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Nishihara, Kenji; Fukushima, Masahiro; Abe, Takumi; Katano, Ryota; Yee-Rendon, B.; Iwamoto, Hiroki; Sugawara, Takanori; Obayashi, Hironari; Saito, Shigeru
JAEA-Research 2025-013, 125 Pages, 2026/03
JAEA-Research-2025-013.pdf:4.68MB
A conceptual design for a pilot Accelerator Driven subcritical System (ADS) was developed as a precursor to a commercial ADS aimed at partitioning and transmutation of minor actinides. The output of the pilot ADS was set at 200 MW. Based on safety assessment results, the design incorporates deep subcriticality and safety rods. Core design, accelerator design, target design, and in-vessel equipment design were performed, clarifying the specific concept.
Takahashi, Tone; Mochimaru, Takanori*; Koizumi, Mitsuo; Yoshimi, Yuki*; Yamanishi, Hirokuni*; Wakabayashi, Genichiro*; Ito, Fumiaki*
JAEA-Review 2025-039, 34 Pages, 2025/11
JAEA-Review-2025-039.pdf:2.18MB
To prevent acts of terrorism involving nuclear or radioactive materials at major public events, it is required to have surveillance technologies that either prevent these materials from being brought in or detect quickly if somebody brings them in secretly. Setting radiation gate monitors to survey pedestrians and vehicles is one of the effective methods. However, considering the possibility of individuals bypassing these monitors, complementary technologies are needed to continuously survey areas inside the gates. To survey extensive areas, radiation mapping is effective. By using multiple detectors and aggregating the data, the survey becomes much more efficient. We have developed mobile detectors capable of simultaneously measuring location data and radiation levels outdoors, with the ability to aggregate measurement results via a network and immediately visualize them on a map. For indoor environments, we have developed a technology that integrates radiation measurement results with environmental mapping created using SLAM (Simultaneous Localization and Mapping) to produce 3D maps of the surveyed areas. Additionally, we have been working on the development of a source search technology using a fast neutron detector to quickly detect neutron sources, including nuclear materials. In this report, we describe a concept of the wide area survey system and report technology development results so far.
Liu, Y.*; Otani, Masashi*; Miyao, Tomoaki*; Nakazawa, Yuga*; Shibata, Takanori*; Nammo, Kesao*; Fang, Z.*; Futatsukawa, Kenta*; Fukui, Yuji*; Mizobata, Satoshi*; et al.
Proceedings of 16th International Particle Accelerator Conference (IPAC25) (Internet), p.855 - 857, 2025/11
Saito, Hiroyukki*; Machida, Akihiko*; Hattori, Takanori; Sano, Asami; Funakoshi, Kenichi*; Sato, Toyoto*; Orimo, Shinichi*; Aoki, Katsutoshi*
Physica B; Condensed Matter, 714, p.417234_1 - 417234_3, 2025/10
Times Cited Count：0 Percentile：0.00(Physics, Condensed Matter)Corrigendum to "Neutron diffraction study on the deuterium composition of nickel deuteride at high temperatures and high pressures" [Phys. B Condens. Matter. 587 (2020) 412153] was reported.
Machida, Akihiko*; Saito, Hiroyuki*; Aoki, Katsutoshi*; Komatsu, Kazuki*; Hattori, Takanori; Sano, Asami; Funakoshi, Kenichi*; Machida, Shinichi*; Sato, Toyoto*; Orimo, Shinichi*
Physical Review B, 111(22), p.224413_1 - 224413_6, 2025/06
Times Cited Count：1 Percentile：47.59(Materials Science, Multidisciplinary)The crystal and magnetic structures of antiferromagnetic Mn deuterides formed by hydrogenating Mn metal at high temperature and high pressure, fcc 
-MnDx and hcp 
-MnDx, were investigated by in-situ neutron powder diffraction. Deuterium atoms partially occupied the octahedral interstitial positions of the fcc and hcp metal lattices. The site occupancies increased rapidly with decreasing temperature from 
700 to 450 K and remained down to 300 K. N
el temperature of 543(10) K was determined for -MnD
. For -MnD
, saturation magnetic moment and Nel temperature were determined to be 0.82(1) 
and 347(3) K, respectively. The Nel temperatures determined for -MnD and -MnD are consistent with those predicted by the respective Slater-Pauling curves proposed in previous studies. The updated Nel temperatures provide insights into the development of more accurate Slater-Pauling curves based on electronic band structure calculations.
