaction. However, the spectroscopy method has not been established yet due to the difficulty of the 
detection. Therefore, we have proposed a new detection method where 
and from the decay are measured by a forward magnetic spectrometer and a detector cluster surrounding the target, respectively. The feasibility of the detection method was confirmed by analyzing the J-PARC E40 data taken with such a detector system. In the analysis, 's were successfully identified in the missing mass spectrum of the 
reaction.
and 
mesons in polarized 
collisions at 
GeVAcharya, U. A.*; 長谷川 勝一; 今井 憲一*; 佐甲 博之; 佐藤 進; 谷田 聖; PHENIX Collaboration*; 他309名*
Physical Review D, 103(5), p.052009_1 - 052009_10, 2021/03
被引用回数：5 パーセンタイル：45.23(Astronomy & Astrophysics)We present a measurement of the transverse single-spin asymmetry for and mesons in 
collisions in the pseudorapidity range 
and at a center-of-mass energy of 200 GeV with the PHENIX detector at the Relativistic Heavy Ion Collider. In comparison with previous measurements in this kinematic region, these results have a factor of 3 smaller uncertainties. As hadrons, and mesons are sensitive to both initial- and final-state nonperturbative effects for a mix of parton flavors. Comparisons of the differences in their transverse single-spin asymmetries have the potential to disentangle the possible effects of strangeness, isospin, or mass. These results can constrain the twist-3 trigluon collinear correlation function as well as the gluon Sivers function.
武田 哲明*; 稲垣 嘉之; 相原 純; 青木 健; 藤原 佑輔; 深谷 裕司; 後藤 実; Ho, H. Q.; 飯垣 和彦; 今井 良行; et al.
High Temperature Gas-Cooled Reactors; JSME Series in Thermal and Nuclear Power Generation, Vol.5, 464 Pages, 2021/02
本書は、原子力機構における今までの高温ガス炉の研究開発の総括として、HTTRの設計、燃料、炉内構造物や中間熱交換器などの要素技術の開発、出力上昇試験、950
Cの高温運転、安全性実証試験などの運転経験及び成果についてまとめたものである。また、HTTRでの知見をもとに、商用炉の設計、高性能燃料、ヘリウムガスタービン、ISプロセスによる水素製造などの要素技術開発の現状について記述しており、今後の高温ガス炉の開発に非常に有用である。本書は、日本機械学会の動力エネルギーシステム部門による化石燃料及び原子力によるエネルギーシステムの技術書のシリーズの一冊として刊行されるものである。
collisions at GeVAcharya, U. A.*; 長谷川 勝一; 今井 憲一*; 佐甲 博之; 佐藤 進; 谷田 聖; PHENIX Collaboration*; 他308名*
Physical Review D, 103(3), p.032007_1 - 032007_8, 2021/02
被引用回数：2 パーセンタイル：20.63(Astronomy & Astrophysics)In 2015, the PHENIX collaboration has measured very forward (
) single-spin asymmetries of inclusive neutrons in transversely polarized proton-proton and proton-nucleus collisions at a center of mass energy of 200 GeV. A previous publication from this data set concentrated on the nuclear dependence of such asymmetries. In this measurement the explicit transverse-momentum dependence of inclusive neutron single spin asymmetries for proton-proton collisions is extracted using a bootstrapping-unfolding technique on the transverse momenta. This explicit transverse-momentum dependence will help improve the understanding of the mechanisms that create these asymmetries.
-N system早川 修平; 藤田 真奈美; 長谷川 勝一; 橋本 直; 細見 健二; 市川 裕大; 今井 憲一*; 七村 拓野; 成木 恵; 佐甲 博之; et al.
Physical Review Letters, 126(6), p.062501_1 - 062501_6, 2021/02
被引用回数：34 パーセンタイル：95.34(Physics, Multidisciplinary)In an emulsion-counter hybrid experiment performed at J-PARC, a absorption event was observed which decayed into twin single- hypernuclei. Kinematic calculations enabled a unique identification of the reaction process as 
N
Be + 
He. For the binding energy of the 
hyperon in the -N system a value of 
MeV was deduced. The energy level of is likely a nuclear state which indicates a weak 
-
coupling.
hypernuclear spectroscopy with the 
reaction後神 利志*; 藤田 真奈美; 長谷川 勝一; 細見 健二; 今井 憲一*; 市川 裕大; 七村 拓野; 成木 恵; 佐甲 博之; 佐藤 進; et al.
Journal of Physics; Conference Series, 1643, p.012133_1 - 012133_6, 2020/12
被引用回数：2 パーセンタイル：84.57(Astronomy & Astrophysics)We performed hypernuclear spectroscopy with the reaction at J-PARC to investigate the interaction (J-PARC E05). A new experiment (J-PARC E70) in which a better energy resolution could be achieved is now being prepared. In this article, an analysis status of J-PARC E05 and a preparation status of J-PARC E70 are described.
interaction from the scattering experiment at J-PARC三輪 浩司*; 藤田 真奈美; 長谷川 勝一; 細見 健二; 市川 真也; 市川 裕大; 今井 憲一*; 七村 拓野; 成木 恵; 佐甲 博之; et al.
