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Journal Articles

Development of regional downscaling capability in STEAMER ocean prediction system based on multi-nested ROMS model

Kamidaira, Yuki; Kawamura, Hideyuki; Kobayashi, Takuya; Uchiyama, Yusuke*

Journal of Nuclear Science and Technology, 56(8), p.752 - 763, 2019/08

 Times Cited Count:1 Percentile:19.54(Nuclear Science & Technology)

Oceanic regional downscaling capability was implemented into Short-Term Emergency Assessment system of Marine Environmental Radioactivity (STEAMER) developed by Japan Atomic Energy Agency to enable us to predict more realistically the oceanic dispersion of radionuclides at higher spatiotemporal resolutions for broader applications. The system consisted of a double-nested oceanic downscaling circulation model with tidal forcing and an oceanic radionuclide dispersion model. This system was used to comparatively examine downscaling and tidal effects on the dispersion of radionuclides hypothetically released from the Fukushima Daiichi Nuclear Power Plant in the colder season. The simulated dissolved $$^{137}$$Cs distribution was different from that obtained using coarser-resolution models because downscaling enhanced both horizontal and vertical mixing. The suppression of horizontal mixing and the promotion of vertical mixing by tidal forcing synergistically reduced offshore $$^{137}$$Cs transport. In addition, the submesoscale effects strengthened the three-dimensional $$^{137}$$Cs fluctuations by $$<$$10 times, while the tidal effects promoted slightly increased the intensity of three-dimensional $$^{137}$$Cs fluctuations by approximately 3%. This indicated that the submesoscale effects substantially surpassed tidal forcing in oceanic mixing in the coastal margin off Fukushima in the colder season.

Journal Articles

Localized magnetic excitations in the fully frustrated dimerized magnet Ba$$_{2}$$CoSi$$_{2}$$O$$_{6}$$Cl$$_{2}$$

Kurita, Nubuyuki*; Yamamoto, Daisuke*; Kanesaka, Takuya*; Furukawa, Nobuo*; Kawamura, Seiko; Nakajima, Kenji; Tanaka, Hidekazu*

Physical Review Letters, 123(2), p.027206_1 - 027206_6, 2019/07

 Times Cited Count:0 Percentile:100(Physics, Multidisciplinary)

Journal Articles

Penetration of $$^{129}$$I released from Fukushima Daiichi Nuclear Power Plant accident in the western North Pacific Ocean

Suzuki, Takashi; Otosaka, Shigeyoshi; Kuwabara, Jun; Kawamura, Hideyuki; Kobayashi, Takuya

JAEA-Conf 2018-002, p.103 - 106, 2019/02

To investigate the dynamics of radionuclides in the ocean released by the accident at Fukushima Daiichi Nuclear Power Plant (1F), vertical distributions of $$^{129}$$ I at three stations in the western North Pacific was revealed. The 1F accident-derived $$^{129}$$ I existed within the mixed layer at 3 stations. The maximum layer of the 1F accident-derived $$^{129}$$ I existed at the depth of 370 m - 470 m at the most southern station. Considering the dissolved oxygen concentration and the current velocity arround the station, the maximum layer of the 1F accident-derived $$^{129}$$ I would be fromed that $$^{129}$$I which existed in the surface seawater at other area of observation point was carried to the depth of 370 m - 470 m by the fast downward flow.

Journal Articles

Quantum paramagnet near spin-state transition

Tomiyasu, Keisuke*; Ito, Naoko*; Okazaki, Ryuji*; Takahashi, Yuki*; Onodera, Mitsugi*; Iwasa, Kazuaki*; Nojima, Tsutomu*; Aoyama, Takuya*; Ogushi, Kenya*; Ishikawa, Yoshihisa*; et al.

Advanced Quantum Technologies (Internet), 1(3), p.1800057_1 - 1800057_7, 2018/12

Spin-state transition, also known as spin crossover, plays a key role in diverse systems. In theory, the boundary range between the low- and high-spin states is expected to enrich the transition and give rise to unusual physical states. However, no compound that realizes a nearly degenerate critical range as the ground state without requiring special external conditions has yet been experimentally identified. This study reports that the Sc substitution in LaCoO3 destabilizes its nonmagnetic low-spin state and generates an anomalous paramagnetic state accompanied by the enhancement of transport gap and magneto-lattice-expansion as well as the contraction of Co-O distance with the increase of electron site transfer. These phenomena are not well described by the mixture of conventional low- and high-spin states, but by their quantum superposition occurring on the verge of a spin-state transition.

