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Journal Articles

High-sensitive XANES analysis at Ce L$$_{2}$$-edge for Ce in bauxites using transition-edge sensors; Implications for Ti-rich geological samples

Li, W.*; Yamada, Shinya*; Hashimoto, Tadashi; Okumura, Takuma*; Hayakawa, Ryota*; Nitta, Kiyofumi*; Sekizawa, Oki*; Suga, Hiroki*; Uruga, Tomoya*; Ichinohe, Yuto*; et al.

Analytica Chimica Acta, 1240, p.340755_1 - 340755_9, 2023/02

no abstracts in English

Journal Articles

Reducing the effect of noise generated from stepper motor for H0 collimator in J-PARC RCS

Fujiyama, Hiroki*; Takahashi, Hiroki; Okabe, Kota; Ito, Yuichi*; Hatakeyama, Shuichiro; Suzuki, Takahiro*; Otsu, Satoru*; Yamakawa, Ryuto*

Proceedings of 19th Annual Meeting of Particle Accelerator Society of Japan (Internet), p.529 - 531, 2023/01

Stepper motors are used for mechanical drive in collimators and wire scanner monitors of J-PARC accelerators. Many of these drive unit hardware have been used since the beginning of J-PARC construction, and it is necessary to take measures against aging deterioration. Therefore, we started updating the motor and control system from around 2017. However, when the stepper motor was updated to the current product in the RCS H0 collimator, a malfunction occurred. This is because the drive unit control system cannot correctly recognize the state of the LS (limit switch) due to the noise generated by the motor driver, which hinders the operation. When the noise generated from the old and new stepper motors was measured in a simple test environment for confirmation, it was found that the current product was clearly larger. As a countermeasure, when the wiring of the stepper motor, which was bundled in a single multi-core cable, was separated into separate cables for the power system and LS signal system, the noise level was reduced to about 1/10 and normal operation was restored. I was able to. In this case, we report on noise countermeasures for the RCS H0 collimator drive unit.

Journal Articles

New $$K$$ isomers in $$^{248}$$Cf

Orlandi, R.; Makii, Hiroyuki; Nishio, Katsuhisa; Hirose, Kentaro; Asai, Masato; Tsukada, Kazuaki; Sato, Tetsuya; Ito, Yuta; Suzaki, Fumi; Nagame, Yuichiro*; et al.

Physical Review C, 106(6), p.064301_1 - 064301_11, 2022/12

 Times Cited Count:0 Percentile:0.02(Physics, Nuclear)

Journal Articles

Structure and magnetic properties of Fe nanoparticles in amorphous silica implanted with Fe ions and effect of subsequent energetic heavy ion irradiation

Iwase, Akihiro*; Fukuda, Kengo*; Saito, Yuichi*; Okamoto, Yoshihiro; Semboshi, Satoshi*; Amekura, Hiroshi*; Matsui, Toshiyuki*

Journal of Applied Physics, 132(16), p.163902_1 - 163902_10, 2022/10

Amorphous SiO$$_{2}$$ samples were implanted with 380 keV Fe ions at room temperature. After implantation, some of the samples were irradiated with 16 MeV Au ions. magnetic properties were investigated using a SQUID magnetometer, and the morphology of the Fe-implanted SiO$$_{2}$$ samples was examined using transmission electron microscopy and X-ray absorption spectroscopy (EXAFS and XANES), which showed that the size of Fe nanoparticles was increasing The size of Fe nanoparticles increased with increasing Fe implantation amount; some of the Fe nanoparticles consisted of Fe oxides, and the valence and structure of Fe atoms became closer to that of metallic $$alpha$$-Fe with increasing Fe injection amount. The magnetization-field curve of the sample implanted with a small amount of Fe was reproduced by Langevin's equation, suggesting that the Fe nanoparticles behave in a superparamagnetic manner. In addition, when a large amount of Fe was implanted, the magnetization-magnetic field curve shows a ferromagnetic state. These magnetic property results are consistent with the X-ray absorption results. Subsequent 16 MeV Au irradiation crushed the Fe nanoparticles, resulting in a decrease in magnetization.

