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Toigawa, Tomohiro; Hotoku, Shinobu; Kumagai, Yuta; Abe, Yuma*; Oyama, Kanichi*; Fukaya, Hiroyuki; Tsubata, Yasuhiro; Ban, Yasutoshi; Kida, Takashi; Hasegawa, Satoshi*; et al.
Journal of Nuclear Science and Technology, 63(8), p.969 - 975, 2026/08
Times Cited Count：0 Percentile：0.00(Nuclear Science & Technology)The effect of temperature on hydrogen generated from radiolysis was investigated to determine the safety implications in nuclear fuel reprocessing. Radiolytic hydrogen production poses a risk due to its flammability, especially when it accumulates in confined spaces without ventilation. Herein, generation of radiolytic hydrogen from an actual nuclear fuel-derived solution is investigated. Compared to previous studies using a plutonium nitric acid solution, this study evaluates radiolytic hydrogen yield under more realistic conditions, reflecting post-irradiation fuel composition. G-values of H
are determined at multiple temperatures, and the impact of alpha, beta, and gamma radiation doses is evaluated using PHITS-based simulations. Findings from this study confirmed a reduction in hydrogen yield due to scavenging effects of high-concentration nitric acid and metal ions dissolved in the solution, and temperature dependence appeared to be minor. A weak decreasing trend of G-values with temperature under agitated conditions might be related to hydrogen consumption by palladium species.
Toigawa, Tomohiro; Hotoku, Shinobu; Kumagai, Yuta; Abe, Yuma*; Oyama, Kanichi*; Fukaya, Hiroyuki; Ban, Yasutoshi; Kida, Takashi; Hasegawa, Satoshi*; Nakano, Masanao*; et al.
Journal of Nuclear Science and Technology, 63(3), p.322 - 327, 2026/03
Times Cited Count：1 Percentile：46.18(Nuclear Science & Technology)The effect of temperature on hydrogen production generated from radiolysis was investigated to determine the associated implications for nuclear fuel reprocessing safety. The hydrogen yield from radiolysis of plutonium nitric acid solution was measured at temperatures up to the boiling temperature of the solution. The results showed no notable temperature dependence even under boiling conditions. The impact of solution agitation on hydrogen production was also assessed, which revealed minor differences in the hydrogen yield between static and agitated conditions at room temperature. These findings suggest that high temperatures or boiling the solution do not considerably enhance hydrogen generation, and provide crucial information for accurately modeling hydrogen risks under severe accidents.
Fuwa, Yasuhiro; Mizobata, Satoshi*; Nakano, Hideto; Shinozaki, Shinichi; Takayanagi, Tomohiro; Asano, Hiroyuki; Iwama, Yuhei*
Proceedings of 22nd Annual Meeting of Particle Accelerator Society of Japan (Internet), p.389 - 391, 2026/03
no abstracts in English
Kondo, Yasuhiro; Chimura, Motoki; Cicek, E.*; Fukui, Yuji*; Futatsukawa, Kenta*; Fuwa, Yasuhiro; Goto, Rikuto*; Hirano, Koichiro; Ishikawa, Masaki*; Ito, Takashi; et al.
Proceedings of 22nd Annual Meeting of Particle Accelerator Society of Japan (Internet), p.124 - 129, 2026/03
Various upgrade plans of the J-PARC linac are underway, and repetition-rate doubling project is one of the most important part. Currently, the linac supplies a 400~MeV H
ion beam to the 3~GeV synchrotron (RCS) at a repetition rate of 25~Hz. However, to deliver the beam to both RCS and proton-beam irradiation facility under planning, it is necessary to raise the repetition rate from 25~Hz to 50~Hz. Prior to construction of the beamline to the irradiation facility, we conducted a verification of the 50~Hz operation of all the linac apparatus simultaneously within the current operational limits in May 2025. And also, the verification of the 50~Hz operation of the particle counter system, which is one of the most important safety device of the J-PARC accelerator, was conducted. As a result, any significant problems were not found out, and it is now ready for the upcoming 50~Hz-beam acceleration demonstration. This paper describes this details of the demonstration of the 50~Hz operation, without beam acceleration, of the J-PARC linac.
Hanasaki, Noriaki*; Hattori, Takayuki*; Komoda, Takumi*; Minamoto, Kakuei*; Torigoe, Shuhei*; Yamashita, Satoshi*; Nakazawa, Yasuhiro*; Nakano, Takehito*; Yoshimi, Kohei*; Yashima, Mitsuharu*; et al.
