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JAEA Reports

Annual report on the effluent control of low level liquid waste in Nuclear Fuel Cycle Engineering Laboratories FY2022

Kokubun, Yuji; Nakada, Akira; Seya, Natsumi; Nagaoka, Mika; Koike, Yuko; Kubota, Tomohiro; Hirao, Moe; Yoshii, Hideki*; Otani, Kazunori*; Hiyama, Yoshinori*; et al.

JAEA-Review 2023-052, 118 Pages, 2024/03

JAEA-Review-2023-052.pdf:3.67MB

Based on the regulations (the safety regulation of Tokai Reprocessing Plant, the safety regulation of nuclear fuel material usage facilities, the radiation safety rule, the regulation about prevention from radiation hazards due to radioisotopes, which are related with the nuclear regulatory acts, the local agreement concerning with safety and environment conservation around nuclear facilities, the water pollution control law, and by law of Ibaraki Prefecture), the effluent control of liquid waste discharged from the Nuclear Fuel Cycle Engineering Laboratories of Japan Atomic Energy Agency has been performed. This report describes the effluent control results of the liquid waste in the fiscal year 2022. In this period, the concentrations and the quantities of the radioactivity in liquid waste discharged from the reprocessing plant, the plutonium fuel fabrication facilities, and the other nuclear fuel material usage facilities were much lower than the limits authorized by the above regulations.

Journal Articles

Thermophysical properties of dense molten Al$$_{2}$$O$$_{3}$$ determined by aerodynamic levitation

Sun, Y.*; Takatani, Tomoya*; Muta, Hiroaki*; Fujieda, Shun*; Kondo, Toshiki; Kikuchi, Shin; Kargl, F.*; Oishi, Yuji*

International Journal of Thermophysics, 45(1), p.11_1 - 11_19, 2024/01

 Times Cited Count:0 Percentile:0.07(Thermodynamics)

no abstracts in English

Journal Articles

Development of a D$$_2$$O/H$$_2$$O vapor generator for contrast-variation neutron scattering

Arima-Osonoi, Hiroshi*; Takata, Shinichi; Kasai, Satoshi*; Ouchi, Keiichi*; Morikawa, Toshiaki*; Miyata, Noboru*; Miyazaki, Tsukasa*; Aoki, Hiroyuki; Iwase, Hiroki*; Hiroi, Kosuke; et al.

Journal of Applied Crystallography, 56(6), p.1802 - 1812, 2023/12

 Times Cited Count:0 Percentile:0.02(Chemistry, Multidisciplinary)

Journal Articles

Study on criticality safety control of fuel debris for validation of methodology applied to the safety regulation

Suyama, Kenya; Ueki, Taro; Gunji, Satoshi; Watanabe, Tomoaki; Araki, Shohei; Fukuda, Kodai; Yamane, Yuichi; Izawa, Kazuhiko; Nagaya, Yasunobu; Kikuchi, Takeo; et al.

Proceedings of 12th International Conference on Nuclear Criticality Safety (ICNC2023) (Internet), 6 Pages, 2023/10

To remove and store safely the fuel debris generated by the severe accident of the Fukushima Daiichi Nuclear Power Station in 2011 is one of the most important and challenging topics for decommissioning of the damaged reactors in Fukushima. To validate the adopted method for the evaluation of criticality safety control of the fuel debris through comparison with the experimental data obtained by the criticality experiments, the Nuclear Regulation Authority (NRA) of Japan funds a research and development project which was entrusted to the Nuclear Safety Research Center (NSRC) of Japan Atomic Energy Agency (JAEA) from 2014. In this project, JAEA has been conducting such activities as i) comprehensive computation of the criticality characteristics of the fuel debris and making database (criticality map of the fuel debris), ii) development of new continuous energy Monte Carlo code, iii) evaluation of criticality accident and iv) modification of the critical assembly STACY for the experiments for validation of criticality safety control methodology. After the last ICNC2019, the project has the substantial progress in the modification of STACY which will start officially operation from May 2024 and the development of the Monte Carlo Code "Solomon" suitable for the criticality calculation for materials having spatially random distribution complies with the power spectrum. We present the whole picture of this research and development project and status of each technical topics in the session.

Journal Articles

Development of safety design technologies for sodium-cooled fast reactor coupled to thermal energy storage system with sodium-molten salt heat exchanger; Project overview

Yamano, Hidemasa; Kurisaka, Kenichi; Takano, Kazuya; Kikuchi, Shin; Kondo, Toshiki; Umeda, Ryota; Shirakura, Shota*

Dai-27-Kai Doryoku, Enerugi Gijutsu Shimpojiumu Koen Rombunshu (Internet), 5 Pages, 2023/09

This project studies investigation on safety design guideline and risk assessment technology for sodium-cooled fast reactor with the molten-salt heat storage system, development of evaluation method for heat transferring performance between sodium and molten-salt and improvement of the performance, and evaluation of chemical reaction characteristic between sodium and molten-salt and improvement of its safety. The project overview is presented in this report.