Journal Articles

New insights into the Cs adsorption on montmorillonite clay from $$^{133}$$Cs solid-state NMR and density functional theory calculations

Okubo, Takahiro*; Okamoto, Takuya*; Kawamura, Katsuyuki*; Gu$'e$gan, R.*; Deguchi, Kenzo*; Oki, Shinobu*; Shimizu, Tadashi*; Tachi, Yukio; Iwadate, Yasuhiko*

Journal of Physical Chemistry A, 122(48), p.9326 - 9337, 2018/12

 Times Cited Count:0 Percentile:100(Chemistry, Physical)

The structures of Cs adsorption on montmorillonite were investigated by the nuclear magnetic resonance (NMR) spectroscopy. The NMR spectra of Cs adsorbed on montmorillonite samples were measured under different Cs contents and relative humidity levels. NMR parameters were evaluated by the first principle calculations in order to identify the relationship between adsorbed Cs structures and NMR parameters. The comparisons between experimental and theoretical NMR spectra revealed that Cs is preferentially adsorbed at sites near Al for low Cs substituted montmorillonites, and that non-hydrated Cs present in partially Cs substituted samples, even after being hydrated under high relative humidity.

Journal Articles

Extended X-ray absorption fine structure study on gel/liquid extraction of f-block elements

Nakase, Masahiko*; Kobayashi, Toru; Shiwaku, Hideaki; Kawamura, Takuya*; Takeshita, Kenji*; Yamamura, Tomoo*; Yaita, Tsuyoshi

Progress in Nuclear Science and Technology (Internet), 5, p.56 - 60, 2018/11

Gel/liquid extraction was investigated to achieve selective separation of trivalent actinides over lanthanides. In this study, thermosensitive hydrogel including N,N,N',N'-tetraallylpyridine-2,6-dicarboxamine (PDA) was synthesized, and its complexation with lanthanide was investigated by extended X-ray absorption fine structure experiments at SPring-8. The radial structure functions (RSF) of solution with gels with and without ligands at different temperatures showed slight differences. As the temperature increased, the RSF decreased owing to the increase in thermal vibration, but PDA-gel showed a shift in the first peak toward the shorter direction. This shift was attributed to the change in stoichiometry of PDA-Ln(III) complexes or coordination number of water molecules affected by the change of conformation of polymer chains and the hydrophilic/hydrophobic properties in the hydrogel.

Journal Articles

Vertical distribution of $$^{129}$$I released from the Fukushima Daiichi Nuclear Power Plant in the Kuroshio and Oyashio current areas

Suzuki, Takashi; Otosaka, Shigeyoshi; Kuwabara, Jun; Kawamura, Hideyuki; Kobayashi, Takuya

Marine Chemistry, 204, p.163 - 171, 2018/08

 Times Cited Count:0 Percentile:100(Chemistry, Multidisciplinary)

To investigate the penetration of radionuclides released from Fukushima Daiichi Nuclear Power Plant (FDNPP), depth profiles were revealed at Kuroshio current, transition, and Oyashio current areas. The FDNPP-derived $$^{129}$$I was found in surface layer at Oyashio current and transition areas and in sub-surface layer at Kuroshio current area. Moreover, it was found that the FDNPP-derived $$^{129}$$I/$$^{134}$$Cs ratios in the Oyashio current and transition areas were higher than that in the FDNPP reactor. The higher FDNPP-derived $$^{129}$$I/$$^{134}$$Cs ratios suggest three potential mechanisms for the migration of radionuclides in the environment: (1) radioiodine was released more easily than radiocesium by the FDNPP accident, (2) $$^{129}$$I was supplied from the atmosphere by re-emitted $$^{129}$$I from contaminated areas around Fukushima, (3) leaked water that removed radiocesium reached the sampling stations. The FDNPP-derived $$^{129}$$I in sub-surface layer would be transported by the meander of the Kuroshio Extension current.

