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Journal Articles

Predictive modeling of a simple field matrix diffusion experiment addressing radionuclide transport in fractured rock. Is it so straightforward?

Soler, J. M.*; Neretnieks, I.*; Moreno, L.*; Liu, L.*; Meng, S.*; Svensson, U.*; Iraola, A.*; Ebrahimi, K.*; Trinchero, P.*; Molinero, J.*; et al.

Nuclear Technology, 208(6), p.1059 - 1073, 2022/06

 Times Cited Count:0 Percentile:0.01(Nuclear Science & Technology)

The SKB Task Force is an international forum on modelling of groundwater flow and solute transport in fractured rock. The WPDE experiments are matrix diffusion experiments in gneiss performed at the ONKALO underground facility in Finland. Synthetic groundwater containing several conservative and sorbing tracers was injected along a borehole interval. The objective of Task 9A was the predictive modelling of the tracer breakthrough curves from the WPDE experiments. Several teams, using different modelling approaches and codes, participated in this exercise. An important conclusion from this exercise is that the modelling results were very sensitive to the magnitude of dispersion in the borehole opening, which is related to the flow of water. Focusing on the tails of the breakthrough curves, which are more directly related to matrix diffusion and sorption, the results from the different teams were more comparable.

Journal Articles

Achieving excellent mechanical properties in type 316 stainless steel by tailoring grain size in homogeneously recovered or recrystallized nanostructures

Liu, M.*; Gong, W.; Zheng, R.*; Li, J.*; Zhang, Z.*; Gao, S.*; Ma, C.*; Tsuji, Nobuhiro*

Acta Materialia, 226, p.117629_1 - 117629_13, 2022/03

 Times Cited Count:1 Percentile:0.01(Materials Science, Multidisciplinary)

Journal Articles

Effect of hydrogen on evolution of deformation microstructure in low-carbon steel with ferrite microstructure

Okada, Kazuho*; Shibata, Akinobu*; Gong, W.; Tsuji, Nobuhiro*

Acta Materialia, 225, p.117549_1 - 117549_13, 2022/02

 Times Cited Count:1 Percentile:81.79(Materials Science, Multidisciplinary)

Journal Articles

Evaluation report of Task 9C based on comparisons and analyses of modelling results for the ONKALO REPRO-TDE experiment

Soler, J. M.*; Kek$"a$l$"a$inen, P.*; Pulkkanen, V.-M.*; Moreno, L.*; Iraola, A.*; Trinchero, P.*; Hokr, M.*; $v{R}$$'i$ha, J.*; Havlov$'a$, V.*; Trpko$v{s}$ov$'a$, D.*; et al.

SKB TR-21-09, 204 Pages, 2021/11

Journal Articles

Half-integer Shapiro steps in strong ferromagnetic Josephson junctions

Yao, Y.*; Cai, R.*; Yang, S.-H.*; Xing, W.*; Ma, Y.*; Mori, Michiyasu; Ji, Y.*; Maekawa, Sadamichi; Xie, X.-C.*; Han, W.*

Physical Review B, 104(10), p.104414_1 - 104414_6, 2021/09

 Times Cited Count:0 Percentile:0(Materials Science, Multidisciplinary)

Journal Articles

Evaluation report of Task 9B based on comparisons and analyses of modelling results for the $"A$sp$"o$ HRL LTDE-SD experiments

Soler, J. M.*; Meng, S.*; Moreno, L.*; Neretnieks, I.*; Liu, L.*; Kek$"a$l$"a$inen, P.*; Hokr, M.*; $v{R}$$'i$ha, J.*; Vete$v{s}$n$'i$k, A.*; Reimitz, D.*; et al.

SKB TR-20-17, 71 Pages, 2021/07

Task 9B of the SKB Task Force on Modelling of Groundwater Flow and Transport of Solutes in fractured rock focused on the modelling of experimental results from the LTDE-SD in situ tracer test performed at the $"A$sp$"o$ Hard Rock Laboratory in Sweden. Ten different modelling teams provided results for this exercise, using different concepts and codes. Three main types of modelling approaches were used: (1) analytical solutions to the transport-retention equations, (2) continuum-porous-medium numerical models, and (3) microstructure-based models accounting for small-scale heterogeneity (i.e. mineral grains and microfracture distributions). The modelling by the different teams allowed the comparison of many different model concepts, especially in terms of potential zonations of rock properties (porosity, diffusion, sorption), such as the presence of a disturbed zone at the rock and fracture surface, the potential effects of micro- and cm-scale fractures.

