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Journal Articles

R&D status of digital technology on inverse estimation of radioactive source distributions and related source countermeasures; Fast Digital Twin Tech. in Decommissioning Field: 3D-ADRES-Indoor FrontEnd

Machida, Masahiko; Yamada, Susumu; Kim, M.; Tanaka, Satoshi*; Tobita, Yasuhiro*; Iwata, Ayako*; Aoki, Yuto; Aoki, Kazuhisa; Yanagisawa, Kenichi*; Yamaguchi, Takashi; et al.

RIST News, (70), p.3 - 22, 2024/09

Inside the Fukushima Daiichi Nuclear Power Plant (1F), there are many locations with high radiation levels due to contamination by radioactive materials that leaked from the reactor. These pose a significant obstacle to the smooth progress of decommissioning work. To help solve this issue, the Japan Atomic Energy Agency (JAEA), under a subsidy from the Ministry of Economy, Trade, and Industry's decommissioning and contaminated water management project, is conducting research and development on digital technologies to improve the radiation environment inside the decommissioning site. This project, titled "Development of Technology to Improve the Environment Inside Reactor Buildings (Enhancing Digital Technology for Environment and Source Distribution to Reduce Radiation Exposure)," began in April of FY 2023. In this project, the aim is to develop three interconnected systems: FrontEnd, Pro, and BackEnd. The FrontEnd system, based on the previously developed 3D-ADRES-Indoor (prototype) from FY 2021-2022, will be upgraded to a high-speed digital twin technology usable on-site. The Pro system will carry out detailed analysis in rooms such as the new office building at 1F, while the BackEnd system will serve as a database to centrally manage the collected and analyzed data. This report focuses on the FrontEnd system, which will be used on-site. After point cloud measurement, the system will quickly create a 3D mesh model, estimate the radiation source from dose rate measurements, and refine the position and intensity of the estimated source using recalculation techniques (re-observation instructions and re-estimation). The results of verification tests conducted on Unit 5 are also presented. Furthermore, the report briefly discusses the future research and development plans for this project.

Journal Articles

Experimental visualization of water/ice phase distribution at cold start for practical-sized polymer electrolyte fuel cells

Higuchi, Yuki*; Yoshimune, Wataru*; Kato, Satoru*; Hibi, Shogo*; Setoyama, Daigo*; Isegawa, Kazuhisa*; Matsumoto, Yoshihiro*; Hayashida, Hirotoshi*; Nozaki, Hiroshi*; Harada, Masashi*; et al.

Communications Engineering (Internet), 3, p.33_1 - 33_7, 2024/02

Journal Articles

Development of time-series point cloud data changes and automatic structure recognition system using Unreal Engine

Kato, Toru*; Takahashi, Hiroki*; Yamashita, Meguru*; Doi, Akio*; Imabuchi, Takashi

Proceedings of 29th International Symposium on Artificial Life and Robotics (AROB 29th 2024) (Internet), p.1097 - 1100, 2024/01

Journal Articles

Development of a virtual 3D scanner for data augmentation in point cloud shape recognition

Takahashi, Hiroki*; Kato, Toru*; Yamashita, Meguru*; Doi, Akio*; Imabuchi, Takashi

Proceedings of 29th International Symposium on Artificial Life and Robotics (AROB 29th 2024) (Internet), p.1093 - 1096, 2024/01

Journal Articles

Development of time-series point cloud data changes and automatic structure recognition system using Unreal Engine

Kato, Toru*; Takahashi, Hiroki*; Yamashita, Meguru*; Doi, Akio*; Imabuchi, Takashi

Artificial Life and Robotics, 10 Pages, 2024/00

Journal Articles

3D water management in polymer electrolyte fuel cells toward fuel cell electric vehicles

Yoshimune, Wataru*; Higuchi, Yuki*; Kato, Akihiko*; Hibi, Shogo*; Yamaguchi, Satoshi*; Matsumoto, Yoshihiro*; Hayashida, Hirotoshi*; Nozaki, Hiroshi*; Shinohara, Takenao; Kato, Satoru*

ACS Energy Letters (Internet), 8(8), p.3485 - 3487, 2023/08

 Times Cited Count:11 Percentile:86.16(Chemistry, Physical)

Journal Articles

Design and actual performance of J-PARC 3 GeV rapid cycling synchrotron for high-intensity operation

Yamamoto, Kazami; Kinsho, Michikazu; Hayashi, Naoki; Saha, P. K.; Tamura, Fumihiko; Yamamoto, Masanobu; Tani, Norio; Takayanagi, Tomohiro; Kamiya, Junichiro; Shobuda, Yoshihiro; et al.

