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Toyoda, Satoshi*; Yamamoto, Tomoki*; Yoshimura, Masashi*; Sumida, Hirosuke*; Mineoi, Susumu*; Machida, Masatake*; Yoshigoe, Akitaka; Suzuki, Satoru*; Yokoyama, Kazushi*; Ohashi, Yuji*; et al.
Vacuum and Surface Science, 64(2), p.86 - 91, 2021/02
We have developed measurement and analysis techniques in X-ray photoelectron spectroscopy. To begin with, time-division depth profiles of gate stacked film interfaces have been achieved by NAP-HARPES (Near Ambient Pressure Hard X-ray Angle-Resolved Photo Emission Spectroscopy) data. We then have promoted our methods to quickly perform peak fittings and depth profiling from time-division ARPES data, which enables us to realize 4D-XPS analysis. It is found that the traditional maximum entropy method (MEM) combined with Jackknife averaging of sparse modeling in NAP-HARPES data is effective to perform dynamic measurement of depth profiles with high precision.
Shikaze, Yoshiaki; Nishizawa, Yukiyasu; Sanada, Yukihisa; Torii, Tatsuo; Jiang, J.*; Shimazoe, Kenji*; Takahashi, Hiroyuki*; Yoshino, Masao*; Ito, Shigeki*; Endo, Takanori*; et al.
Journal of Nuclear Science and Technology, 53(12), p.1907 - 1918, 2016/12
Times Cited Count:37 Percentile:96.33(Nuclear Science & Technology)The Compton camera was improved for use with the unmanned helicopter. Increase of the scintillator array from 44 to 8
8 and expanse of the distance between the two layers contributed to the improvements of detection efficiency and angular resolution, respectively. Measurements were performed over the riverbed of the Ukedo river of Namie town in Fukushima Prefecture. By programming of flight path and speed, the areas of 65 m
60 m and 65 m
180 m were measured during about 20 and 30 minutes, respectively. By the analysis the air dose rate maps at 1 m height were obtained precisely with the angular resolution corresponding to the position resolution of about 10 m from 10 m height. Hovering flights were executed over the hot spot areas for 10-20 minutes at 5-20 m height. By using the reconstruction software the
-ray images including the hot spots were obtained with the angular resolution same as that evaluated in the laboratory (about 10
).
Isayama, Akihiko; Suzuki, Takahiro; Hayashi, Nobuhiko; Ide, Shunsuke; Hamamatsu, Kiyotaka; Fujita, Takaaki; Hosoyama, Hiroki; Kamada, Yutaka; Nagasaki, Kazunobu*; Oyama, Naoyuki; et al.
AIP Conference Proceedings 933, p.229 - 236, 2007/10
no abstracts in English
Nakamura, Hiroo; Tsuji, Shunji; ; Ozeki, Takahisa; Ishida, Shinichi; Azumi, Masafumi; Akiba, Masato; Ando, Toshiro; Fujii, Tsuneyuki; Fukuda, Takeshi; et al.
Nuclear Fusion, 30(2), p.235 - 250, 1990/02
Times Cited Count:16 Percentile:53.11(Physics, Fluids & Plasmas)no abstracts in English
Nakamura, Hiroo; Tsuji, Shunji; ; Ozeki, Takahisa; Ishida, Shinichi; Azumi, Masafumi; Akiba, Masato; Ando, Toshiro; Fujii, Tsuneyuki; Fukuda, Takeshi; et al.
JAERI-M 89-106, 52 Pages, 1989/08
no abstracts in English
Kaneya, Yusuke*; Tomitsuka, Tomohiro; Sato, Tetsuya; Asai, Masato; Tsukada, Kazuaki; Toyoshima, Atsushi; Mitsukai, Akina; Makii, Hiroyuki; Hirose, Kentaro; Osa, Akihiko; et al.
no journal, ,
Kaneya, Yusuke*; Asai, Masato; Sato, Tetsuya; Tomitsuka, Tomohiro; Tsukada, Kazuaki; Toyoshima, Atsushi; Mitsukai, Akina; Makii, Hiroyuki; Hirose, Kentaro; Osa, Akihiko; et al.
no journal, ,
To study the influence of the valence 7p electronic orbital on chemical properties of lawrencium, a measurement of the adsorption enthalpy of lawrencium was carried out. A new method using a surface ionization technique coupled to an on-line isotope separator was developed, which enabled one to measure temperature dependence of lawrencium surface adsorption on a metallic tantalum surface at high temperature up to 2800 K. The temperature dependences of adsorption of lawrencium as well as various lanthanide elements were investigated with this method, and the adsorption enthalpy of lawrencium was successfully extracted.
