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Kinoshita, Norikazu*; Noto, Takuma*; Nakajima, Hitoshi*; Kosako, Kazuaki*; Kato, Takahiro*; Kuroiwa, Yoichi*; Kurabe, Misako*; Sasaki, Yuki*; Torii, Kazuyuki*; Maeda, Makoto; et al.
Journal of Radioanalytical and Nuclear Chemistry, 332(2), p.479 - 486, 2023/02
Nakamura, Shoji; Shibahara, Yuji*; Kimura, Atsushi; Endo, Shunsuke; Shizuma, Toshiyuki*
Journal of Nuclear Science and Technology, 10 Pages, 2023/00
In recent years, research has been advanced on lead-cooled fast reactors and accelerator drive systems, and it is required to improve the accuracy of the neutron capture cross section of Pb isotopes. Although Pb has a small natural abundance, it is of importance because it produces the long-lived radionuclide
Pb (17.3 million years) by neutron capture reaction. However, it is difficult to measure its cross section by a conventional activation method using a nuclear reactor because the induced radioactivity of
Pb is weak. Hence, the cross-section measurement was performed by applying mass spectrometry. This presentation gives the details of the experiment and the results obtained in the neutron capture cross-section measurement of
Pb using mass spectroscopy.
Endo, Shunsuke; Okudaira, Takuya*; Abe, Ryota*; Fujioka, Hiroyuki*; Hirota, Katsuya*; Kimura, Atsushi; Kitaguchi, Masaaki*; Oku, Takayuki; Sakai, Kenji; Shima, Tatsushi*; et al.
Physical Review C, 106(6), p.064601_1 - 064601_7, 2022/12
Times Cited Count:0 Percentile:0.02(Physics, Nuclear)no abstracts in English
Nakamura, Shoji; Shibahara, Yuji*; Endo, Shunsuke; Kimura, Atsushi
Journal of Nuclear Science and Technology, 59(11), p.1388 - 1398, 2022/11
Times Cited Count:0 Percentile:0.01(Nuclear Science & Technology)The present study selected Np among radioactive nuclides and aimed to measure the thermal-neutron capture cross-section for
Np in a well-thermalized neutron field by an activation method. A
Np standard solution was used for irradiation samples. A thermal-neutron flux at an irradiation position was measured with neutron flux monitors:
Sc,
Co,
Mo,
Ta and
Au. The
Np sample and flux monitors were irradiated together for 30 minutes in the graphite thermal column equipped with the Kyoto University Research Reactor. The similar irradiation was carried out twice. After the irradiations, the
Np samples were quantified using 312-keV gamma ray emitted from
Pa in a radiation equilibrium with
Np. The reaction rates of
Np were obtained from gamma-ray peak net counts given by
Np, and then the thermal-neutron capture cross-section of
Np was found to be 173.8
4.4 barn by averaging the results obtained by the two irradiations. The present result was in agreement with the reported data given by a time-of-flight method within the limit of uncertainty.
Iwamoto, Osamu; Iwamoto, Nobuyuki; Kimura, Atsushi; Tada, Kenichi; Sugawara, Takanori; Yokoyama, Kenji
Kaku Deta Nyusu (Internet), (133), p.1 - 6, 2022/10
no abstracts in English
Shizuma, Toshiyuki*; Endo, Shunsuke; Kimura, Atsushi; Massarczyk, R.*; Schwengner, R.*; Beyer, R.*; Hensel, T.*; Hoffmann, H.*; Junghans, A.*; Rmer, K.*; et al.
