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平田 芳信*; 中川 洋; 山内 宏樹; 金子 耕士; 萩原 雅人; 山口 秀幸*; 大元 智絵*; 勝野 那嘉子*; 今泉 鉄平*; 西津 貴久*
Food Hydrocolloids, 141, p.108728_1 - 108728_7, 2023/08
結晶化度は食品や材料の機械的性質に反映される。結晶化度は澱粉の構造ダイナミクスと関係しているはずである。本研究では、中性子準弾性散乱(QENS)を用いて、炊飯澱粉の老化に伴う分子ダイナミクスの変化を調べた。測定されたQENSの幅は老化に伴い狭くなった。また、弾性非干渉散乱構造因子(EISF)は増加し、老化現象に伴い分子ダイナミクスが空間的に抑制されることが示された。低移動度と高移動度をそれぞれ結晶相と非晶質相に対応させた2値分布の連続拡散モデルを用いてEISFを解析したところ、低移動度成分の割合が老化によって増加することが示された。
金子 耕士; 田端 千紘; 萩原 雅人; 山内 宏樹; 久保田 正人; 長壁 豊隆; 大貫 惇睦*
Journal of the Physical Society of Japan, 92(8), p.085001_1 - 085001_2, 2023/08
被引用回数：0 パーセンタイル：0(Physics, Multidisciplinary)A magnetic order in orthorhombic GdCu was investigated by a single crystal neutron diffraction with thermal neutron. Magnetic peaks were observed at incommensurate positions described by the ordering vector 
=(
~1~0) with =0.678 at 4~K. This ordering vector is close to the commensurate one with 
=(2/3~1~0) reported earlier, but clearly deviates. The incommensurate nature of the magnetic order in GdCu is further corroborated by the peak shift with temperature below 
.
森下 祐樹; 高崎 浩司; 北山 佳治; 田川 明広; 柴田 卓弥; 星 勝也; 金子 純一*; 樋口 幹雄*; 大浦 正利*
Radiation Measurements, 160, p.106896_1 - 106896_10, 2023/01
被引用回数：0 パーセンタイル：0.01(Nuclear Science & Technology)福島第一原子力発電所のアルファおよびベータ汚染をリアルタイム弁別測定するためのPhoswichアルファ/ベータ検出器を開発した。検出器は、アルファ線とベータ線を検出する2層のシンチレータ(プラスチックシンチレータ及びGPSシンチレータ)で構成した。パルス波形弁別(PSD)法を使用して、高ベータ線および高ガンマ線環境でアルファ線をリアルタイムを弁別測定できた。さらに、この検出器は、最大9.0mSv/hのバックグラウンド線量下でアルファ線を識別することができた。
; 
SR studies and charge-spin percolation modelSheng, Q.*; 金子 竜也*; Yamakawa, Kohtaro*; Guguchia, Z.*; Gong, Z.*; Zhao, G.*; Dai, G.*; Jin, C.*; Guo, S.*; Fu, L.*; et al.
Physical Review Research (Internet), 4(3), p.033172_1 - 033172_14, 2022/09
A pyrite system NiS
Se
exhibits a bandwidth controlled Mott transition via (S,Se) substitutions in a two-step process: the antiferromagnetic insulator (AFI) to antiferromagnetic metal (AFM) transition at 
0.45 followed by the AFM to paramagnetic metal (PMM) transition at 1.0. Among a few other Mott systems which exhibit similar two-step transitions, Ni(S,Se) is of particular interest because a large intermediate AFM region in the phase diagram would provide unique opportunities to study the interplay between the spin and charge order. By comparing and combining our muon spin relaxation studies and previous neutron scattering studies, here we propose a picture where the spin order is maintained by the percolation of "nonmetallic" localized and dangling Ni moments surrounded by S, while the charge transition from AFI to AFM is caused by the percolation of the conducting paths generated by the Ni-Se-Ni bonds.
