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Journal Articles

Solvent extraction of tin in nitric acids; Evaluation of multiple extractants

Ito, Kengo*; Takahashi, Shin*; Kato, Chizu*; Fukutani, Satoshi*; Matsumura, Tatsuro; Fujii, Toshiyuki*

Journal of Radioanalytical and Nuclear Chemistry, 334, p.2467 - 2475, 2025/02

 Times Cited Count:0 Percentile:0.00(Chemistry, Analytical)

In this study, the solvent extraction behavior of tin (Sn), specifically $$^{126}$$Sn, from high-level radioactive waste was evaluated using six different extractants in a HNO$$_{3}$$ system. Among the tested extractants, N,N-Didodecyl-2-hydroxyacetoamide (HAA) exhibited higher efficiency, still not sufficient for industrial implementation. In systems where HCl was added to HNO$$_{3}$$, both tributyl phosphate (TBP) and N,N,N,N'-tetra-2-ethylhexyl diglycolamide (TEHDGA) achieved D$$_{Sn}$$ values greater than 1 at $$>$$ 1 M HCl. However, due to practical challenges in industrial applications, HAA extraction in HNO$$_{3}$$ systems, particularly at low Sn concentrations (0.0008 M), may provide a more effective solution for Sn recovery.

Journal Articles

Tensile properties of irradiated modified 316 stainless steel (PNC316) at slow strain rates

Yano, Yasuhide; Miyazawa, Takeshi; Tanno, Takashi; Akasaka, Naoaki; Yoshitake, Tsunemitsu; Kaito, Takeji; Otsuka, Satoshi

Journal of Nuclear Science and Technology, 8 Pages, 2025/00

 Times Cited Count:0 Percentile:0.00(Nuclear Science & Technology)

The effects of strain rate on tensile properties of irradiated modified 316 stainless steel (PNC316) claddings were investigated. PNC316 claddings were irradiated at the experimental fast reactor Joyo using CRT402 control rod assembly at 400$$^{circ}$$C up to 25 dpa. Post-irradiation ring tensile tests were carried out at strain rates of 3.3$$times$$10$$^{-6}$$, 3.3$$times$$10$$^{-7}$$ and 3.3$$times$$10$$^{-8}$$ s$$^{-1}$$ at a test temperature of 350$$^{circ}$$C. The results showed no obvious dependence of all strain rates on tensile properties, although a slight decrease in total elongation was observed at the slowest strain rate of 3.3$$times$$10$$^{-8}$$ s$$^{-1}$$. In addition, only a part of fracture surface at the slowest strain rate showed intergranular type region in the inner surface area, although the grain boundary separation occurred on inner surfaces near the fracture region at all strain rates. It is suggested that presence of a high content of helium near the inner surfaces would be related to the fracture behavior.

Journal Articles

Solvent extraction behaviors of rhodium and palladium in nitric acid solutions using amide extractants

Ito, Kengo*; Morita, Misaki*; Araki, Yuta*; Kato, Chizu*; Fukutani, Satoshi*; Matsumura, Tatsuro; Fujii, Toshiyuki*

Solvent Extraction Research and Development, Japan, 32(1), p.53 - 62, 2025/00

Rhodium (Rh) and Palladium (Pd) in high-level radioactive waste are primarily fission products. This Study focused on understanding the extraction behavior of these platinum group elements (PGEs) using the novel extractants ${it N,N,N',N',N'',N''}$-hexaoctylnitriloacetamide (HONTA) and alkyl diamideamine (ADAAM). Both extractants showed affinity for Pd, with distribution coefficients significantly exceeding 1, demonstrating their effectiveness in Pd separation. In contrast, the distribution coefficients for Rh were consistently below 10 $$^{-1}$$, indicating low extraction efficiency from nitric acid. However, by leveraging the salting-out effect with calcium nitrate hydrate, a distribution coefficient of $$sim$$570 for Rh was achieved using HONTA. To overcome the difficult back-extraction of PGEs with HONTA, experiments were conducted using HEDTA and thiourea. Back-extraction with HEDTA in high-concentration nitric acid ($$>$$2M) resulted in $$sim$$90% extraction of Pd, while thiourea-based back-extraction with nitric acid yielded over 40% extraction for Rh, with the maximum of 62.7% achieved using hydrochloric acid.

