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Journal Articles

Consequence analysis of a postulated nuclear excursion in BWR spent fuel pool using 1/$$f^{beta}$$ spectrum model of randomization

Simanullang, I.; Yamane, Yuichi; Kikuchi, Takeo; Tonoike, Kotaro

Annals of Nuclear Energy, 147, p.107675_1 - 107675_6, 2020/11

 Times Cited Count:2 Percentile:18.47(Nuclear Science & Technology)

Journal Articles

Corrosion behavior of Fe, Cr, Ni and their alloys in sodium molybdate melts

Nagai, Takayuki; Kikuchi, Kotaro*; Kano, Yoshiharu*

Nihon Genshiryoku Gakkai Wabun Rombunshi, 12(1), p.76 - 88, 2013/03

To understand the corrosion behavior of stainless steel and Ni-Cr alloys in sodium molybdate melts, the immersed corrosion tests of Fe, Cr, Ni, SUS316, 55Ni-45Cr, and Inconel 690 specimens were carried out in Na$$_{2}$$MoO$$_{4}$$ and Na$$_{2}$$Mo$$_{2}$$O$$_{7}$$ melts at 750 $$^{circ}$$C. The results of the immersed test, it was found that the corrosion rate decreased with an increase of chromium content in chemical composition of specimens. It was observed that Cr$$_{2}$$O$$_{3}$$ formed on the surface of Cr, 55Ni-45Cr, and Inconel 690 specimens by immersed in Na$$_{2}$$Mo$$_{2}$$O$$_{7}$$ melt, which corrosion rates were low in the melt, and we presumed that this Cr$$_{2}$$O$$_{3}$$ on the surface controlled the corrosion behavior of their material in the melt.

Journal Articles

Identified charged hadron production in $$p + p$$ collisions at $$sqrt{s}$$ = 200 and 62.4 GeV

Adare, A.*; Afanasiev, S.*; Aidala, C.*; Ajitanand, N. N.*; Akiba, Yasuyuki*; Al-Bataineh, H.*; Alexander, J.*; Aoki, Kazuya*; Aphecetche, L.*; Armendariz, R.*; et al.

Physical Review C, 83(6), p.064903_1 - 064903_29, 2011/06

 Times Cited Count:191 Percentile:99.41(Physics, Nuclear)

Transverse momentum distributions and yields for $$pi^{pm}, K^{pm}, p$$, and $$bar{p}$$ in $$p + p$$ collisions at $$sqrt{s}$$ = 200 and 62.4 GeV at midrapidity are measured by the PHENIX experiment at the RHIC. We present the inverse slope parameter, mean transverse momentum, and yield per unit rapidity at each energy, and compare them to other measurements at different $$sqrt{s}$$ collisions. We also present the scaling properties such as $$m_T$$ and $$x_T$$ scaling and discuss the mechanism of the particle production in $$p + p$$ collisions. The measured spectra are compared to next-to-leading order perturbative QCD calculations.

Journal Articles

Azimuthal correlations of electrons from heavy-flavor decay with hadrons in $$p+p$$ and Au+Au collisions at $$sqrt{s_{NN}}$$ = 200 GeV

Adare, A.*; Afanasiev, S.*; Aidala, C.*; Ajitanand, N. N.*; Akiba, Yasuyuki*; Al-Bataineh, H.*; Alexander, J.*; Aoki, Kazuya*; Aphecetche, L.*; Aramaki, Y.*; et al.

Physical Review C, 83(4), p.044912_1 - 044912_16, 2011/04

 Times Cited Count:10 Percentile:54.89(Physics, Nuclear)

Measurements of electrons from the decay of open-heavy-flavor mesons have shown that the yields are suppressed in Au+Au collisions compared to expectations from binary-scaled $$p+p$$ collisions. Here we extend these studies to two particle correlations where one particle is an electron from the decay of a heavy flavor meson and the other is a charged hadron from either the decay of the heavy meson or from jet fragmentation. These measurements provide more detailed information about the interaction between heavy quarks and the quark-gluon matter. We find the away-side-jet shape and yield to be modified in Au+Au collisions compared to $$p+p$$ collisions.

