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Moro, Takuya*; Kim, J.*; Yamanaka, Satoru*; Murayama, Ichiro*; Kato, Takanori*; Nakayama, Tadachika*; Takeda, Masatoshi*; Yamada, Noboru*; Nishihata, Yasuo; Fukuda, Tatsuo; et al.
Journal of Alloys and Compounds, 768, p.22 - 27, 2018/11
Times Cited Count:17 Percentile:66.2(Chemistry, Physical)Ishida, Takuya; Suzuki, Yoshitaka; Nishikata, Kaori; Yonekawa, Minoru; Kato, Yoshiaki; Shibata, Akira; Kimura, Akihiro; Matsui, Yoshinori; Tsuchiya, Kunihiko; Sano, Tadafumi*; et al.
KURRI Progress Report 2015, P. 64, 2016/08
no abstracts in English
Suzuki, Yumi*; Nakano, Hiroko; Suzuki, Yoshitaka; Ishida, Takuya; Shibata, Akira; Kato, Yoshiaki; Kawamata, Kazuo; Tsuchiya, Kunihiko
JAEA-Technology 2015-031, 58 Pages, 2015/11
Technetium-99m (Tc) is one of the most commonly used radioisotopes in the field of nuclear medicine. In the Japan Atomic Energy Agency (JAEA), the research and development (R&D) have been carried out for production of molybdenum-99 (Mo) by (n, ) method, a parent nuclide of Tc, with the Japan Material Testing Reactor (JMTR). On the other hand, the new project as "Domestic Production of Medical Radioisotope (Technetium preparation) in Japan" was adopted in the Tsukuba International Strategic Zone on October, 2013 and the demonstration tests will be planned for the domestic production of Mo/Tc with the JMTR. Thus, new facilities and analysis devices were equipped in the JMTR Hot Laboratory in 2014 as the part of this project. As the part of the analytical device equipment, the -TLC analyzer and the radiation detector connected with the High Performance Liquid Chromatography (HPLC) were installed for quality inspection of the Mo/Tc solution and the extracted Tc solution in the JMTR Hot Laboratory. The performance tests of these devices such as detection sensitivity, resolution, linearity and selectivity of energy range were carried out with Cs and Eu as alternative radionuclides of Mo and Tc, respectively. In the results, bright prospects were obtained concerning the quality inspection of the Mo/Tc and Tc solutions using these devices. This report describes the results of those performance tests.
Nishikata, Kaori; Ishida, Takuya; Yonekawa, Minoru; Kato, Yoshiaki; Kurosawa, Makoto; Kimura, Akihiro; Matsui, Yoshinori; Tsuchiya, Kunihiko; Sano, Tadafumi*; Fujihara, Yasuyuki*; et al.
KURRI Progress Report 2014, P. 109, 2015/07
As one of effective applications of the Japan Materials Testing Reactor (JMTR), JAEA has a plan to produce Mo by (n,) method ((n,)Mo production), a parent nuclide of Tc. In this study, preliminary irradiation test was carried out with the high-density molybdenum trioxide (MoO) pellets in the hydraulic conveyer (HYD) of the Kyoto University Research Reactor (KUR) and the Tc solution extracted from Mo was evaluated. After the irradiation test of the high-density MoO pellets in the KUR, Tc was extracted from the Mo solution and the recovery rate of Tc achieved the target values. The Tc solution also got the value that satisfied the standard value for Tc radiopharmaceutical products by the solvent extraction method.
Nishikata, Kaori; Ishida, Takuya; Yonekawa, Minoru; Kato, Yoshiaki; Kurosawa, Makoto; Kimura, Akihiro; Matsui, Yoshinori; Tsuchiya, Kunihiko; Sano, Tadafumi*; Fujihara, Yasuyuki*; et al.
KURRI Progress Report 2013, P. 242, 2014/10
As one of effective applications of the Japan Materials Testing Reactor (JMTR), JAEA has a plan to produce Mo-99 (Mo) by (n,) method ((n,)Mo production), a parent nuclide of Tc. In this study, preliminary irradiation tests were carried out with the high-density MoO pellets in the KUR and the Mo production amount was evaluated between the calculation results and measurement results.