Journal Articles

Submesoscale mixing on initial dilution of radionuclides released from the Fukushima Daiichi Nuclear Power Plant

Kamidaira, Yuki; Uchiyama, Yusuke*; Kawamura, Hideyuki; Kobayashi, Takuya; Furuno, Akiko

Journal of Geophysical Research; Oceans (Internet), 123(4), p.2808 - 2828, 2018/04

 Times Cited Count:6 Percentile:8.53(Oceanography)

We developed a submesoscale eddy-resolving oceanic dispersal modeling system consisting of a double nested oceanic downscaling model and an offline oceanic radionuclides dispersion model to investigate influences of submesoscale coherent structures (SCSs) and associated ageostrophic secondary circulations (ASCs) on the three-dimensional (3D) dispersal and initial dilution of the dissolved radioactive $$^{137}$$Cs accidentally released from the Fukushima Daiichi Nuclear Power Plant (FNPP1) occurred since March 2011. The extensive model-data comparison demonstrates that the elaborated innermost high-resolution model at a lateral grid resolution of 1 km successfully reproduces transient mesoscale oceanic structures, the Kuroshio path and stratification, and spatiotemporal variations of 3D $$^{137}$$Cs concentrations. These SCSs and ASCs occurred primarily due to shear instability with baroclinic instability as the secondary mechanism, according to energy conversion and spectral analyses. The vertical $$^{137}$$Cs flux analysis was performed with decomposition of the variables into the mean, mesoscale, and submesoscale components using frequency and wavenumber filters. The vertical $$^{137}$$Cs flux analysis explained that 84% of the FNPP1-derived $$^{137}$$Cs was transported downward below the mixed layer by eddies, with the major contributions from ASCs induced by submesoscale eddies.

Journal Articles

Oceanic dispersion of Fukushima-derived Cs-137 simulated by multiple oceanic general circulation models

Kawamura, Hideyuki; Furuno, Akiko; Kobayashi, Takuya; In, Teiji*; Nakayama, Tomoharu*; Ishikawa, Yoichi*; Miyazawa, Yasumasa*; Usui, Norihisa*

Journal of Environmental Radioactivity, 180, p.36 - 58, 2017/12

 Times Cited Count:3 Percentile:65.3(Environmental Sciences)

This study simulates the oceanic dispersion of Fukushima-derived Cs-137 by an oceanic dispersion model and multiple oceanic general circulation models. The models relatively well reproduced the observed Cs-137 concentrations in the coastal, offshore, and open oceans. Multiple simulations in the coastal, offshore, and open oceans consistently suggested that Cs-137 dispersed along the coast in the north-south direction during the first few months post-disaster, and were subsequently dispersed offshore by the Kuroshio Current and Kuroshio Extension. Quantification of the Cs-137 amounts suggested that Cs-137 actively dispersed from the coastal and offshore oceans to the open ocean, and from the surface layer to the deeper layers in the North Pacific.

Journal Articles

Development of a short-term emergency assessment system of the marine environmental radioactivity around Japan

Kobayashi, Takuya; Kawamura, Hideyuki; Fujii, Katsuji*; Kamidaira, Yuki

Journal of Nuclear Science and Technology, 54(5), p.609 - 616, 2017/05

 Times Cited Count:4 Percentile:26.08(Nuclear Science & Technology)

The Japan Atomic Energy Agency has, for many years, been developing a radionuclide dispersion model for the ocean, and has validated the model through application in many sea areas using oceanic flow fields calculated by the ocean model. The Fukushima Dai-ichi Nuclear Power Station accident caused marine pollution by artificial radioactive materials to the North Pacific, especially to coastal waters northeast of mainland Japan. In order to investigate the migration of radionuclides in the ocean caused by this severe accident, studies using marine dispersion simulations have been carried out by JAEA. Based on these as well as the previous studies, JAEA has developed the Short-Term Emergency Assessment system of Marine Environmental Radioactivity (STEAMER) to immediately predict the radionuclide concentration around Japan in case of a nuclear accident.

