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Otosaka, Shigeyoshi*; Kamidaira, Yuki; Ikenoue, Tsubasa; Kawamura, Hideyuki
Journal of Nuclear Science and Technology, 59(4), p.409 - 423, 2022/04
Times Cited Count：3 Percentile：45.99(Nuclear Science & Technology)After the accident at Fukushima Daiichi Nuclear Power Plant (FDNPP), many oceanographic observations were carried out from various perspectives. Numerical simulations were also effectively applied to understand the distribution of radionunclides. By integrating these results, the dynamics of the accident-derived radionuclides in the ocean were highlighted. The transport processes of the accident-derived radionuclides to the ocean include (1) direct discharge to the ocean, (2) deposition in the ocean via the atmosphere, and (3) inflow from rivers after deposition to the land surface. In the case of 
Cs, one of major accident-derived radionuclides, most of the supply to the ocean immediately after the accident (8-21 PBq) was estimated to be due to processes (1) and (2). The amount of Cs accumulated on the seafloor is only about 1% (0.2PBq) of the amount carried to the ocean, but it remains in the sediments in the coastal area for a long period of time and gradually migrates to the seawater and ecosystems near the seafloor.
Kamidaira, Yuki; Uchiyama, Yusuke*; Kawamura, Hideyuki; Kobayashi, Takuya; Otosaka, Shigeyoshi*
Journal of Environmental Radioactivity, 238-239, p.106724_1 - 106724_16, 2021/11
Times Cited Count：11 Percentile：64.14(Environmental Sciences)A three-dimensional oceanic dispersion model considering the migration of radionuclides between seawater and sediments was developed. The migration mechanism of dissolved Cs-137 originating from the Fukushima Daiichi Nuclear Power Plant accident to sediments was investigated. The comparison between the model and the observed data showed that the model can adequately reproduce the ocean structure and the concentration of Cs-137 in seawater and sediments. Cs-137 distribution in the sediment off the Fukushima coast was formed mainly owing to adsorption from the dissolved phase by June 2011, when the impact of the direct oceanic Cs-137 release from FNPP1 was remarkable.
I released from Fukushima Daiichi Nuclear Power Plant accident in the western North Pacific OceanSuzuki, Takashi; Otosaka, Shigeyoshi; Kuwabara, Jun; Kawamura, Hideyuki; Kobayashi, Takuya
JAEA-Conf 2018-002, p.103 - 106, 2019/02
To investigate the dynamics of radionuclides in the ocean released by the accident at Fukushima Daiichi Nuclear Power Plant (1F), vertical distributions of I at three stations in the western North Pacific was revealed. The 1F accident-derived I existed within the mixed layer at 3 stations. The maximum layer of the 1F accident-derived I existed at the depth of 370 m - 470 m at the most southern station. Considering the dissolved oxygen concentration and the current velocity arround the station, the maximum layer of the 1F accident-derived I would be fromed that I which existed in the surface seawater at other area of observation point was carried to the depth of 370 m - 470 m by the fast downward flow.
I released from the Fukushima Daiichi Nuclear Power Plant in the Kuroshio and Oyashio current areasSuzuki, Takashi; Otosaka, Shigeyoshi; Kuwabara, Jun; Kawamura, Hideyuki; Kobayashi, Takuya
Marine Chemistry, 204, p.163 - 171, 2018/08
Times Cited Count：2 Percentile：10.86(Chemistry, Multidisciplinary)To investigate the penetration of radionuclides released from Fukushima Daiichi Nuclear Power Plant (FDNPP), depth profiles were revealed at Kuroshio current, transition, and Oyashio current areas. The FDNPP-derived I was found in surface layer at Oyashio current and transition areas and in sub-surface layer at Kuroshio current area. Moreover, it was found that the FDNPP-derived I/
Cs ratios in the Oyashio current and transition areas were higher than that in the FDNPP reactor. The higher FDNPP-derived I/Cs ratios suggest three potential mechanisms for the migration of radionuclides in the environment: (1) radioiodine was released more easily than radiocesium by the FDNPP accident, (2) I was supplied from the atmosphere by re-emitted I from contaminated areas around Fukushima, (3) leaked water that removed radiocesium reached the sampling stations. The FDNPP-derived I in sub-surface layer would be transported by the meander of the Kuroshio Extension current.