Nakayama, Takuya; Suzuki, Shinji; Hanada, Keiji; Tomioka, Osamu; Sato, Junya; Irisawa, Keita; Kato, Jun; Kawato, Yoshimi; Meguro, Yoshihiro
Proceedings of 2nd International Symposium on Cement-based Materials for Nuclear Wastes (NUWCEM 2014) (CD-ROM), 12 Pages, 2014/06
Taguchi, Taketoshi; Yonekawa, Minoru; Kato, Yoshiaki; Kurosawa, Makoto; Nishikata, Kaori; Ishida, Takuya; Kawamata, Kazuo
UTNL-R-0483, p.10_5_1 - 10_5_13, 2013/03
JMTR focus on the activation method. By carrying out the preliminary tests using irradiation facilities existing, and verification tests using the irradiation facility that has developed in the cutting-edge research and development strategic strengthening business, as irradiation tests towards the production of Mo, we have been conducting research and development that can contribute to supply about 25% for Mo demand in Japan and the stable supply of radiopharmaceutical. This report describes a summary of the status of the preliminary tests for the production of Mo: Maintenance of test equipment in the facility in JMTR Hot Laboratory in preparation for research and development for the production of Mo in JMTR and using MoO pellet irradiated at Kyoto University Research Reactor Institute (KUR).
Faenov, A. Ya.*; Skobelev, I. Yu.*; Pikuz, T.; Pikuz, S. A.*; Fortov, V. E.*; Fukuda, Yuji; Hayashi, Yukio; Pirozhkov, A. S.; Kotaki, Hideyuki; Shimomura, Takuya; et al.
Laser and Particle Beams, 30(3), p.481 - 488, 2012/09
Times Cited Count:11 Percentile:43.57(Physics, Applied)Pikuz, T.; Faenov, A.*; Skobelev, I.*; Fortov, V. E.*; Boldarev, A.*; Gasilov, V.*; Chen, L. M.*; Zhang, L.*; Yan, W.*; Yuan, D.*; et al.
AIP Conference Proceedings 1465, p.181 - 201, 2012/07
Times Cited Count:0 Percentile:0.13(Physics, Applied)Colgan, J.*; Abdallah, J. Jr.*; Faenov, A. Ya.*; Pikuz, T. A.*; Skobelev, I. Yu.*; Fukuda, Yuji; Hayashi, Yukio; Pirozhkov, A. S.; Kawase, Keigo*; Shimomura, Takuya; et al.
High Energy Density Physics, 7(2), p.77 - 83, 2011/06
Times Cited Count:21 Percentile:65.79(Physics, Fluids & Plasmas)A study is made of the ultra-short laser pulse irradiation of Ar cluster targets. Experiments have been performed with large cluster sizes and using very high laser contrasts, which have allowed clear and unambiguous observation of exotic inner-shell transitions in near-neutral Ar ions. The interaction of the main laser pulse with the unperturbed target is a necessary requirement for observing these lines. Our measurements are supported by kinetics calculations in which a very detailed atomic model is used. The calculations predict all of the spectral features found experimentally, and support the notion that the X-ray emission arises from many ion stages of the Ar plasma, from near-neutral through He-like ions, and from a range of plasma temperatures and densities.
Kushida, Hiroaki*; Fukuda, Kodai*; Terai, Tomoyuki*; Fukuda, Takashi*; Kakeshita, Tomoyuki*; Oba, Takuya*; Osakabe, Toyotaka; Kakurai, Kazuhisa; Kato, Kenichi*
Journal of Physics; Conference Series, 165, p.012054_1 - 012054_4, 2009/06
Katsumura, Soichiro; Kitabata, Takuya; Irie, Tsutomu; Suzuki, Mitsutoshi; Hashimoto, Yu; Kato, Keiji*
Transactions of the American Nuclear Society, 99(1), P. 780, 2008/11
Kushida, Hiroaki*; Fukuda, Kodai*; Terai, Tomoyuki*; Fukuda, Takashi*; Kakeshita, Tomoyuki*; Oba, Takuya*; Osakabe, Toyotaka; Kakurai, Kazuhisa; Kato, Kenichi*
European Physical Journal; Special Topics, 158(1), p.87 - 92, 2008/05
Times Cited Count:22 Percentile:72.02(Physics, Multidisciplinary)Kato, Harukazu*; Tsuruta, Takuya*; Nishioka, Takashi*; Matsumura, Masahiro*; Sakai, Hironori; Kambe, Shinsaku
Journal of Physics and Chemistry of Solids, 68(11), p.2187 - 2190, 2007/11
Times Cited Count:8 Percentile:38.69(Chemistry, Multidisciplinary)Cu nuclear quadrupole resonance (NQR) studies have been carried out for CaCuRuO,which has been suggested to show a heavy-fermion-like behavioral though it possess no f electron. A Lorentzian shape of the Cu NQR line with a narrow width implies that no magnetic ordering appears, at least, down to 5 K. The spin-lattice relaxation rate of the Cu nuclei probes a change of the Cu 3 electron nature, resulting in the Fermi liquid state at a low temperature. These facts strongly support that the heavy fermion picture is available in the concerned compound.