Journal Articles

Magnetic excitation in the $$S$$=1/2 Ising-like antiferromagnetic chain CsCoCl$$_{3}$$ in longitudinal magnetic fields studied by high-field ESR measurements

Kimura, Shojiro*; Onishi, Hiroaki; Okunishi, Koichi*; Akaki, Mitsuru*; Narumi, Yasuo*; Hagiwara, Masayuki*; Kindo, Koichi*; Kikuchi, Hikomitsu*

Journal of the Physical Society of Japan, 92(9), p.094701_1 - 094701_9, 2023/09

 Times Cited Count:0 Percentile:0(Physics, Multidisciplinary)

Journal Articles

Validation practices of multi-physics core performance analysis in an advanced reactor design study

Doda, Norihiro; Kato, Shinya; Hamase, Erina; Kuwagaki, Kazuki; Kikuchi, Norihiro; Ohgama, Kazuya; Yoshimura, Kazuo; Yoshikawa, Ryuji; Yokoyama, Kenji; Uwaba, Tomoyuki; et al.

Proceedings of 20th International Topical Meeting on Nuclear Reactor Thermal Hydraulics (NURETH-20) (Internet), p.946 - 959, 2023/08

An innovative design system named ARKADIA is being developed to realize the design of advanced nuclear reactors as safe, economical, and sustainable carbon-free energy sources. This paper focuses on ARKADIA-Design for design studies as a part of ARKADIA and introduces representative verification methods for numerical analysis methods of the core design. ARKADIA-Design performs core performance analysis of sodium-cooled fast reactors using a multiphysics approach that combines neutronics, thermal-hydraulics, core mechanics, and fuel pin behavior analysis codes. To confirm the validity of these analysis codes, validation matrices are identified with reference to experimental data and reliable numerical analysis results. The analysis models in these codes and the representative practices for the validation matrices are described.

Journal Articles

Thermophysical properties of molten (Fe$$_{2}$$O$$_{3}$$)$$_{0.95}$$-(SiO$$_{2}$$)$$_{0.05}$$ measured by aerodynamic levitation

Kondo, Toshiki; Toda, Taro*; Takeuchi, Junichi*; Kikuchi, Shin; Kargl, F.*; Muta, Hiroaki*; Oishi, Yuji*

High Temperatures-High Pressures, 52(3-4), p.307 - 321, 2023/06

 Times Cited Count:0 Percentile:0.02(Thermodynamics)

In order to establish an evaluation method/numerical simulation for nuclear reactor safety under severe accidental conditions, it is necessary to obtain the physical properties, especially fluidity of the relevant molten materials at very high temperatures. In this study, thermophysical properties such as density and viscosity were obtained for (Fe$$_{2}$$O$$_{3}$$)$$_{0.95}$$-(SiO$$_{2}$$)$$_{0.05}$$, which is a representative composition in the early stage of severe accident. (Fe$$_{2}$$O$$_{3}$$)$$_{0.95}$$-(SiO$$_{2}$$)$$_{0.05}$$ is produced by the contact between the molten oxide of steel, which is the main component of the reactor, and SiO$$_{2}$$, which is the main component of concrete. As a result, the physical properties of the (Fe$$_{2}$$O$$_{3}$$)$$_{0.95}$$-(SiO$$_{2}$$)$$_{0.05}$$ mixture were almost the same as those of Fe$$_{2}$$O$$_{3}$$ obtained in previous studies, and it could be concluded that a small amount of SiO$$_{2}$$ (about 5 mol.%) did not significantly affect the fluidity of Fe$$_{2}$$O$$_{3}$$.

JAEA Reports

Annual report on the effluent control of low level liquid waste in Nuclear Fuel Cycle Engineering Laboratories FY2021

Nakada, Akira; Kanai, Katsuta; Kokubun, Yuji; Nagaoka, Mika; Koike, Yuko; Yamada, Ryohei*; Kubota, Tomohiro; Hirao, Moe; Yoshii, Hideki*; Otani, Kazunori*; et al.

JAEA-Review 2022-079, 116 Pages, 2023/03

JAEA-Review-2022-079.pdf:2.77MB

Based on the regulations (the safety regulation of Tokai Reprocessing Plant, the safety regulation of nuclear fuel material usage facilities, the radiation safety rule, the regulation about prevention from radiation hazards due to radioisotopes, which are related with the nuclear regulatory acts, the local agreement concerning with safety and environment conservation around nuclear facilities, the water pollution control law, and by law of Ibaraki Prefecture), the effluent control of liquid waste discharged from the Nuclear Fuel Cycle Engineering Laboratories of Japan Atomic Energy Agency has been performed. This report describes the effluent control results of the liquid waste in the fiscal year 2021. In this period, the concentrations and the quantities of the radioactivity in liquid waste discharged from the reprocessing plant, the plutonium fuel fabrication facilities, and the other nuclear fuel material usage facilities were much lower than the limits authorized by the above regulations.