Journal Articles

$$^{149}$$Sm synchrotron-radiation-based M$"{o}$ssbauer spectroscopy of Sm-based heavy fermion compounds

Tsutsui, Satoshi; Higashinaka, Ryuji*; Mizumaki, Masaichiro*; Kobayashi, Yoshio*; Nakamura, Jin*; Ito, Takashi; Yoda, Yoshitaka*; Matsuda, Tatsuma*; Aoki, Yuji*; Sato, Hideyuki*

Interactions (Internet), 245(1), p.9_1 - 9_10, 2024/12

Journal Articles

$$^{149}$$Sm synchrotron-radiation-based M$"{o}$ssbauer and $$mu^+$$SR studies of Sm$$_3$$Ru$$_4$$Ge$$_{13}$$

Tsutsui, Satoshi; Ito, Takashi; Nakamura, Jin*; Yoshida, Mio*; Kobayashi, Yoshio*; Yoda, Yoshitaka*; Nakamura, Jumpei*; Koda, Akihiro*; Higashinaka, Ryuji*; Aoki, Dai*; et al.

Interactions (Internet), 245(1), p.55_1 - 55_9, 2024/12

Journal Articles

Application of indentation technique to material degradation evaluation in the mercury target vessel for spallation neutron sources

Wakui, Takashi; Saito, Shigeru; Futakawa, Masatoshi

Jikken Rikigaku, 24(4), p.212 - 218, 2024/12

Irradiation damage is one of the main factors determining the lifetime of the mercury target vessel for spallation neutron source in J-PARC. To understand material degradation of the used vessels, it is planned to conduct an evaluation using inverse analyses with indentation tests on the structural materials of the used vessels and numerical experiments. This evaluation technique was applied to two kinds of ion-irradiated materials with different displacement damage doses, in which the irradiation condition was simulated. It could be confirmed that the ultimate strength increased, and the total elongation decreased with increasing irradiation. These trends are like the material degradation behaviors which have been reported by using small specimen's tensile tests.

Journal Articles

Quantitative evaluation of irradiated ductility degradation using the indentation technique combined with numerical experiments

Wakui, Takashi; Saito, Shigeru; Futakawa, Masatoshi

Materials, 17(23), p.5925_1 - 5925_14, 2024/12

 Times Cited Count:0 Percentile:0.00(Chemistry, Physical)

The ductile properties of irradiated materials are one of the important indicators related to their structural integrity. Indentation tests are used for evaluating the ductile properties easily and rapidly. Constants in the material constitutive equation were identified via inverse analysis using the Kalman filter, such that the numerical experimental results reproduced the indentation test results. Numerical tensile experiments were conducted using stress-strain curves with the identified constants to obtain nominal stress-strain curves. Furthermore, two methods were proposed for evaluating the total elongation. Evaluated minimum total elongation was 10 %. The evaluation results of ion-irradiated materials were similar to the tensile test results of irradiated materials.

Journal Articles

Development of a nondestructive assay technique using a laser-driven neutron source

Koizumi, Mitsuo; Ito, Fumiaki*; Lee, J.; Hironaka, Kota; Takahashi, Tone; Suzuki, Satoshi*; Arikawa, Yasunobu*; Abe, Yuki*; Wei, T.*; Yogo, Akifumi*; et al.

Dai-45-Kai Nihon Kaku Busshitsu Kanri Gakkai Nenji Taikai Kaigi Rombunshu (Internet), 4 Pages, 2024/11

JAEA Reports

High-temperature strength of modified type 316 steel for fast reactor fuel before and after neutron irradiation

Miyazawa, Takeshi; Uwaba, Tomoyuki; Yano, Yasuhide; Tanno, Takashi; Otsuka, Satoshi; Onizawa, Takashi; Ando, Masanori; Kaito, Takeji

