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Journal Articles

Microphase separation of cationic homopolymers bearing alkyl ammonium salts into sub-4 nm lamellar materials with water intercalation channels

Sujita, Ryota*; Imai, Sahori*; Ouchi, Makoto*; Aoki, Hiroyuki; Terashima, Takaya*

Macromolecules, 56(23), p.9738 - 9749, 2023/12

Journal Articles

Water-assisted microphase separation of cationic random copolymers into sub-5 nm lamellar materials and thin films

Imai, Sahori*; Arakawa, Masato*; Nakanishi, Yohei*; Takenaka, Mikihito*; Aoki, Hiroyuki; Ouchi, Makoto*; Terashima, Takaya*

Macromolecules, 55(20), p.9113 - 9125, 2022/10

Journal Articles

High temperature gas-cooled reactors

Takeda, Tetsuaki*; Inagaki, Yoshiyuki; Aihara, Jun; Aoki, Takeshi; Fujiwara, Yusuke; Fukaya, Yuji; Goto, Minoru; Ho, H. Q.; Iigaki, Kazuhiko; Imai, Yoshiyuki; et al.

High Temperature Gas-Cooled Reactors; JSME Series in Thermal and Nuclear Power Generation, Vol.5, 464 Pages, 2021/02

As a general overview of the research and development of a High Temperature Gas-cooled Reactor (HTGR) in JAEA, this book describes the achievements by the High Temperature Engineering Test Reactor (HTTR) on the designs, key component technologies such as fuel, reactor internals, high temperature components, etc., and operational experience such as rise-to-power tests, high temperature operation at 950$$^{circ}$$C, safety demonstration tests, etc. In addition, based on the knowledge of the HTTR, the development of designs and component technologies such as high performance fuel, helium gas turbine and hydrogen production by IS process for commercial HTGRs are described. These results are very useful for the future development of HTGRs. This book is published as one of a series of technical books on fossil fuel and nuclear energy systems by the Power Energy Systems Division of the Japan Society of Mechanical Engineers.

Journal Articles

Measurement of Auger electrons emitted through Coster-Kronig transitions under irradiation of fast C$$_{2}$$$$^{+}$$ ions

Shiina, Yoko*; Kinoshita, Ryo*; Funada, Shuhei*; Matsuda, Makoto; Imai, Makoto*; Kawatsura, Kiyoshi*; Sataka, Masao*; Sasa, Kimikazu*; Tomita, Shigeo*

Nuclear Instruments and Methods in Physics Research B, 460, p.30 - 33, 2019/12

 Times Cited Count:2 Percentile:23.44(Instruments & Instrumentation)

Journal Articles

Effect of the headgroup structure on counterion binding in adsorbed surfactant films investigated by total reflection X-ray absorption fine structure spectroscopy

Imai, Yosuke*; Tokiwa, Yuhei*; Ueno, Shusaku*; Tanida, Hajime; Watanabe, Iwao*; Matsubara, Hiroki*; Takiue, Takanori*; Aratono, Makoto*

Bulletin of the Chemical Society of Japan, 91(10), p.1487 - 1494, 2018/10

 Times Cited Count:2 Percentile:8.33(Chemistry, Multidisciplinary)

Competitive binding of binary mixed counterions to the headgroups of adsorbed surfactant films has been investigated at solution surfaces by total reflection X-ray absorption fine structure (XAFS) spectroscopy. The obtained extended XAFS $$chi$$ spectra for bromide counterions are linear combinations of the spectra of fully hydrated bromide ions (free Br) and partially dehydrated bromide ions bound to the headgroups of the surfactant ions (bound Br). From the fraction of bound Br in counterion mixed systems, two series of the relative strengths of counterion binding are proposed for the trimethylammonium (TA$$^{+}$$) and 3-methylimidazolium (MIM$$^{+}$$) headgroups: (a) TA-SO$$_{4}$$ $$<$$ TA-Cl $$<$$ TA-Br $$<$$ TA-BF$$_{4}$$ and (b) MIM-Br $$<$$ TA-Br $$<$$ TA-BF$$_{4}$$ $$<$$ MIM-BF$$_{4}$$. For the TA headgroup, matching the hydration of the headgroups and counterions gives series (a) according to Collins' law, which states that the tendency of contact ion pair formation becomes larger when the absolute values of the hydration enthalpies of the ions match. For the MIM headgroup, the number of binding sites of hydrogen bonds between the MIM headgroup and counterion is essential, which leads to series (b) because of competition between the counterion and water for interaction with the MIM headgroup.

