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Journal Articles

PANDORA Project for the study of photonuclear reactions below $$A=60$$

Tamii, Atsushi*; Pellegri, L.*; S$"o$derstr$"o$m, P.-A.*; Allard, D.*; Goriely, S.*; Inakura, Tsunenori*; Khan, E.*; Kido, Eiji*; Kimura, Masaaki*; Litvinova, E.*; et al.

European Physical Journal A, 59(9), p.208_1 - 208_21, 2023/09

 Times Cited Count:1 Percentile:0.02(Physics, Nuclear)

no abstracts in English

Journal Articles

Neutron-hole states in $$^{131}$$Sn and spin-orbit splitting in neutron-rich nuclei

Orlandi, R.; Pain, S. D.*; Ahn, S.*; Jungclaus, A.*; Schmitt, K. T.*; Bardayan, D. W.*; Catford, W. N.*; Chapman, R.*; Chipps, K. A.*; Cizewski, J. A.*; et al.

Physics Letters B, 785, p.615 - 620, 2018/10

 Times Cited Count:7 Percentile:53.6(Astronomy & Astrophysics)

Journal Articles

First prompt in-beam $$gamma$$-ray spectroscopy of a superheavy element; The $$^{256}$$Rf

Rubert, J.*; Dorvaux, O.*; Gall, B. J. P.*; Greenlees, P. T.*; Asfari, Z.*; Piot, J.*; Andersson, L. L.*; Asai, Masato; Cox, D. M.*; Dechery, F.*; et al.

Journal of Physics; Conference Series, 420, p.012010_1 - 012010_10, 2013/03

 Times Cited Count:0 Percentile:0.04(Physics, Nuclear)

The first prompt in-beam $$gamma$$-ray spectroscopy of a superheavy element, $$^{256}$$Rf, has been performed successfully. A development of an intense isotopically enriched $$^{50}$$Ti beam using the MIVOC method enabled us to perform this experiment. A rotational band up to a spin of 20 $$hbar$$ has been discovered in $$^{256}$$Rf, and its moment of inertia has been extracted. These data suggest that there is no evidence of a significant deformed shell gap at $$Z$$ = 104.

Journal Articles

Shell-structure and pairing interaction in superheavy nuclei; Rotational properties of the $$Z$$=104 nucleus $$^{256}$$Rf

Greenlees, P. T.*; Rubert, J.*; Piot, J.*; Gall, B. J. P.*; Andersson, L. L.*; Asai, Masato; Asfari, Z.*; Cox, D. M.*; Dechery, F.*; Dorvaux, O.*; et al.

Physical Review Letters, 109(1), p.012501_1 - 012501_5, 2012/07

 Times Cited Count:58 Percentile:88.75(Physics, Multidisciplinary)

Rotational band structure of the $$Z$$=104 nucleus $$^{256}$$Rf has been observed for the first time using an in-beam $$gamma$$-ray spectroscopic technique. This nucleus is the heaviest among the nuclei whose rotational band structure has ever been observed. Thus, the present result provides valuable information on the single-particle shell structure and pairing interaction in the heaviest extreme of nuclei. The deduced moment of inertia indicates that there is no deformed shell gap at $$Z$$=104, which is predicted in a number of current self-consistent mean-field models.

Journal Articles

Bacterial production of organic acids enhances H$$_{2}$$O$$_{2}$$-dependent iodide oxidation

Li, H.-P.*; Yeager, C. M.*; Brinkmeyer, R.*; Zhang, S.*; Ho, Y.-F.*; Xu, C.*; Jones, W. L.*; Schwehr, K. A.*; Otosaka, Shigeyoshi; Roberts, K. A.*; et al.

