Initialising ...
Initialising ...
Initialising ...
Initialising ...
Initialising ...
Initialising ...
Initialising ...
molecule generation from dissociatively adsorbed water on TiO
through photoexcitationKato, Koichi*; Nagatsuka, Naoki*; Fukutani, Katsuyuki
Journal of Physical Chemistry C, 128(20), p.8188 - 8198, 2024/05
Times Cited Count:2 Percentile:19.40(Chemistry, Physical)Kato, Atsushi; Yamamoto, Tomohiko; Ando, Masato; Chikazawa, Yoshitaka; Murakami, Hisatomo*; Oyama, Kazuhiro*; Kaneko, Fumiaki*; Higurashi, Koichi*; Chanteclair, F.*; Chenaud, M.-S.*; et al.
EPJ Nuclear Sciences & Technologies (Internet), 8, p.11_1 - 11_10, 2022/06
This paper provides an overview of plant system studies to establish a common technical view for Sodium-cooled Fast Reactor concept between France and Japan based on ASTRID600 and the new concept with downsized output called ASTRID150. One of important issues on a reactor structure design is to enhance seismic resistance to be tolerable against strong earthquake such that postulated in Japan. A concept of High Frequency Design is shared, and the design options related to HFD have been examined and design recommendations are established. In addition, this paper include results of studies for a steam generator, a decay heat removal system, a fuel handling system and a containment vessel.
-ironHirayama, Shintaro*; Sato, Koichi*; Kato, Daiji*; Iwakiri, Hirotomo*; Yamaguchi, Masatake; Watanabe, Yoshiyuki*; Nozawa, Takashi*
Nuclear Materials and Energy (Internet), 31, p.101179_1 - 101179_9, 2022/06
Times Cited Count:9 Percentile:72.04(Nuclear Science & Technology)no abstracts in English
X raysOkumura, Takuma*; Azuma, Toshiyuki*; Bennet, D. A.*; Caradonna, P.*; Chiu, I. H.*; Doriese, W. B.*; Durkin, M. S.*; Fowler, J. W.*; Gard, J. D.*; Hashimoto, Tadashi; et al.
Physical Review Letters, 127(5), p.053001_1 - 053001_7, 2021/07
Times Cited Count:20 Percentile:77.04(Physics, Multidisciplinary)We observed electronic
X rays emitted from muonic iron atoms using a superconducting transition-edge-type sensor microcalorimeter. The energy resolution of 5.2 eV in FWHM allowed us to observe the asymmetric broad profile of the electronic characteristic 
and 
X rays together with the hypersatellite 
X rays around 6 keV. This signature reflects the time-dependent screening of the nuclear charge by the negative muon and the
-shell electrons, accompanied by electron side-feeding. Assisted by a simulation, this data clearly reveals the electronic
- and
-shell hole production and their temporal evolution during the muon cascade process.
Segawa, Tomoomi; Kawaguchi, Koichi; Ishii, Katsunori; Suzuki, Masahiro; Tachihara, Joji; Takato, Kiyoto; Okita, Takatoshi; Satone, Hiroshi*; Suzuki, Michitaka*
Mechanical Engineering Journal (Internet), 8(3), p.21-00022_1 - 21-00022_9, 2021/06
To reduce the hold-up of the nuclear fuel materials in the glove box and the external exposure dose, the technology of the MOX powder adhesion prevention by the nanoparticle coating to the acrylic panels of the glove box has been developed. The surface analysis by means of atomic force microscopy (AFM) showed that the acrylic test piece surface coated with nanoparticles had a higher root mean square roughness value than that non-coated with nanoparticles. Due to the formation of nano-sized tiny rugged surface, the nanoparticle coating reduced the minimum adhesion force between the UO
particles and the acrylic test piece surface with the smallest particle size of about 5
m where desorption was observed, by about one-tenth. Moreover, the nanoparticle coating reduced the amount of the MOX powder adhering to the acrylic test piece to about one-tenth. In this study, it was found that applying the nanoparticle coating to the acrylic panels of glove box can prevent the adhesion of nuclear fuel materials. This method is effective for reducing the hold-up of the nuclear fuel materials in the glove box, the external exposure dose and improving the visibility of the acrylic panels.
