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Journal Articles

The $$f$$-electron state of the heavy fermion superconductor NpPd$$_5$$Al$$_2$$ and the isostructural family

Metoki, Naoto; Aczel, A. A.*; Aoki, Dai*; Chi, S.*; Fernandez-Baca, J. A.*; Griveau, J.-C.*; Hagihara, Masato*; Hong, T.*; Haga, Yoshinori; Ikeuchi, Kazuhiko*; et al.

JPS Conference Proceedings (Internet), 30, p.011123_1 - 011123_6, 2020/03

Rare earths (4$$f$$) and actinides (5$$f$$) provide variety of interesting states realized with competing interactions between the increasing number of $$f$$ electrons. Since crystal field splitting of many-body $$f$$ electron system is smaller than the bandwidth, (1) high resolution experiments are needed, (2) essentially no clear spectrum with well defined peaks is expected in itinerant Ce and U compounds, and (3) Np and Pu is strictly regulated. Therefore, systematic research on magnetic excitations by neutron scattering experiments of localized compounds and rare earth iso-structural reference is useful. We describe the $$f$$ electron states of heavy electron compounds NpPd$$_5$$Al$$_2$$ and actinide and rare earth based iso-structural family.

Journal Articles

MAGIC chopper; Basic concept and experimental evaluation

Nakamura, Mitsutaka; Ikeuchi, Kazuhiko*; Kajimoto, Ryoichi; Kambara, Wataru; Krist, T.*; Shinohara, Takenao; Arai, Masatoshi; Iida, Kazuki*; Kamazawa, Kazuya*; Inamura, Yasuhiro; et al.

JAEA-Conf 2015-002, p.339 - 348, 2016/02

We have developed a new Fermi chopper referred to as Magic chopper to realize the full optimization of the experimental condition for Multi-Ei method in a chopper spectrometer. In this study, the theoretical aspects of MAGIC chopper concept will be initially presented, and the performances of MAGIC chopper will be evaluated by both Monte Carlo simulation and neutron transmission experiment.

Journal Articles

Structure and dynamics of solid electrolyte (LiI)$$_{0.3}$$(LiPO$$_{3}$$)$$_{0.7}$$

Kartini, E.*; Nakamura, Mitsutaka; Arai, Masatoshi; Inamura, Yasuhiro; Nakajima, Kenji; Maksum, T.*; Hoggowiranto, W.*; Putra, T. Y. S. P.*

Solid State Ionics, 262, p.833 - 836, 2014/09

 Times Cited Count:19 Percentile:60.77(Chemistry, Physical)

We present the neutron scattering study of superionic glass (LiI)$$_{0.3}$$(LiPO$$_{3}$$)$$_{0.7}$$ by using the inelastic neutron spectrometer AMATERAS at J-PARC. From the inelastic scattering, low energy excitation or the Boson Peak appears at $$sim$$ 6.5 meV. The extra quasielastic scattering was observed in the energy range 1 meV $$<$$ E $$<$$ 3 meV at 285 K but not at 20 K. The Q dependence of the dynamical structure factor S(Q,E) can be approximated to the long-wave acoustic like density fluctuation.

Journal Articles

Precision hfs of $$^{126}$$Cs($$T$$$$_{1/2}$$ = 1.63 m) by ABMR

Pinard, J.*; Duong, H. T.*; Marescaux, D.*; Stroke, H. H.*; Redi, O.*; Gustafsson, M.*; Nilsson, T.*; Matsuki, S.*; Kishimoto, Yasuaki*; Kominato, K.*; et al.

Nuclear Physics A, 753(1-2), p.3 - 12, 2005/05

 Times Cited Count:4 Percentile:36.02(Physics, Nuclear)

The hfs separation $$Deltanu$$ of $$^{126}$$Cs($$T$$$$_{1/2} = 1.63$$ m) in the 6s $$^2$$S$$_{1/2}$$ ground state was obtained in a precision measurement near zero magnetic field by means of atomic beam magnetic resonance with laser optical pumping on-line with the CERN-PSB-ISOLDE mass separator. The result, $$Deltanu = 3629.514(0.001)$$ MHz, corrects significantly a previous published value from a high-field experiment. With our result, the precision of the nuclear magnetic moment, $$mu(^{126}$$Cs)$$sim 0.776 mu_N$$, is now limited by the influence of extended nuclear structure on the hfs (the Bohr-Weisskopf effect).