Proceedings of the National Academy of Sciences of the United States of America, 123(1), p.e2517926123_1 - e2517926123_6, 2026/01
Times Cited Count：1 Percentile：80.48(Multidisciplinary Sciences)Liu, Y.*; Otani, Masashi*; Miyao, Tomoaki*; Nakazawa, Yuga*; Shibata, Takanori*; Nammo, Kesao*; Fang, Z.*; Futatsukawa, Kenta*; Fukui, Yuji*; Mizobata, Satoshi*; et al.
Proceedings of 16th International Particle Accelerator Conference (IPAC25) (Internet), p.855 - 857, 2025/11
Nakano, Hideto; Mizobata, Satoshi*; Futatsukawa, Kenta*; Fuwa, Yasuhiro; Fang, Z.*; Fukui, Yuji*; Sato, Yoshikatsu*; Cicek, E.*; Kitamura, Ryo
Journal of Physics; Conference Series, 3094(1), p.012049_1 - 012049_6, 2025/09
Nakamura, Satoshi; Ishii, Sho*; Kato, Hitoshi*; Ban, Yasutoshi; Hiruta, Kenta; Yoshida, Takuya; Uehara, Hiroyuki; Obata, Hiroki; Kimura, Yasuhiko; Takano, Masahide
Journal of Nuclear Science and Technology, 62(1), p.56 - 64, 2025/01
Times Cited Count：1 Percentile：19.36(Nuclear Science & Technology)A dissolution method for analyzing the elemental composition of fuel debris using the sodium peroxide (NaO) fusion technique has been developed. Herein, two different types of simulated debris materials (such as solid solution of (Zr,RE)O and molten core-concrete interaction products (MCCI)) were taken. At various temperatures, these debris materials were subsequently fused with NaO in crucibles, which are made of different materials, such as Ni, AlO
, Fe, and Zr. Then, the fused samples are dissolved in nitric acid. Furthermore, the effects of the experimental conditions on the elemental composition analysis were evaluated using inductively coupled plasma-atomic emission spectroscopy (ICP-AES), which suggested the use of a Ni crucible at 923 K as an optimum testing condition. The optimum testing condition was then applied to the demonstration tests with Three Mile Island unit-2 (TMI-2) debris in a shielded concrete cell, thereby achieving complete dissolution of the debris. The elemental composition of TMI-2 debris revealed by the proposed dissolution method has good reproducibility and has an insignificant contradiction in the mass balance of the sample. Therefore, this newly developed reproducible dissolution method can be effectively utilized in practical applications by dissolving fuel debris and estimating its elemental composition.
He, X.*; Kagi, Hiroyuki*; Komatsu, Kazuki*; Sano, Asami; Abe, Jun*; Fukuyama, Ko*; Shimmei, Toru*; Nakano, Satoshi*
Inorganic Chemistry, 63(47), p.22349 - 22360, 2024/11
Times Cited Count：4 Percentile：37.51(Chemistry, Inorganic & Nuclear)Brucite, Mg(OH), is a key material for studying hydrogen bonds in solid hydroxides. This study explored how fluorine (F) substitution affects hydrogen-bonding in hydrogenated and deuterated brucite under ambient and high-pressure conditions using neutron powder diffraction, Raman, and IR spectroscopy. At ambient conditions, F substitution shortened donor- acceptor distances and elongated hydroxyl bonds, strengthening hydrogen bonds, as evidenced by red shifts in hydroxyl stretching modes. High-pressure experiments showed that F doping suppressed pressure-induced hydrogen-bond strengthening, reducing changes in hydroxyl bond length, bond angle, and cone angle. Spectroscopic measurements confirmed that F substitution limits pressure-induced hydroxyl elongation.
revealed by inelastic X-ray and neutron scatteringKimura, Koji*; Tsutsui, Satoshi*; Yamamoto, Yuta*; Nakano, Akitoshi*; Kawamura, Keisuke*; Kajimoto, Ryoichi; Kamazawa, Kazuya*; Martin, A.*; Webber, K. G.*; Kakimoto, Kenichi*; et al.
Physical Review B, 110(13), p.134314_1 - 134314_10, 2024/10
Times Cited Count：4 Percentile：41.54(Materials Science, Multidisciplinary)Machida, Shinichi*; Hattori, Takanori; Nakano, Satoshi*; Sano, Asami; Funakoshi, Kenichi*; Abe, Jun*
Koatsuryoku No Kagaku To Gijutsu, 34(3), p.134 - 142, 2024/09
A diamond anvil cell (DAC) for high-pressure neutron diffraction experiments has been developed at the PLANET beamline, Materials and Life Science Experimental Facility, in J-PARC. The conically supported diamond anvils were used for high-pressure generation. We succeeded in obtaining the neutron data for D
O ice up to 69.4 GPa. In addition, the gasket materials suitable for the neutron diffraction measurements were investigated. 11 kinds of alloys were tested and SUS304, Inconel718 and M2052 (73Mn-20Cu-5Ni-2Fe, at%) alloys showed excellent performance. Especially, M2052 null-matrix alloy has proven to be useful for neutron diffraction experiments where the beam inevitably hits the gasket. We then obtained refinable neutron diffraction profiles in Rietveld analysis from DO ice at least up to 43.3 GPa.