Segawa, Tomoomi; Kawaguchi, Koichi; Ishii, Katsunori; Suzuki, Masahiro; Tachihara, Joji; Takato, Kiyoto; Okita, Takatoshi; Satone, Hiroshi*; Suzuki, Michitaka*
Proceedings of 2020 International Conference on Nuclear Engineering (ICONE 2020) (Internet), 6 Pages, 2020/08
To reduce the hold-up of the nuclear fuel materials in the glove box and the external exposure dose, the technology of the MOX powder adhesion prevention by the nanoparticle coating to the acrylic panels of the glove box has been developed. Due to the formation of nano-sized tiny rugged surface, the nanoparticle coating reduced the minimum adhesion force between the UO
particles and the acrylic test piece surface with the smallest particle size of about 5
m where desorption was observed, by about one-tenth. Moreover, the nanoparticle coating reduced the amount of the MOX powder adhering to the acrylic test piece to about one-tenth. In this study, it was found that applying the nanoparticle coating to the acrylic panels of glove box can prevent the adhesion of nuclear fuel materials. This method is effective for reducing the hold-up of the nuclear fuel materials in the glove box, the external exposure dose and improving the visibility of the acrylic panels.
Kondo, Yasuhiro; Hirano, Koichiro; Ito, Takashi; Kikuzawa, Nobuhiro; Kitamura, Ryo; Morishita, Takatoshi; Oguri, Hidetomo; Okoshi, Kiyonori; Shinozaki, Shinichi; Shinto, Katsuhiro; et al.
Journal of Physics; Conference Series, 1350, p.012077_1 - 012077_7, 2019/12
Times Cited Count:3 Percentile:76.63(Physics, Particles & Fields)We have upgraded a 3-MeV linac at J-PARC. The ion source is same as the J-PARC linac's, and the old 30-mA RFQ is replaced by a spare 50-mA RFQ, therefore, the beam energy is 3 MeV and the nominal beam current is 50 mA. The main purpose of this system is to test the spare RFQ, but also used for testing of various components required in order to keep the stable operation of the J-PARC accelerator. The accelerator has been already commissioned, and measurement programs have been started. In this paper, present status of this 3-MeV linac is presented.
Segawa, Tomoomi; Kawaguchi, Koichi; Kato, Yoshiyuki; Ishii, Katsunori; Suzuki, Masahiro; Fujita, Shunya*; Kobayashi, Shohei*; Abe, Yutaka*; Kaneko, Akiko*; Yuasa, Tomohisa*
Proceedings of 2019 International Congress on Advances in Nuclear Power Plants (ICAPP 2019) (Internet), 9 Pages, 2019/05
A solution of plutonium nitrate and uranyl nitrate is converted into a mixed oxide by microwave heating denitration method. In the present study, for improving the efficiency of microwave heating and achieving high-temperature uniformity to produce homogeneous UO
powder, the microwave heating test of potassium chloride and uranyl nitrate solution, and numerical simulation analysis were conducted. The potassium chloride agar was adjusted to the dielectric loss, which is close to that of the uranyl nitrate solution and the optimum support table height was estimated to be 50 mm for denitration of the uranyl nitrate solution by microwave heating. The adiabator improved the efficiency of microwave heating denitration. Moreover, the powder yield was improved by using the adiabator owing to ease of scraping of the denitration product from the bottom of the denitration vessel.
Kishi, Hirofumi*; Sakamoto, Tomokazu*; Asazawa, Koichiro*; Yamaguchi, Susumu*; Kato, Takeshi*; Zulevi, B.*; Serov, A.*; Artyushkova, K.*; Atanassov, P.*; Matsumura, Daiju; et al.