Journal Articles

Coordination number regulation of molybdenum single-atom nanozyme peroxidase-like specificity

Wang, Y.*; Jia, G.*; Cui, X.*; Zhao, X.*; Zhang, Q.*; Gu, L.*; Zheng, L.*; Li, L. H.*; Wu, Q.*; Singh, D. J.*; et al.

Chem, 7(2), p.436 - 449, 2021/02

 Times Cited Count:58 Percentile:99.74(Chemistry, Multidisciplinary)

Journal Articles

Study of quasielastic barrier distributions as a step towards the synthesis of superheavy elements with hot fusion reactions

Tanaka, Taiki*; Morita, Kosuke*; Morimoto, Koji*; Kaji, Daiya*; Haba, Hiromitsu*; Boll, R. A.*; Brewer, N. T.*; Van Cleve, S.*; Dean, D. J.*; Ishizawa, Satoshi*; et al.

Physical Review Letters, 124(5), p.052502_1 - 052502_6, 2020/02

 Times Cited Count:6 Percentile:62.45(Physics, Multidisciplinary)

Journal Articles

Organ and detriment-weighted dose rate coefficients for exposure to radionuclide-contaminated soil considering body morphometries that differ from reference conditions; Adults and children

Kofler, C.*; Domal, S.*; Satoh, Daiki; Dewji, S.*; Eckerman, K.*; Bolch, W. E.*

Radiation and Environmental Biophysics, 58(4), p.477 - 492, 2019/11

 Times Cited Count:4 Percentile:41.11(Biology)

In the current radiation protection system, the International Commission on Radiological Protection (ICRP) recommends to use the effective dose for dose estimation. The effective dose is derived from the organ doses calculated using the computational human models (phantoms) defined by the ICRP to represent the reference person at each age. Questions arise, however, among the general public regarding the accuracy of organ and effective dose estimates based upon reference phantom methodologies, especially for those individuals with heights and/or weights that differ from the nearest age-matched reference person. In this paper, the detriment-weighted dose was defined for non-reference persons as the same manner to the effective dose for reference person. The doses were calculated for external exposure to radionuclides in a soil using 351-member phantom library based on the data of the U.S. population reported by the U.S. National Center for Health Statistics. The results for 33 nuclides were listed in the paper. Especially, for the environmental relevant radionuclides of $$^{89}$$Sr, $$^{90}$$Sr, $$^{137}$$Cs, and $$^{131}$$I, the detriment-weighted dose of 1-year-old phantom agreed with the effective dose within 5%, while the range of percent differences in these two quantities increased with increases the body size and age, e.g. +15% to -40% for adults.

Journal Articles

Nature of dynamic ferrite transformation revealed by ${it in-situ}$ neutron diffraction analysis during thermomechanical processing

Shibata, Akinobu*; Takeda, Yasunari*; Park, N.*; Zhao, L.*; Harjo, S.; Kawasaki, Takuro; Gong, W.*; Tsuji, Nobuhiro*

Scripta Materialia, 165, p.44 - 49, 2019/05

 Times Cited Count:17 Percentile:83.71(Nanoscience & Nanotechnology)

Journal Articles

In situ neutron diffraction study on microstructure evolution during thermo-mechanical processing of medium manganese steel

Nakamura, Yoshihiko*; Shibata, Akinobu*; Gong, W.*; Harjo, S.; Kawasaki, Takuro; Ito, Atsushi*; Tsuji, Nobuhiro*

Proceedings of International Conference on Martensitic Transformations: Chicago, p.155 - 158, 2018/04

Journal Articles

$$beta$$-delayed fission of $$^{230}$$Am

Wilson, G. L.*; Takeyama, Mirei*; Andreyev, A. N.; Andel, B.*; Antalic, S.*; Catford, W. N.*; Ghys, L.*; Haba, Hiromitsu*; He${ss}$berger, F. P.*; Huang, M.*; et al.

Physical Review C, 96(4), p.044315_1 - 044315_7, 2017/10

 Times Cited Count:5 Percentile:47.75(Physics, Nuclear)

Journal Articles

Complex chemistry with complex compounds

Eichler, R.*; Asai, Masato; Brand, H.*; Chiera, N. M.*; Di Nitto, A.*; Dressler, R.*; D$"u$llmann, Ch. E.*; Even, J.*; Fangli, F.*; Goetz, M.*; et al.