Journal Articles

Thinning behavior of solid boron carbide immersed in molten stainless steel for core disruptive accident of sodium-cooled fast reactor

Emura, Yuki; Takai, Toshihide; Kikuchi, Shin; Kamiyama, Kenji; Yamano, Hidemasa; Yokoyama, Hiroki*; Sakamoto, Kan*

Journal of Nuclear Science and Technology, 10 Pages, 2023/00

 Times Cited Count:0 Percentile:0.01(Nuclear Science & Technology)

Journal Articles

Development of safety design technologies for sodium-cooled fast reactor coupled to thermal energy storage system with sodium-molten salt heat exchanger

Yamano, Hidemasa; Kurisaka, Kenichi; Takano, Kazuya; Kikuchi, Shin; Kondo, Toshiki; Umeda, Ryota; Shirakura, Shota*; Hayashi, Masaaki*

Proceedings of 8th International Conference on New Energy and Future Energy Systems (NEFES 2023) (Internet), p.27 - 34, 2023/00

 Times Cited Count:0

This project studies investigation on safety design guideline and risk assessment technology for sodium-cooled fast reactor with the molten-salt heat storage system, development of evaluation method for heat transferring performance between sodium and molten-salt and improvement of the performance, and evaluation of chemical reaction characteristic between sodium and molten-salt and improvement of its safety. The project overview is presented in this report.

Journal Articles

Possible options for efficient wide-band polychromatic measurements using chopper spectrometers at pulsed sources

Nakajima, Kenji; Kikuchi, Tatsuya*; Kawamura, Seiko; Kambara, Wataru*

EPJ Web of Conferences, 272, p.02012_1 - 02012_8, 2022/11

We will present some of attempts on AMATEAS, a cold-neutron chopper spectrometer at a pulsed source, to increase time-windows at a single-measurement condition. One of ways is that, by allowing interveined trajectories on the time-of-flight diagram, the usable width selectable for $$E$$$$_{rm is}$$ is can be increased. Based on our experiences, the conditions of pulse repetition rate multiplication based polychromatic $$E$$$$_{rm i}$$ measurements on chopper spectrometers at pulsed sources will be discussed. Optimization of wide-band polychromatic $$E$$$$_{rm i}$$ measurements and a generalized formulated condition will be proposed. Application of our idea to existing spectrometers and to the criteria design of an optimized chopper spectrometer will be also discussed with suggesting further possibility to improve efficiency by modifying the pulse shaping chopper.

Journal Articles

Thermophysical properties of molten FeO$$_{1.5}$$, (FeO$$_{1.5}$$)$$_{0.86}$$-(ZrO$$_{2}$$)$$_{0.14}$$ and (FeO$$_{1.5}$$)$$_{0.86}$$-(UO$$_{2}$$)$$_{0.14}$$

Kondo, Toshiki; Toda, Taro*; Takeuchi, Junichi*; Kargl, F.*; Kikuchi, Shin; Muta, Hiroaki*; Oishi, Yuji*

Journal of Nuclear Science and Technology, 59(9), p.1139 - 1148, 2022/09

 Times Cited Count:1 Percentile:31.61(Nuclear Science & Technology)

no abstracts in English

Journal Articles

Sodium-cooled Fast Reactors

Ohshima, Hiroyuki; Morishita, Masaki*; Aizawa, Kosuke; Ando, Masanori; Ashida, Takashi; Chikazawa, Yoshitaka; Doda, Norihiro; Enuma, Yasuhiro; Ezure, Toshiki; Fukano, Yoshitaka; et al.

Sodium-cooled Fast Reactors; JSME Series in Thermal and Nuclear Power Generation, Vol.3, 631 Pages, 2022/07

This book is a collection of the past experience of design, construction, and operation of two reactors, the latest knowledge and technology for SFR designs, and the future prospects of SFR development in Japan. It is intended to provide the perspective and the relevant knowledge to enable readers to become more familiar with SFR technology.