Journal Articles

Direct measurement of nanoscale lithium diffusion in solid battery materials using radioactive tracer of $$^{8}$$Li

Ishiyama, Hironobu*; Jeong, S.-C.*; Watanabe, Yutaka*; Hirayama, Yoshikazu*; Imai, Nobuaki*; Jung, H. S.*; Miyatake, Hiroari*; Oyaizu, Mitsuhiro*; Osa, Akihiko; Otokawa, Yoshinori; et al.

Nuclear Instruments and Methods in Physics Research B, 376, p.379 - 381, 2016/06

 Times Cited Count:7 Percentile:60.71(Instruments & Instrumentation)

Journal Articles

Progress of divertor simulation research toward the realization of detached plasma using a large tandem mirror device

Nakashima, Yosuke*; Takeda, Hisahito*; Ichimura, Kazuya*; Hosoi, Katsuhiro*; Oki, Kensuke*; Sakamoto, Mizuki*; Hirata, Mafumi*; Ichimura, Makoto*; Ikezoe, Ryuya*; Imai, Tsuyoshi*; et al.

Journal of Nuclear Materials, 463, p.537 - 540, 2015/08

 Times Cited Count:18 Percentile:82.74(Materials Science, Multidisciplinary)

Journal Articles

Equilibrium and non-equilibrium charge-state distributions of 2.0 MeV/u carbon ions passing through carbon foils

Imai, Makoto*; Sataka, Masao*; Matsuda, Makoto; Okayasu, Satoru; Kawatsura, Kiyoshi*; Takahiro, Katsumi*; Komaki, Kenichiro*; Shibata, Hiromi*; Nishio, Katsuhisa

Nuclear Instruments and Methods in Physics Research B, 354, p.172 - 176, 2015/07

 Times Cited Count:14 Percentile:75.73(Instruments & Instrumentation)

Both equilibrium and non-equilibrium charge-state distributions were studied experimentally for 2.0 MeV/u carbon ions after passing through carbon foils. Measured charge-state distribution established the equilibrium at a target thickness of 10 $$mu$$g/cm$$^{2}$$ and this remained unchanged until a maximum target thickness of 98 $$mu$$g/cm$$^{2}$$. The equilibrium charge-state distribution, the equilibrium mean charge-state, and the width and skewness of the equilibrium distribution were compared with predictions using existing semi-empirical formulae as well as simulation results, including the ETACHA code. It was found that charge-state distributions, mean charge states, and distribution widths for C$$^{2+}$$, C$$^{3+}$$, and C$$^{4+}$$ incident ions merged into quasi-equilibrium values at a target thickness of 5.7 $$mu$$g/cm$$^{2}$$ in the pre-equilibrium region and evolved simultaneously to the "real equilibrium" values for all of the initial charge states, including C$$^{5+}$$ and C$$^{6+}$$ ions. Two kinds of simulation, ETACHA and solution of rate equations taking only single electron transfers into account, were used, and both of them reproduced the measured charge evolution qualitatively. The quasi-equilibrium behavior could be reproduced with the ETACHA code, but not with solution of elementary rate equations.

Journal Articles

$$^{57}$$Fe polarization dependent synchrotron M$"o$ssbauer spectroscopy using a diamond phase plate and an iron borate nuclear Bragg monochromator

Mitsui, Takaya; Imai, Yasuhiko*; Masuda, Ryo*; Seto, Makoto*; Mibu, Ko*

Journal of Synchrotron Radiation, 22(2), p.427 - 435, 2015/03

 Times Cited Count:10 Percentile:49.93(Instruments & Instrumentation)

Journal Articles

Nanoscale diffusion tracing by radioactive $$^{8}$$Li tracer

Ishiyama, Hironobu*; Jeong, S.-C.*; Watanabe, Yutaka*; Hirayama, Yoshikazu*; Imai, Nobuaki*; Miyatake, Hiroari*; Oyaizu, Mitsuhiro*; Katayama, Ichiro*; Osa, Akihiko; Otokawa, Yoshinori; et al.