Environmental Science & Technology, 46(9), p.4837 - 4844, 2012/03

 Times Cited Count:52 Percentile:77.77(Engineering, Environmental)

In order to develop an understanding of the role that microorganisms play in the transport of $$^{129}$$I in soil-water systems, naturally occurring bacteria isolated from the F-area subsurface of the Savannah River Site (SRS) were assessed for iodide oxidizing activity. Spent liquid medium from a number of SRS bacterial cultures enhanced iodide oxidation 2-10 fold in the presence of hydrogen peroxide (H$$_{2}$$O$$_{2}$$). From a time-series measurements of peroxidase activities and organic acid concentrations, it was hypothesized that microbial organic acid exudate promoted iodide oxidation via following mechanisms; (1) organic acids interact with H$$_{2}$$O$$_{2}$$ to form strong iodide oxidizing agents, peroxy carboxylic acids, and (2) organic acid secretion led to enhanced rates of H$$_{2}$$O$$_{2}$$-dependent iodide oxidation by lowering the pH of the culture medium.

Journal Articles

Isomeric states observed in heavy neutron-rich nuclei populated in the fragmentation of a $$^{208}$$Pb beam

Steer, S. J.*; Podoly$'a$k, Z.*; Pietri, S.*; G$'o$rska, M.*; Grawe, H.*; Maier, K.*; Regan, P. H.*; Rudolph, D.*; Garnsworthy, A. B.*; Hoischen, R.*; et al.

Physical Review C, 84(4), p.044313_1 - 044313_22, 2011/10

 Times Cited Count:65 Percentile:94.74(Physics, Nuclear)

Heavy neutron-rich nuclei were populated via the fragmentation of a E/A=1 GeV $$_{82}^{208}$$Pb beam. Secondary fragments were separated and identified and subsequently implanted in a passive stopper. By the detection of delayed $$gamma$$ rays, isomeric decays associated with these nuclei have been identified. A total of 49 isomers were detected, with the majority of them observed for the first time. Possible level schemes are constructed and the structure of the nuclei discussed. To aid the interpretation, shell-model as well as BCS calculations were performed.

Journal Articles

Search for a 2-quasiparticle high-$$K$$ isomer in $$^{256}$$Rf

Robinson, A. P.*; Khoo, T. L.*; Seweryniak, D.*; Ahmad, I.*; Asai, Masato; Back, B. B.*; Carpenter, M. P.*; Chowdhury, P.*; Davids, C. N.*; Greene, J.*; et al.

Physical Review C, 83(6), p.064311_1 - 064311_7, 2011/06

 Times Cited Count:32 Percentile:84.86(Physics, Nuclear)

We have identified an isomer with a half-life of 17 $$mu$$s in $$^{256}$$Rf through a calorimetric conversion electron measurement tagged with implanted $$^{256}$$Rf nuclei using the fragment mass analyzer at Argonne National Laboratory. The low population yield for this isomer suggests that this isomer should not be a 2-quasiparticle high-$$K$$ isomer which is typically observed in the N = 152 isotones, but should be a 4-quasiparticle one. Possible reasons of the non-observation of a 2-quasiparticle isomer are this isomer decays by fission with a half-life similar to that of the ground state of $$^{256}$$Rf. Another possibility, that there is no 2-quasiparticle isomer at all, would imply an abrupt termination of axially symmetric deformed shape at Z=104.

Journal Articles

Bridging the nuclear structure gap between stable and super heavy nuclei

Seweryniak, D.*; Khoo, T. L.*; Ahmad, I.*; Kondev, F. G.*; Robinson, A.*; Tandel, S. K.*; Asai, Masato; Back, B. B.*; Carpenter, M. P.*; Chowdhury, P.*; et al.

Nuclear Physics A, 834(1-4), p.357c - 361c, 2010/03

 Times Cited Count:7 Percentile:47.82(Physics, Nuclear)

Experimental data on single-particle energies in nuclei around Z=100 and N=152 play an important role to test validity of theoretical predictions for shell structure of superheavy nuclei. We found high-K two-quasiparticle isomers in $$^{252}$$No and $$^{254}$$No, and evaluated energies of proton single-particle orbitals around Z=100. We also found a new high-K three quasiparticle isomer in $$^{257}$$Rf. Energies of neutron single-particle orbitals were also evaluated from experimental data of the $$alpha$$ decay of $$^{257}$$Rf. Comparisons between the present experimental data and various theoretical calculations for the proton single-particle orbitals indicate that the calculation by using the Woods-Saxon potential gives the best agreement with the data.