Journal Articles

Design and actual performance of J-PARC 3 GeV rapid cycling synchrotron for high-intensity operation

Yamamoto, Kazami; Kinsho, Michikazu; Hayashi, Naoki; Saha, P. K.; Tamura, Fumihiko; Yamamoto, Masanobu; Tani, Norio; Takayanagi, Tomohiro; Kamiya, Junichiro; Shobuda, Yoshihiro; et al.

Journal of Nuclear Science and Technology, 59(9), p.1174 - 1205, 2022/09

 Times Cited Count:1 Percentile:71.47(Nuclear Science & Technology)

In the Japan Proton Accelerator Research Complex, the purpose of the 3 GeV rapid cycling synchrotron (RCS) is to accelerate a 1 MW, high-intensity proton beam. To achieve beam operation at a repetition rate of 25 Hz at high intensities, the RCS was elaborately designed. After starting the RCS operation, we carefully verified the validity of its design and made certain improvements to establish a reliable operation at higher power as possible. Consequently, we demonstrated beam operation at a high power, namely, 1 MW. We then summarized the design, actual performance, and improvements of the RCS to achieve a 1 MW beam.

Journal Articles

Status of decommissioning for prototype ATR Fugen and FBR Monju

Ito, Kenji; Kondo, Tetsuo; Nakamura, Yasuyuki; Matsuno, Hiroki; Nagaoki, Yoshihiro; Sakuma, Yuichi

Dekomisshoningu Giho, (63), p.1 - 26, 2022/05

The prototype advanced thermal reactor Fugen entered into the decommissioning phases with the approval of the decommissioning plan in February 2008. The prototype fast breeder reactor Monju entered into the decommissioning stage with the approval of the decommissioning plan in March 2018. In April 2018, the head office of Tsuruga decommissioning demonstration was newly established to oversee the decommissioning operations in Tsuruga area, and decommissioning projects for two unique reactors have progressed safely and steadily.

Journal Articles

A Storm-induced flood and associated nearshore dispersal of the river-derived suspended $$^{137}$$Cs

Uchiyama, Yusuke*; Tokunaga, Natsuki*; Azuma, Kohei*; Kamidaira, Yuki; Tsumune, Daisuke*; Iwasaki, Toshiki*; Yamada, Masatoshi*; Tateda, Yutaka*; Ishimaru, Takashi*; Ito, Yukari*; et al.

Science of the Total Environment, 816, p.151573_1 - 151573_13, 2022/04

 Times Cited Count:3 Percentile:85.21(Environmental Sciences)

no abstracts in English

Journal Articles

Magnetic Bragg peak enhancement under ultrasound injection

Shamoto, Shinichi*; Akatsu, Mitsuhiro*; Matsuura, Masato*; Kawamura, Seiko; Harii, Kazuya*; Ono, Masao*; Chang, L.-J.*; Ito, Takashi; Nemoto, Yuichi*; Ieda, Junichi

Physical Review Research (Internet), 4(1), p.013245_1 - 013245_7, 2022/03

Ultrasound injection effect on a magnetic Bragg peak of yttrium iron garnet has been studied by quasielastic neutron scattering. The magnetic Bragg peak is vastly enhanced with decreasing temperature. The energy width increases proportionally to the square root of the sample temperature increase induced by the ultrasound injection. Because the magnetic Bragg peak is enhanced by the lattice vibration, the enhancement is expected to relate to the spin-lattice coupling closely. An observed sharp drop above 100 K in the longitudinal mode suggests the degradation of the spin-lattice coupling. It is consistent with the decline of spin Seebeck effect with increasing temperature above 100 K, proving the degradation mechanism by the spin-lattice coupling.