Journal of Nuclear Science and Technology, 59(9), p.1174 - 1205, 2022/09

 Times Cited Count:7 Percentile:80.72(Nuclear Science & Technology)

In the Japan Proton Accelerator Research Complex, the purpose of the 3 GeV rapid cycling synchrotron (RCS) is to accelerate a 1 MW, high-intensity proton beam. To achieve beam operation at a repetition rate of 25 Hz at high intensities, the RCS was elaborately designed. After starting the RCS operation, we carefully verified the validity of its design and made certain improvements to establish a reliable operation at higher power as possible. Consequently, we demonstrated beam operation at a high power, namely, 1 MW. We then summarized the design, actual performance, and improvements of the RCS to achieve a 1 MW beam.

Journal Articles

${it Operando}$ structure observation of pyroelectric ceramics during power generation cycle

Kawasaki, Takuro; Fukuda, Tatsuo; Yamanaka, Satoru*; Sakamoto, Tomokazu*; Murayama, Ichiro*; Kato, Takanori*; Baba, Masaaki*; Hashimoto, Hideki*; Harjo, S.; Aizawa, Kazuya; et al.

Journal of Applied Physics, 131(13), p.134103_1 - 134103_7, 2022/04

 Times Cited Count:1 Percentile:9.28(Physics, Applied)

Journal Articles

PSTEP: Project for solar-terrestrial environment prediction

Kusano, Kanya*; Ichimoto, Kiyoshi*; Ishii, Mamoru*; Miyoshi, Yoshizumi*; Yoden, Shigeo*; Akiyoshi, Hideharu*; Asai, Ayumi*; Ebihara, Yusuke*; Fujiwara, Hitoshi*; Goto, Tadanori*; et al.

Earth, Planets and Space (Internet), 73(1), p.159_1 - 159_29, 2021/12

 Times Cited Count:7 Percentile:44.49(Geosciences, Multidisciplinary)

The PSTEP is a nationwide research collaboration in Japan and was conducted from April 2015 to March 2020, supported by a Grant-in-Aid for Scientific Research on Innovative Areas from the Ministry of Education, Culture, Sports, Science and Technology of Japan. It has made a significant progress in space weather research and operational forecasts, publishing over 500 refereed journal papers and organizing four international symposiums, various workshops and seminars, and summer school for graduate students at Rikubetsu in 2017. This paper is a summary report of the PSTEP and describes the major research achievements it produced.

Journal Articles

Thermally altered subsurface material of asteroid (162173) Ryugu

Kitazato, Kohei*; Milliken, R. E.*; Iwata, Takahiro*; Abe, Masanao*; Otake, Makiko*; Matsuura, Shuji*; Takagi, Yasuhiko*; Nakamura, Tomoki*; Hiroi, Takahiro*; Matsuoka, Moe*; et al.

Nature Astronomy (Internet), 5(3), p.246 - 250, 2021/03

 Times Cited Count:51 Percentile:96.49(Astronomy & Astrophysics)

Here we report observations of Ryugu's subsurface material by the Near-Infrared Spectrometer (NIRS3) on the Hayabusa2 spacecraft. Reflectance spectra of excavated material exhibit a hydroxyl (OH) absorption feature that is slightly stronger and peak-shifted compared with that observed for the surface, indicating that space weathering and/or radiative heating have caused subtle spectral changes in the uppermost surface. However, the strength and shape of the OH feature still suggests that the subsurface material experienced heating above 300 $$^{circ}$$C, similar to the surface. In contrast, thermophysical modeling indicates that radiative heating does not increase the temperature above 200 $$^{circ}$$C at the estimated excavation depth of 1 m, even if the semimajor axis is reduced to 0.344 au. This supports the hypothesis that primary thermal alteration occurred due to radiogenic and/or impact heating on Ryugu's parent body.

Journal Articles

Complexation and bonding studies on [Ru(NO)(H$$_{2}$$O)$$_{5}$$]$$^{3+}$$ with nitrate ions by using density functional theory calculation

Kato, Akane*; Kaneko, Masashi; Nakashima, Satoru*

RSC Advances (Internet), 10(41), p.24434 - 24443, 2020/06

 Times Cited Count:6 Percentile:26.41(Chemistry, Multidisciplinary)