Journal Articles

New muonium HFS measurements at J-PARC/MUSE

Strasser, P.*; Aoki, Masaharu*; Fukao, Yoshinori*; Higashi, Yoshitaka*; Higuchi, Takashi*; Iinuma, Hiromi*; Ikedo, Yutaka*; Ishida, Keiichi*; Ito, Takashi; Iwasaki, Masahiko*; et al.

Hyperfine Interactions, 237(1), p.124_1 - 124_9, 2016/12

 Times Cited Count:4 Percentile:7.76

Journal Articles

Development of a prediction system for radionuclide dispersion in Fukushima coast

Kamidaira, Yuki; Kawamura, Hideyuki; Kobayashi, Takuya; Uchiyama, Yusuke*

Doboku Gakkai Rombunshu, B2 (Kaigan Kogaku) (Internet), 72(2), p.I_451 - I_456, 2016/11

no abstracts in English

Journal Articles

Technical estimation for mass production of highly-concentrated $$^{rm 99m}$$Tc solution from $$^{99}$$Mo to be obtained by ($$n,gamma$$) reaction; A Preliminary study using inactive Re instead of $$^{rm 99m}$$Tc

Tanase, Masakazu*; Fujisaki, Saburo*; Ota, Akio*; Shiina, Takayuki*; Yamabayashi, Hisamichi*; Takeuchi, Nobuhiro*; Tsuchiya, Kunihiko; Kimura, Akihiro; Suzuki, Yoshitaka; Ishida, Takuya; et al.

Radioisotopes, 65(5), p.237 - 245, 2016/05

no abstracts in English

Journal Articles

Chromatographic separation of nuclear rare metals by highly functional xerogels

Onishi, Takashi; Koyama, Shinichi; Masud, R. S.*; Kawamura, Takuya*; Mimura, Hitoshi*; Niibori, Yuichi*

Nippon Ion Kokan Gakkai-Shi, 25(4), p.220 - 227, 2014/11

no abstracts in English

Journal Articles

Numerical simulation on the long-term variation of radioactive cesium concentration in the North Pacific due to the Fukushima disaster

Kawamura, Hideyuki; Kobayashi, Takuya; Furuno, Akiko; Usui, Norihisa*; Kamachi, Masafumi*

Journal of Environmental Radioactivity, 136, p.64 - 75, 2014/10

 Times Cited Count:18 Percentile:32.84(Environmental Sciences)

Numerical simulations on oceanic radioactive cesium dispersions in the North Pacific were conducted with a focus on the long-term variation of the radioactive cesium concentration after the Fukushima disaster. It was suggested that the $$^{137}$$Cs concentration had already been reduced to the pre-Fukushima background value in the wide area within the North Pacific 2.5 years after the Fukushima disaster.

Journal Articles

Drift simulation of tsunami debris in the North Pacific

Kawamura, Hideyuki; Kobayashi, Takuya; Nishikawa, Shiro*; Ishikawa, Yoichi*; Usui, Norihisa*; Kamachi, Masafumi*; Aso, Noriko*; Tanaka, Yusuke*; Awaji, Toshiyuki*

Global Environmental Research (Internet), 18(1), p.81 - 96, 2014/09

A drift simulation of tsunami debris flushed out from the Tohoku district, Japan, into the North Pacific due to the tsunami on March 11, 2011, has been conducted to monitor and forecast the drift path over the North Pacific. Results showed that tsunami debris was first transported eastward by the intense Kuroshio Extension and westerly, spreading in the north and south directions by both an energetic ocean eddy and a storm track over the ocean. Tsunami debris with larger windage was transported over the North Pacific by ocean surface wind rather than ocean current and arrived at the west coast of the North American Continent in the fall of 2011. Tsunami debris located near the North American Continent migrated, associated with the basin-scale seasonal change in the atmospheric pressure pattern. Our forecast run suggested that the tsunami debris belt will be formed from the North American Continent in the east to the Philippines in the west.