Journal Articles

Corrosion behavior of SUS316 clad in alkalis molybdate melt

Nagai, Takayuki; Kikuchi, Kotaro*; Kano, Yoshiharu*; Fukushima, Mineo

Nihon Genshiryoku Gakkai Wabun Rombunshi, 7(4), p.370 - 379, 2008/12

Study of a new pyrochemical processing using alkaline molybdate melt has been carrying out as a candidate reprocessing process for spent oxide fuels. In our previous study, we had confirmed that melting of UO$$_{2}$$ pellet into a molten Na$$_{2}$$MoO$$_{4}$$-MoO$$_{3}$$ and electrolytic recovering of UO$$_{2}$$ from the melt included uranyl ions. In this report, the corrosion behavior of the SUS316 cladding tube in molten Na$$_{2}$$MoO$$_{4}$$-MoO$$_{3}$$ was evaluated, and we confirmed the dissolution of SUS316 elements into the melt when the amount of additional MoO$$_{3}$$ was excess. And, it is necessary to understand an appropriate amount of additional MoO$$_{3}$$ since the result of this study.

Journal Articles

Progress in R&D efforts on the energy recovery linac in Japan

Sakanaka, Shogo*; Ago, Tomonori*; Enomoto, Atsushi*; Fukuda, Shigeki*; Furukawa, Kazuro*; Furuya, Takaaki*; Haga, Kaiichi*; Harada, Kentaro*; Hiramatsu, Shigenori*; Honda, Toru*; et al.

Proceedings of 11th European Particle Accelerator Conference (EPAC '08) (CD-ROM), p.205 - 207, 2008/06

Future synchrotron light sources based on the energy-recovery linacs (ERLs) are expected to be capable of producing super-brilliant and/or ultra-short pulses of synchrotron radiation. Our Japanese collaboration team is making efforts for realizing an ERL-based hard X-ray source. We report recent progress in our R&D efforts.

Journal Articles

Kinetic parameter $$beta_{rm eff}/ell$$ measurement on low enriched uranyl nitrate solution with single unit cores (600$$phi$$, 280T, 800$$phi$$) of STACY

Tonoike, Kotaro; Miyoshi, Yoshinori; Kikuchi, Tsukasa*; Yamamoto, Toshihiro

Journal of Nuclear Science and Technology, 39(11), p.1227 - 1236, 2002/11

 Times Cited Count:21 Percentile:76.73(Nuclear Science & Technology)

Kinetic parameter $$beta_{rm eff}/ell$$ of low enriched uranyl nitrate solution was measured by the pulsed neutron source method in the STACY. This measurement was repeated systematically over several uranium concentrations from 193.7 gU/$$ell$$ to 432.1 gU/$$ell$$. Used core tanks were two cylindrical tanks whose diameters are 600 mm and 800 mm and one slab tank which has 280 mm thickness and 700 mm width. In this report, experimental data such as solution conditions, critical solution level for each solution condition, subcritical solution levels where measurements were conducted, measured decay time constants of prompt neutron and extrapolated $$beta_{rm eff}/ell$$ values are described as well as basic principle of the pulsed neutron source method. $$beta_{rm eff}/ell$$ values were evaluated also by computation with the diffusion code CITATION in SRAC and the nuclear data library JENDL 3.2. Both experimental and computational $$beta_{rm eff}/ell$$ values show good agreement.

Oral presentation

Measurement and analysis by SWAT4.0 of isotopic composition of PWR high-burnup lead use assembly

Watanabe, Tomoaki; Kikuchi, Takeo; Tonoike, Kotaro; Suyama, Kenya

no journal, , 

In order to obtain new post irradiation examination data for validation of burnup calculation codes, isotopic compositions of 9 samples obtained from a 17$$times$$17 high-burnup lead use assembly (53 GWd/t), which was irradiated in Ohi Nuclear Power Station Unit 4, were measured. The isotopic compositions were also evaluated by burnup calculations with SWAT4.0 code and compared with the measurements.