Nanomaterials (Internet), 8(12), p.965_1 - 965_13, 2018/12
Times Cited Count:15 Percentile:50.94(Chemistry, Multidisciplinary)Fujita, Shunya*; Abe, Yutaka*; Kaneko, Akiko*; Yuasa, Tomohisa*; Segawa, Tomoomi; Kato, Yoshiyuki; Kawaguchi, Koichi; Ishii, Katsunori
Proceedings of 11th Korea-Japan Symposium on Nuclear Thermal Hydraulics and Safety (NTHAS-11) (Internet), 7 Pages, 2018/11
Mixed uranium oxide and plutonium oxide powder is produced from uranyl nitrate and plutonium nitrate mixed solution by the microwave heating denitration method in the spent fuel reprocessing process. Since the microwave heating method is accompanied by a boiling phenomenon, it is necessary to fully grasp the operating conditions in order to avoid flashing and spilling in the mass production of denitrification technology for the future. In this research, it was clarified that the heat transfer coefficient became lower as the dielectric constant increased. The dominant factor of the blowing up phenomena is supposed to be generation of the innumerable bubble rather than bubble's growth.
Machida, Masahiko; Kato, Koichiro*; Shiga, Motoyuki
Journal of Chemical Physics, 148(10), p.102324_1 - 102324_11, 2018/03
Times Cited Count:28 Percentile:76.31(Chemistry, Physical)The isotopologs of liquid water, H
O, D
O, and T
O, are studied systematically by first principles PIMD simulations, in which the whole entity of the electrons and nuclei are treated quantum mechanically. The simulation results are in reasonable agreement with available experimental data on isotope effects, in particular, on the peak shift in the radial distributions of H
O and D
O and the shift in the evaporation energies. It is found that, due to differences in nuclear quantum effects, the H atoms in the OH bonds more easily access the dissociative region up to the hydrogen bond center than the D (T) atoms in the OD (OT) bonds. The accuracy and limitation in the use of the current density-functional-theory-based first principles PIMD simulations are also discussed. It is argued that the inclusion of the dispersion correction or relevant improvements in the density functionals are required for the quantitative estimation of isotope effects.
Kim, J.*; Yamanaka, Satoru*; Nakajima, Akira*; Kato, Takanori*; Kim, Y.*; Fukuda, Tatsuo; Yoshii, Kenji; Nishihata, Yasuo; Baba, Masaaki*; Takeda, Masatoshi*; et al.
Ferroelectrics, 512(1), p.92 - 99, 2017/08
Times Cited Count:15 Percentile:51.85(Materials Science, Multidisciplinary)Yamanaka, Satoru*; Kim, J.*; Nakajima, Akira*; Kato, Takanori*; Kim, Y.*; Fukuda, Tatsuo; Yoshii, Kenji; Nishihata, Yasuo; Baba, Masaaki*; Yamada, Noboru*; et al.
Advanced Sustainable Systems (Internet), 1(3-4), p.1600020_1 - 1600020_6, 2017/04
no abstracts in English
Sawabe, Yuki*; Ishiyama, Tatsuya; Takahashi, Daisuke; Kato, Yuko; Suzuki, Takahiro*; Hirano, Koichiro; Takei, Hayanori; Meigo, Shinichiro; Kikuzawa, Nobuhiro; Hayashi, Naoki
Proceedings of 13th Annual Meeting of Particle Accelerator Society of Japan (Internet), p.647 - 651, 2016/11
In the J-PARC, a 3 MeV linac has been developed for the tests of beam scraper irradiation and charge exchange by high-power laser. To accomplish tests efficiently and safely, the control system for 3 MeV was designed and developed, and this system consists of four subsystems, personal protection system, machine protection system, timing system, and remote control system using the EPICS. In this paper, the details of control system for a 3 MeV linac are presented.
Pirozhkov, A. S.; Kando, Masaki; Esirkepov, T. Z.; Faenov, A. Y.*; Pikuz, T. A.*; Kawachi, Tetsuya; Sagisaka, Akito; Koga, J. K.; Mori, Michiaki; Kawase, Keigo*; et al.
RAL-TR-2015-025, P. 22, 2015/00
Oguri, Hidetomo; Hasegawa, Kazuo; Ito, Takashi; Chishiro, Etsuji; Hirano, Koichiro; Morishita, Takatoshi; Shinozaki, Shinichi; Ao, Hiroyuki; Okoshi, Kiyonori; Kondo, Yasuhiro; et al.