松村 武*; 塚越 舜*; 上田 祥央*; 比嘉 野乃花*; 中尾 朗子*; 金子 耕士; 垣花 将司*; 辺土 正人*; 仲間 隆男*; 大貫 惇睦*
Journal of the Physical Society of Japan, 91(7), p.073703_1 - 073703_5, 2022/07
被引用回数：6 パーセンタイル：78.27(Physics, Multidisciplinary)Successive magnetic phase transitions in EuIrGe, an intermetallic compound with a body centered tetragonal lattice belonging to a polar space group I4mm, has been investigated by neutron diffraction and resonant X-ray diffraction. It is shown that EuIrGe exhibits an incommensurate longitudinal sinusoidalorder with 
(0, 0, 0.792) and m
c-axis in the high temperature phase, which changes to a cycloidal order with = (
, 0, 0.8) (
0.017) and m ac-plane in the intermediate phase. In the low temperature phase, the cycloidal plane rotates by 45
to have =(
, 0.8) (
0.012). It is also pointed out that the X-ray scattering amplitude from odd-parity magnetic quadrupole due to the polar environment interfere with that from normal even-parity magnetic dipole in the magnetic ordered phase.
加藤 篤志; 山本 智彦; 安藤 将人; 近澤 佳隆; 村上 久友*; 大山 一弘*; 金子 文彰*; 日暮 浩一*; Chanteclair, F.*; Chenaud, M.-S.*; et al.
EPJ Nuclear Sciences & Technologies (Internet), 8, p.11_1 - 11_10, 2022/06
本稿はナトリウム冷却炉のプラントシステムに採用する技術について、仏国のアストリッド炉等を基にして日仏の技術仕様共通化を検討し、共通プラントの構築に係る検討の成果をまとめている。特に地震条件の違いに対応した原子炉構造設計では、日本側で採用している高周波設計を日仏で共有し、適応を試みている。その他、蒸気発生器、崩壊熱除去システム、燃料取り扱いシステム、および格納容器の仕様共通化の検討を紹介する。
金子 耕士; 川崎 卓郎; 仲村 愛*; 宗像 孝司*; 中尾 朗子*; 花島 隆泰*; 鬼柳 亮嗣; 大原 高志; 辺土 正人*; 仲間 隆男*; et al.
Journal of the Physical Society of Japan, 90(6), p.064704_1 - 064704_6, 2021/06
被引用回数：37 パーセンタイル：95.85(Physics, Multidisciplinary)Multiple transition phenomena in divalent Eu compound EuAl with the tetragonal structure were investigated via single crystal time-of-flight neutron Laue technique. At 30 K below a charge-density-wave (CDW) transition, superlattice peaks emerge near nuclear Bragg peaks described by an ordering vector 
= (0 0 
). In contrast, magnetic peaks appear at 
with 
= 0.09 below 
= 15.4 K, and moves to 
with 
= 0.19 below 
=12.2 K, whereas no distinct change in the magnetic Bragg peak was detected at 
and 
. The structural modification with is characterized by an absence of the superlattice peak in (0 0 
). Considering an absence of splitting in magnetic peaks along , the structural transition is mainly ascribed to a displacement of Al ions within the tetragonal 
-plane. Complex incommensurate magnetic transitions are in stark contrast to a simple collinear commensurate structure in isovalent EuGa. This could stem from incompatible electronic structures with the CDW transition between two compounds.