Suzuki, Takashi; Otosaka, Shigeyoshi; Kuwabara, Jun; Kawamura, Hideyuki; Kobayashi, Takuya
Biogeosciences, 10(6), p.3839 - 3847, 2013/06
Times Cited Count：24 Percentile：57.84(Ecology)no abstracts in English
Kawamura, Hideyuki; Ito, Toshimichi; Kobayashi, Takuya; Otosaka, Shigeyoshi; Hirose, Naoki*; Togawa, Orihiko
Journal of Oceanography, 66(5), p.649 - 662, 2010/10
Times Cited Count：2 Percentile：6.22(Oceanography)A numerical experiment is performed to reproduce a distribution of concentrations of 
Sr and Cs and estimate their total amounts in the Japan Sea. The concentrations of Sr and Cs in the surface layer is in the range of 1.0-1.5 Bq/m
and 2.0-2.5 Bq/m. The concentrations in the intermediate and deep layer are higher than those observed in the northwestern Pacific Ocean, indicating active winter convection in the Japan Sea. The total amounts of Sr and Cs in the seawater is evaluated to be 1.34 PBq (1 PBq = 10
Bq) and 2.02 PBq, which demonstrates an estimation by observational data in the Japan Sea expeditions between 1997 and 2002 by Japan Atomic Energy Agency. The total amounts of Sr and Cs vary corresponding to deposition at the sea surface with the maximums of 4.86 PBq for Sr and 7.33 PBq for Cs in the mid-1960s.
Kawamura, Hideyuki; Ito, Toshimichi; Kobayashi, Takuya; Otosaka, Shigeyoshi; Hirose, Naoki*; Togawa, Orihiko
Proceedings of Joint International Conference of 7th Supercomputing in Nuclear Application and 3rd Monte Carlo (SNA + MC 2010) (USB Flash Drive), 4 Pages, 2010/10
This study aims to demonstrate many findings in the Japan Sea expeditions by Japan Atomic Energy Agency between 1997 and 2002 making use of an ocean general circulation model. A numerical experiment is performed between 1945 and 2000 with deposition at the sea surface by global fallout as main source of anthropogenic radionuclides. The concentrations of Sr and Cs in the surface layer are approximately in the range of 1.0-1.5 Bq/m and 2.0-2.5 Bq/m and they exponentially decrease with depth from the sea surface to the sea bottom. Total amounts of Sr and Cs in the seawater of the Japan Sea are estimated to be about 1.34 PBq (1 PBq = 10 Bq) and 2.02 PBq in the numerical experiment, which demonstrates observational estimations in the Japan Sea expeditions. Time series of the total amounts show that they attain the maximums of 4.86 PBq for Sr and 7.33 PBq for Cs in 1964.
Otosaka, Shigeyoshi; Suzuki, Takashi; Tanaka, Takayuki; Ito, Toshimichi; Kobayashi, Takuya; Kawamura, Hideyuki; Minakawa, Masayuki*; Aramaki, Takafumi*; Senju, Tomoharu*; Togawa, Orihiko
JAEA-Data/Code 2009-020, 27 Pages, 2010/02
JAEA-Data-Code-2009-020.pdf:2.45MB
The database for the Japan Sea parameters on marine environment and radionuclides (JASPER) has been established by the Japan Atomic Energy Agency as a product of the Japan Sea Expeditions. By the previous version of the database, data for representative anthropogenic radionuclides were opened to public. And now, data for radiocarbon and fundamental oceanographic properties (salinity, temperature, dissolved oxygen) including nutrients (silicate, phosphate, nitrate and nitrite) are released as the second volume of the database. In the second volume, 20,398 data records are stored including 2,695 data for temperature, 2,883 data for salinity, 2,109 data for dissolved oxygen, 11,051 data for the nutrients, and 1,660 data for radiocarbon. The database will be a strong tool for the continuous monitoring for contamination by anthropogenic radionuclides, studies on biogeochemical cycle, and development and validation of models for numerical simulations in the sea.
Kobayashi, Takuya; Togawa, Orihiko; Ito, Toshimichi; Otosaka, Shigeyoshi; Kawamura, Hideyuki; Hayashi, Keisuke*; Shima, Shigeki*; Nakayama, Tomoharu*; In, Teiji*
JAEA-Research 2009-040, 63 Pages, 2009/12
JAEA-Research-2009-040.pdf:12.19MB
A spent nuclear fuel reprocessing plant has the possibility of routine releases of liquid radioactive wastes from a discharge pipe to the off Shimokita region during its operations. Thus, for environmental safety, it is important to assess the migration processes of released radionuclides from the plant. Therefore, an ocean circulation prediction code and an oceanic radionuclides migration prediction code, which were developed by Japan Atomic Energy Agency, has been improved to describe the migration behavior of radionuclides in the off Shimokita region. Parameters on characteristics and dynamics of particulate materials in seawater have also been obtained in the study area for the adjustment and verification of the oceanic radionuclides migration prediction code. This report summarizes the primary results of the study which was carried out at the off Shimokita region from FY2003 to 2008.