Journal Articles

State-of-the-art report on nuclear aerosols

Allelein, H.-J.*; Auvinen, A.*; Ball, J.*; G$"u$ntay, S.*; Herranz, L. E.*; Hidaka, Akihide; Jones, A. V.*; Kissane, M.*; Powers, D.*; Weber, G.*

NEA/CSNI/R(2009)5, 388 Pages, 2009/12

Journal Articles

ERL09 WG1 summary; DC gun technological challenges

Nishimori, Nobuyuki; Bazarov, I.*; Dunham, B.*; Grames, J.*; Hernandez-Garcia, C.*; Jones, L.*; Militsyn, B.*; Poelker, M.*; Surles-Law, K.*; Yamamoto, Masahiro*

Proceedings of 45th Advanced ICFA Beam Dynamics Workshop on Energy Recovery Linacs (ERL '09) (Internet), p.6 - 23, 2009/06

Journal Articles

Weakly deformed oblate structures in $$^{198}_{76}$$Os$$_{122}$$

Podoly$'a$k, Zs.*; Steer, S. J.*; Pietri, S.*; Xu, F. R.*; Liu, H. J.*; Regan, P. H.*; Rudolph, D.*; Garnsworthy, A. B.*; Hoischen, R.*; G$'o$rska, M.*; et al.

Physical Review C, 79(3), p.031305_1 - 031305_4, 2009/03

 Times Cited Count:35 Percentile:86.28(Physics, Nuclear)

$$gamma$$ rays de-exciting isomeric states in the neutron-rich nucleus $$_{76}^{198}$$Os$$_{122}$$ have been observed following relativistic projectile fragmentation of a 1 GeV per nucleon $$^{208}$$Pb beam. The ground-state band has properties compatible with oblate deformation. The evolution of the structure of Os isotopes characterized by sudden prolate-oblate shape change is discussed and contrasted with the smooth change known in the Pt chain.

Journal Articles

$$K^{pi}=8^{-}$$ isomers and $$K^{pi}=2^{-}$$ octupole vibrations in $$N=150$$ shell-stabilized isotones

Robinson, A. P.*; Khoo, T. L.*; Ahmad, I.*; Tandel, S. K.*; Kondev, F. G.*; Nakatsukasa, Takashi*; Seweryniak, D.*; Asai, Masato; Back, B. B.*; Carpenter, M. P.*; et al.

Physical Review C, 78(3), p.034308_1 - 034308_6, 2008/09

 Times Cited Count:49 Percentile:90.87(Physics, Nuclear)

Isomers have been identified in $$^{246}$$Cm and $$^{252}$$No with quantum number $$K^{pi}=8^{-}$$, which decay through $$K^{pi}=2^{-}$$ rotational bands built on octupole vibrational states. For $$N=150$$ isotones with atomic number $$Z=94$$$$sim$$102, the $$K^{pi}=8^{-}$$ and 2$$^{-}$$ states have remarkably stable energies, indicating neutron excitations. An exception is a singular minimum in the 2$$^{-}$$ energy at $$^{246}$$Cm, due to the additional role of proton configurations.

Journal Articles

Neutron-proton pairing competition in $$N=Z$$ nuclei; Metastable state decays in the proton dripline nuclei $$^{82}_{41}$$Nb and $$^{86}_{43}$$Tc

Garnsworthy, A. B.*; Regan, P. H.*; C$'a$ceres, L.*; Pietri, S.*; Sun, Y.*; Rudolph, D.*; G$'o$rska, M.*; Podoly$'a$k, Z.*; Steer, S. J.*; Hoischen, R.*; et al.