Aoki, Katsutoshi*; Machida, Akihiko*; Saito, Hiroyuki*; Hattori, Takanori
Koatsuryoku No Kagaku To Gijutsu, 35(1), p.4 - 11, 2025/03
Iron reacts with hydrogen to form solid solutions with body-centered cubic, face-centered cubic, hexagonal close packed, and double hexagonal close packed structures at high temperatures and high pressures. Neutron diffraction is the most powerful tool for determining the occupation sites and occupancies of hydrogen atoms dissolved in a metal lattice. Structural parameters, including hydrogen occupation sites and occupancies, are refined via Rietveld analysis for neutron diffraction data. We present our expertise in Rietveld refinement of iron hydrides accumulated over 10 years.
Sb
with a honeycomb networkAdachi, Tadashi*; Ogawa, Taiki*; Komiyama, Yota*; Sumura, Takuya*; Saito-Tsuboi, Yuki*; Takeuchi, Takaaki*; Mano, Kohei*; Manabe, Kaoru*; Kawabata, Koki*; Imazu, Tsuyoshi*; et al.
Physical Review B, 111(10), p.L100508_1 - L100508_6, 2025/03
Times Cited Count：1 Percentile：0.00(Materials Science, Multidisciplinary)Machida, Akihiko*; Saito, Hiroyuki*; Sugimoto, Hidehiko*; Hattori, Takanori; Sano, Asami; Endo, Naruki*; Katayama, Yoshinori*; Iizuka, Riko*; Sato, Toyoto*; Matsuo, Motoaki*; et al.
Nature Communications (Internet), 15, p.8861_1 - 8861_2, 2024/10
Times Cited Count：2 Percentile：0.00(Multidisciplinary Sciences)In our previous article (Nature Commun. 5, 5063 (2014)), the site occupancies of D atoms dissolved in an fcc Fe metal lattice were investigated via Rietveld refinement of neutron powder diffraction patterns collected at 988 K and 6.3 GPa. The fcc metal lattice has two interstitial sites available for accommodating D atoms: octahedral and tetrahedral sites. The Rietveld refinement revealed that D atoms occupied mainly the octahedral sites with occupancy of 0.532 and slightly the tetrahedral sites with occupancy of 0.056. Subsequent density-functional-theory (DFT) calculations by Antonov (Phys. Rev. Mater. 2019)) showed that the occupation energy on the tetrahedral site was significantly higher than that on the octahedral site; the tetrahedral site occupation was unlikely to occur even at temperatures as high as 988 K. We reexamined the site occupancies of D-atom by Rietveld refinement including extinction correction. As a result, the octahedral occupancy was increased to 0.60 and the tetrahedral occupancy was reduced to zero. The occupation of only the octahedral site for D atom is consistent with the DFT calculation, although in contrast to the previous results.
Hattori, Takanori; Suzuki, Koji*; Miyo, Tatsuya*; Ito, Takayoshi*; Machida, Shinichi*
Nuclear Instruments and Methods in Physics Research A, 1064, p.169448_1 - 169448_9, 2024/07
Times Cited Count：0 Percentile：0.00(Instruments & Instrumentation)The authors regret that the abstract and summary explain that the cup diameter of a standard double-toroidal anvils is 1.5 mm. This is incorrect; the standard diameter is 4.0 mm. The authors would like to apologise for any inconvenience caused.
Li-glass detector to gamma rays by a coincidence methodIto, Fumiaki*; Lee, J.; Hironaka, Kota; Takahashi, Tone; Suzuki, Satoshi*; Mochimaru, Takanori*; Hori, Junichi*; Terada, Kazushi*; Koizumi, Mitsuo
Nuclear Instruments and Methods in Physics Research A, 1064, p.169465_1 - 169465_9, 2024/07
Times Cited Count：0 Percentile：0.00(Instruments & Instrumentation)
O ice observed by neutron diffractionKomatsu, Kazuki*; Hattori, Takanori; Klotz, S.*; Machida, Shinichi*; Yamashita, Keishiro*; Ito, Hayate*; Kobayashi, Hiroki*; Irifune, Tetsuo*; Shimmei, Toru*; Sano, Asami; et al.
Nature Communications (Internet), 15, p.5100_1 - 5100_7, 2024/06
Times Cited Count：21 Percentile：85.99(Multidisciplinary Sciences)Hydrogen bond symmetrisation is the phenomenon where a hydrogen atom is located at the centre of a hydrogen bond. Theoretical studies predict that hydrogen bonds in ice VII eventually undergo symmetrisation upon increasing pressure, involving nuclear quantum effect with significant isotope effect and drastic changes in the elastic properties through several intermediate states with varying hydrogen distribution. Despite numerous experimental studies conducted, the location of hydrogen and hence the transition pressures reported up to date remain inconsistent. Here we report the atomic distribution of deuterium in DO ice using neutron diffraction above 100 GPa and observe for the first time the transition from a bimodal to a unimodal distribution of deuterium at around 80 GPa. At the transition pressure, a significant narrowing of the peak widths of 110 was also observed, attributed to the structural relaxation by the change of elastic properties.