Journal Articles

${it In situ}$ spectrometry of terrestrial gamma rays using portable germanium detectors in area of 80 km radius around the Fukushima Daiichi Nuclear Power Plant

Mikami, Satoshi; Tanaka, Hiroyuki*; Okuda, Naotoshi*; Sakamoto, Ryuichi*; Ochi, Kotaro; Uno, Kiichiro*; Matsuda, Norihiro; Saito, Kimiaki

Nihon Genshiryoku Gakkai Wabun Rombunshi, 20(4), p.159 - 178, 2021/12

In order to know the background radiation level where the area affected by the Fukushima Daiichi Nuclear Power Plant accident in 2011, terrestrial gamma rays had been measured by using portable germanium detectors repeatedly from 2013 through 2019, at 370 locations within 80 km radius area centered on the Fukushima Daiichi Nuclear Power Plant. Radioactive concentrations of Uranium 238, Thorium 232, Potassium 40 and kerma rates in air due to terrestrial gamma rays were obtained at those locations based on the method of ICRU report 53. Averaged concentrations of $$^{238}$$U, $$^{232}$$Th and $$^{40}$$K were 18.8, 22.7, 428 Bq/kg, respectively, and kerma rate in air over the area was found to be 0.0402 $$mu$$Gy/h. The obtained kerma rates in air were compared to those reported in literatures. It was confirmed that the data were correlated with each other, and were agreed within the range of their uncertainty. This is because the kerma rate in air due to terrestrial gamma rays is depend on geology. The similar trend to previous findings was observed that the kerma rate in air at locations geologically classified as Mesozoic era, Granite and Rhyolite were statistically significantly higher than the others.

Journal Articles

Chiral-spin rotation of non-collinear antiferromagnet by spin-orbit torque

Takeuchi, Yutaro*; Yamane, Yuta*; Yoon, J.-Y.*; Ito, Ryuichi*; Jinnai, Butsurin*; Kanai, Shun*; Ieda, Junichi; Fukami, Shunsuke*; Ohno, Hideo*

Nature Materials, 20(10), p.1364 - 1370, 2021/10

 Times Cited Count:44 Percentile:98.8(Chemistry, Physical)

Journal Articles

Update of MPS modules for J-PARC linac and RCS, 2

Takahashi, Hiroki; Suzuki, Takahiro*; Ishiyama, Tatsuya*; Ito, Yuichi*

Proceedings of 18th Annual Meeting of Particle Accelerator Society of Japan (Internet), p.914 - 917, 2021/10

In the event of an abnormal situation, a machine protection system (MPS) that immediately inhibits the beam is indispensable to minimize the damage and the radioactivation by beam loss. The existing MPS was developed during the construction period, and there are many MPS modules that have been used from the beginning of J-PARC operation, Therefore, as a measure against aging, we started designing, manufacturing and updating the new MPS module in 2018. In this paper, the specifications and the results of performance test about the newly designed and manufactured the MPS signal aggregation module and the E/O converter module will be described.

Journal Articles

Chemical characterization of a volatile dubnium compound, DbOCl$$_3$$

Chiera, N. M.*; Sato, Tetsuya; Eichler, R.*; Tomitsuka, Tomohiro; Asai, Masato; Adachi, Sadia*; Dressler, R.*; Hirose, Kentaro; Inoue, Hiroki*; Ito, Yuta; et al.

Angewandte Chemie; International Edition, 60(33), p.17871 - 17874, 2021/08

 Times Cited Count:2 Percentile:30.08(Chemistry, Multidisciplinary)

The formation and the chemical characterization of single atoms of dubnium (Db, element 105), in the form of its volatile oxychloride, was investigated using the on-line gas phase chromatography technique, in the temperature range 350 - 600 $$^circ$$C. Under the exact same chemical conditions, comparative studies with the lighter homologs of group-5 in the Periodic Table clearly indicate the volatility sequence being NbOCl$$_3 > $$ TaOCl$$_3 geq$$ DbOCl$$_3$$. From the obtained experimental results, thermochemical data for DbOCl$$_3$$ were derived. The present study delivers reliable experimental information for theoretical calculations on the chemical properties of transactinides.

