Nakamura, Shoji; Kimura, Atsushi; Iwamoto, Osamu; Shibahara, Yuji*; Uehara, Akihiro*; Fujii, Toshiyuki*
KURNS Progress Report 2018, P. 106, 2019/08
Under the ImPACT project, the neutron capture cross-section measurements of Cesium-135 (Cs) among the long-lived fission products have been performed at Kyoto University. This paper reports measurements of the thermal-neutron capture cross-section of Cs at the Kyoto University Research Reactor (KUR).
Kimura, Atsushi; Nakamura, Shoji; Terada, Kazushi*; Nakao, Taro*; Mizuyama, Kazuhito*; Iwamoto, Nobuyuki; Iwamoto, Osamu; Harada, Hideo; Katabuchi, Tatsuya*; Igashira, Masayuki*; et al.
Journal of Nuclear Science and Technology, 56(6), p.479 - 492, 2019/06
Nakamura, Shoji; Kitatani, Fumito; Kimura, Atsushi; Uehara, Akihiro*; Fujii, Toshiyuki*
Journal of Nuclear Science and Technology, 56(6), p.493 - 502, 2019/06
The thermal-neutron capture cross-section()and resonance integral(I) were measured for the Np(n,)Np reaction by an activation method. A method with a Gadolinium filter, which is similar to the Cadmium difference method, was used to measure the with paying attention to the first resonance at 0.489 eV of Np, and a value of 0.133 eV was taken as a cut-off energy. Neptunium-237 samples were irradiated at the pneumatic tube of the Kyoto University Research Reactor in Institute for Integral Radiation and Nuclear Science, Kyoto University. Wires of Co/Al and Au/Al alloys were used as monitors to determine thermal-neutron fluxes and epi-thermal Westcott's indices at an irradiation position. A -ray spectroscopy was used to measure activities of Np, Np and neutron monitors. On the basis of Westcott's convention, the and I values were derived as 186.96.2 barn, and 100990 barn, respectively.
Lederer-Woods, C.*; Battino, U.*; Ferreira, P.*; Gawlik, A.*; Kimura, Atsushi; n_TOF Collaboration*; 128 of others*
Physics Letters B, 790, p.458 - 465, 2019/03
Hagiwara, Kaito*; Yano, Takatomi*; Das, P. K.*; Lorenz, S.*; Ou, Iwa*; Sakuda, Makoto*; Kimura, Atsushi; Nakamura, Shoji; Iwamoto, Nobuyuki; Harada, Hideo; et al.
Progress of Theoretical and Experimental Physics (Internet), 2019(2), p.023D01_1 - 023D01_26, 2019/02
Mastromarco, M.*; Manna, A.*; Aberle, O.*; Andrzejewski, J.*; Harada, Hideo; Kimura, Atsushi; n_TOF Collaboration*; 116 of others*
European Physical Journal A, 55(1), p.9_1 - 9_20, 2019/01
Nakamura, Shoji; Terada, Kazushi*; Kimura, Atsushi; Nakao, Taro*; Iwamoto, Osamu; Harada, Hideo; Uehara, Akihiro*; Takamiya, Koichi*; Fujii, Toshiyuki*
Journal of Nuclear Science and Technology, 56(1), p.123 - 129, 2019/01
Accurate data of -ray emission probabilities are frequently needed when one quantitatively determines the amount of isotope by -ray measurements or obtains neutron capture cross-sections using them. Americium-243, one of the most important minor actinides, produces Am after neutron capture. The 744-keV -ray decaying from the ground state of Am has a relatively large -ray emission probability c.a. 66%, however, its uncertainty is as large as 29%. The uncertainty of the -ray emission probability leads to a major factor of the systematic uncertainty on determining an amount of isotope, and therefore the -ray emission probability was measured by using an activation method and an examined level structure of Cm. In this study, the emission probability of 744-keV ray was derived as 66.51.1%, and its uncertainty was improved from 29% to 2%.
Nakamura, Shoji; Kimura, Atsushi; Hales, B. P.; Iwamoto, Osamu; Shibahara, Yuji*; Uehara, Akihiro*; Fujii, Toshiyuki*
JAEA-Conf 2018-001, p.199 - 203, 2018/12
Study on cross-section measurements has been promoted for Cs among long-lived fission products in ImPACT Project. The feasibility study on Se sample preparation also has been conducted to measure its cross sections in future. During the feasibility study, we started the neutron-capture cross-section measurements of stable Se isotopes. This paper reports research progresses on preparation of a radioactive Cs sample, neutron irradiation experiments with the Cs sample, and cross-section measurements of stable Se isotopes.
Shibahara, Yuji*; Uehara, Akihiro*; Fujii, Toshiyuki*; Nakamura, Shoji; Kimura, Atsushi; Hales, B. P.; Iwamoto, Osamu
JAEA-Conf 2018-001, p.205 - 210, 2018/12
In the ImPACT project, high-precision mass analysis was performed on a Cs standard solution for using Cs included in the standard solution as an impurity to measure the Cs cross-sections. A Cs standard solution of only 10Bq (pg order) was analyzed, and the isotope ratio of Cs and Cs was obtained with an accuracy of 0.5%.