Physical Review C, 106(4), p.044326_1 - 044326_11, 2022/10
Times Cited Count:0 Percentile:0.02(Physics, Nuclear)no abstracts in English
Mastromarco, M.*; Amaducci, S.*; Colonna, N.*; Kimura, Atsushi; 118 of others*
European Physical Journal A, 58(8), p.147_1 - 147_13, 2022/08
Times Cited Count:0 Percentile:0.02(Physics, Nuclear)no abstracts in English
Nakamura, Shoji; Toh, Yosuke; Kimura, Atsushi; Hatsukawa, Yuichi*; Harada, Hideo
Journal of Nuclear Science and Technology, 59(7), p.851 - 865, 2022/07
Times Cited Count:0 Percentile:0.01(Nuclear Science & Technology)The present study performed integral experiments of I using a fast-neutron source reactor "YAYOI" of the University of Tokyo to validate evaluated nuclear data libraries. The iodine-129 sample and flux monitors were irradiated by fast neutrons in the Glory hole of the YAYOI reactor. Reaction rates of
I were obtained by measurement of decay gamma-rays emitted from
I. The validity of the fast-neutron flux spectrum in the Glory hole was confirmed by the
ratios of the reaction rates of flux monitors. The experimental reaction rate of
I was compared with that calculated with both the fast-neutron flux spectrum and evaluated nuclear data libraries. The present study revealed that the evaluated nuclear data of
I cited in JENDL-4.0 should be reduced as much as 18% in neutron energies ranging from 10 keV to 3 MeV, and supported the reported data by Noguere
below 100 keV.
Nakamura, Shoji; Endo, Shunsuke; Kimura, Atsushi; Shibahara, Yuji*
KURNS Progress Report 2021, P. 93, 2022/07
In terms of nuclear transmutation studies of minor actinides in nuclear wastes, the present work selected Np among them and aimed to measure the thermal-neutron capture cross-section of
Np using a well-thermalized neutron field by a neutron activation method because there have been discrepancies among reported cross-section data. A
Np standard solution was used for irradiation samples. The thermal-neutron flux at an irradiation position was measured with flux monitors:
Sc,
Co,
Mo,
Ta and
Au. The
Np sample was irradiated together with the flux monitors for 30 minutes in the graphite thermal column equipped in the Kyoto University Research Reactor. The similar irradiation was repeated once more to confirm the reproducibility of the results. After irradiation, the
Np samples were quantified using 312-keV gamma-ray emitted from
Pa in radiation equilibrium with
Np. The reaction rates of
Np were obtained from the peak net counts of gamma-rays emitted from generated
Np, and then the thermal-neutron capture cross-section of
Np was found to be 173.8
4.7 barn by averaging the results obtained by the two irradiations. The present result was in agreement with the reported data given by a time-of-flight method within a limit of uncertainty.
Maeda, Makoto; Segawa, Mariko; Toh, Yosuke; Endo, Shunsuke; Nakamura, Shoji; Kimura, Atsushi
Scientific Reports (Internet), 12(1), p.6287_1 - 6287_8, 2022/06
Times Cited Count:1 Percentile:59.33(Multidisciplinary Sciences)Rovira Leveroni, G.; Kimura, Atsushi; Nakamura, Shoji; Endo, Shunsuke; Iwamoto, Osamu; Iwamoto, Nobuyuki; Katabuchi, Tatsuya*; Kodama, Yu*; Nakano, Hideto*; Sato, Yaoki*; et al.
Journal of Nuclear Science and Technology, 59(5), p.647 - 655, 2022/05
Times Cited Count:1 Percentile:30.57(Nuclear Science & Technology)Koga, Jun*; Takada, Shusuke*; Endo, Shunsuke; Fujioka, Hiroyuki*; Hirota, Katsuya*; Ishizaki, Kohei*; Kimura, Atsushi; Kitaguchi, Masaaki*; Niinomi, Yudai*; Okudaira, Takuya*; et al.
Physical Review C, 105(5), p.054615_1 - 054615_5, 2022/05
Times Cited Count:1 Percentile:67.14(Physics, Nuclear)no abstracts in English
Segawa, Mariko; Toh, Yosuke; Kai, Tetsuya; Kimura, Atsushi; Nakamura, Shoji
Annals of Nuclear Energy, 167, p.108828_1 - 108828_5, 2022/03
Times Cited Count:0 Percentile:0.01(Nuclear Science & Technology)Endo, Shunsuke; Kimura, Atsushi; Nakamura, Shoji; Iwamoto, Osamu; Iwamoto, Nobuyuki; Rovira Leveroni, G.; Terada, Kazushi*; Meigo, Shinichiro; Toh, Yosuke; Segawa, Mariko; et al.