金子 耕士; 垣花 将司*; 辺土 正人*; 仲間 隆男*; 大貫 惇睦*
波紋, 30(3), p.160 - 165, 2020/08
MnSiと同じ空間群に属する4
電子系化合物EuPtSiについて、磁気特性を調べた。単結晶中性子回折実験の結果、MnSiとEuPtSiの磁気構造に多くの共通点を見出した。この結果は、EuPtSiが4電子系で初めて磁気スキルミオン格子を示す物質であることを示している。
電子系化合物EuPtSiにおける磁気スキルミオン金子 耕士; 垣花 将司*; 辺土 正人*; 仲間 隆男*; 大貫 惇睦*
固体物理, 54(12), p.757 - 766, 2019/12
MnSiと同じ空間群に属する4電子系化合物EuPtSiについて、磁気特性を調べた。単結晶中性子回折実験の結果、MnSiとEuPtSiの磁気構造に多くの共通点を見出した。この結果は、EuPtSiが4電子系で初めて磁気スキルミオン格子を示す物質であることを示している。
concentration大谷 恭平; Islam, M. S.*; 坂入 正敏*; 兼子 彬*
Surface and Interface Analysis, 51(12), p.1207 - 1213, 2019/12
被引用回数：1 パーセンタイル：2.04(Chemistry, Physical)異なる亜鉛イオン濃度の模擬淡水中でA3003アルミニウム合金に形成した腐食生成物の形態および組成をオージェ電子分光分析装置(AES)により明らかにした。試料断面の観察より、浸漬した模擬淡水の亜鉛イオン濃度が増加するほどA3003に形成した腐食生成物の厚さは減少することがわかった。試料断面の分析より、溶液中の亜鉛イオン濃度が0.1mMを超えると腐食生成物は多層構造になり、内側の亜鉛の豊富な層は高耐食性を有することが示唆された。
magnetic order in trillium lattice antiferromagnet EuPtSi studied by resonant X-ray scattering田端 千紘*; 松村 武*; 中尾 裕則*; 道村 真司*; 垣花 将司*; 稲見 俊哉*; 金子 耕士; 辺土 正人*; 仲間 隆男*; 大貫 惇睦*
Journal of the Physical Society of Japan, 88(9), p.093704_1 - 093704_5, 2019/09
被引用回数：34 パーセンタイル：88.7(Physics, Multidisciplinary)The magnetic order in the magnetic-fild-induced so-called A phase of cubic chiral antiferromagnet EuPtSi was investigated by resonant X-ray scattering (RXS) near the Eu 
edge. The high flux RXS signal under the magnetic field applied along [111] revealed the first and second order satellite magnetic reflections, indicating that the A phase is a triple- magnetic ordered state that is described by three propagation vectors lying in the plane normal to the magnetic field direction; 
, 
, and 
. With the high resolution in the reciprocal space achieved in the RXS measurement, it is suggested that the triple- order strongly couples with the underlying crystal lattice. The triple- magnetic order is discussed in the context of a magnetic skyrmion lattice on which the geometrical frustration may play a crucial role.
金子 耕士; Frontzek, M. D.*; 松田 雅昌*; 中尾 朗子*; 宗像 孝司*; 大原 高志; 垣花 将司*; 芳賀 芳範; 辺土 正人*; 仲間 隆男*; et al.
Journal of the Physical Society of Japan, 88, p.013702_1 - 013702_5, 2019/01
被引用回数：60 パーセンタイル：95.02(Physics, Multidisciplinary)Magnetic transitions in chiral antiferromagnet EuPtSi were investigated by means of single crystal neutron diffraction. In the ground state, magnetic peaks emerge at positions represented by 
=
. Upon heating, an additional magnetic peak splitting around 2.5 K was uncovered, indicating a presence of a first-order transition with 
=
. An half-polarized neutron scattering for polarization parallel to Q reveled that polarization antiparallel to Q has stronger intensity in both magnetic phases. This feature clarifies single chiral character of helical structure with moments normal to the ordering vector in both ordered states. Under vertical magnetic field along [1,1,1] in the 
phase, magnetic peaks form hexagonal patterns in the equatorial scattering plane around nuclear. An ordering vector 
of the -phase has the similar size in the periodicity to , and could be a hallmark of a formation of skyrmion lattice in EuPtSi.
studied by single-crystal time-of-flight neutron diffraction川崎 卓郎; 金子 耕士; 仲村 愛*; 阿曽 尚文*; 辺土 正人*; 仲間 隆男*; 大原 高志; 鬼柳 亮嗣; 及川 健一; 田村 格良; et al.