Oral presentation

Cyclic voltammetry for high concentration lanthanide ions in molten LiCl-KCl eutectic

Nagai, Takayuki; Kikuchi, Kotaro*; Hirano, Hiroyasu; Fukasawa, Kazuhito*; Uehara, Akihiro*; Yamana, Hajimu*

no journal, , 

In the dry reprocessing process for spent nuclear fuel by the electro-metallurgical method, we are studying the online monitoring technique of dissolved ion concentration in molten LiCl-KCl eutectic. In this study, the cyclic voltammetry was carried out in the molten LiCl-KCl eutectic added lanthanide chlorides (NdCl$$_{3}$$, etc.) and we confirmed that the peak current density by the reductive reaction of dissolved ions increased in proportion to the dissolved ion concentration until about 4 mol%.

Oral presentation

Development of measurement techniques for density and liquid level of molten salt to assess an inventory in equipment of Pyro-proccesing

Fukushima, Mineo; Nagai, Takayuki; Kikuchi, Kotaro*; Hirano, Hiroyasu; Myochin, Munetaka

no journal, , 

Measurement techniques for density and liquid level of molten salt are very important elements in material accountancy system for pyro-processing and also in process control system. Test equipments were developed for the in-situ measurement of density and liquid level of molten salt and provided to the measurement experiments. Measurement of the density of LiCl-KCl eutectic showed a good agreement with published data in an error of 0.2%. Measurement of the liquid level of LiCl-KCl eutectic showed an error of 0.5 mm against theoretical values. From these results, both techniques were considered to be promising although the additional data accumulation is needed to estimate the performance statistically by using practical equipment.

Oral presentation

Corrosion behavior of Fe, Cr, and Ni in molten sodium molybdate

Nagai, Takayuki; Kikuchi, Kotaro*; Kano, Yoshiharu*; Hirano, Hiroyasu

no journal, , 

On the dry reprocessing process study by using a molten sodium molybdate, the SUS316 stainless steel of clad material was dissolved into the melt. In this study, we carried out the immersed corrosion test of Fe, Cr, and Ni in molten sodium molybdate, and estimated the corrosion behavior of these material and dissolution content in the melt.

Oral presentation

Consequence analysis of postulated criticality in SFP using the randomized model of fuel debris

Simanullang, I.; Yamane, Yuichi; Kikuchi, Takeo; Tonoike, Kotaro

no journal, , 

Oral presentation

Corrosion behavior of SUS316 stainless steel in molten sodium molybdate

Nagai, Takayuki; Kikuchi, Kotaro*; Kano, Yoshiharu*; Fukushima, Mineo

no journal, , 

The study of a pyrochemical process by using molten alkaline molybdate has been carried out as a candidate reprocessing process for spent oxide fuels. In this study, the immersed corrosion tests of SUS316 tube were carried out in molten Na$$_{2}$$MoO$$_{4}$$-MoO$$_{3}$$ mixtures with MoO$$_{3}$$ mole fractions. Results showed that the concentration of dissolved iron and nickel species in the melt increased with the increase of the MoO$$_{3}$$ mole fraction, whereas the concentrations of dissolved chromium species remained constant at low values, independent of the MoO$$_{3}$$ content. It is found that the corrosion of SUS316 specimens in molten Na$$_{2}$$MoO$$_{4}$$-MoO$$_{3}$$ mixtures proceeds with the iron and nickel preferably dissolved into the melt and with chromium-rich corrosion films formed at the surface.

Oral presentation

Consequence analysis of a postulated nuclear excursion in BWR spent fuel pool using 1/$$f^{beta}$$ spectrum model of randomization

Simanullang, I.; Yamane, Yuichi; Kikuchi, Takeo; Tonoike, Kotaro

no journal, , 

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