Hatsukawa, Yuichi*; Hayakawa, Takehito*; Tsukada, Kazuaki; Hashimoto, Kazuyuki*; Sato, Tetsuya; Asai, Masato; Toyoshima, Atsushi; Tanimori, Toru*; Sonoda, Shinya*; Kabuki, Shigeto*; et al.
PLOS ONE (Internet), 13(12), p.e0208909_1 - e0208909_12, 2018/12
Imaging of Tc radioisotope was conducted using an electron tracking-Compton camera (ETCC). Tc emits 204, 582, and 835 keV rays, and was produced in the Mo(p,n)Tc reaction with a Mo-enriched target. The recycling of the Mo-enriched molybdenum trioxide was investigated, and the recycled yield of Mo was achieved to be 70% - 90%. The images were obtained with each of the three rays. Results showed that the spatial resolution increases with increasing -ray energy, and suggested that the ETCC with high-energy -ray emitters such as Tc is useful for the medical imaging of deep tissue and organs in the human body.
Terada, Kazushi*; Kimura, Atsushi; Nakao, Taro*; Nakamura, Shoji; Mizuyama, Kazuhito*; Iwamoto, Nobuyuki; Iwamoto, Osamu; Harada, Hideo; Katabuchi, Tatsuya*; Igashira, Masayuki*; et al.
Journal of Nuclear Science and Technology, 55(10), p.1198 - 1211, 2018/10
Harada, Masahide; Teshigawara, Makoto; Oi, Motoki; Klinkby, E.*; Zanini, L.*; Batkov, K.*; Oikawa, Kenichi; Toh, Yosuke; Kimura, Atsushi; Ikeda, Yujiro
Nuclear Instruments and Methods in Physics Research A, 903, p.38 - 45, 2018/09
Damone, L.*; Barbagallo, M.*; Mastromarco, M.*; Cosentino, L.*; Harada, Hideo; Kimura, Atsushi; n_TOF Collaboration*; 152 of others*
Physical Review Letters, 121(4), p.042701_1 - 042701_7, 2018/07
Iwamoto, Osamu; Iwamoto, Nobuyuki; Kimura, Atsushi; Yokoyama, Kenji; Tada, Kenichi
Kaku Deta Nyusu (Internet), (120), p.35 - 46, 2018/06
We report 30th WPEC meeting, expert group meeting, and subgroup meeting in Paris, May 14-18, 2018.
Meigo, Shinichiro; Matsuda, Hiroki; Iwamoto, Yosuke; Iwamoto, Hiroki; Hasegawa, Shoichi; Maekawa, Fujio; Yoshida, Makoto*; Ishida, Taku*; Makimura, Shunsuke*; Nakamoto, Tatsushi*
Proceedings of 9th International Particle Accelerator Conference (IPAC '18) (Internet), p.499 - 501, 2018/06
no abstracts in English
Kumagai, Yuta; Kimura, Atsushi*; Taguchi, Mitsumasa*; Watanabe, Masayuki
Journal of Radioanalytical and Nuclear Chemistry, 316(1), p.341 - 348, 2018/04
We studied effect of adsorption and condensation by zeolites on radiation-induced degradation of aqueous 2-chlorophenol (2-ClPh). This study aims to demonstrate that the solid-phase extraction using zeolites has potential advantage in treatments of aqueous organic pollutants. Among three zeolites examined in this study, a mordenite type zeolite (HMOR) that has a high Si to Al ratio (127 3) exhibited preferable performance as the matrix for the 2-ClPh degradation. HMOR adsorbed far more 2-ClPh than the other zeolites, which have lower Si/Al ratios. The irradiation of HMOR induced degradation of adsorbed 2-ClPh into Cl and organic by-products. We found a significant increase in Cl production by HMOR. The yield of Cl production in the presence of HMOR was as high as the yield in aqueous solution of 2-ClPh at a concentration 10 times higher. The increased Cl production indicates that the high concentration of adsorbed 2-ClPh led to effective use of the adsorbed energy of HMOR.
Barbagallo, M.*; Andrzejewski, J.*; Mastromarco, M.*; Perkowski, J.*; Damone, L. A.*; Gawlik, A.*; Kimura, Atsushi; n_TOF Collaboration*; 122 of others*
Nuclear Instruments and Methods in Physics Research A, 887, p.27 - 33, 2018/04
Okudaira, Takuya*; Takada, Shusuke*; Hirota, Katsuya*; Kimura, Atsushi; Kitaguchi, Masaaki*; Koga, Jun*; Nagamoto, Kosuke*; Nakao, Taro*; Okada, Anju*; Sakai, Kenji; et al.
Physical Review C, 97(3), p.034622_1 - 034622_15, 2018/03
Takada, Shusuke*; Okudaira, Takuya*; Goto, Fumiya*; Hirota, Katsuya*; Kimura, Atsushi; Kitaguchi, Masaaki*; Koga, Jun*; Nakao, Taro*; Sakai, Kenji; Shimizu, Hirohiko*; et al.
Journal of Instrumentation (Internet), 13(2), p.P02018_1 - P02018_21, 2018/02
Lerendegui-Marco, J.*; Guerrero, C.*; Mendoza, E.*; Quesada, J. M.*; Eberhardt, K.*; Junghans, A. R.*; Kimura, Atsushi; n_TOF Collaboration*; 126 of others*
Physical Review C, 97(2), p.024605_1 - 024605_21, 2018/02