Oral presentation

Current status of software development for chopper spectrometer in MLF

Inamura, Yasuhiro; Nakajima, Kenji; Kajimoto, Ryoichi; Otomo, Toshiya*; Nakatani, Takeshi; Suzuki, Jiro*; Arai, Masatoshi; So, J.-Y.*; Park, J.-G.*; Perring, T.*; et al.

no journal, , 

We report the plan and current status of development for software used on high-intensity chopper spectrometer, 4SEASONS, and Cold Neutron Disk-Chopper Spectrometer, CNDCS, at Materials and Life Science Facility(MLF), J-PARC. We begin to design software packages based on many required functions for performing experiments and analysis, for example control spectrometer system (data acquisition, devices), suggestion of experiment conditions, visualization and so on. This project progresses with software company. On the other hand, we started to collaborate with Korean group about the development of analysis software for inelastic scattering. In this presentation, we will present the current status and plan for software development including collaboration with Korean group.

Oral presentation

Low energy inelastic neutron scattering on LaFePO$$_{0.9}$$

Ishikado, Motoyuki*; Kodama, Katsuaki; Kajimoto, Ryoichi*; Nakamura, Mitsutaka; Inamura, Yasuhiro; Wakimoto, Shuichi; Iyo, Akira*; Eisaki, Hiroshi*; Arai, Masatoshi; Shamoto, Shinichi; et al.

no journal, , 

no abstracts in English

Oral presentation

Low energy inelastic neutron scattering on LaFePO$$_{0.9}$$

Ishikado, Motoyuki*; Kodama, Katsuaki; Kajimoto, Ryoichi*; Nakamura, Mitsutaka; Inamura, Yasuhiro; Wakimoto, Shuichi; Iyo, Akira*; Eisaki, Hiroshi*; Arai, Masatoshi; Shamoto, Shinichi; et al.

no journal, , 

We report results of inelastic neutron scattering measurement on powder sample of relatively low-Tc LaFePO$$_{0.9}$$ ($$T_{rm c}$$ $$sim$$ 5 K). Spin fluctuation arising from $$Gamma$$-M point FS nesting was not clearly observed on LaFePO$$_{0.9}$$. This feature is similar with LaFeAsO1-xFx (x = 15.8%, $$T_{rm c}$$ 7 K). Considering the fact that the magnetic fluctuation is also observed on high-$$T_{rm c}$$ material of x=8.2% ($$T_{rm c}$$=29 K), it indicates strong correlation between magnetic fluctuation arising from $$Gamma$$-M FS nesting and high-$$T_{rm c}$$. Furthermore, we also report recent experimental results performed by using CTAX (Triple Axis Spectrometer) at HFIR in ORNL and IN5 (chopper spectrometer) in ILL in order to see magnetic excitation and resonance mode at lower $$Q$$-$$E$$ space and temperature region on LaFePO$$_{0.9}$$.

Oral presentation

Nodal superconductivity and spin excitation on iron-based superconductors

Shamoto, Shinichi; Ishikado, Motoyuki*; Kodama, Katsuaki; Kajimoto, Ryoichi; Nakamura, Mitsutaka; Inamura, Yasuhiro; Iyo, Akira*; Eisaki, Hiroshi*; Hong, T.*; Mutka, H.*; et al.

no journal, , 

Some nodal iron-based superconductors such as LaFePO have been discovered. Their spin excitation spectra will be discussed in relation to their superconducting gap symmetries.

Oral presentation

$$f$$-electron states in RPd$$_5$$Al$$_2$$ (R: Pr, Nd)

Metoki, Naoto; Yamauchi, Hiroki; Kitazawa, Hideaki*; Suzuki, Hiroyuki*; Hagihara, Masato*; Masuda, Takatsugu*; Matsuda, Masaaki*; Aczel, A. A.*; Songxue, C.*; Hong, T.*; et al.

no journal, , 

In order to elucidate the 5$$f$$-electron states in the heavy electron superconductor NpPd$$_5$$Al$$_2$$, neutron scattering experiments of the rare earth based iso-structural family have been carried out. The observed crystal field excitations of PrPd$$_5$$Al$$_2$$ and NdPd$$_5$$Al$$_2$$ were analyzed via the crystal field Hamiltonian with tetragonal symmetry, diagonalized analytically. The experimentally obtained crystal field parameters $$A_{lm}$$were very similar in CePd$$_5$$Al$$_2$$, PrPd$$_5$$Al$$_2$$, and NdPd$$_5$$Al$$_2$$, indicating a common effective charge potential in this series. We succeeded to clarify the 5$$f$$ electron states of NpPd$$_5$$Al$$_2$$ and UPd$$_5$$Al$$_2$$ in comparison with these results.

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