Journal of Physics; Conference Series, 1643, p.012174_1 - 012174_6, 2020/12
被引用回数：2 パーセンタイル：84.57(Astronomy & Astrophysics)A high statistics scattering experiment has been performed at the K1.8 beamline in the J-PARC Hadron Experimental Facility. Data for momentum-tagged beam running in a liquid hydrogen target were accumulated by detecting the 
reaction with a high intensity beam of 20 M/spill. The number of the beam was about 
in total. The elastic scattering and the 
inelastic scattering events were successfully observed with about 100 times larger statistics than that in past experiments.
and mesons in UU collisions at 
GeVAcharya, U.*; 長谷川 勝一; 今井 憲一*; 永宮 正治*; 佐甲 博之; 佐藤 進; 谷田 聖; PHENIX Collaboration*; 他397名*
Physical Review C, 102(6), p.064905_1 - 064905_13, 2020/12
被引用回数：5 パーセンタイル：52.72(Physics, Nuclear)The PHENIX experiment at the Relativistic Heavy Ion Collider measured and mesons at midrapidity in UU collisions at GeV in a wide transverse momentum range. Measurements were performed in the 
decay modes. A strong suppression of and meson production at high transverse momentum was observed in central UU collisions relative to binary scaled results. Yields of and mesons measured in UU collisions show similar suppression pattern to the ones measured in AuAu collisions at 
GeV for similar numbers of participant nucleons. The / ratios do not show dependence on centrality or transverse momentum, and are consistent with previously measured values in hadron-hadron, hadron-nucleus, nucleus-nucleus, and 
collisions.
+Au collisions at GeVAcharya, U.*; 長谷川 勝一; 今井 憲一*; 永宮 正治*; 佐甲 博之; 佐藤 進; 谷田 聖; PHENIX Collaboration*; 他572名*
Physical Review C, 102(5), p.054910_1 - 054910_11, 2020/11
被引用回数：3 パーセンタイル：36.4(Physics, Nuclear)We present direct photon-hadron correlations in 200 GeV/A AuAu, Au and collisions, for direct photon 
from 5 - 12 GeV/, collected by the PHENIX Collaboration in the years from 2006 to 2011. We observe no significant modification of jet fragmentation in Au collisions, indicating that cold nuclear matter effects are small or absent. Hadrons carrying a large fraction of the quark's momentum are suppressed in AuAu compared to and Au. As the momentum fraction decreases, the yield of hadrons in AuAu increases to an excess over the yield in collisions. The excess is at large angles and at low hadron and is most pronounced for hadrons associated with lower momentum direct photons. Comparison to theoretical calculations suggests that the hadron excess arises from medium response to energy deposited by jets.
at forward rapidity in 
collisions at 
GeVAcharya, U.*; 長谷川 勝一; 今井 憲一*; 永宮 正治*; 佐甲 博之; 佐藤 進; 谷田 聖; PHENIX Collaboration*; 他344名*
Physical Review D, 102(9), p.092002_1 - 092002_14, 2020/11
被引用回数：0 パーセンタイル：0.01(Astronomy & Astrophysics)The cross section of bottom quark-antiquark () production in collisions at GeV is measured with the PHENIX detector at the Relativistic Heavy Ion Collider. The results are based on the yield of high mass, like-sign muon pairs measured within the PHENIX muon arm acceptance (
). The signal is extracted from like-sign dimuons by utilizing the unique properties of neutral 
meson oscillation. We report a differential cross section of 
nb for like-sign muons in the rapidity and ranges and 
GeV/, and dimuon mass of 5 - 10 GeV/
. The extrapolated total cross section at this energy for production is 
b. The total cross section is compared to a perturbative quantum chromodynamics calculation and is consistent within uncertainties. The azimuthal opening angle between muon pairs from decays and their distributions are compared to distributions generated using 
, which includes next-to-leading order processes. The azimuthal correlations and pair distribution are not very well described by 
calculations, but are still consistent within uncertainties. Flavor creation and flavor excitation subprocesses are favored over gluon splitting.
production in collisions at GeVAcharya, U.*; 長谷川 勝一; 今井 憲一*; 永宮 正治*; 佐甲 博之; 佐藤 進; 谷田 聖; PHENIX Collaboration*; 他344名*
Physical Review D, 102(7), p.072008_1 - 072008_13, 2020/10
被引用回数：2 パーセンタイル：16.06(Astronomy & Astrophysics)The PHENIX experiment has measured the spin alignment for inclusive 
decays in collisions at GeV at midrapidity. The angular distributions have been measured in three different polarization frames, and the three decay angular coefficients have been extracted in a full two-dimensional analysis. Previously, PHENIX saw large longitudinal net polarization at forward rapidity at the same collision energy. This analysis at midrapidity, complementary to the previous PHENIX results, sees no sizable polarization in the measured transverse momentum range of 
GeV/. The results are consistent with a previous one-dimensional analysis at midrapidity at GeV. The transverse-momentum-dependent cross section for midrapidity production has additionally been measured, and after comparison to world data we find a simple logarithmic dependence of the cross section on .