Ito, Toshimichi; Otosaka, Shigeyoshi; Kawamura, Hideyuki
Journal of Nuclear Science and Technology, 44(6), p.912 - 922, 2007/06
Times Cited Count：11 Percentile：61.1(Nuclear Science & Technology)The total amount of anthropogenic radionuclides - Sr, Cs and 
Pu - in the Japan Sea were estimated for the first time. Inventories of seawater, seabed sediment and total at each sampling site varied depending on the water depth of the sites, and the total inventories for Sr, Cs and Pu were in the range of 0.52-2.8 kBqm
, 0.64-4.1 kBqm and 27-122 Bqm, respectively. Using the dependency of the seawater and seabed sediment and gridded water depth data, the total amounts in the Japan Sea were estimated to be about 1.2
0.4 PBq for Sr, 1.80.7 PBq for Cs and 6914 TBq for Pu, and their total was about 3.1 PBq. The amount ratio of these radionuclides (Sr : Cs : Pu) became to be 1.0 : 1.6 : 0.059 implying selective accumulation of the plutonium isotopes. This implication was supported by the balance between the existing and supplied amounts, in which the existing Sr and Cs were comparable for the supplied while the existing Pu exceeded the supplied in nearly 40 %. This work were performed using the observation data obtained through a wide-area research project, "Japan Sea Expeditions", carried out during 1997-2003 and covered the Japanese and Russian exclusive economic zones.
Otosaka, Shigeyoshi; Amano, Hikaru; Ito, Toshimichi; Kawamura, Hideyuki; Kobayashi, Takuya; Suzuki, Takashi; Togawa, Orihiko; Chaykovskaya, E. L.*; Lishavskaya, T. S.*; Novichkov, V. P.*; et al.
Journal of Environmental Radioactivity, 91(3), p.128 - 145, 2006/00
Times Cited Count：20 Percentile：42.21(Environmental Sciences)Distributions of radionuclides (Sr, Cs and Pu) in seabed sediment in the Japan Sea were observed during 1998-2002. Observed inventories of anthropogenic radionuclides in sediment ranged 0.1-86 Bq m for Sr, 23-379 Bq m for Cs and 0.1-86 Bq m for Pu. In the deep part (
2 km depth) of the western Japan Basin, Pu/Cs inventory ratios were larger than those in the central Yamato Basin although inventories of radionuclides were not different between basins. The higher Pu/Cs ratios in the western Japan Basin were derived by the production of Pu-enriched particle in the surface layer and effective sinking of particulate materials in this region. In the marginal Yamato Basin and the Ulleung Basin, both inventories and Pu/Cs ratios in sediment were larger than those in the central Yamato Basin. In the eastern/southern Japan Sea, it was suggested that the supply of particulate radionuclides by the TWC enhanced accumulation of radionuclides in this region.
Ito, Toshimichi; Aramaki, Takafumi*; Otosaka, Shigeyoshi; Suzuki, Takashi; Togawa, Orihiko; Kobayashi, Takuya; Kawamura, Hideyuki; Amano, Hikaru; Senju, Tomoharu*; Chaykovskaya, E. L.*; et al.
Journal of Nuclear Science and Technology, 42(1), p.90 - 100, 2005/01
Times Cited Count：14 Percentile：67.84(Nuclear Science & Technology)During 1996-2002, a wide-area research project on anthropogenic radionuclides was done in the Japanese and Russian EEZ of the Japan Sea to investigate their migration. As the results of expeditions in 2001 and 2002, (1) the concentrations and distributions of radionuclides are similar to the results of previous, (2) inventories of these radionuclides indicate accumulation in the Japan Sea seawater compared to the amounts supplied by global fallout, (3) Sr and Cs concentrations in intermediate layer show temporal variations, and 4) the variations may reflect the water mass movement in upper part of the Japan Sea.
Otosaka, Shigeyoshi; Ito, Toshimichi; Kawamura, Hideyuki; Kobayashi, Takuya; Suzuki, Takashi; Togawa, Orihiko
Dai-45-Kai Kankyo Hoshano Chosa Kenkyu Seika Rombun Shorokushu (Heisei-14-Nendo), p.77 - 78, 2003/12
no abstracts in English
Yokoyama, Hiroomi*; Kanazawa, Toshio*; Fukuma, Tadashi*; Tamekiyo, Kozo*; Yanagida, Koji*; Furuya, Takashi*; Kono, Hiroshi*; Ito, Keiji*; Shirakura, Takao*; Kashiwara, Shinichiro*; et al.