JAEA-Technology 2024-009, 140 Pages, 2024/10

JAEA-Technology-2024-009.pdf:8.03MB

For the purpose of enhancing the reliability of fast reactor fuel designing using modified type 316 steel, the out-of-pile and in-pile mechanical data of modified type 316 steel cladding tubes and wrapper tubes were statistically analyzed with the knowledge on material science and engineering; the high-temperature strength equations of modified type 316 steel, which can be applied to high-dose neutron irradiation environment, were derived. The out-of-pile high-temperature tensile and creep data of modified type 316 steel cladding tubes and wrapper tubes were derived up to 900$$^{circ}$$C, which is higher than the upper limit temperature of anticipated transient event of fast reactor. Using the extended database, the best-fit equation and the lower limit equation were derived for out-of-pile 0.2% proof strength, ultimate tensile strength and creep rupture strength while the best-fit equation and the upper and lower limit equations for creep strain. Furthermore, the degradation factors for tensile and creep strength, which will be produced by in-reactor environment (i.e., neutron irradiation in liquid sodium), were evaluated using the existing neutron irradiation data of modified type 316 steel, which were derived using the experimental fast reactor Joyo, the French proto-type fast reactor Phenix, the American experimental fast reactor FFTF. The derived equations were validated by the comparison with the experimental data.

Journal Articles

Oxide particles in oxide dispersion strengthened steel neutron-irradiated up to 158 dpa at Joyo

Toyama, Takeshi*; Tanno, Takashi; Yano, Yasuhide; Inoue, Koji*; Nagai, Yasuyoshi*; Otsuka, Satoshi; Miyazawa, Takeshi; Mitsuhara, Masatoshi*; Nakashima, Hideharu*; Onuma, Masato*; et al.

Journal of Nuclear Materials, 599, p.155252_1 - 155252_14, 2024/10

 Times Cited Count:0 Percentile:0.00(Materials Science, Multidisciplinary)

We investigated the stability of oxide nano particles in oxide dispersion-strengthened (ODS) steel, which is a promising candidate material for next-generation reactors, under neutron irradiation at high temperature to high doses. MA957, a 14Cr-ODS steel, was irradiated with Joyo in Japan Atomic Energy Agency under irradiation conditions of 130 dpa at 502$$^{circ}$$C, 154 dpa at 589$$^{circ}$$C, and 158 dpa at 709$$^{circ}$$C. Three-dimensional atom probe (3D-AP) and transmission electron microscope (TEM) observation were performed to characterize the oxide particles in the ODS steels. A high number density of Y-Ti-O particle was observed in the unirradiated and irradiated samples. Almost no change in the morphology of the oxide particles, i.e. average diameter, number density, and chemical composition, has been observed in the samples irradiated to 130 dpa at 502$$^{circ}$$C and to 154 dpa at 589$$^{circ}$$C. A slight decrease in number density was observed in the sample irradiated to 158 dpa at 709$$^{circ}$$CC. The hardness of any of the irradiated samples was almost unchanged from that of the unirradiated sample. It was revealed that the oxide particles existed stable, and the strength of the material was sufficiently maintained even after being neutron irradiated to high dose of $$sim$$160 dpa at high temperature up to 700$$^{circ}$$C. A part of this study includes the results of MEXT Innovative Nuclear Research and Development Program Grant Number JPMXD0219214482.

Journal Articles

Solvent extraction of selenium in nitric acid; Evaluation of multiple extractants and proposal of a novel separation process

Ito, Kengo*; Kawakami, Takahiro*; Kato, Chizu*; Fukutani, Satoshi*; Matsumura, Tatsuro; Fujii, Toshiyuki*

Journal of Radioanalytical and Nuclear Chemistry, 333(10), p.5183 - 5189, 2024/10

 Times Cited Count:1 Percentile:62.55(Chemistry, Analytical)

Solvent extraction behaviors of Se (VI) from nitric acid solutions were investigated with multiple extractants used for uranium, plutonium, minor actinides, and rare earthelements separation processes from high-level liquid waste. During the processes, Se remained in the residual aqueous solutions, as all extractants showed distributionratios $$<$$ 1. In contrast, Se showed distribution ratios $$>$$ 1 with $$o$$-phenylenediamine in dilute nitric acid ($$<$$ 2 M HNO$$_{3}$$), octanol as the organic phase, and concentrated nitric acid (8 M HNO$$_{3}$$) for back extraction, suggesting a potential new single separation process and recovery of Se.