Journal Articles

Thermal decomposition of perlite concrete under different water vapor pressures

Iwasaki, Shun*; Sakai, Yasuhiro*; Kikuchi, Shin; Koga, Nobuyoshi*

Journal of Thermal Analysis and Calorimetry, 147(11), p.6309 - 6322, 2022/06

 Times Cited Count:5 Percentile:41.15(Thermodynamics)

The influence of atmospheric water vapor on the multistep thermal decomposition of perlite concrete was investigated in detail by separating the component reaction steps using kinetic deconvolution analysis (KDA). The retardation of thermal decomposition of Ca(OH)$$_{2}$$ and the acceleration of thermal decomposition of CaCO$$_{3}$$ were identified as specific effect of atmospheric water vapor.

Journal Articles

Urea-introduced ionic liquid for the effective extraction of Pt(IV) and Pd(II) ions

Ueda, Yuki; Eguchi, Ayano; Tokunaga, Kohei; Kikuchi, Kei*; Sugita, Tsuyoshi; Okamura, Hiroyuki; Naganawa, Hirochika

Industrial & Engineering Chemistry Research, 61(19), p.6640 - 6649, 2022/05

 Times Cited Count:1 Percentile:12.67(Engineering, Chemical)

no abstracts in English

Journal Articles

Influence of atmospheric CO$$_{2}$$ on the thermal decomposition of perlite concrete

Sakai, Yasuhiro*; Iwasaki, Shun*; Kikuchi, Shin; Koga, Nobuyoshi*

Journal of Thermal Analysis and Calorimetry, 147(10), p.5801 - 5813, 2022/05

 Times Cited Count:8 Percentile:59.41(Thermodynamics)

The influence of atmospheric CO$$_{2}$$ on the multistep thermal decomposition of perlite concrete was investigated in detail by separating the component reaction steps using kinetic deconvolution analysis (KDA). The carbonation of Ca(OH)$$_{2}$$ and the retardation of the thermal decomposition of CaCO$$_{3}$$ were identified as specific effect of atmospheric CO$$_{2}$$.

Journal Articles

Thermal behavior and kinetics of the reaction between liquid sodium and calcium hydroxide

Kikuchi, Shin; Koga, Nobuyoshi*

Journal of Thermal Analysis and Calorimetry, 147(7), p.4635 - 4643, 2022/04

 Times Cited Count:1 Percentile:7.32(Thermodynamics)

In a sodium-cooled fast reactor (SFR), sodium-concrete reaction (SCR) may probably occur when liquid sodium from cooling system spilled into the floor may lead to fail the steel liner as protector of the structural concretes. The structural concretes of SFR comprises siliceous concreate as main body of reactor structure and perlite concrete placed between the steel liner and the siliceous concrete serving as a protector and an insulator, respectively. Therefore, the reaction behaviour between the perlite concrete and liquid sodium in the early stage of SCR should be focused. In this study, for the first step of elucidation on SCR, thermal behaviour of sodium-calcium hydroxide reaction was investigated using a differential scanning calorimetry (DSC). It was revealed that the reaction between Na(l) and Ca(OH)$$_{2}$$(s) initiates at approximately 550 K, producing the product layer composed of CaO(s) and NaOH(s), which is evident from XRD pattern of solid product after DSC measurement. The kinetic consideration of the cited reaction was carried out to obtain the activation energy.

JAEA Reports

Radiation monitoring using manned helicopter around the Nuclear Power Station in the fiscal year 2020 (Contract research)

Futemma, Akira; Sanada, Yukihisa; Ishizaki, Azusa; Kawasaki, Yoshiharu*; Iwai, Takeyuki*; Hiraga, Shogo*; Sato, Kazuhiko*; Haginoya, Masashi*; Matsunaga, Yuki*; Kikuchi, Hikaru*; et al.

JAEA-Technology 2021-029, 132 Pages, 2022/02

JAEA-Technology-2021-029.pdf:24.58MB

By the nuclear disaster of Fukushima Daiichi Nuclear Power Station (FDNPS), Tokyo Electric Power Company (TEPCO), caused by the Great East Japan Earthquake and the following tsunami on March 11, 2011, a large amount of radioactive material was released from the FDNPS. After the nuclear disaster, airborne radiation monitoring using manned helicopter has been conducted around FDNPS. The results of the airborne radiation monitoring and the evaluation for temporal change of dose rate in the fiscal 2020 were summarized in this report. Analysis considering topographical effects was applied to the result of the airborne monitoring to improve the accuracy of conventional method. In addition, technique for discriminating gamma rays from the ground and those from the airborne Rn-progenies was also utilized to evaluate their effect on airborne radiation monitoring.

Journal Articles

Thermally stimulated liquid Na-CaCO$$_{3}$$ reaction; A Physicogeometrical kinetic approach toward the safety assessment of Na-cooled fast reactors

Koga, Nobuyoshi*; Kikuchi, Shin

Industrial & Engineering Chemistry Research, 61(7), p.2759 - 2770, 2022/02

 Times Cited Count:0 Percentile:0(Engineering, Chemical)

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