He, X.*; Kagi, Hiroyuki*; Komatsu, Kazuki*; Iizuka, Riko*; Okajima, Hajime*; Hattori, Takanori; Sano, Asami; Machida, Shinichi*; Abe, Jun*; Goto, Hirotada*; et al.
Journal of Molecular Structure, 1310, p.138271_1 - 138271_8, 2024/08
Times Cited Count：0 Percentile：0.00(Chemistry, Physical)High-pressure responses of the O-D
F hydrogen bonds in deuterated magnesium hydroxyfluoride were investigated using neutron powder diffraction and Raman spectroscopy. The Rietveld analysis at ambient conditions revealed a chemical formula of Mg(OD)
F
and hydroxyl group/fluorine disorder (OD/F disorder) in the crystal structure, which gave rise to two hydrogen-bonding configurations. The Rietveld analysis showed the hydrogen-bonding geometries remains up to 9.8 GPa, indicating no pressure-induced strengthening of hydrogen bonds. The Raman spectra at ambient conditions showed three hydroxyl stretching bands at 2613, 2694, and 2718 cm
. The high frequencies of the O-D stretching modes indicated that the hydroxyls should be involved in weak or none hydrogen-bonding interactions. Up to 20.2 GPa, the mode initially centered at 2694 cm displayed a pressure-induced blue shift, revealing no strengthening of hydrogen bonds under compression. We discuss the existence of hydrogen bonds and the causes of the blue-shifting hydroxyls at ambient and at high pressures.
shetta lakes in the Soya Coast region and their paleoenvironmental significance with glacial isostatic adjustment in East AntarcticaInoue, Genki*; Honda, Eisuke*; Ito, Keisuke*; Kang, I.*; Seto, Koji*; Tani, Yukinori*; Watanabe, Takahiro; Kashima, Kaoru*; Otani, Shuji*; Yamanaka, Toshiro*; et al.
Quaternary Science Reviews, 338, p.108822_1 - 108822_18, 2024/08
Times Cited Count：0 Percentile：0.00(Geography, Physical)We studied Holocene paleolimnological changes inferred from biomarkers and microscopic observation of microalgae and cyanobacteria in sediment cores from Rundvshetta lakes (Maruwanminami-ike and Maruwan o-ike) in the Soya Coast of East Antarctica, along with sedimentary facies and radiocarbon dating. Coastal marine environment: Maruwanminami-ike (147-72.5 cm, 5,010-2,590 cal BP) and Maruwan-oike (226-47.2 cm, 5,700-3,190 cal BP) were characterized by low biological production with the predominance of diatoms. Transition period of stratified brackish lake environment: Maruwanminami-ike (72.5-65.6 cm, 2,590-2,500 cal BP) and Maruwan-oike (47.2-28.8 cm, 3,190-2,890 cal BP) were characterized by stratified conditions with marine water overlain by freshwater, and a chemocline developed together with an anoxic layer in the bottom of photic zone.
Miyazaki, Kanako*; Takehara, Masato*; Minomo, Kenta*; Horie, Kenji*; Takehara, Mami*; Yamasaki, Shinya*; Saito, Takumi*; Onuki, Toshihiko*; Takano, Masahide; Shiotsu, Hiroyuki; et al.
Journal of Hazardous Materials, 470(15), p.134104_1 - 134104_11, 2024/05
Times Cited Count：4 Percentile：34.74(Engineering, Environmental)Koyama, Shinichi; Ikeuchi, Hirotomo; Mitsugi, Takeshi; Maeda, Koji; Sasaki, Shinji; Onishi, Takashi; Tsai, T.-H.; Takano, Masahide; Fukaya, Hiroyuki; Nakamura, Satoshi; et al.
Hairo, Osensui, Shorisui Taisaku Jigyo Jimukyoku Homu Peji (Internet), 216 Pages, 2023/11
In FY 2021 and 2022, JAEA perfomed the subsidy program for "the Project of Decommissioning and Contaminated Water Management (Development of Analysis and Estimation Technology for Characterization of Fuel Debris (Development of Technologies for Enhanced Analysis Accuracy, Thermal Behavior Estimation, and Abbreviated Analysis))" started in FY 2021. This presentation material summarized the results of the project, which will be available shortly on the website of Management Office for the Project of Decommissioning, Contaminated Water and Treated Water Management.