Physics Letters B, 660(4), p.326 - 330, 2008/02

 Times Cited Count:25 Percentile:79.09(Astronomy & Astrophysics)

The low-lying structures of the self-conjugate ($$N=Z$$) nuclei $$^{82}_{41}$$Nb and $$^{86}_{43}$$Tc have been investigated using isomeric-decay spectroscopy following the projectile fragmentation of a $$^{107}$$Ag beam. These represent the heaviest odd-odd $$N=Z$$ nuclei in which internal decays have been identified to date. The resulting level schemes shed light on the shape evolution along the $$N=Z$$ line between the doubly-magic systems $$^{56}_{28}$$Ni and $$^{100}_{50}$$Sn and support a preference for $$T=1$$ states in $$T_z=0$$ odd-odd nuclei at low excitation energies associated with a $$T=1$$ neutron-proton pairing gap. Comparison with Projected Shell Model calculations suggests that the decay in $$^{82}$$Nb may be interpreted as an isospin-changing $$K$$ isomer.

Journal Articles

Isomeric decay studies around $$^{204}$$Pt and $$^{148}$$Tb

Podoly$'a$k, Zs.*; Steer, S. J.*; Pietri, S.*; Werner-Malento, E.*; Regan, P. H.*; Rudolph, D.*; Garnsworthy, A. B.*; Hoischen, R.*; G$'o$rska, M.*; Gerl, J.*; et al.

European Physical Journal; Special Topics, 150(1), p.165 - 168, 2007/11

 Times Cited Count:11 Percentile:55.68(Physics, Multidisciplinary)

Relativistic energy projectile fragmentation of $$^{208}$$Pb has been used to produce a range of exotic nuclei. The nuclei of interest were studied by detecting delayed $$gamma$$ rays following the decay of isomeric states. Experimental information on the excited states of the neutron-rich $$^{204}$$Pt N=126 nucleus, following internal decay of two isomeric states, was obtained for the first time. In addition, decays from the previously reported isomeric $$I=27hbar$$ and $$I=(49/2)hbar$$ states in $$^{148}$$Tb and $$^{147}$$Gd, respectively, have been observed. These isomeric decays represent the highest discrete states observed to date following a prejectile fragmentation reaction, and opens up the possibilty of doing "high-spin physics" using this technique.

Journal Articles

Design progress of the ITER vacuum vessel sectors and port structures

Utin, Y.*; Ioki, Kimihiro; Alekseev, A.*; Bachmann, C.*; Cho, S. Y.*; Chuyanov, V.*; Jones, L.*; Kuzmin, E.*; Morimoto, Masaaki; Nakahira, Masataka; et al.

Fusion Engineering and Design, 82(15-24), p.2040 - 2046, 2007/10

 Times Cited Count:2 Percentile:18.73(Nuclear Science & Technology)

Recent progress of the ITER vacuum vessel (VV) design is presented. As the ITER construction phase approaches, the VV design has been improved and developed in more detail with the focus on better performance, improved manufacture and reduced cost. Based on achievements of manufacturing studies, design improvement of the typical VV sector (#1) has been nearly finalized. Design improvement of other sectors is in progress - in particular, of the VV sector #2 and #3 which interface with the ports for the neutral beam injection. For all sectors, the concept for the in-wall shielding has progressed and developed in more detail. The design progress of the VV sectors has been accompanied by the progress of the port structures. In particular, design of the NB Ports was advanced with the focus on the heat-flux components to handle the heat input of the neutral beams. Structural analyses have been performed to validate all design improvements.

Journal Articles

Recent results in fragmentation isomer spectroscopy with rising

Pietri, S.*; Regan, P. H.*; Podoly$'a$k, Zs.*; Rudolph, D.*; Steer, S. J.*; Garnsworthy, A. B.*; Werner-Malento, E.*; Hoischen, R.*; G$'o$rska, M.*; Gerl, J.*; et al.