Journal Articles

Development of next-generation timing system for the Japan Proton Accelerator Research Complex

Tamura, Fumihiko; Takahashi, Hiroki; Kamikubota, Norihiko*; Ito, Yuichi*; Hayashi, Naoki

IEEE Transactions on Nuclear Science, 68(8), p.2043 - 2050, 2021/08

 Times Cited Count:0 Percentile:0.01(Engineering, Electrical & Electronic)

A precise and stable timing system is necessary for high intensity proton accelerators such as the J-PARC. The existing timing system, which was developed during the construction period of the-PARC, has been working without major issues since 2006. After a decade of operation, the optical modules, which are key components for signal transfer, were discontinued already. Thus, the next-generation timing system for the J-PARC is under development. The new system is designed to be compatible with the existing system in terms of the operating principle. The new system utilizes modern high speed signal communication for the transfer of the clock, trigger, and type code. We present the system configuration of the next-generation timing system and current status.

Journal Articles

Correction to Transport and redistribution of radiocesium in Fukushima fallout through rivers

Taniguchi, Keisuke*; Onda, Yuichi*; Smith, H. G.*; Blake, W.*; Yoshimura, Kazuya; Yamashiki, Yosuke*; Kuramoto, Takayuki*; Saito, Kimiaki

Environmental Science & Technology, 55(13), P. 9394, 2021/07

 Times Cited Count:0 Percentile:0.24(Engineering, Environmental)

no abstracts in English

Journal Articles

Observation of longitudinal magnetic fluctuations at a first-order ferromagnetic quantum phase transition in UGe$$_2$$

Noma, Yuichiro*; Kotegawa, Hisashi*; Kubo, Tetsuro*; To, Hideki*; Harima, Hisatomo*; Haga, Yoshinori; Yamamoto, Etsuji; Onuki, Yoshichika*; Ito, Kohei*; Nakamura, Ai*; et al.

Journal of the Physical Society of Japan, 90(7), p.073707_1 - 073707_5, 2021/07

 Times Cited Count:0 Percentile:0(Physics, Multidisciplinary)

Journal Articles

Behavior of light elements in iron-silicate-water-sulfur system during early Earth's evolution

Iizuka, Riko*; Goto, Hirotada*; Shito, Chikara*; Fukuyama, Ko*; Mori, Yuichiro*; Hattori, Takanori; Sano, Asami; Funakoshi, Kenichi*; Kagi, Hiroyuki*

Scientific Reports (Internet), 11(1), p.12632_1 - 12632_10, 2021/06

 Times Cited Count:2 Percentile:41.71(Multidisciplinary Sciences)

The Earth's core consist of Fe-Ni alloy with some light elements (H, C, O, Si, S etc.). Hydrogen (H) is the most abundant element in the universe and one of the promising candidates. In this study, we have investigated the effects of sulfur(S) on hydrogenation of iron-hydrous silicate system containing saturated water in the ideal composition of the primitive Earth. We observed a series of phase transitions of Fe, dehydration of the hydrous mineral, and formation of olivine and enstatite with increasing temperature. The FeS formed as the coexisting phase of Fe under high-pressure and temperature condition, but its unit cell volume did not increase, suggesting that FeS is hardly hydrogenated. Recovered samples exhibited that H and S can be incorporated into solid Fe, which lowers the melting temperature as Fe(H$$_{x}$$)-FeS system. No detection of other light elements (C, O, Si) in solid Fe suggests that they dissolve into molten iron hydride and/or FeS in the later process of Earth's core-mantle differentiation.

Journal Articles

First isolation and analysis of caesium-bearing microparticles from marine samples in the Pacific coastal area near Fukushima Prefecture

Miura, Hikaru*; Ishimaru, Takashi*; Ito, Yukari*; Kuribara, Yuichi; Otosaka, Shigeyoshi*; Sakaguchi, Aya*; Misumi, Kazuhiro*; Tsumune, Daisuke*; Kubo, Atsushi*; Higaki, Shogo*; et al.