Complexation reactions of ruthenium-nitrosyl complexes in HNO$$_{3}$$ solution were investigated by density functional theory (DFT) calculations in order to predict the stability of Ru species in high-level radioactive liquid waste (HLLW) solution. Equilibrium structure of [Ru(NO)(NO$$_{3}$$)$$_{3}$$(H$$_{2}$$O)$$_{2}$$] obtained by DFT calculations reproduced the experimental Ru-ligands bond lengths and IR frequencies reported previously. Comparison of the Gibbs energies among the geometrical isomers revealed that the complexation reactions of the ruthenium-nitrosyl complexes with NO$$_{3}$$$$^{-}$$ proceed via the NO$$_{3}$$$$^{-}$$ coordination to the equatorial plane toward the Ru-NO axis. We also estimated Gibbs energy differences on the stepwise complexation reactions to succeed in reproducing the fraction of Ru-NO species in 6 M HNO$$_{3}$$ solution, such as in HLLW, by considering the association energy between the Ru-NO species and the substituting ligands. Electron density analyses of the complexes indicated that the strength of the Ru-ligands coordination bonds depends on the stability of the Ru species and the Ru complex without NO$$_{3}$$$$^{-}$$ at the axial position is more stable than that wit NO$$_{3}$$$$^{-}$$, which might attribute to the difference in the trans influence between H$$_{2}$$O and NO$$_{3}$$$$^{-}$$. Finally, we demonstrated the complexation kinetics in the reactions $$x = 1 rightarrow x = 2$$. The present study is expected to enable us to model the precise complexation reactions of platinum-group metals in HNO$$_{3}$$ solution.

Journal Articles

Pyroelectric power generation from the waste heat of automotive exhaust gas

Kim, J.*; Yamanaka, Satoru*; Murayama, Ichiro*; Kato, Takanori*; Sakamoto, Tomokazu*; Kawasaki, Takuro; Fukuda, Tatsuo; Sekino, Toru*; Nakayama, Tadachika*; Takeda, Masatoshi*; et al.

Sustainable Energy & Fuels (Internet), 4(3), p.1143 - 1149, 2020/03

 Times Cited Count:20 Percentile:65.42(Chemistry, Physical)

Journal Articles

Density Functional Theory (DFT)-based bonding analysis correlates ligand field strength with $$^{99}$$Ru M$"o$ssbauer parameters of ruthenium-nitrosyl complexes

Kaneko, Masashi; Kato, Akane*; Nakashima, Satoru*; Kitatsuji, Yoshihiro

Inorganic Chemistry, 58(20), p.14024 - 14033, 2019/10

 Times Cited Count:12 Percentile:58.77(Chemistry, Inorganic & Nuclear)

We applied density functional theory calculations to ruthenium-nitrosyl complexes, which are known to exist in high-level radioactive waste, to give a theoretical correlation between $$^{99}$$Ru M$"o$ssbauer spectroscopic parameters ($$delta$$ and $$Delta$$$$E_{rm Q}$$) and ligand field strength ($$Delta$$$$_{rm o}$$) for the first time. The structures of the series of complexes, [Ru(NO)L$$_{5}$$] (L = Br$$^{-}$$, Cl$$^{-}$$, NH$$_{3}$$, CN$$^{-}$$), were modeled based on the corresponding single-crystal X-ray coordinates. The comparisons of the geometries and total energies between the different spin states suggested that the singlet spin state of [Ru(II)(NO$$^{+}$$)L$$_{5}$$] complexes were the most stable. The calculated results of both the $$delta$$ and $$Delta$$$$E_{rm Q}$$ values reproduced the experimental results by reported previously and increased in the order of L = Br$$^{-}$$, Cl$$^{-}$$, NH$$_{3}$$, CN$$^{-}$$. Finally, we estimated the ligand field strength ($$Delta$$$$_{rm o}$$) based on molecular orbitals, assuming C$$_{rm 4v}$$ symmetry and showed the increase of $$Delta$$$$_{rm o}$$ values in that order, being consistent with well-known spectrochemical series of ligands. The increase attributes to the strengthening of the abilities of $$sigma$$-donor and $$pi$$-acceptor of the L-ligands to the Ru atom, resulting in the increase of the $$delta$$ values.

Journal Articles

The Surface composition of asteroid 162173 Ryugu from Hayabusa2 near-infrared spectroscopy

Kitazato, Kohei*; Milliken, R. E.*; Iwata, Takahiro*; Abe, Masanao*; Otake, Makiko*; Matsuura, Shuji*; Arai, Takehiko*; Nakauchi, Yusuke*; Nakamura, Tomoki*; Matsuoka, Moe*; et al.