Japanese Journal of Applied Physics, 53(11), p.110303_1 - 110303_4, 2014/11

 Times Cited Count:4 Percentile:18.27(Physics, Applied)

Journal Articles

Development of divertor simulation research in the GAMMA 10/PDX tandem mirror

Nakashima, Yosuke*; Sakamoto, Mizuki*; Yoshikawa, Masayuki*; Oki, Kensuke*; Takeda, Hisahito*; Ichimura, Kazuya*; Hosoi, Katsuhiro*; Hirata, Mafumi*; Ichimura, Makoto*; Ikezoe, Ryuya*; et al.

Proceedings of 25th IAEA Fusion Energy Conference (FEC 2014) (CD-ROM), 8 Pages, 2014/10

Journal Articles

Coordinated Research Projects (CRP) on atomic and molecular data at IAEA, 3; Data evaluation of code comparison activities

Ichikawa, Yukikazu*; Takagi, Shuichi*; Nakamura, Yoshiharu*; Imai, Makoto*; Sasaki, Akira

Purazuma, Kaku Yugo Gakkai-Shi, 89(9), p.600 - 610, 2013/09

no abstracts in English

Journal Articles

Present status of hydrogen production and the ammonia production by the thermochemical cycle; Introduction of IS cycle and ISN cycle

Kameyama, Hideo*; Sakurai, Makoto*; Masuda, Akiyuki*; Fukui, Tomoaki*; Onuki, Kaoru; Kubo, Shinji; Imai, Yoshiyuki

Suiso Enerugi Shisutemu, 37(1), p.3 - 10, 2012/03

The technical present status of hydrogen production process using IS thermochemical cycle was introduced. This process is experimentally investigated in Japan, U.S.A., Germany, France, Italy, India, China and Korea. Japan Atomic Energy Agency succeeded in consecutive hydrogen production as a proof examination. The trend of the research and development about the reactions, separation technology, device materials and the process equipment were reported. Thermochemical ammonia production cycle was also introduced. This new cycle is named ISN cycle which was modified from IS cycle in order to produce ammonia from water and nitrogen.

Journal Articles

Observation of ion cyclotron emission owing to DD fusion product H ions in JT-60U

Sato, Shoichi*; Ichimura, Makoto*; Yamaguchi, Yusuke*; Katano, Makoto*; Imai, Yasutaka*; Murakami, Tatsuya*; Miyake, Yuichiro*; Yokoyama, Takuro*; Moriyama, Shinichi; Kobayashi, Takayuki; et al.

Plasma and Fusion Research (Internet), 5, p.S2067_1 - S2067_4, 2010/12

Ion cyclotron emissions (ICEs) due to deuterium-deuterium fusion-product (FP) ions on JT-60U are studied. ICE due to H-ions is identified from the difference of the toroidal wave number of 2nd ICE(D). The parameter dependence for the appearance of ICE(H) is investigated from the experimental conditions and also is studied by using "Escape Particle Orbit analysis Code (EPOC)".

Journal Articles

A New measurement of the astrophysical $$^8$$Li(d,t)$$^7$$Li reaction

Hashimoto, Takashi; Ishiyama, Hironobu*; Watanabe, Yutaka*; Hirayama, Yoshikazu*; Imai, Nobuaki*; Miyatake, Hiroari; Jeong, S.-C.*; Tanaka, Masahiko*; Yoshikawa, Nobuharu*; Nomura, Toru*; et al.

Physics Letters B, 674(4-5), p.276 - 280, 2009/04

 Times Cited Count:6 Percentile:43.52(Astronomy & Astrophysics)

The excitation function of the $$^8$$Li(d,t)$$^7$$Li reaction was directly measured using $$^8$$Li beams at E$$_{mathrm{cm}}$$ = 0.3, 0.4, 0.5, 0.7, 0.8, 1.0, 1.1, and 1.2 MeV with CD$$_2$$ targets. The beam energies covered the Gamow peaks for 1$$sim$$3$$times$$10$$^9$$ K. Large cross sections were observed at around E$$_{mathrm{cm}}$$ = 0.8 MeV, implying a resonance state located at 22.4 MeV in $$^{10}$$Be. The present astrophysical reaction rate is higher in one order magnitude than the presently adopted rate at around 1$$times$$10$$^9$$ K.