EPJ Web of Conferences, 131, p.07005_1 - 07005_7, 2016/12

 Times Cited Count:2 Percentile:65

In recent years gas-phase chemical studies assisted by physical pre-separation allowed for the productions and investigations of fragile single molecular species of superheavy elements. The latest highlight is the formation of very volatile hexacarbonyl compound of element 106, Sg(CO)$$_{6}$$. Following this success, second-generation experiments were performed to measure the first bond dissociation energy between the central metal atom and the surrounding ligand. The method using a tubular decomposition reactor was developed and successfully applied to short-lived Mo(CO)$$_{6}$$, W(CO)$$_{6}$$, and Sg(CO)$$_{6}$$.

Journal Articles

Study on spray cooling capability for spent fuel pool at coolant loss accident, 1; Research plan

Liu, W.; Nagatake, Taku; Shibata, Mitsuhiko; Koizumi, Yasuo; Yoshida, Hiroyuki; Nemoto, Yoshiyuki; Kaji, Yoshiyuki

Proceedings of 10th Japan-Korea Symposium on Nuclear Thermal Hydraulics and Safety (NTHAS-10) (USB Flash Drive), 4 Pages, 2016/11

The Fukushima Daiichi NPP accident asks that the accident management of the LOCA in the SFPs must be considered to avoid occurrences of severe accident in the SFPs. To prevent the failure of the spent fuel assemblies at the LOCA, transportable spray systems are expected to be put into use to discharge water into fuel assemblies to moderate the temperature increase. To apply the spray system as a countermeasure for the LOCA of the SFP, the capability of the spray cooling system must be evaluated to keep the spent fuel rods safety. JAEA has started the research project to investigate the spray cooling capability for the SFP. In this research project, we aim to construct a numerical simulation method for evaluating the capability of the spray cooling. To develop the method, the basic key phenomena that affect the cooling performance must be clarified and the validation data required for the code development. To clarify the basic key phenomena that affect the cooling performance, that is, the CCFL and the drop size effect on the CCFL, and to obtain the code validation data, we are planning to carry out 2 experiments with two test sections, the spray visualization experiment and the spray cooling experiment. The spray visualization test section aims to get CCFL data in air-water two-phase flow and to understand the two-phase flow behavior over the upper tie plate. The spray cooling test section aims to get the CCFL data in steam-water two-phase flow and to obtain the validation data. This paper focus on the outline of the research plan for the whole research project.

Journal Articles

Visualization study on two-phase flow behavior at spray cooling for spent fuel pool

Nagatake, Taku; Liu, W.; Uesawa, Shinichiro; Koizumi, Yasuo; Shibata, Mitsuhiko; Yoshida, Hiroyuki; Nemoto, Yoshiyuki; Kaji, Yoshiyuki

Konsoryu Shimpojiumu 2016 Koen Rombunshu (USB Flash Drive), 2 Pages, 2016/08

no abstracts in English

Journal Articles

Decomposition studies of group 6 hexacarbonyl complexes, 1; Production and decomposition of Mo(CO)$$_6$$ and W(CO)$$_6$$

Usoltsev, I.*; Eichler, R.*; Wang, Y.*; Even, J.*; Yakushev, A.*; Haba, Hiromitsu*; Asai, Masato; Brand, H.*; Di Nitto, A.*; D$"u$llmann, Ch. E.*; et al.

Radiochimica Acta, 104(3), p.141 - 151, 2016/03

 Times Cited Count:28 Percentile:96.25(Chemistry, Inorganic & Nuclear)

Conditions of the production and decomposition of hexacarbonyl complexes of short-lived Mo and W isotopes were investigated to study thermal stability of the heaviest group 6 hexacarbonyl complex Sg(CO)$$_6$$. A tubular flow reactor was tested to decompose the hexacarbonyl complexes and to extract the first bond dissociation energies. A silver was found to be the most appropriate reaction surface to study the decomposition of the group 6 hexacarbonyl. It was found that the surface temperature at which the decomposition occurred was correlated to the first bond dissociation energy of Mo(CO)$$_6$$ and W(CO)$$_6$$, indicating that the first bond dissociation energy of Sg(CO)$$_6$$ could be determined with this technique.