Journal Articles

Intercomparison of numerical simulations on oceanic dispersion of the radioactive cesium released because of the Fukushima disaster

Kawamura, Hideyuki; Kobayashi, Takuya; Furuno, Akiko; Usui, Norihisa*; Kamachi, Masafumi*; Nishikawa, Shiro*; Ishikawa, Yoichi*

Proceedings of 19th Pacific Basin Nuclear Conference (PBNC 2014) (USB Flash Drive), 7 Pages, 2014/08

Numerical simulations on oceanic dispersion of the radioactive cesium in the North Pacific from March 2011 to September 2013 were conducted to clarify the concentration of the radioactive cesium released from the Fukushima Daiichi Nuclear Power Plant. We implemented the oceanic dispersion simulations with two independent ocean reanalysis dataset. It was suggested that the $$^{137}$$Cs concentration in the North Pacific was lower than the pre-Fukushima background level about two years after the Fukushima disaster. The intercomparison revealed that meso-scale eddies in the Kuroshio Extension region may have efficiently diluted the radioactive cesium concentration at the sea surface. In addition, it was suggested that the enhanced downward current accompanied by the meso-scale eddies played an important role in transporting the radioactive cesium into the intermediate layer.

Journal Articles

Iodine-129 concentration in seawater near Fukushima before and after the accident at the Fukushima Daiichi Nuclear Power Plant

Suzuki, Takashi; Otosaka, Shigeyoshi; Kuwabara, Jun; Kawamura, Hideyuki; Kobayashi, Takuya

Biogeosciences, 10(6), p.3839 - 3847, 2013/06

 Times Cited Count:17 Percentile:36.38(Ecology)

no abstracts in English

Journal Articles

Source term estimation of atmospheric release due to the Fukushima Dai-ichi Nuclear Power Plant accident by atmospheric and oceanic dispersion simulations

Kobayashi, Takuya; Nagai, Haruyasu; Chino, Masamichi; Kawamura, Hideyuki

Journal of Nuclear Science and Technology, 50(3), p.255 - 264, 2013/03

AA2012-0777.pdf:1.24MB

 Times Cited Count:101 Percentile:0.17(Nuclear Science & Technology)

The source term of the atmospheric release of $$^{131}$$I and $$^{137}$$Cs due to the Fukushima Dai-ichi Nuclear Power Plant accident estimated by previous studies was validated and refined by coupling atmospheric and oceanic dispersion simulations with observed $$^{134}$$Cs in seawater collected from the Pacific Ocean. By assuming the same release rate for $$^{134}$$Cs and $$^{137}$$Cs, the sea surface concentration of $$^{134}$$Cs was calculated using the previously estimated source term and was compared with measurement data. The release rate of $$^{137}$$Cs was refined to reduce underestimation of measurements, which resulted in a larger value than that previously estimated. In addition, the release rate of $$^{131}$$I was refined to follow the radioactivity ratio of $$^{137}$$Cs. As a result, the total amounts of $$^{131}$$I and $$^{137}$$Cs discharged into the atmosphere from 5 JST on March 12 to 0 JST on March 20 were estimated to be approximately 2.0$$times$$10$$^{17}$$ and 1.3$$times$$10$$^{16}$$ Bq, respectively.

Journal Articles

Numerical experiments on dispersion of radionuclides in the ocean released from the Fukushima Daiichi Nuclear Power Plant

Kawamura, Hideyuki; Kobayashi, Takuya; Furuno, Akiko; In, Teiji*; Ishikawa, Yoichi*; Nakayama, Tomoharu*; Shima, Shigeki*; Awaji, Toshiyuki*

Reports of Research Institute for Applied Mechanics, Kyushu University, (143), p.111 - 117, 2012/09

Because of the Fukushima Dai-ichi Nuclear Power Plant disaster, some radionuclides were released into the ocean from the Fukushima Dai-ichi Nuclear Power Plant. In response to this situation, numerical experiments were carried out at Japan Atomic Energy Agency using an oceanic dispersion model and an ocean general circulation model to estimate an effect of the radionuclides on marine environment. It was suggested that the radionuclides deposited from the atmosphere mainly in the middle of March after the disaster spread over a comparatively wide area of the Pacific Ocean east of Japan. On the other hand the radionuclides directly released into the ocean from the Fukushima Dai-ichi Nuclear Power Plant were carried along the coast and then spread along the Kuroshio extension.

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