Journal Articles

Charge state evolution of 2MeV/u sulfur ion passing through thin carbon foil

Imai, Makoto*; Sataka, Masao; Kawatsura, Kiyoshi*; Takahiro, Katsumi*; Komaki, Kenichiro*; Shibata, Hiromi*; Sugai, Hiroyuki; Nishio, Katsuhisa

Nuclear Instruments and Methods in Physics Research B, 256(1), p.11 - 15, 2007/03

 Times Cited Count:6 Percentile:45.71(Instruments & Instrumentation)

no abstracts in English

Journal Articles

High-energy-resolution monochromator for nuclear resonant scattering of synchrotron radiation by Te-125 at 35.49 keV

Imai, Yasuhiko*; Yoda, Yoshitaka*; Kitao, Shinji*; Masuda, Ryo; Higashitaniguchi, Satoshi*; Inaba, Chika*; Seto, Makoto

Advances in X-ray/EUV Optics and Components II (Proceedings of SPIE Vol.6705), p.670512_1 - 670512_7, 2007/00

We have developed a high-resolution monochromator (HRM) for the measurement of nuclear resonant scattering of synchrotron radiation by $$^{125}$$Te at 35.49 keV using the backscattering of sapphire (9 1 -10 68). The relative energy resolution of $$2.1times10^{-7}$$ is achieved, that is 7.5 meV in energy bandwidth. A new HRM has been desired at this energy region because of the low efficiency of usual Si HRMs. This HRM opens studies on element-specific dynamics and electronic state of substances containing $$^{125}$$Te.

Journal Articles

Overview of national centralized tokamak program; Mission, design and strategy to contribute ITER and DEMO

Ninomiya, Hiromasa; Akiba, Masato; Fujii, Tsuneyuki; Fujita, Takaaki; Fujiwara, Masami*; Hamamatsu, Kiyotaka; Hayashi, Nobuhiko; Hosogane, Nobuyuki; Ikeda, Yoshitaka; Inoue, Nobuyuki; et al.

Journal of the Korean Physical Society, 49, p.S428 - S432, 2006/12

To contribute DEMO and ITER, the design to modify the present JT-60U into superconducting coil machine, named National Centralized Tokamak (NCT), is being progressed under nationwide collaborations in Japan. Mission, design and strategy of this NCT program is summarized.

Journal Articles

Production of a low-energy radioactive nuclear beam with high purity using JAERI-RMS

Ishiyama, Hironobu*; Ishikawa, Tomoko*; Hashimoto, Takashi; Watanabe, Yutaka*; Hirayama, Yoshikazu*; Imai, Nobuaki*; Miyatake, Hiroari; Tanaka, Masahiko*; Fuchi, Yoshihide*; Yoshikawa, Nobuharu*; et al.

Nuclear Instruments and Methods in Physics Research A, 560(2), p.366 - 372, 2006/05

 Times Cited Count:7 Percentile:47.55(Instruments & Instrumentation)

Thanks to the nature of inverse transfer-reactions, low-energy radioactive nuclear beams in light neutron-rich region were produced. The mass-separation and velocity-separation of the JAERI recoil mass-separator help to form high purity beams. The beams of $$^8$$Li, $$^{12}$$B, and $$^{16}$$N-RNBs are utilized to the experiments, so far, with those beam intensities and purities of 1.4$$times$$10$$^4$$ pps and 99$$%$$, 7.8$$times$$10$$^3$$ pps and 98$$%$$, and 4.7$$times$$10$$^3$$ pps and 98.5$$%$$, respectively.

Journal Articles

Overview of the national centralized tokamak programme

Kikuchi, Mitsuru; Tamai, Hiroshi; Matsukawa, Makoto; Fujita, Takaaki; Takase, Yuichi*; Sakurai, Shinji; Kizu, Kaname; Tsuchiya, Katsuhiko; Kurita, Genichi; Morioka, Atsuhiko; et al.

Nuclear Fusion, 46(3), p.S29 - S38, 2006/03

 Times Cited Count:13 Percentile:41.84(Physics, Fluids & Plasmas)

The National Centralized Tokamak (NCT) facility program is a domestic research program for advanced tokamak research to succeed JT-60U incorporating Japanese university accomplishments. The mission of NCT is to establish high beta steady-state operation for DEMO and to contribute to ITER. The machine flexibility and mobility is pursued in aspect ratio and shape controllability, feedback control of resistive wall modes, wide current and pressure profile control capability for the demonstration of the high-b steady state.

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