Journal Articles

Carrier-mediated ferromagnetism in the magnetic topological insulator Cr-doped (Sb,Bi)$$_{2}$$Te$$_{3}$$

Ye, M.*; Li, W.*; Zhu, S.-Y.*; Takeda, Yukiharu; Saito, Yuji; Wang, J.*; Pan, H.*; Nurmamat, M.*; Sumida, Kazuki*; Ji, F.*; et al.

Nature Communications (Internet), 6, p.8913_1 - 8913_7, 2015/11

AA2015-0647.pdf:0.64MB

 Times Cited Count:46 Percentile:90.21(Multidisciplinary Sciences)

Magnetically doped topological insulators are predicted to exhibit exotic phenomena including the quantized anomalous Hall effect and a dissipationless transport, which facilitate the development of low-power-consumption devices using electron spins. The realization of the quantized anomalous Hall effect is so far restricted to the Cr-doped (Sb,Bi)$$_{2}$$Te$$_{3}$$ system at extremely low temperature; however, the microscopic origin of its ferromagnetism is poorly understood. Here we present an element-resolved study for Cr-doped (Sb,Bi)$$_{2}$$Te$$_{3}$$ using X-ray magnetic circular dichroism to unambiguously show that the long-range magnetic order is mediated by the p-hole carriers of the host lattice, and the interaction between the Sb(Te) p and Cr d states is crucial.

Journal Articles

Atom-photon coupling from nitrogen-vacancy centres embedded in tellurite microspheres

Ruan, Y.*; Gibson, B. C.*; Lau, D. W. M.*; Greentree, A. D.*; Ji, H.*; Ebendorff-Heidepriem, H.*; Johnson, B. C.*; Oshima, Takeshi; Monro, T. M.*

Scientific Reports (Internet), 5, p.11486_1 - 11486_7, 2015/06

 Times Cited Count:4 Percentile:27.29(Multidisciplinary Sciences)

Journal Articles

Identification of deformed intruder states in semi-magic $$^{70}$$Ni

Chiara, C. J.*; Weisshaar, D.*; Janssens, R. V. F.*; Tsunoda, Yusuke*; Otsuka, Takaharu*; Harker, J. L.*; Walters, W. B.*; Recchia, F.*; Albers, M.*; Alcorta, M.*; et al.

Physical Review C, 91(4), p.044309_1 - 044309_10, 2015/04

 Times Cited Count:33 Percentile:91.67(Physics, Nuclear)

The neutron-rich isotope $$^{70}$$Ni was produced by multi-nucleon transfer reactions of $$^{70}$$Zn in the Argonne National Laboratory, and an in-beam $$gamma$$-ray experiment were performed using the GRETINA array. The $$2^+_2$$ and $$4^+_2$$ levels of $$^{70}$$Ni were observed for the first time. Those levels are regarded as large deformed states associated with proton excitation from the $$f_{7/2}$$ orbit because they cannot be reproduced by a shell-model calculation assuming a small valence space without $$f_{7/2}$$. A theoretical analysis based on the Monte Carlo shell model published in 2014 indicates that those levels corresponds to a prolate deformed band. The present result demonstrates the occurrence of shape coexistence in neutron-rich Ni isotopes other than a known case of $$^{68}$$Ni, and confirms the predictive power of the Monte Carlo shell-model calculation.

Journal Articles

In situ synthesis of volatile carbonyl complexes with short-lived nuclides

Even, J.*; Ackermann, D.*; Asai, Masato; Block, M.*; Brand, H.*; Di Nitto, A.*; D$"u$llmann, Ch. E.*; Eichler, R.*; Fan, F.*; Haba, Hiromitsu*; et al.

Journal of Radioanalytical and Nuclear Chemistry, 303(3), p.2457 - 2466, 2015/03

 Times Cited Count:13 Percentile:78.31(Chemistry, Analytical)

Rapid In situ synthesis of metal carbonyl complexes has been demonstrated using short-lived isotopes produced in nuclear fission and fusion reactions. The short-lived isotopes with high recoil energy directly react with carbon-monoxides and form carbonyl complexes. Only highly volatile complexes were fast transported in a gas stream to counting and chemistry devices. Short-lived Mo, Tc, Ru, Rh, W, Re, Os, and Ir were found to form volatile carbonyl complexes, while no volataile complex of Hf and Ta were detected. This technique has been applied to a chemical investigation of the superheavy element Sg (atomic number 106), and will be applicable to various fields of nuclear science with short-lived transition metal isotopes.

62 (Records 1-20 displayed on this page)