Oxide particles in oxide dispersion strengthened steel neutron-irradiated up to 158 dpa at Joyo

Toyama, Takeshi*; Tanno, Takashi; Yano, Yasuhide; Inoue, Koji*; Nagai, Yasuyoshi*; Otsuka, Satoshi; Miyazawa, Takeshi; Mitsuhara, Masatoshi*; Nakashima, Hideharu*; Onuma, Masato*; et al.

Journal of Nuclear Materials, 599, p.155252_1 - 155252_14, 2024/10

https://doi.org/10.1016/j.jnucmat.2024.155252

We investigated the stability of oxide nano particles in oxide dispersion-strengthened (ODS) steel, which is a promising candidate material for next-generation reactors, under neutron irradiation at high temperature to high doses. MA957, a 14Cr-ODS steel, was irradiated with Joyo in Japan Atomic Energy Agency under irradiation conditions of 130 dpa at 502C, 154 dpa at 589C, and 158 dpa at 709C. Three-dimensional atom probe (3D-AP) and transmission electron microscope (TEM) observation were performed to characterize the oxide particles in the ODS steels. A high number density of Y-Ti-O particle was observed in the unirradiated and irradiated samples. Almost no change in the morphology of the oxide particles, i.e. average diameter, number density, and chemical composition, has been observed in the samples irradiated to 130 dpa at 502C and to 154 dpa at 589C. A slight decrease in number density was observed in the sample irradiated to 158 dpa at 709CC. The hardness of any of the irradiated samples was almost unchanged from that of the unirradiated sample. It was revealed that the oxide particles existed stable, and the strength of the material was sufficiently maintained even after being neutron irradiated to high dose of 160 dpa at high temperature up to 700C. A part of this study includes the results of MEXT Innovative Nuclear Research and Development Program Grant Number JPMXD0219214482.

Formulation of high-temperature strength equation of 9Cr-ODS tempered martensitic steels using the Larson-Miller parameter and life-fraction rule for rupture life assessment in steady-state, transient, and accident conditions of fast reactor fuel

Miyazawa, Takeshi; Tanno, Takashi; Imagawa, Yuya; Hashidate, Ryuta; Yano, Yasuhide; Kaito, Takeji; Otsuka, Satoshi; Mitsuhara, Masatoshi*; Toyama, Takeshi*; Onuma, Masato*; et al.

Journal of Nuclear Materials, 593, p.155008_1 - 155008_16, 2024/05

https://doi.org/10.1016/j.jnucmat.2024.155008

High-temperature creep properties of 9Cr-ODS tempered martensitic steel and quantitative correlation with its nanometer-scale structure

Otsuka, Satoshi; Shizukawa, Yuta; Tanno, Takashi; Imagawa, Yuya; Hashidate, Ryuta; Yano, Yasuhide; Onizawa, Takashi; Kaito, Takeji; Onuma, Masato*; Mitsuhara, Masatoshi*; et al.

Journal of Nuclear Science and Technology, 60(3), p.288 - 298, 2023/03

https://doi.org/10.1080/00223131.2022.2096147

JAEA has been developing 9Cr-oxide dispersion strengthened (ODS) tempered martensitic steel(TMS) as a candidate material for the fuel cladding tubes of sodium-cooled fast reactors(SFRs). The reliable prediction of in-reactor creep-rupture strength is critical for implementing the 9Cr-ODS TMS cladding tube in the SFR. This study investigated the quantitative correlation between the creep properties of 9Cr-ODS TMS at 700 C and the dispersions of nanosized oxides by analyzing the creep data and the material's nanostructure. The possibility of deriving a formula for estimating the in-reactor creep properties of 9Cr-ODS TMSs based on an analysis of the nanostructure of neutron-irradiated 9Cr-ODS TMSs was also discussed. The creep properties of 9Cr-ODS TMS at 700 C closely correlated with the dispersion of nanosized oxide particles. The correlation between creep-rupture lives and nanosized oxide particle dispersion was determined using existing creep models. The elucidation of correlation between the stress exponent of secondary creep rate and the nanostructure is essential to enhance future modeling reliability and formulation.

Estimated isotopic compositions of Yb in enriched Yb for producing Lu with high radionuclide purity by Yb()Lu

Nagai, Yasuki*; Kawabata, Masako*; Hashimoto, Shintaro; Tsukada, Kazuaki; Hashimoto, Kazuyuki*; Motoishi, Shoji*; Saeki, Hideya*; Motomura, Arata*; Minato, Futoshi; Ito, Masatoshi*

Journal of the Physical Society of Japan, 91(4), p.044201_1 - 044201_10, 2022/04

https://doi.org/10.7566/JPSJ.91.044201

Recently, Lu is considered as one of the most important medical RIs for treating neuroendocrine tumors. A plan to produce Lu with high purity by using enriched Yb samples with irradiation of deuteron beams in accelerators has been discussed. However, since the other Yb isotopes contained in the Yb sample interacts with deuterons, Lu isotopes other than Lu are produced as impurities. Since the purity of Lu is important for medical use, a method to evaluate the impurity of Lu has been required. In this study, we proposed a new method to estimate production yields of each Lu isotopes in Yb samples with arbitrary isotopic compositions by using excitation functions of Yb()Lu reactions and the particle transport calculation code PHITS. The method plays an important role in discussing the isotopic composition of enriched samples to produce high-purity Lu using accelerators.