PNC TN8410 87-086VOL2, 944 Pages, 1986/09
Yokoyama, Hiroomi*; Kanazawa, Toshio*; Fukuma, Tadashi*; Tamekiyo, Kozo*; Yanagida, Koji*; Furuya, Takashi*; Kono, Hiroshi*; Ito, Keiji*; Shirakura, Takao*; Kashiwara, Shinichiro*; et al.
PNC TN8410 87-086VOL1, 1037 Pages, 1986/09
PNC-TN8410-87-086VOL1.pdf:34.39MB
A detailed design for a New Material Nitric Acid Recovery Evaporator was carried out with a plan to use it to replace an already constructed stainless steel Nitric Acid Recovery Evaporator at the Power Reactor and Nuclear Fuel Development Corporation's Tokai Works. Most of the original Evaporator's conditions such as compliance with applicable laws, standards, structure, treatment performance and operating conditions were maintained when designing the new machine. The material is titanium with the addition of 5% tantalum. The Evaporator was designed with an operational life expectance of 10 years. We have calculated that the new Evaporator will have sufficient strength (including a seismatic design) and have the same evaporative performance as the already constructed one. During design, we referred to the results of already completed basic designs (Phase 1) of New Material Nitric Acid Recovery Evaporators, design and production of small-scale test equipment units, and the development of successful joints between different materials. We also considered manufacturing, installation, trial runs, maintenance, and the specifications for materials used for manufacturing, installation, piping and operation of the new Evaporator.
Ito, Toshimichi; Otosaka, Shigeyoshi; Kawamura, Hideyuki
no journal, ,
no abstracts in English
Kawamura, Hideyuki; Ito, Toshimichi; Kobayashi, Takuya; Otosaka, Shigeyoshi; Hirose, Naoki*
no journal, ,
Observation had been carried out to clarify distribution of anthropogenic radionuclides in the Japan Sea in the period between 1997 and 2002 by Japan Atomic Energy Agency. This study aims at reproducing the distribution of anthropogenic radionuclides with a numerical model and clarifying their movement in the Japan Sea. Deposition densities by global fallout are applied as boundary conditions for strontium 90 and cesium 137 at the sea surface. Numerical results show that concentration of strontium 90 and cesium 137 is compared with the observed one in the surface layer and the intermediate layer, although the concentration below 1000 m depth is quite low. More numerical experiments will be performed modifying parameters and boundary conditions of the numerical model in the future.
Kawamura, Hideyuki; Kobayashi, Takuya; Ito, Toshimichi; Otosaka, Shigeyoshi; Togawa, Orihiko; Onitsuka, Go*; Hirose, Naoki*
no journal, ,
Japan Atomic Energy Agency has been developing a material circulation model in the Japan Sea to confirm aspect of observational results. The material circulation model consists of three numerical models, an ocean general circulation model, a particle random-walk model and a lower trophic ecosystem model. A preliminary numerical experiment shows that vertical profile and total amount of Sr-90 and Cs-137 are well compared with observational results.
Otosaka, Shigeyoshi; Kobayashi, Takuya; Kawamura, Hideyuki; Suzuki, Takashi
no journal, ,
Based on oceanographic observations and numerical simulations, dispersion and sedimentation processes of radionuclides released from the Fukushima Dai-ichi NPP were summarized. An oceanic dispersion simulation indicated that, (1) in the middle of March, 2011, radionuclides released to the atmosphere mainly deposited on the surface of the northeastern regions of Fukushima Prefecture, and (2) radionuclides released directly to the ocean were transported southward along the coast of Fukushima and Ibaraki Prefectures. Observational results indicated that (3) most radiocesium in seabed sediment was transported by the above-mentioned process (2), and adsorbed on sediments in the coastal regions within 6 months after the accident.
Kobayashi, Takuya; Kawamura, Hideyuki; Otosaka, Shigeyoshi
no journal, ,
Some radioactive material was discharged into the Pacific Ocean because of the Fukushima Daiichi Nuclear Power Plant disaster. High concentrations of Cs were found in the seawater and the seabed sediment along the coastline of Fukushima Prefecture. Numerical experiments on oceanic dispersion of Cs-137 discharged from the Fukushima Dai-ichi Nuclear Power Plant were carried out with an oceanic dispersion model SEA-GEARN developed in Japan Atomic Energy Agency. Radionuclides in the ocean are modeled in three phases, i.e., the dissolved phase in seawater, the adsorbed with large particulate matter (LPM) and the adsorbed with active bottom sediment.