Journal Articles

Chapter 9, Advanced materials; Oxide-dispersion strengthened steels

Otsuka, Satoshi; Tanno, Takashi; Yano, Yasuhide; Kaito, Takeji

Materials and Processes for Nuclear Energy Today and in the Future, p.279 - 297, 2024/10

The oxide dispersion strengthening is an effective technique for improving the mechanical strength of the steel. The dispersed oxides prevent the gliding motion of dislocations, thus remarkably enhancing the resistance to high-temperature deformation and rupture of steels. Extensive efforts have been made to develop ODS steels in the fields of nuclear and fusion engineering. Research has been done to improve their performance and meet the requirements such as irradiation resistance, high-temperature strength, and corrosion resistance. Based on recent research, the high-density dispersion of nanosized oxides could improve the irradiation resistance of the steels in addition to high-temperature strength because the interface between oxide and matrix could act as sink sites for point defects. This section overviews the ODS steel development for nuclear application.

Journal Articles

Demonstration of shape analysis of neutron resonance transmission spectrum measured with a laser-driven neutron source

Koizumi, Mitsuo; Ito, Fumiaki*; Lee, J.; Hironaka, Kota; Takahashi, Tone; Suzuki, Satoshi*; Arikawa, Yasunobu*; Abe, Yuki*; Lan, Z.*; Wei, T.*; et al.

Scientific Reports (Internet), 14, p.21916_1 - 21916_9, 2024/09

 Times Cited Count:0 Percentile:0.00(Multidisciplinary Sciences)

Journal Articles

Holocene paleolimnological changes in Rundv${aa}$shetta lakes in the Soya Coast region and their paleoenvironmental significance with glacial isostatic adjustment in East Antarctica

Inoue, Genki*; Honda, Eisuke*; Ito, Keisuke*; Kang, I.*; Seto, Koji*; Tani, Yukinori*; Watanabe, Takahiro; Kashima, Kaoru*; Otani, Shuji*; Yamanaka, Toshiro*; et al.

Quaternary Science Reviews, 338, p.108822_1 - 108822_18, 2024/08

 Times Cited Count:0 Percentile:0.00(Geography, Physical)

We studied Holocene paleolimnological changes inferred from biomarkers and microscopic observation of microalgae and cyanobacteria in sediment cores from Rundv${aa}$shetta lakes (Maruwanminami-ike and Maruwan o-ike) in the Soya Coast of East Antarctica, along with sedimentary facies and radiocarbon dating. Coastal marine environment: Maruwanminami-ike (147-72.5 cm, 5,010-2,590 cal BP) and Maruwan-oike (226-47.2 cm, 5,700-3,190 cal BP) were characterized by low biological production with the predominance of diatoms. Transition period of stratified brackish lake environment: Maruwanminami-ike (72.5-65.6 cm, 2,590-2,500 cal BP) and Maruwan-oike (47.2-28.8 cm, 3,190-2,890 cal BP) were characterized by stratified conditions with marine water overlain by freshwater, and a chemocline developed together with an anoxic layer in the bottom of photic zone.

Journal Articles

Measurement of the response of a $$^6$$Li-glass detector to gamma rays by a coincidence method

Ito, Fumiaki*; Lee, J.; Hironaka, Kota; Takahashi, Tone; Suzuki, Satoshi*; Mochimaru, Takanori*; Hori, Junichi*; Terada, Kazushi*; Koizumi, Mitsuo

Nuclear Instruments and Methods in Physics Research A, 1064, p.169465_1 - 169465_9, 2024/07

 Times Cited Count:0 Percentile:0.00(Instruments & Instrumentation)

Journal Articles

Lattice dynamics of CH(NH$$_{2}$$)$$_{2}$$PbI$$_{3}$$ and CH(NH$$_{2}$$)$$_{2}$$SnI$$_{3}$$ investigated by inelastic X-ray scattering and comparison of their elastic properties