Ichikawa, Tsubasa*; Hakoshima, Hideaki*; Inui, Koji*; Ito, Kosuke*; Matsuda, Ryo*; Mitarai, Kosuke*; Miyamoto, Koichi*; Mizukami, Wataru*; Mizuta, Kaoru*; Mori, Toshio*; et al.
Nature Reviews Physics (Internet), 6(6), p.345 - 347, 2024/06
Times Cited Count：13 Percentile：98.48(Physics, Applied)Hattori, Takanori; Suzuki, Koji*; Miyo, Tatsuya*; Ito, Takayoshi*; Machida, Shinichi*
Nuclear Instruments and Methods in Physics Research A, 1059, p.168956_1 - 168956_9, 2024/02
Times Cited Count：2 Percentile：32.62(Instruments & Instrumentation)Radial collimators (RC) with a 0.5 mm gauge size (GS) were specially designed for high-pressure neutron diffraction experiments and their performance and efficacy were investigated. The RCs with nominal GS of 0.75 mm, 1.5 mm, and 3.0 mm effectively exhibited GS of 0.50 mm, 1.07 mm, and 2.78 mm, respectively. The transmissions of all three RCs were almost equivalent. The assessment using a P-E press and a DAC revealed that the anvil scattering was considerably minimized and the sample-to-anvil signal ratio reached values of 0.5 and 2.0 for the PE press and DAC, respectively, when using the 0.5 mm-GS RCs. These results indicate that the 0.5mm-GS RCs have been fabricated as intended and exhibit efficacy for the high-pressure-neutron diffraction experiments, specifically those exceeding 30 GPa. Among those ever manufactured for neutron scattering experiments, the RCs display the smallest GS.
neutron diffractionKobayashi, Hiroki*; Komatsu, Kazuki*; Ito, Hayate*; Machida, Shinichi*; Hattori, Takanori; Kagi, Hiroyuki*
Journal of Physical Chemistry Letters (Internet), 14(47), p.10664 - 10669, 2023/11
Times Cited Count：3 Percentile：26.53(Chemistry, Physical)Ice IV is a metastable high-pressure phase of ice in which the water molecules exhibit orientational disorder. Although orientational ordering is commonly observed for other ice phases, it has not been reported for ice IV. We conducted powder neutron diffraction experiments for DCl-doped D
O ice IV to investigate hydrogen ordering in ice IV. We found abrupt changes in the temperature derivative of unit cell volume, dV/dT, at about 120 K, and revealed their slightly ordered structure at low temperatures based on the Rietveld method. The occupancy of the D1 site deviates from 0.5; it increased when samples were cooled at higher pressures and reached 0.282(5) at 2.38 GPa, 58 K. Our results evidence the presence of a low-symmetry hydrogen-ordered state corresponding to ice IV. It seems, however, difficult to experimentally access the completely ordered phase corresponding to ice IV by slow cooling at high pressure.
Ni
D at high 
conditionsShito, Chikara*; Kagi, Hiroyuki*; Kakizawa, Sho*; Aoki, Katsutoshi*; Komatsu, Kazuki*; Iizuka, Riko*; Abe, Jun*; Saito, Hiroyuki*; Sano, Asami; Hattori, Takanori
American Mineralogist, 108(4), p.659 - 666, 2023/04
Times Cited Count：6 Percentile：50.61(Geochemistry & Geophysics)The phase relation and crystal structure of FeNiH (D) at high pressures and temperatures up to 12 GPa and 1000 K were clarified by in-situ X-ray and neutron diffraction measurements. Under conditions of the present study, no deuterium atoms occupied tetragonal (
) sites of face-centered cubic (fcc) FeNiD unlike fcc FeH(D). The deuterium-induced volume expansion per deuterium 
was determined as 2.45(4) 
and 3.31(6) for fcc and hcp phases, respectively, which were significantly larger than the corresponding values for FeD. The value slightly increased with increasing temperature. This study suggests that only 10% of nickel in iron drastically changes the behaviors of hydrogen in metal. Assuming that is constant regardless of pressure, the maximum hydrogen content in the Earth's inner core is estimated to be one to two times the amount of hydrogen in the oceans.
-type La
Eu
CuO
and NdCuOAsano, Shun*; Ishii, Kenji*; Matsumura, Daiju; Tsuji, Takuya; Kudo, Kota*; Taniguchi, Takanori*; Saito, Shin*; Sunohara, Toshiki*; Kawamata, Takayuki*; Koike, Yoji*; et al.