Scientific Reports (Internet), 11, p.5664_1 - 5664_11, 2021/03

 Times Cited Count:7 Percentile:70.79(Multidisciplinary Sciences)

For the first time, we isolated and investigated seven CsMPs (radioactive caesium-bearing microparticles) from marine particulate matter and sediment. From the elemental composition, the $$^{134}$$Cs/$$^{137}$$Cs activity ratio, and the $$^{137}$$Cs activity per unit volume results, we inferred that the five CsMPs collected from particulate matter were emitted from Unit 2 of the FDNPP, whereas the two CsMPs collected from marine sediment were possibly emitted from Unit 3. The presence of CsMPs can cause overestimation of the solid-water distribution coefficient of Cs in marine sediments and particulate matter and a high apparent radiocaesium concentration factor for marine biota. CsMPs emitted from Unit 2, which were collected from the estuary of a river that flowed through a highly contaminated area, may have been deposited on land and then transported by the river. By contrast, CsMPs emitted from Unit 3 were possibly transported eastward by the wind and deposited directly onto the ocean surface.

Journal Articles

Ion tracks in silicon formed by much lower energy deposition than the track formation threshold

Amekura, Hiroshi*; Toulemonde, M.*; Narumi, Kazumasa*; Li, R.*; Chiba, Atsuya*; Hirano, Yoshimi*; Yamada, Keisuke*; Yamamoto, Shunya*; Ishikawa, Norito; Okubo, Nariaki; et al.

Scientific Reports (Internet), 11(1), p.185_1 - 185_11, 2021/01

 Times Cited Count:7 Percentile:77.36(Multidisciplinary Sciences)

We report the track formation of 10 nm in diameter in silicon irradiated with 6 MeV C$$_{60}$$, i.e., much lower energy than the previously reported energy threshold.

Journal Articles

Neutron diffraction study of hydrogen site occupancy in Fe$$_{0.95}$$Si$$_{0.05}$$ at 14.7 GPa and 800 K

Mori, Yuichiro*; Kagi, Hiroyuki*; Kakizawa, Sho*; Komatsu, Kazuki*; Shito, Chikara*; Iizuka, Riko*; Aoki, Katsutoshi*; Hattori, Takanori; Sano, Asami; Funakoshi, Kenichi*; et al.

Journal of Mineralogical and Petrological Sciences, 116(6), p.309 - 313, 2021/00

 Times Cited Count:0 Percentile:0.02(Mineralogy)

The Earth's core is believed to contain some light elements because it is 10% less dense than pure Fe under the corresponding pressure and temperature conditions. Hydrogen, a promising candidate among light elements, has phase relations and physical properties that have been investigated mainly for the Fe-H system. This study specifically examined an Fe-Si-H system using in-situ neutron diffraction experiments to investigate the site occupancy of deuterium of hcp-Fez$$_{0.95}$$Si$$_{0.05}$$ hydride at 14.7 GPa and 800 K. Results of Rietveld refinement indicate hcp-Fe$$_{0.95}$$Si$$_{0.05}$$ hydride as having deuterium (D) occupancy of 0.24(2) exclusively at the interstitial octahedral site in the hcp lattice. The effect on the site occupancy of D by addition of 2.6 wt% Si into Fe (Fe$$_{0.95}$$Si$$_{0.05}$$) was negligible compared to results obtained from an earlier study of an Fe-D system (Machida et al., 2019).

Journal Articles

Experimental validation of tensile properties measured with thick samples taken from MEGAPIE target

Saito, Shigeru; Suzuki, Kazuhiro; Hatakeyama, Yuichi; Suzuki, Miho; Dai, Y.*

Journal of Nuclear Materials, 534, p.152146_1 - 152146_16, 2020/06

 Times Cited Count:1 Percentile:17.77(Materials Science, Multidisciplinary)

A post-irradiation examination (PIE) was performed on the tensile specimens prepared from the MEGAPIE (MEGAwatt Pilot Experiment) target which were irradiated in flowing lead-bismuth eutectic (LBE). Thicknesses of the specimens were over two times larger than that of the standard specimen. The PIE revealed that the T91 specimens showed a 1.5-2.0 times larger total elongation (TE) compared to the literature values for a specimen with standard t/w (ratio of thickness to width). It could be suggested that the t/w and TE were strongly correlated. Then, we tried to investigate the effects of the t/w on the TE by comparing unirradiated specimens. We found that there was no t/w dependence on the strength and uniform elongation. On the other hand, the TE increases with increasing t/w. Based on the experimental data, we correlated the TE with various specimens t/w to estimate appropriate TE values, including that for the standard specimen.

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