Tamatsukuri, Hiromu; Murakami, Yoichi*; Saito, Noriko*; Ohashi, Naoki*; Tsutsui, Satoshi*

Physical Review B, 110(2), p.024301_1 - 024301_8, 2024/07

 Times Cited Count:0 Percentile:0.00(Materials Science, Multidisciplinary)

Journal Articles

Creep deformation and rupture behavior of 9Cr-ODS steel cladding tube at high temperatures from 700$$^{circ}$$C to 1000$$^{circ}$$C

Imagawa, Yuya; Hashidate, Ryuta; Miyazawa, Takeshi; Onizawa, Takashi; Otsuka, Satoshi; Yano, Yasuhide; Tanno, Takashi; Kaito, Takeji; Onuma, Masato*; Mitsuhara, Masatoshi*; et al.

Journal of Nuclear Science and Technology, 61(6), p.762 - 777, 2024/06

 Times Cited Count:3 Percentile:65.16(Nuclear Science & Technology)

The Japan Atomic Energy Agency has been developing 9Cr-oxide dispersion strengthened (ODS) steel as a fuel cladding material for sodium-cooled fast reactors (SFRs). Previous studies have formulated the creep rupture equation for 650$$^{circ}$$C to 850$$^{circ}$$C. However, little data have been obtained above 850$$^{circ}$$C, and no equation has been formulated. This study conducted creep tests to evaluate creep strength at 700$$^{circ}$$C to 1000$$^{circ}$$C. Two creep test methods, the internal pressure and ring creep tests under development, were used, and the validation of the ring creep test method was conducted. The results showed that 9Cr-ODS steel undergoes almost no strength change due to the matrix's phase transformation, and a single equation can express a creep rupture strength from 700$$^{circ}$$C to 1000$$^{circ}$$C. In validating the ring creep test method, analysis clarified the effect of stress concentration on the specimen. Plastic deformation occurs at high initial stress and may lead to early rupture. The results will be essential for future creep testing and evaluation of neutron-irradiated 9Cr-ODS steel.

Journal Articles

"Invisible" radioactive cesium atoms revealed; Pollucite inclusion in cesium-rich microparticles (CsMPs) from the Fukushima Daiichi Nuclear Power Plant

Miyazaki, Kanako*; Takehara, Masato*; Minomo, Kenta*; Horie, Kenji*; Takehara, Mami*; Yamasaki, Shinya*; Saito, Takumi*; Onuki, Toshihiko*; Takano, Masahide; Shiotsu, Hiroyuki; et al.

Journal of Hazardous Materials, 470(15), p.134104_1 - 134104_11, 2024/05

 Times Cited Count:1 Percentile:0.00(Engineering, Environmental)

Journal Articles

Formulation of high-temperature strength equation of 9Cr-ODS tempered martensitic steels using the Larson-Miller parameter and life-fraction rule for rupture life assessment in steady-state, transient, and accident conditions of fast reactor fuel

Miyazawa, Takeshi; Tanno, Takashi; Imagawa, Yuya; Hashidate, Ryuta; Yano, Yasuhide; Kaito, Takeji; Otsuka, Satoshi; Mitsuhara, Masatoshi*; Toyama, Takeshi*; Onuma, Masato*; et al.

Journal of Nuclear Materials, 593, p.155008_1 - 155008_16, 2024/05

 Times Cited Count:1 Percentile:0.00(Materials Science, Multidisciplinary)

Journal Articles

Microbiome analysis of the restricted bacteria in radioactive element-containing water at the Fukushima Daiichi Nuclear Power Station

Warashina, Tomoro*; Sato, Asako*; Hinai, Hiroshi; Shaikhutdinov, N.*; Shagimardanova, E.*; Mori, Hiroshi*; Tamaki, Satoshi*; Saito, Motofumi*; Sanada, Yukihisa; Sasaki, Yoshito; et al.

Applied and Environmental Microbiology, 90(4), p.e02113-23_1 - e02113-23_23, 2024/04

 Times Cited Count:0 Percentile:0.00(Biotechnology & Applied Microbiology)

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