Physical Review B, 104(21), p.214504_1 - 214504_7, 2021/12
Times Cited Count：2 Percentile：8.39(Materials Science, Multidisciplinary)Iizuka, Riko*; Goto, Hirotada*; Shito, Chikara*; Fukuyama, Ko*; Mori, Yuichiro*; Hattori, Takanori; Sano, Asami; Funakoshi, Kenichi*; Kagi, Hiroyuki*
Scientific Reports (Internet), 11(1), p.12632_1 - 12632_10, 2021/06
Times Cited Count：7 Percentile：33.19(Multidisciplinary Sciences)The Earth's core consist of Fe-Ni alloy with some light elements (H, C, O, Si, S etc.). Hydrogen (H) is the most abundant element in the universe and one of the promising candidates. In this study, we have investigated the effects of sulfur(S) on hydrogenation of iron-hydrous silicate system containing saturated water in the ideal composition of the primitive Earth. We observed a series of phase transitions of Fe, dehydration of the hydrous mineral, and formation of olivine and enstatite with increasing temperature. The FeS formed as the coexisting phase of Fe under high-pressure and temperature condition, but its unit cell volume did not increase, suggesting that FeS is hardly hydrogenated. Recovered samples exhibited that H and S can be incorporated into solid Fe, which lowers the melting temperature as Fe(H
)-FeS system. No detection of other light elements (C, O, Si) in solid Fe suggests that they dissolve into molten iron hydride and/or FeS in the later process of Earth's core-mantle differentiation.
Sano, Asami; Kakizawa, Sho*; Shito, Chikara*; Hattori, Takanori; Machida, Shinichi*; Abe, Jun*; Funakoshi, Kenichi*; Kagi, Hiroyuki*
High Pressure Research, 41(1), p.65 - 74, 2021/03
Times Cited Count：4 Percentile：34.03(Physics, Multidisciplinary)We applied Kawai-type multi-anvil assemblies (MA6-8) for time-of-flight neutron-diffraction experiments to achieve high pressures and high temperatures simultaneously. To achieve sufficient signal intensities, the angular access to the sample was enlarged using slits and tapers on the first-stage anvils. Using SiC-binder sintered diamond for the second-stage anvils that transmits neutrons, sufficient signal intensities were achieved at a high-pressure of 23.1 GPa. A high-temperature experiment was also conducted at 16.2 GPa and 973 K, validating the use of tungsten carbide for the second-stage anvils. The present study reveals the capability of the MA6-8 cells in neutron-diffraction experiments to attain pressures and temperatures beyond the limits of the conventional MA6-6 cells used in the high-pressure neutron diffractometer PLANET at the MLF, J-PARC.
Shibata, Takanori*; Sugimura, Takashi*; Ikegami, Kiyoshi*; Takagi, Akira*; Sato, Masaharu*; Naito, Fujio*; Okoshi, Kiyonori; Hasegawa, Kazuo
JPS Conference Proceedings (Internet), 33, p.011009_1 - 011009_6, 2021/03
Upgrade of beam current in the Linac of Ibaraki Boron Neutron Capture Therapy (iBNCT) is one of the most important requirements to realize clinical trial. By 2018, the measurement of the produced neutrons characteristics and the neutron irradiation experiment for living cells have been done by producing 8-MeV proton beam current at the beryllium target with average current up to 2 mA. In order to satisfy the original clinical trial conditions, 5 mA average beam current is required at the target. For this goal, peak beam current extracted from the ion source should be increased to 60 mA from the present 30 mA with duty factor up to more than 10% (pulse width up to 1 ms and repetition rate up to more than 100 Hz). Stability of the peak current in the macro pulse is also important for the clinical application.
beam with orifice in J-PARC front-endShibata, Takanori*; Ikegami, Kiyoshi*; Nammo, Kesao*; Liu, Y.*; Otani, Masashi*; Naito, Fujio*; Shinto, Katsuhiro; Okoshi, Kiyonori; Okabe, Kota; Kondo, Yasuhiro; et al.
JPS Conference Proceedings (Internet), 33, p.011010_1 - 011010_6, 2021/03
Together with the intensity upgrade in J-PARC Linac Front-End, improvement of RFQ transmission ratio is an important task. This RFQ transmission ratio depends strongly upon the solenoid current settings in the low energy beam transport line (LEBT). In the present study, high beam current cases (72 mA and 88 mA H beam current in LEBT) are investigated at a test-stand. Phase space distributions of the H beam particles at the RFQ entrance are measured and compared with numerical results by Particle-In-Cell simulation. As a result, it has been clarified that a 15 mm 
orifice for differential pumping of H gas coming from the ion source plays a role as a collimator in these beam conditions. This leads to change the beam emittance and Twiss parameters at the RFQ entrance. Especially in the condition with the beam current up to 88 mA in LEBT, the beam collimation contributes to optimize the phase space distribution to the RFQ acceptance with relatively low solenoid current settings. As a higher solenoid current setting would be necessary to suppress the beam expansion due to high space charge effect, these results suggest that current-saving of the solenoids can be possible even in the higher beam intensity operations.
