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Journal Articles

Quasifree neutron knockout reaction reveals a small $$s$$-Orbital component in the Borromean nucleus $$^{17}$$B

Yang, Z. H.*; Kubota, Yuki*; Corsi, A.*; Yoshida, Kazuki; Sun, X.-X.*; Li, J. G.*; Kimura, Masaaki*; Michel, N.*; Ogata, Kazuyuki*; Yuan, C. X.*; et al.

Physical Review Letters, 126(8), p.082501_1 - 082501_8, 2021/02

AA2020-0819.pdf:1.29MB

 Times Cited Count:43 Percentile:96.7(Physics, Multidisciplinary)

A quasifree ($$p$$,$$pn$$) experiment was performed to study the structure of the Borromean nucleus $$^{17}$$B, which had long been considered to have a neutron halo. By analyzing the momentum distributions and exclusive cross sections, we obtained the spectroscopic factors for $$1s_{1/2}$$ and $$0d_{5/2}$$ orbitals, and a surprisingly small percentage of 9(2)% was determined for $$1s_{1/2}$$. Our finding of such a small $$1s_{1/2}$$ component and the halo features reported in prior experiments can be explained by the deformed relativistic Hartree-Bogoliubov theory in continuum, revealing a definite but not dominant neutron halo in $$^{17}$$B. The present work gives the smallest $$s$$- or $$p$$-orbital component among known nuclei exhibiting halo features and implies that the dominant occupation of $$s$$ or $$p$$ orbitals is not a prerequisite for the occurrence of a neutron halo.

Journal Articles

Detailed structural study on the poly(vinyl alcohol) adsorption layers on a Si substrate with solvent vapor-induced swelling

Miyazaki, Tsukasa*; Miyata, Noboru*; Yoshida, Tessei*; Arima, Hiroshi*; Tsumura, Yoshihiro*; Torikai, Naoya*; Aoki, Hiroyuki; Yamamoto, Katsuhiro*; Kanaya, Toshiji*; Kawaguchi, Daisuke*; et al.

Langmuir, 36(13), p.3415 - 3424, 2020/04

 Times Cited Count:14 Percentile:58.64(Chemistry, Multidisciplinary)

Journal Articles

Elucidation of a heterogeneous layered structure in the thickness direction of poly(vinyl alcohol) films with solvent vapor-induced swelling

Miyazaki, Tsukasa*; Miyata, Noboru*; Asada, Mitsunori*; Tsumura, Yoshihiro*; Torikai, Naoya*; Aoki, Hiroyuki; Yamamoto, Katsuhiro*; Kanaya, Toshiji*; Kawaguchi, Daisuke*; Tanaka, Keiji*

Langmuir, 35(34), p.11099 - 11107, 2019/08

 Times Cited Count:22 Percentile:67.64(Chemistry, Multidisciplinary)

Journal Articles

Determination of fusion barrier distributions from quasielastic scattering cross sections towards superheavy nuclei synthesis

Tanaka, Taiki*; Narikiyo, Yoshihiro*; Morita, Kosuke*; Fujita, Kunihiro*; Kaji, Daiya*; Morimoto, Koji*; Yamaki, Sayaka*; Wakabayashi, Yasuo*; Tanaka, Kengo*; Takeyama, Mirei*; et al.

Journal of the Physical Society of Japan, 87(1), p.014201_1 - 014201_9, 2018/01

 Times Cited Count:18 Percentile:74.47(Physics, Multidisciplinary)

Excitation functions of quasielastic scattering cross sections for the $$^{48}$$Ca + $$^{208}$$Pb, $$^{50}$$Ti + $$^{208}$$Pb, and $$^{48}$$Ca + $$^{248}$$Cm reactions were successfully measured by using the gas-filled recoil-ion separator GARIS. Fusion barrier distributions were extracted from these data, and compared with the coupled-channels calculations. It was found that the peak energies of the barrier distributions for the $$^{48}$$Ca + $$^{208}$$Pb and $$^{50}$$Ti + $$^{208}$$Pb systems coincide with those of the 2n evaporation channel cross sections for the systems, while that of the $$^{48}$$Ca + $$^{248}$$Cm is located slightly below the 4n evaporation ones. This results provide us helpful information to predict the optimum beam energy to synthesize superheavy nuclei.

Journal Articles

Non-destructive examination of jacket sections for ITER central solenoid conductors

Takahashi, Yoshikazu; Suwa, Tomone; Nabara, Yoshihiro; Ozeki, Hidemasa; Hemmi, Tsutomu; Nunoya, Yoshihiko; Isono, Takaaki; Matsui, Kunihiro; Kawano, Katsumi; Oshikiri, Masayuki; et al.