Science, 364(6437), p.272 - 275, 2019/04

 Times Cited Count:284 Percentile:99.69(Multidisciplinary Sciences)

The near-Earth asteroid 162173 Ryugu, the target of Hayabusa2 sample return mission, is believed to be a primitive carbonaceous object. The Near Infrared Spectrometer (NIRS3) on Hayabusa2 acquired reflectance spectra of Ryugu's surface to provide direct measurements of the surface composition and geological context for the returned samples. A weak, narrow absorption feature centered at 2.72 micron was detected across the entire observed surface, indicating that hydroxyl (OH)-bearing minerals are ubiquitous there. The intensity of the OH feature and low albedo are similar to thermally- and/or shock-metamorphosed carbonaceous chondrite meteorites. There are few variations in the OH-band position, consistent with Ryugu being a compositionally homogeneous rubble-pile object generated from impact fragments of an undifferentiated aqueously altered parent body.

Journal Articles

Electrical and crystallographic study of an electrothermodynamic cycle for a waste heat recovery

Kim, J.*; Yamanaka, Satoru*; Nakajima, Akira*; Kato, Takanori*; Kim, Y.*; Fukuda, Tatsuo; Yoshii, Kenji; Nishihata, Yasuo; Baba, Masaaki*; Takeda, Masatoshi*; et al.

Advanced Sustainable Systems (Internet), 2(11), p.1800067_1 - 1800067_8, 2018/11

 Times Cited Count:7 Percentile:25.35(Green & Sustainable Science & Technology)

Journal Articles

Temperature stability of PIN-PMN-PT ternary ceramics during pyroelectric power generation

Moro, Takuya*; Kim, J.*; Yamanaka, Satoru*; Murayama, Ichiro*; Kato, Takanori*; Nakayama, Tadachika*; Takeda, Masatoshi*; Yamada, Noboru*; Nishihata, Yasuo; Fukuda, Tatsuo; et al.

Journal of Alloys and Compounds, 768, p.22 - 27, 2018/11

 Times Cited Count:17 Percentile:61.62(Chemistry, Physical)

Journal Articles

Incorporation of multinuclear copper active sites into nitrogen-doped graphene for electrochemical oxygen reduction

Kato, Masaru*; Muto, Marika*; Matsubara, Naohiro*; Uemura, Yohei*; Wakisaka, Yuki*; Yoneuchi, Tsubasa*; Matsumura, Daiju; Ishibara, Tomoko*; Tokushima, Takashi*; Noro, Shinichiro*; et al.

ACS Applied Energy Materials (Internet), 1(5), p.2358 - 2364, 2018/05

 Times Cited Count:14 Percentile:44.80(Chemistry, Physical)

Journal Articles

A Failure investigation of the beam collimator system in the J-PARC 3 GeV rapid cycling synchrotron

Okabe, Kota; Yamamoto, Kazami; Kamiya, Junichiro; Takayanagi, Tomohiro; Yamamoto, Masanobu; Yoshimoto, Masahiro; Takeda, Osamu*; Horino, Koki*; Ueno, Tomoaki*; Yanagibashi, Toru*; et al.

Proceedings of 14th Annual Meeting of Particle Accelerator Society of Japan (Internet), p.853 - 857, 2017/12

The most important issue is to reduce the uncontrolled beam loss in the high intensity hadron accelerator such as J-PARC proton accelerators. The J-PARC 3 GeV Synchrotron (RCS) has a collimator system which narrows a high intensity beam in the RCS. After startup of RCS in 2007, the collimator system of the RCS worked well. However, in April 2016, vacuum leakage at the collimator system occurred during the maintenance operation. To investigate a cause of the failure, we took apart iron shields of the collimator reducing exposed dose of operators. As a result of inspection, we succeeded to identify the cause of the vacuum leakage failure. In this presentation, we report the failure investigation of the beam collimator system in the RCS.

Journal Articles

Pyroelectric power generation with ferroelectrics (1-x)PMN-xPT

Kim, J.*; Yamanaka, Satoru*; Nakajima, Akira*; Kato, Takanori*; Kim, Y.*; Fukuda, Tatsuo; Yoshii, Kenji; Nishihata, Yasuo; Baba, Masaaki*; Takeda, Masatoshi*; et al.

Ferroelectrics, 512(1), p.92 - 99, 2017/08

 Times Cited Count:14 Percentile:53.37(Materials Science, Multidisciplinary)

Journal Articles

Relationship between the material properties and pyroelectric-generating performance of PZTs

Yamanaka, Satoru*; Kim, J.*; Nakajima, Akira*; Kato, Takanori*; Kim, Y.*; Fukuda, Tatsuo; Yoshii, Kenji; Nishihata, Yasuo; Baba, Masaaki*; Yamada, Noboru*; et al.

Advanced Sustainable Systems (Internet), 1(3-4), p.1600020_1 - 1600020_6, 2017/04

no abstracts in English

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