Nakano, Hideto; Fuwa, Yasuhiro; Shinozaki, Shinichi; Mizobata, Satoshi*
Proceedings of 20th Annual Meeting of Particle Accelerator Society of Japan (Internet), p.577 - 578, 2023/11
In the J-PARC linac, klystrons are used as RF source. To improve the stability of RF power supply, the replacement of klystrons with semiconductor amplifiers is under consideration. Since the output of a semiconductor amplifier is relatively small, klystrons were installed in high power sections. Progresses of semiconductor production technology have allowed to manufacture semiconductor amplifiers that are expected be practical use. In the J-PARC linac, the installation in a debuncher 2 cavity with relatively small output power is planed. Characteristics test of a prototype semiconductor amplifier were conducted before full scale installation.
OKondo, Yosuke*; Achouri, N. L.*; Al Falou, H.*; Atar, L.*; Aumann, T.*; Baba, Hidetada*; Boretzky, K.*; Caesar, C.*; Calvet, D.*; Chae, H.*; et al.
Nature, 620(7976), p.965 - 970, 2023/08
Times Cited Count：55 Percentile：95.68(Multidisciplinary Sciences)no abstracts in English
Ne at the transition into the island of inversion; Detailed structure study of NeWang, H.*; Yasuda, Masahiro*; Kondo, Yosuke*; Nakamura, Takashi*; Tostevin, J. A.*; Ogata, Kazuyuki*; Otsuka, Takaharu*; Poves, A.*; Shimizu, Noritaka*; Yoshida, Kazuki; et al.
Physics Letters B, 843, p.138038_1 - 138038_9, 2023/08
Times Cited Count：8 Percentile：73.64(Astronomy & Astrophysics)Detailed 
-ray spectroscopy of the exotic neon isotope Ne has been performed using the one-neutron removal reaction from Ne. Based on an analysis of parallel momentum distributions, a level scheme with spin-parity assignments has been constructed for Ne and the negative-parity states are identified for the first time. The measured partial cross sections and momentum distributions reveal a significant intruder p-wave strength providing evidence of the breakdown of the N = 20 and N = 28 shell gaps. Only a weak, possible f-wave strength was observed to bound final states. Large-scale shell-model calculations with different effective interactions do not reproduce the large p-wave and small f-wave strength observed experimentally, indicating an ongoing challenge for a complete theoretical description of the transition into the island of inversion along the Ne isotopic chain.
Onuki, Toshihiko*; Ye, J.*; Kato, Tomoaki; Liu, J.; Takano, Masahide; Kozai, Naofumi; Utsunomiya, Satoshi*
Environmental Science; Processes & Impacts, 25(7), p.1204 - 1212, 2023/07
Times Cited Count：2 Percentile：11.36(Chemistry, Analytical)To elucidate chemical forms of Cs and I in microparticles produced via the Fukushima Daiichi Nuclear Power Plant accident and released into the atmosphere, we analyzed Cs and I in condensed vaporized particles (CVP) produced by melting experiments using nuclear fuel components containing CsI with concrete. CVPs consisted of many round particles containing Cs and I of diameters less than several tens of micrometers. Two kinds of particles were present: one containing large amounts of Cs and I, suggesting the presence of CsI, and the other containing small amounts of Cs and I with large Si contents. Most of CsI from both particles were dissolved in water. On the contrary, some fractions of Cs remained from the latter particles. These results suggest that Cs was incorporated in CVPs along with Si to form water low-soluble CVPs
Ikeuchi, Hirotomo; Koyama, Shinichi; Osaka, Masahiko; Takano, Masahide; Nakamura, Satoshi; Onozawa, Atsushi; Sasaki, Shinji; Onishi, Takashi; Maeda, Koji; Kirishima, Akira*; et al.
JAEA-Technology 2022-021, 224 Pages, 2022/10
JAEA-Technology-2022-021.pdf:12.32MB
A set of technology, including acid dissolving, has to be established for the analysis of content of elements/nuclides in the fuel debris samples. In this project, a blind test was performed for the purpose of clarifying the current level of analytical accuracy and establishing the alternative methods in case that the insoluble residue remains. Overall composition of the simulated fuel debris (homogenized powder having a specific composition) were quantitatively determined in the four analytical institutions in Japan by using their own dissolving and analytical techniques. The merit and drawback for each technique were then evaluated, based on which a tentative flow of the analyses of fuel debris was constructed.