Journal of the Physical Society of Japan, 85(11), p.114711_1 - 114711_5, 2016/11
被引用回数：13 パーセンタイル：60.51(Physics, Multidisciplinary)The magnetic structure of the intermetallic compound EuGa was investigated using single-crystal neutron diffraction with TOF Laue technique on the new diffractometer SENJU at MLF of J-PARC. Despite of the high neutron absorption of Eu, a vast number of diffraction spots were observed without isotope enrichment. The magnetic reflections appeared at 
2
below 16 K, indicating that the ordering vector is = (0, 0, 0). The continuous evolution of the magnetic reflection intensity below T
follows a squared Brillouin function for 
= 7/2. By adopting a wavelength-dependent absorption collection, the magnetic structure of EuGa revealed that a nearly full magnetic moment of 6.4 B of Eu lies within the basal plane of the lattice.
大原 高志; 鬼柳 亮嗣; 及川 健一; 金子 耕士; 川崎 卓郎; 田村 格良; 中尾 朗子*; 花島 隆泰*; 宗像 孝司*; 茂吉 武人*; et al.
Journal of Applied Crystallography, 49(1), p.120 - 127, 2016/02
被引用回数：51 パーセンタイル：95.86(Chemistry, Multidisciplinary)SENJU, a time-of-flight Laue-type single-crystal neutron diffractometer, was developed at the Materials and Life Science Experimental Facility (MLF) of the Japan Accelerator Research Complex (J-PARC). Molecular structure analysis of a sub-millimeter taurine crystal and magnetic structure analysis of a MnF
crystal were performed to evaluate its performance.
川崎 卓郎; 金子 耕士; 阿曽 尚文*; 仲村 愛*; 辺土 正人*; 仲間 隆男*; 大貫 惇睦*; 大原 高志; 鬼柳 亮嗣; 及川 健一; et al.
JPS Conference Proceedings (Internet), 1, p.014009_1 - 014009_4, 2014/03
Single crystal neutron diffraction measurement of EuGa has been carried out using time-of-flight single crystal neutron diffractometer SENJU at BL18 in MLF/J-PARC. In spite of extremely high neutron absorption of natural Eu, significant numbers of Bragg reflection were observed. Lattice parameters and Bravais lattice at above 
(=15 K) obtained from the positions and systematic extinction of the reflections were well agreed with the result of single crystal X-ray diffraction. Further, magnetic reflections were clearly observed at below at the positions of forbidden reflections of body-centered lattice of EuGa. An antiferromagnetic structure with the propagation vector = 0 was clarified.
武田 全康; 山崎 大; 曽山 和彦; 丸山 龍治; 林田 洋寿; 朝岡 秀人; 山崎 竜也; 久保田 正人; 相澤 一也; 新井 正敏; et al.
Chinese Journal of Physics, 50(2), p.161 - 170, 2012/04
The construction of a new polarized neutron reflectometer is now in progress at the Materials and Life Science Experimental Facility (MLF) of the Japan Proton Accelerator Research Complex (J-PARC). MLF has the world's brightest pulsed neutron and muon sources (JSNS and MUSE). The user program of MLF has been already started in 2008, and now nine neutron and two muon spectrometers are in operation. Installation of the new reflectometer was expected to be completed in March 2011. However, the construction was interrupted by the massive earthquake hitting northeast Japan, including Tokai-mura where J-PARC is located. We expect to restart the user program of the new polarized neutron reflectometer at the beginning of next year (2012).
田村 格良; 及川 健一; 川崎 卓郎; 大原 高志; 金子 耕士; 鬼柳 亮嗣; 木村 宏之*; 高橋 美和子; 清谷 多美子*; 新井 正敏; et al.