Local structure study of the iron-based systems of BaFeAs and LiFeAs by X-ray PDF and XAFS analyses

Li, S.*; Toyoda, Masayuki*; Kobayashi, Yoshiaki*; Ito, Masayuki*; Ikeuchi, Kazuhiko*; Yoneda, Yasuhiro; Otani, Akira*; Matsumura, Daiju; Asano, Shun*; Mizuki, Junichiro*; et al.

Physica C, 555, p.45 - 53, 2018/12

https://doi.org/10.1016/j.physc.2018.10.003

-dependence of local distortions in BaFeAs and LiFeAs by X-ray PDF and XAFS methods. Although PDF data exhibit anomaly at the structure transition temperature, EXAFS data exhibit no anomaly. Data supporting the local orthorhombicity at 300 K in the tetragonal phase for BaFeAs. Arguments on the origins of the 4-fold symmetry breaking in the ground average structure of the tetragonal phase.

Mo yield using large sample mass of MoO for sustainable production of Mo

Tsukada, Kazuaki; Nagai, Yasuki*; Hashimoto, Kazuyuki*; Kawabata, Masako*; Minato, Futoshi; Saeki, Hideya*; Motoishi, Shoji*; Ito, Masatoshi*

Journal of the Physical Society of Japan, 87(4), p.043201_1 - 043201_5, 2018/04

https://doi.org/10.7566/JPSJ.87.043201

Progress report of Japanese simulation research projects using the high-performance computer system Helios in the International Fusion Energy Research Centre

Ishizawa, Akihiro*; Idomura, Yasuhiro; Imadera, Kenji*; Kasuya, Naohiro*; Kanno, Ryutaro*; Satake, Shinsuke*; Tatsuno, Tomoya*; Nakata, Motoki*; Nunami, Masanori*; Maeyama, Shinya*; et al.

Purazuma, Kaku Yugo Gakkai-Shi, 92(3), p.157 - 210, 2016/03

http://www.jspf.or.jp/Journal/PDF_JSPF/jspf2016_03/jspf2016_03-157.pdf

The high-performance computer system Helios which is located at The Computational Simulation Centre (CSC) in The International Fusion Energy Research Centre (IFERC) started its operation in January 2012 under the Broader Approach (BA) agreement between Japan and the EU. The Helios system has been used for magnetised fusion related simulation studies in the EU and Japan and has kept high average usage rate. As a result, the Helios system has contributed to many research products in a wide range of research areas from core plasma physics to reactor material and reactor engineering. This project review gives a short catalogue of domestic simulation research projects. First, we outline the IFERC-CSC project. After that, shown are objectives of the research projects, numerical schemes used in simulation codes, obtained results and necessary computations in future.

Nitrogen K-edge X-ray absorption near edge structure of pyrimidine-containing nucleotides in aqueous solution

Shimada, Hiroyuki*; Minami, Hirotake*; Okuizumi, Naoto*; Sakuma, Ichiro*; Ukai, Masatoshi*; Fujii, Kentaro; Yokoya, Akinari; Fukuda, Yoshihiro*; Saito, Yuji

Journal of Chemical Physics, 142(17), p.175102_1 - 175102_9, 2015/05

AA2015-0073.pdf:1.15MB

https://doi.org/10.1063/1.4919744

Nuclear resonant scattering measurements on Fe by multichannel scaling with a 64 pixel silicon avalanche photodiode linear-array detector

Kishimoto, Shunji*; Mitsui, Takaya; Haruki, Rie*; Yoda, Yoshitaka*; Taniguchi, Takashi*; Shimazaki, Shoichi*; Ikeno, Masahiro*; Saito, Masatoshi*; Tanaka, Manobu*

Review of Scientific Instruments, 85(11), p.113102_1 - 113102_5, 2014/11

https://doi.org/10.1063/1.4900862

High power laser developments with femtosecond to nanosecond pulse durations for laser shock science and engineering

Kiriyama, Hiromitsu; Mori, Michiaki; Suzuki, Masayuki*; Daito, Izuru*; Okada, Hajime; Ochi, Yoshihiro; Tanaka, Momoko; Sato, Masatoshi*; Tamaoki, Yoshinori*; Yoshii, Takehiro*; et al.

Reza Kenkyu, 42(6), p.441 - 447, 2014/06

http://ci.nii.ac.jp/naid/40020137371

We describe three specific high power laser systems that are being developed in our laboratory for many applications in high field science, nonlinear optics and material processing. We report on a femtosecond petawatt-class Ti:sapphire chirped-pulse amplification laser system that can produce a pulse energy of 20 J of 40 fs pulse duration, a picosecond high intensity Yb:YAG chirped-pulse amplification laser system that can generate a pulse energy of 100 mJ of 0.5 ps pulse duration, and a nanosecond high repetition rate Nd:YAG laser system that can provide an average power of 360 W with a pulse duration of 30 ns delivered at a 1 kHz repetition rate. We discuss the basic design aspects and present the results from our experimental investigations of these laser systems.