Tomitsuka, Tomohiro; Tokoi, Katsuyuki*; Sato, Tetsuya; Asai, Masato; Tsukada, Kazuaki; Toyoshima, Atsushi; Chiera, N. M.; Kamada, Hiroki; Nagame, Yuichiro; Goto, Shinichi*
no journal, ,
no abstracts in English
Sato, Tetsuya; Kaneya, Yusuke*; Asai, Masato; Tsukada, Kazuaki; Toyoshima, Atsushi; Mitsukai, Akina*; Osa, Akihiko; Makii, Hiroyuki; Hirose, Kentaro; Nagame, Yuichiro; et al.
no journal, ,
Our experimental results on the first ionization potential measurement of lawrencium (Lr, element 103) have strongly suggested that the Lr atom has a [Rn] configuration as a result of the influence of strong relativistic effects. The configuration is different from that expected from the lanthanide homologue, lutetium (Lu). According to a semi-empirical consideration, it is expected that the change of the electronic configuration leads higher volatility of Lr than that of Lu. In this work, adsorption behaviors of Lr and various short-lived rare earth isotopes on a tantalum surface were investigated via observation of their surface ionization efficiencies. It was found that Lr would behave like low volatile rare earth elements such as Lu contrary to the semi-empirical expectation.
Kamada, Hiroki*; Asai, Masato; Tsukada, Kazuaki; Sato, Tetsuya; Toyoshima, Atsushi; Nagame, Yuichiro; Mitsukai, Akina; Tomitsuka, Tomohiro*; Andreyev, A. N.; Nishio, Katsuhisa; et al.
no journal, ,
Existence of the previously unknown isomer Np was discovered for the first time.
Np was produced by using the JAEA tandem accelerator. Short-lived reaction products were mass-separated by the on-line isotope separator ISOL, and
and X rays originating from the decay of
Np were observed. The half-life of
Np was determined to be approximately 9 min, and
Np was found to decay via the EC decay as well as the isomeric transition. On the basis of the observed
and X rays and the half-life value, we have evaluated level energy, spin-parity, and proton-neutron configuration of
Np.
Asai, Masato; Tsukada, Kazuaki; Hirose, Kentaro; Toyoshima, Atsushi; Tomitsuka, Tomohiro; Chiera, N. M.; Ito, Yuta; Makii, Hiroyuki; Nagame, Yuichiro; Nishio, Katsuhisa; et al.
no journal, ,
Spontaneous fissions of neutron-rich heavy actinide isotopes Fm,
Fm, and
Lr have been measured at the JAEA Tandem accelerator facility.
Fm and
Fm were produced in a multinucleon transfer reaction with an
O beam and an extremely rare
Es target with a half-life of 276 days. Reaction products were mass-separated with an on-line isotope separator (ISOL). A transition between the typical asymmetric mass distribution and a very sharp symmetric one was clearly observed between
Fm and
Fm, while the spontaneous fission of
Lr was found to exhibit mixture of three different fission modes.
Asai, Masato; Suekawa, Yoshihide*; Higashi, Masato*; Kamada, Hiroki*; Tobe, Teruhisa*; Andreyev, A. N.; Hirose, Kentaro; Ito, Yuta; Makii, Hiroyuki; Nishio, Katsuhisa; et al.
no journal, ,
A new isomer Np with a half-life of
9 min has been discovered. It was produced in the reaction of
U target with
Li beam at JAEA tandem accelerator, and was identified through characteristic X-ray measurement and mass separation with an on-line isotope separator (ISOL). Gamma-ray singles, gamma-gamma coincidence, and internal-conversion electron measurements were performed. It was revealed that the
Np decays mostly through an isomeric E4 transition followed by an M1 transition, and that the spin-parity of the
Np should be 5
. The results are introduced in detail, and the nuclear structure of the
Np are discussed.
Asai, Masato; Suekawa, Yoshihide*; Higashi, Masato*; Kamada, Hiroki*; Tobe, Teruhisa*; Andreyev, A. N.; Hirose, Kentaro; Ito, Yuta; Makii, Hiroyuki; Nishio, Katsuhisa; et al.
no journal, ,
We have carried out experiments to study nuclear structure of the new isomer Np which we discovered recently. The
Np was produced in the reaction of
U target with
Li beam at JAEA tandem accelerator, and was mass-separated with an on-line isotope separator (ISOL). The half-life was determined accurately through LX-ray measurements. The
transition emitted by following the isomeric transition was successfully observed through LX-
coincidence measurements. Moreover, the multipolarities of the
transitions were determined with internal-conversion electron measurements. On the basis of these experimental results, We have clarified excitation energy, spin-parity, and nuclear structure of
Np.
Shikaze, Yoshiaki; Torii, Tatsuo; Nishizawa, Yukiyasu; Yoshida, Mami*; Shimazoe, Kenji*; Jiang, J.*; Takahashi, Hiroyuki*; Kurosawa, Shunsuke*; Kamada, Kei*; Yoshikawa, Akira*; et al.
no journal, ,
no abstracts in English
Sato, Tetsuya; Kaneya, Yusuke*; Asai, Masato; Tsukada, Kazuaki; Toyoshima, Atsushi; Mitsukai, Akina*; Osa, Akihiko; Makii, Hiroyuki; Hirose, Kentaro; Nagame, Yuichiro; et al.
no journal, ,
Our experimental results on the first ionization potential measurement of lawrencium (Lr, element 103) have strongly suggested that the Lr atom has a [Rn] configuration as a result of the influence of strong relativistic effects. The configuration is different from that expected from the lanthanide homologue, lutetium (Lu). According to a semi-empirical consideration, it is expected that the change of the electronic configuration leads higher volatility of Lr than that of Lu. In this work, adsorption behaviors of Lr and various short-lived rare earth isotopes on a tantalum surface were investigated via observation of their surface ionization efficiencies. It was found that Lr would behave like low volatile rare earth elements such as Lu contrary to the semi-empirical expectation.