Journal of Physics; Conference Series, 340, p.012040_1 - 012040_4, 2012/02
被引用回数：10 パーセンタイル：93.64(Physics, Condensed Matter)SENJU is a state-of-the-art single crystal time-of-flight Laue diffractometer in Materials and Life Science Experimental Facility at Japan Proton Accelerator Research Complex (J-PARC). The diffractometer is designed for precise crystal and magnetic structure analyses under multiple extreme conditions, such as low temperature, high-pressure, high-magnetic field. A measurement using small sample less than 1.0 mm
will be also realized, which allows us to study wide variety of materials. SENJU is aimed at a poisoned decoupled moderator to obtain peak profiles of Bragg reflection, and intensity distributions of superlattice reflections and diffuse scatterings with good accuracy. At the beginning, the diffractometer will have 31 two-dimensional scintillator detectors to cover wide area of reciprocal lattice space by a single measurement. The instrument is currently under construction and is scheduled to start on-beam commissioning by the end of 2011.
益田 隆嗣*; 萩原 雅人*; 近藤 洋右*; 金子 耕士; 目時 直人
Journal of the Physical Society of Japan, 80(11), p.113705_1 - 113705_4, 2011/11
被引用回数：36 パーセンタイル：81.82(Physics, Multidisciplinary)フラストレート系化合物LiCuVOの磁場誘起秩序相を中性子散乱によって研究し、臨界磁場8.5T以上で、量子揺らぎ,幾何学的なフラストレーション、そしてチェーン間相互作用の拮抗によって安定化した新しい磁場誘起スピン密度状態の長距離秩序相を発見したので報告する。
quasiparticle states in 
Cm by in-beam 
-ray spectroscopy using heavy-ion transfer reactions石井 哲朗; 牧井 宏之*; 浅井 雅人; 塚田 和明; 豊嶋 厚史; 松田 誠; 牧嶋 章泰*; 重松 宗一郎*; 金子 順一*; 静間 俊行; et al.
Physical Review C, 78(5), p.054309_1 - 054309_11, 2008/11
被引用回数：14 パーセンタイル：64.91(Physics, Nuclear)We have measured deexcitation rays in Cm populated by one-neutron stripping reactions with a 
Cm target and a 162 MeV 
O, a 162 MeV 
O, and a 120 MeV 
C beams. rays in Cm were identified by measuring kinetic energies of outgoing particles using Si 
-
detectors. It was demonstrated that high- orbitals were selectively populated in the (O,
O) reaction having a large negative 
value. We have observed eight quasi-particle states above the deformed shell gap of 
. The 1/2
[620], 1/2
[750], and 7/2[613] bands were extended up to 19/2, 19/2, and 13/2 states, respectively. We have established the 9/2 9/2[615] state at 526 keV, the 9/2 9/2[604] state with a short life of 
ps at 1030 keV, and the 11/2 11/2[725] state with 
ns at 375 keV. Furthermore, the 17/2 1/2[880] state, having a large component of the 
spherical single-particle state, has been identified at 1505 keV. We discuss the properties of those quasi-particle states in the framework of a deformed shell model.
-ray spectroscopy of neutron-rich nuclei in the uranium region through the heavy-ion transfer reaction石井 哲朗; 牧井 宏之; 浅井 雅人; 小浦 寛之; 重松 宗一郎*; 塚田 和明; 豊嶋 厚史; 松田 誠; 牧嶋 章泰*; 静間 俊行; et al.
Nuclear Physics A, 805(1-4), p.257 - 259, 2008/06
中性子過剰核
Th, 
U, 
Pu, 
Cmの脱励起線を初めて測定し、それぞれ10, 12, 8, 12, 12状態までの回転バンドを確立した。さらに
Uでは、9状態までの八重極振動バンドを観測した。これらの原子核は、
U, 
Pu, Cm標的とOビームとの(O, O)及び(O, 
Ne)2核子移行反応により生成した。Si-検出器を用いて散乱粒子O及びNeの運動エネルギーを選択することにより、残留核の線を同定した。回転バンドの慣性能率及び中性子軌道のエネルギー準位の系統性より、中性子数152の変形閉殻が、陽子数96以上では存在するが陽子数94のPuでは消失することを明らかにした。また第1励起エネルギーの中性子数依存性より、中性子数164が球形閉殻になる可能性を示唆した。