Journal of Nuclear Science and Technology, 59(3), p.318 - 333, 2022/03
Times Cited Count:0 Percentile:0.01(Nuclear Science & Technology)Kumagai, Yuta; Kimura, Atsushi*; Taguchi, Mitsumasa*; Watanabe, Masayuki
Radiation Physics and Chemistry, 191, p.109831_1 - 109831_8, 2022/02
Times Cited Count:0 Percentile:0.01(Chemistry, Physical)In this study, we investigated and compared the effects of a high-silica zeolite (HMOR) on the radiation-induced degradation of three aromatic chlorides, 2-chlorophenol (2-ClPh), 2-chloroaniline (2-ClAn), and 2-chlorobenzoic acid (2-ClBA), in order to examine its potential to reduce the influence of ions in water matrix in the irradiation treatment of water-soluble organic compounds. In the presence of ions reactive to radicals, the degradation of 2-ClPh in water was inhibited, but the combined use of HMOR much improved the degradation yield. This improvement was attributed to high performance of HMOR in adsorption of 2-ClPh. Similarly, HMOR was effective for adsorption of 2-ClAn and facilitated the 2-ClAn degradation by irradiation. In contrast, HMOR was poor at adsorption of 2-ClBA and consistently the degradation of 2-ClBA in the water-HMOR mixture was inhibited by the radical scavenger. These results demonstrate that HMOR can mitigate the influence of radical scavengers in water.
Rovira Leveroni, G.; Katabuchi, Tatsuya*; Tosaka, Kenichi*; Matsuura, Shota*; Kodama, Yu*; Nakano, Hideto*; Iwamoto, Osamu; Kimura, Atsushi; Nakamura, Shoji; Iwamoto, Nobuyuki
Journal of Nuclear Science and Technology, 59(1), p.110 - 122, 2022/01
Times Cited Count:1 Percentile:30.57(Nuclear Science & Technology)Rovira Leveroni, G.; Kimura, Atsushi; Nakamura, Shoji; Endo, Shunsuke; Iwamoto, Osamu; Iwamoto, Nobuyuki; Katabuchi, Tatsuya*; Kodama, Yu*; Nakano, Hideto*
Journal of Nuclear Science and Technology, 11 Pages, 2022/00
Times Cited Count:0 Percentile:0.01(Nuclear Science & Technology)Nakamura, Shoji; Hatsukawa, Yuichi*; Kimura, Atsushi; Toh, Yosuke; Harada, Hideo
Journal of Nuclear Science and Technology, 58(12), p.1318 - 1329, 2021/12
Times Cited Count:0 Percentile:0.01(Nuclear Science & Technology)The present study performed fast-neutron capture cross-section measurement of Tc by an activation method using a fast-neutron source reactor "YAYOI" of the University of Tokyo. Technetium-99 samples were irradiated with reactor neutrons using a pneumatic system. Reaction rates of
Tc were obtained by measuring decay gamma rays emitted from
Tc. The neutron flux at an irradiation position was monitored with gold foils. The fast-neutron capture cross section of
Tc at neutron energy of 85 keV was derived as 0.432
0.023 barn by using the reaction rates of
Tc, evaluated cross-section data and the fast-neutron flux spectrum of the YAYOI reactor. The present study agreed with the evaluated nuclear data library JENDL-4.0.
Kodama, Yu*; Katabuchi, Tatsuya*; Rovira Leveroni, G.; Kimura, Atsushi; Nakamura, Shoji; Endo, Shunsuke; Iwamoto, Nobuyuki; Iwamoto, Osamu; Hori, Junichi*; Shibahara, Yuji*; et al.
Journal of Nuclear Science and Technology, 58(11), p.1159 - 1164, 2021/11
Times Cited Count:2 Percentile:53.86(Nuclear Science & Technology)Kimura, Kenta*; Yagi, Naoki*; Hasegawa, Shunsuke*; Hagihara, Masato; Miyake, Atsushi*; Tokunaga, Masashi*; Cao, H.*; Masuda, Takatsugu*; Kimura, Tsuyoshi*
Inorganic Chemistry, 60(20), p.15078 - 15084, 2021/10
Times Cited Count:0 Percentile:0.01(Chemistry, Inorganic & Nuclear)