Shikaze, Yoshiaki; Torii, Tatsuo; Shimazoe, Kenji*; Jiang, J.*; Takahashi, Hiroyuki*; Kurosawa, Shunsuke*; Kamada, Kei*; Yoshikawa, Akira*; Yoshino, Masao*; Ito, Shigeki*; et al.
no journal, ,
no abstracts in English
Sato, Tetsuya; Kaneya, Yusuke*; Asai, Masato; Tsukada, Kazuaki; Toyoshima, Atsushi; Mitsukai, Akina*; Osa, Akihiko; Makii, Hiroyuki; Nishio, Katsuhisa; Hirose, Kentaro; et al.
no journal, ,
The ground state electronic configuration of lawrencium (Lr, Z =103) is predicted to be [Rn], which is different from that of the lanthanide homolog Lu [Xe]
due to strong relativistic effects. According to semi-empirical considerations, volatility of Lr is expected to be higher than that of Lu. We have investigated adsorption behavior of
Lr, which was produced in the reaction of
Cf(
B, 4n), on a tantalum (Ta) metal surface using a surface ion-source installed into the isotope separator on-line (ISOL) at the JAEA tandem accelerator facility. The observed adsorption behavior of
Lr was similar to those of Tb and Lu which have relatively higher adsorption enthalpy on Ta surface. It implies that Lr would have low volatility like such as Lu and Tb.
Asai, Masato; Kamada, Hiroki*; Shigekawa, Yudai*; Tsukada, Kazuaki; Sato, Tetsuya; Toyoshima, Atsushi; Mitsukai, Akina; Nagame, Yuichiro; Nishio, Katsuhisa; Hirose, Kentaro; et al.
no journal, ,
To clarify the fission mechanism of mass-symmetric spontaneous fissions observed around the neutron-rich Fm region, we have measured kinetic energies and mass distribution of spontaneous-fission fragments in this nuclear region precisely. The experiment was performed at the JAEA tandem accelerator facility using an on-line isotope separator (ISOL). The mass-separated Lr nuclei were implanted into thin foil, and two fragments of their spontaneous fission were coincidently measured with two Si detectors. The spontaneous fission of
Lr was found to show a narrow symmetric mass distribution. On the other hand, their total kinetic energy TKE was found to be low, which is apparently different from the high-TKE symmetric fissions observed in the Fm isotopes. This indicates that the fission mechanisms of these two symmetric fissions are different.
Asai, Masato; Tsukada, Kazuaki; Hirose, Kentaro; Toyoshima, Atsushi; Tomitsuka, Tomohiro; Chiera, N. M.; Ito, Yuta; Makii, Hiroyuki; Nagame, Yuichiro; Nishio, Katsuhisa; et al.
no journal, ,
Spontaneous fissions of Fm,
Fm, and
Lr have been measured using an
Es target at the JAEA Tandem Accelerator Facility. These three nuclei show different fission properties: the asymmetric fission, the high total-kinetic-energy (TKE) symmetric fission, and the low TKE symmetric fission, and the mechanisms of these three fissions should be very different. It is of great interest to elucidate how these differences occur. We have produced
Fm in multinucleon-transfer reactions with a
Es target and
O projectiles, and produced
Lr in the
Cm(
N,4n) fusion-evaporation reaction. The reaction products were mass-separated with a gas-jet-coupled on-line isotope separator, and were delivered into a rotating wheel alpha- and fission-fragment detection system. By comparing the mass and TKE distributions deduced from the present experimental data, we will discuss the differences in fission mechanism among
Fm,
Fm, and
Lr.
Kodama, Shohei*; Kurosawa, Shunsuke*; Morishita, Yuki; Usami, Hiroshi; Hayashi, Masateru*; Tanaka, Hiroki*; Yoshino, Masao*; Kamada, Kei*; Yoshikawa, Akira*; Torii, Tatsuo
no journal, ,
After Fukushima 1st Nuclear Plant accident, a large number of radioactive pollutants or nuclear debris with very high dose of more than a few Sv/h still have existed. To estimate the dose of such pollutants, a Japan Atomic Energy Agency research group has suggested a new technique to use a long optical fiber and a red-emitting scintillator, and the scintillation photons are read outside of high dose area. We tested the gamma-ray detection performance of a ruby (Cr:AlO
) and a newly developed Cs
HfI
scintillators as a scintillating probe coupled with an optical fiber in this study.