Proceedings of 11th Annual Meeting of Particle Accelerator Society of Japan (Internet), p.389 - 393, 2014/10
no abstracts in English
Kawane, Yusuke*; Miura, Akihiko; Miyao, Tomoaki*; Hirano, Koichiro; Sugimura, Takashi*; Kato, Yuko; Sawabe, Yuki; Fukuda, Shimpei; Ouchi, Nobuo
Proceedings of 11th Annual Meeting of Particle Accelerator Society of Japan (Internet), p.1288 - 1291, 2014/10
In the J-PARC Linac, because an upgrading of a beam current up to 50mA using an RF-driven ion source and a new RFQ Linac cavity is in progress, we have developed a new frontend equipments. In order to protect the scraper against 50 mA, we need to observe the temperature and to avoid the excess heat loading of the scraper surface and to count the irradiated beam particles. We also monitor the beam transmission between the upstream and downstream of the chopper cavity to check the chopping errors using the beam current monitors. We fabricated the interlock system for the temperature, irradiated particle numbers and beam transmission. And we tested them in the test stand with actual beam. This paper describes the interlock system and their test results.
Arifi, E.*; Ishimatsu, Koichi*; Iizasa, Shinya*; Namihira, Takao*; Sakamoto, Hiroyuki*; Tachi, Yukio; Kato, Hiroyasu*; Shigeishi, Mitsuhiro*
Construction and Building Materials, 67(Part B), p.192 - 196, 2014/09
Times Cited Count:7 Percentile:28.21(Construction & Building Technology)The Fukushima Dai-ichi Nuclear Plant accident has resulted in a large amount of radioactively contaminated concrete. The possible application of the pulsed power discharge to reduce the amount of contaminated concrete as radioactive waste was investigated. The contaminated concrete was decontaminated by separating contaminated matrix from uncontaminated coarse aggregate under pulsed power discharge process. In this study, a stable Cs isotope was used to simulate radioactively contaminated concrete. As a result, while the volume of reclaimed aggregate from contaminated concrete could be reproduced was up to 60%, nevertheless Cs detected in the reclaimed aggregate was only approximately 3%. Thus most of the Cs were dissolved in water during the discharge process. It is expected that the pulsed power could reduce the contaminated concrete waste by reusing aggregate. Further investigations are requested to test the applicability of this method under the realistic conditions close to the actual waste.
Pirozhkov, A. S.; Kando, Masaki; Esirkepov, T. Z.; Gallegos, P.*; Ahmed, H.*; Ragozin, E. N.*; Faenov, A. Ya.*; Pikuz, T. A.*; Kawachi, Tetsuya; Sagisaka, Akito; et al.
New Journal of Physics (Internet), 16(9), p.093003_1 - 093003_30, 2014/09
Times Cited Count:31 Percentile:79.23(Physics, Multidisciplinary)Watahiki, Shunsuke; Hanakawa, Hiroki; Imaizumi, Tomomi; Nagata, Hiroshi; Ide, Hiroshi; Komukai, Bunsaku; Kimura, Nobuaki; Miyauchi, Masaru; Ito, Masayasu; Nishikata, Kaori; et al.
JAEA-Technology 2013-021, 43 Pages, 2013/07
The number of research reactors in the world is decreasing because of their aging. On the other hand, the necessity of research reactor, which is used for human resources development, progress of the science and technology, industrial use and safety research is increasing for the countries which are planning to introduce the nuclear power plants. From above background, the Neutron Irradiation and Testing Reactor Center began to discuss a basic concept of Multipurpose Compact Research Reactor (MCRR) for education and training, etc., on 2010 to 2012. This activity is also expected to contribute to design tool improvement and human resource development in the center. In 2011, design study of reactor core, irradiation facilities with high versatility and practicality, and hot laboratory equipment for the production of Mo-99 was carried out. As the result of design study of reactor core, subcriticality and operation time of the reactor in consideration of an irradiation capsule, and about the transient response of the reactor to the reactivity disturbance during automatic control operation, it was possible to do automatic operation of MCRR, was confirmed. As the result of design study of irradiation facilities, it was confirmed that the implementation of an efficient mass production radioisotope Mo-99 can be expected. As the result of design study with hot laboratory facilities, Mo-99 production, RI export devised considered cell and facilities for exporting the specimens quickly was designed.