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Journal Articles

Spin-orbital short-range order on a honeycomb-based lattice

Nakatsuji, Satoru*; Kuga, Kentaro*; Kimura, Kenta*; Satake, Ryuta*; Katayama, Naoyuki*; Nishibori, Eiji*; Sawa, Hiroshi*; Ishii, Rieko*; Hagiwara, Masayuki*; Bridges, F.*; et al.

Science, 336(6081), p.559 - 563, 2012/05

 Times Cited Count:114 Percentile:95.24(Multidisciplinary Sciences)

Frustrated magnetic materials can remain disordered to the lowest temperatures. Such is the case for Ba$$_3$$CuSb$$_2$$O$$_9$$, which is magnetically anisotropic at the atomic scale but curiously isotropic on mesoscopic length and time scales. We find that the frustration on the triangular lattice is imprinted in a nanostructured honeycomb lattice of Cu$$^{2+}$$ ions that resists a coherent static Jahn-Teller distortion. The resulting two-dimensional random-bond spin-1/2 system on the honeycomb lattice has a broad spectrum of spin-dimer like excitations and low-energy spin degrees of freedom that retain.

Journal Articles

Investigation of bulk superconductivity in PrPt$$_5$$

Ito, Takashi; Nishida, Nobuhiko*; Oishi, Kazuki; Higemoto, Wataru; Karaki, Yoshitomo*; Ishimoto, Hidehiko*

Journal of the Physical Society of Japan, 75(Suppl.), p.189 - 191, 2006/08

no abstracts in English

Oral presentation

Hyperfine-enhanced nuclear magnetism in $$^{141}$$Pr-based compounds observed by muon spin relaxation

Ito, Takashi; Higemoto, Wataru; Oishi, Kazuki; Nishida, Nobuhiko*; Karaki, Yoshitomo*; Ishimoto, Hidehiko*

no journal, , 

Several novel phenomena about higher order multipoles have recently been found in $$^{141}$$Pr-based compounds with a nonmagnetic crystalline-electric-field (CEF) ground state. Previous $$mu$$SR studies in such compounds reported an anomalous muon spin relaxation at low temperatures in spite of the CEF ground state with the nonmagnetic nature, and a hyperfine-enhanced nuclear magnetism was discussed as the origin. A Van-Vleck paramagnet PrPt$$_5$$ is a typical system of the enhanced nuclear magnetism, which exhibits a ferromagnetic nuclear ordering at $$T_c$$=1.7 mK. This compound has been well characterized and is an ideal system to clarify a relation between the enhanced nuclear magnetism and the anomalous muon spin relaxation in $$^{141}$$Pr-based compounds. We performed $$mu$$SR measurements down to 50 mK. An internal field observed at the muon site is much larger in magnitude than ones due to bare nuclear dipole moments, suggesting an induction of 4$$f$$ magnetic moments. A fluctuation rate $$nu$$ of the field was estimated in the order of a few MHz and the value for $$nu$$ is consistent with one estimated from $$T_c$$. Our observations demonstrate that the $$mu$$SR is an ideal tool to investigate the dynamics of the hyperfine-enhanced nuclear spins in $$f$$ electron systems.

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