Kato, Harukazu*; Tsuruta, Takuya*; Nishioka, Takashi*; Matsumura, Masahiro*; Sakai, Hironori; Kambe, Shinsaku
Journal of Magnetism and Magnetic Materials, 310(2, Part1), p.251 - 253, 2007/03
Cu NMR measurements have been carried out for CaCuRuO, which shows a heavy-fermion-like behavior although it posseses no f electron moment. The field-sweep spectrum observed can be understood as a powder pattern of a Cu nucleus affected by the quadrupole interaction with no axial symmetry. The quadrupole parameters and the Knight shift of Cu are evaluated.
Minato, Kazuo; Akabori, Mitsuo; Tsuboi, Takashi; Kurobane, Shiro; Hayashi, Hirokazu; Takano, Masahide; Otobe, Haruyoshi; Misumi, Masahiro*; Sakamoto, Takuya*; Kato, Isao*; et al.
JAERI-Tech 2005-059, 61 Pages, 2005/09
An experimental facility called the Module for TRU High Temperature Chemistry (TRU-HITEC) was installed in the Back-end Cycle Key Elements Research Facility (BECKY) of the Nuclear Fuel Cycle Safety Engineering Research Facility (NUCEF) for the basic studies of the behavior of the transuranium elements (TRU) in pyrochemical reprocessing and oxide fuels. TRU-HITEC consists of three alpha/gamma cells shielded by steel and polyethylene and a glove box shielded by leaded acrylic resin, where experimental apparatuses have been equipped and a high purity argon gas atmosphere is maintained. In the facility 10 g of Am as well as the other TRU of Np, Pu and Cm can be handled. This report summarizes the outline, structure, performance and interior apparatuses of the facility, and is the result of the joint research between the Japan Atomic Energy Research Institute and three electric power companies of Tokyo Electric Power Co., Tohoku Electric Power Co. and the Japan Atomic Power Co.
Yamamoto, Yoshihisa*; Togashi, Hideaki*; Kato, Atsushi*; Hasegawa, Satoshi*; Goto, Seiichi*; Nakano, Takuya*; Suemitsu, Maki*; Narita, Yuzuru*; Yoshigoe, Akitaka; Teraoka, Yuden
no journal, ,
We have investigated the initial oxidation process on an Si(110)-162 surface by real time synchrotron radiation photoemission spectroscopy (SR-XPS). As a result, a rapid initial oxidation regime was found to exist on this surface, which is not present on other crystal orientations. Analyses of the O1s spectra suggest insertion of oxygen atoms at the Si-Si bonds as the predominant process during initial oxidation. The rapid initial oxidation is accompanied by decrease of the Si2p subpeak that is related to Si(110)-162 reconstruction, indicating the preferential oxidation at the pentagon pair.
Togashi, Hideaki*; Yamamoto, Yoshihisa*; Goto, Seiichi*; Takahashi, Yuya*; Nakano, Takuya*; Kato, Atsushi*; Hasegawa, Satoshi*; Konno, Atsushi*; Suemitsu, Maki*; Asaoka, Hidehito; et al.
no journal, ,
no abstracts in English
Nakano, Takuya*; Hasegawa, Satoshi*; Togashi, Hideaki*; Kato, Atsushi*; Goto, Seiichi*; Teraoka, Yuden; Yoshigoe, Akitaka; Suemitsu, Maki*
no journal, ,
no abstracts in English
Yamamoto, Yoshihisa*; Togashi, Hideaki*; Kato, Atsushi*; Hasegawa, Satoshi*; Nakano, Takuya*; Goto, Seiichi*; Teraoka, Yuden; Yoshigoe, Akitaka; Suemitsu, Maki*
no journal, ,
In this study, we have investigated adsorption of oxygen molecules on Si(110)-162 clean surface at room temperature by synchrotron radiation photoemission spectros (SR-PES). The SR-PES experiments were conducted at the surface chemistry end-station of BL23SU in the SPring-8. The photon energy was 334 eV. Samples were B-doped p-type Si(110) wafers, and were flash-annealed in an UHV ambient prior to the exposure to oxygen gas at room temperature at the gas pressure of 6.710 Pa. By observing a structural change after a mild annealing, we have confirmed presence of a metastable state of oxidation on this RT-oxidized Si(110) surface.