Nuclear Instruments and Methods in Physics Research B, 261(1-2), p.1079 - 1083, 2007/08

 Times Cited Count:94 Percentile:98.43(Instruments & Instrumentation)

The first results from the stopped beam RISING experimental campaign performed at the GSI laboratory in Darmstadt, Germany, are presented. RISING constitutes a major new experimental program in European nuclear structure physics research aimed at using relativistic energy (typically around 1 GeV per nucleon) projectile fragmentation reactions to populate nuclei with highly exotic proton-to-neutron ratios compared to the line of beta stability. In its high-efficiency stopped beam configuration, the RISING $$gamma$$-ray spectrometer consists of 105 individual germanium crystals which view a focal plane in which the exotic nuclei are brought to rest. Here, decays from metastable states with half-lives in the nano to milliseconds range can be observed. Results of initial commissioning experiments are also shown and details of the planned future experimental program are given.

Journal Articles

ITER nuclear components, preparing for the construction and R&D results

Ioki, Kimihiro*; Akiba, Masato; Barabaschi, P.*; Barabash, V.*; Chiocchio, S.*; Daenner, W.*; Elio, F.*; Enoeda, Mikio; Ezato, Koichiro; Federici, G.*; et al.

Journal of Nuclear Materials, 329-333(1), p.31 - 38, 2004/08

 Times Cited Count:14 Percentile:66.09(Materials Science, Multidisciplinary)

The preparation of the procurement specifications is being progressed for key components. Progress has been made in the preparation of the procurement specifications for key nuclear components of ITER. Detailed design of the vacuum vessel (VV) and in-vessel components is being performed to consider fabrication methods and non-destructive tests (NDT). R&D activities are being carried out on vacuum vessel UT inspection with waves launched at an angle of 20 or 30 degree, on flow distribution tests of a two-channel model, on fabrication and testing of FW mockups and panels, on the blanket flexible support as a complete system including the housing, on the blanket co-axial pipe connection with guard vacuum for leak detection, and on divertor vertical target prototypes. The results give confidence in the validity of the design and identify possibilities of attractive alternate fabrication methods.

Journal Articles

Design improvements and R&D achievements for vacuum vessel and in-vessel components towards ITER construction

Ioki, Kimihiro*; Barabaschi, P.*; Barabash, V.*; Chiocchio, S.*; Daenner, W.*; Elio, F.*; Enoeda, Mikio; Gervash, A.*; Ibbott, C.*; Jones, L.*; et al.

Nuclear Fusion, 43(4), p.268 - 273, 2003/04

 Times Cited Count:21 Percentile:54.59(Physics, Fluids & Plasmas)

Although the basic concept of the vacuum vessel (VV) and in-vessel components of the ITER design has stayed the same, there have been several detailed design improvements resulting from efforts to raise reliability, to improve maintainability and to save money. One of the most important achievements in the VV R&D has been demonstration of the necessary fabrication and assembly tolerances. Recently the deformation due to cutting of the port extension was measured and it was shown that the deformation is small and acceptable. Further development of advanced methods of cutting, welding and NDT on a thick plate have been continued in order to refine manufacturing and improve cost and technical performance. With regard to the related FW/blanket and divertor designs, the R&D has resulted in the development of suitable technologies. Prototypes of the FW panel, the blanket shield block and the divertor components have been successfully fabricated.

Journal Articles

Structure and thermal expansivity of tetrahydrofuran deuterate determined by neutron powder diffraction

Jones, C. Y.*; Marshall, S. L.*; Chakoumakos, B. C.*; Rawn, C. J.*; Ishii, Yoshinobu

Journal of Physical Chemistry B, 107(25), p.6026 - 6031, 2003/03

 Times Cited Count:38 Percentile:68.4(Chemistry, Physical)

no abstracts in English

Journal Articles

The Use of rigid body constraints in Rietveld refinements of neutron diffraction data of clathrate hydrates

Chakoumakos, B. C.*; Rawn, C. J.*; Rondinone, A. J.*; Marshall, S. L.*; Stern, L. A.*; Circone, S.*; Kirby, S. H.*; Jones, C. Y.*; Toby, B. H.*; Ishii, Yoshinobu

Proceedings of 4th International Conference on Gas Hydrates (ICGH-4), p.655 - 658, 2002/05

no abstracts in English

24 (Records 1-20 displayed on this page)