IEEE Transactions on Applied Superconductivity, 25(3), p.4200904_1 - 4200904_4, 2015/06

 Times Cited Count:3 Percentile:20.23(Engineering, Electrical & Electronic)

The Japan Atomic Energy Agency (JAEA) is responsible for procuring all amounts of Central Solenoid (CS) Conductors for ITER, including CS jacket sections. The conductor is cable-in-conduit conductor (CICC) with a central spiral. A total of 576 Nb$$_{3}$$Sn strands and 288 copper strands are cabled around the central spiral. The maximum operating current is 40 kA at magnetic field of 13 T. CS jacket section is circular in square type tube made of JK2LB, which is high manganese stainless steel with boron added. Unit length of jacket sections is 7 m and 6,300 sections will be manufactured and inspected. Outer/inner dimension and weight are 51.3/35.3 mm and around 90 kg, respectively. Eddy Current Test (ECT) and Phased Array Ultrasonic Test (PAUT) were developed for non-destructive examination. The defects on inner and outer surfaces can be detected by ECT. The defects inside jacket section can be detected by PAUT. These technology and the inspected results are reported in this paper.

Journal Articles

Development of a new continuous dissolution apparatus with a hydrophobic membrane for superheavy element chemistry

Oe, Kazuhiro*; Attallah, M. F.*; Asai, Masato; Goto, Naoya*; Gupta, N. S.*; Haba, Hiromitsu*; Huang, M.*; Kanaya, Jumpei*; Kaneya, Yusuke*; Kasamatsu, Yoshitaka*; et al.

Journal of Radioanalytical and Nuclear Chemistry, 303(2), p.1317 - 1320, 2015/02

 Times Cited Count:10 Percentile:64.63(Chemistry, Analytical)

A new technique for continuous dissolution of nuclear reaction products transported by a gas-jet system was developed for superheavy element (SHE) chemistry. In this technique, a hydrophobic membrane is utilized to separate an aqueous phase from the gas phase. With this technique, the dissolution efficiencies of short-lived radionuclides of $$^{91m,93m}$$Mo and $$^{176}$$W were measured. Yields of more than 80% were observed for short-lived radionuclides at aqueous-phase flow rates of 0.1-0.4 mL/s. The gas flow-rate had no influence on the dissolution efficiency within the studied flow range of 1.0-2.0 L/min. These results show that this technique is applicable for on-line chemical studies of SHEs in the liquid phase.

Oral presentation

Chemical studies of Mo and W in preparation of a Seaborgium (Sg) reduction experiment using MDG, FEC, and SISAK

Toyoshima, Atsushi; Miyashita, Sunao*; Asai, Masato; Sato, Tetsuya; Kaneya, Yusuke; Tsukada, Kazuaki; Kitatsuji, Yoshihiro; Nagame, Yuichiro; Sch$"a$del, M.; Lerum, H. V.*; et al.

no journal, , 

To carry out a continuous reduction experiment of Sg with the low production rates and the short half-life, we are developing a new chemistry assembly consisting of a membrane degasser (MDG), a flow electrolytic column (FEC), the continuous liquid-liquid extraction apparatus, and the liquid scintillation counting system (SISAK). Recently, we have begun preparatory studies with Mo and W isotopes. Aqueous solution dissolving Mo and W was successfully separated from a carrier gas. Redox couples of Mo(VI)/Mo(V) and W(VI)/W(V) in HCl have been characterized for their macro amounts. Extraction behavior of Mo(VI) and W(VI) between toluene containing hinokitiol (HT) and HCl was successfully observed by a batch method. On-line extractions of short-lived Mo and W were also carried out using SISAK and MDG. In the symposium, our present status of the preparation with Mo and W will be presented.

Oral presentation

Electrolytic reduction studies of Mo and W towards the reduction of seaborgium

Toyoshima, Atsushi; Asai, Masato; Attallah, M. F.*; Goto, Naoya*; Gupta, N. S.*; Haba, Hiromitsu*; Huang, M.*; Kanaya, Jumpei*; Kaneya, Yusuke; Kasamatsu, Yoshitaka*; et al.

no journal, , 

Towards electrolytic reduction of Sg, batch-wise electrolytic reduction of carrier-free $$^{93m}$$Mo and $$^{176,181}$$W radiotracers was studied using a flow electrolytic column (FEC). The electrolyzed samples from a FEC were chemically analyzed by solvent extraction with TOA and HDEHP to separate and identify reduced species from the stable Mo(VI) and W(VI) ones based on their different extraction behavior. $$^{93m}$$Mo and $$^{176, 181}$$W were applied as radiotracers. We also performed cyclic voltammetry and UV/Vis absorption spectrometry of macro amounts of Mo and W in acidic solutions to obtain information on redox reactions of these elements under given conditions. In the conference, the present status of the preparatory reduction experiments with Mo and W will be presented.

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