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JAEA Reports

Conceptual study of Post Irradiation Examination (PIE) Facility at J-PARC

Saito, Shigeru; Meigo, Shinichiro; Makimura, Shunsuke*; Hirano, Yukinori*; Tsutsumi, Kazuyoshi*; Maekawa, Fujio

JAEA-Technology 2023-025, 48 Pages, 2024/03

JAEA-Technology-2023-025.pdf:3.11MB

JAEA has been developing Accelerator-Driven Systems (ADS) for research and development of nuclear transmutation using accelerators in order to reduce the volume and hazardousness of high-level radioactive waste generated by nuclear power plants. In order to prepare the material irradiation database necessary for the design of ADS and to study the irradiation effects in Lead-Bismuth Eutectic (LBE) alloys, a proton irradiation facility is under consideration at J-PARC. In this proton irradiation facility, 250 kW proton beams will be injected into the LBE spallation target, and irradiation tests under LBE flow will be performed for candidate structural materials for ADS. Furthermore, semiconductor soft-error tests, medical RI production, and proton beam applications will be performed. Among these, Post Irradiation Examination (PIE) of irradiated samples and RI separation and purification will be carried out in the PIE facility to be constructed near the proton irradiation facility. In this PIE facility, PIE of the equipment and samples irradiated in other facilities in J-PARC will also be performed. This report describes the conceptual study of the PIE facility, including the items to be tested, the test flow, the facilities, the test equipment, etc., and the proposed layout of the facility.

Journal Articles

Angular distribution of $$gamma$$ rays from a neutron-induced $$p$$-wave resonance of $$^{132}$$Xe

Okudaira, Takuya*; Tani, Yuika*; Endo, Shunsuke; Doskow, J.*; Fujioka, Hiroyuki*; Hirota, Katsuya*; Kameda, Kento*; Kimura, Atsushi; Kitaguchi, Masaaki*; Luxnat, M.*; et al.

Physical Review C, 107(5), p.054602_1 - 054602_7, 2023/05

 Times Cited Count:1 Percentile:68.16(Physics, Nuclear)

no abstracts in English

Journal Articles

Measurement of the transverse asymmetry of $$gamma$$ rays in the $$^{117}$$Sn($$n,gamma$$)$$^{118}$$Sn reaction

Endo, Shunsuke; Okudaira, Takuya*; Abe, Ryota*; Fujioka, Hiroyuki*; Hirota, Katsuya*; Kimura, Atsushi; Kitaguchi, Masaaki*; Oku, Takayuki; Sakai, Kenji; Shima, Tatsushi*; et al.

Physical Review C, 106(6), p.064601_1 - 064601_7, 2022/12

 Times Cited Count:2 Percentile:52.69(Physics, Nuclear)

no abstracts in English

Journal Articles

Angular distribution of $$gamma$$ rays from the $$p$$-wave resonance of $$^{118}$$Sn

Koga, Jun*; Takada, Shusuke*; Endo, Shunsuke; Fujioka, Hiroyuki*; Hirota, Katsuya*; Ishizaki, Kohei*; Kimura, Atsushi; Kitaguchi, Masaaki*; Niinomi, Yudai*; Okudaira, Takuya*; et al.

Physical Review C, 105(5), p.054615_1 - 054615_5, 2022/05

 Times Cited Count:3 Percentile:66.85(Physics, Nuclear)

no abstracts in English

Journal Articles

Energy-dependent angular distribution of individual $$gamma$$ rays in the $$^{139}$$La($$n, gamma$$)$$^{140}$$La$$^{ast}$$ reaction

Okudaira, Takuya*; Endo, Shunsuke; Fujioka, Hiroyuki*; Hirota, Katsuya*; Ishizaki, Kohei*; Kimura, Atsushi; Kitaguchi, Masaaki*; Koga, Jun*; Niinomi, Yudai*; Sakai, Kenji; et al.

Physical Review C, 104(1), p.014601_1 - 014601_6, 2021/07

 Times Cited Count:4 Percentile:57.13(Physics, Nuclear)

Journal Articles

Measurement of displacement cross section for proton in the kinetic energy range from 0.4 GeV to 3 GeV

Meigo, Shinichiro; Matsuda, Hiroki; Iwamoto, Yosuke; Yoshida, Makoto*; Hasegawa, Shoichi; Maekawa, Fujio; Iwamoto, Hiroki; Nakamoto, Tatsushi*; Ishida, Taku*; Makimura, Shunsuke*

JPS Conference Proceedings (Internet), 33, p.011050_1 - 011050_6, 2021/03

R&D of the beam window is crucial in the ADS, which serves as a partition between the accelerator and the target region. Although the displacement per atom (DPA) is used to evaluate the damage on the window, experimental data on the displacement cross section is scarce in the energy region above 20 MeV. We started to measure the displacement cross section for the protons in the energy region between 0.4 to 3 GeV. The displacement cross section can be derived by resistivity change divided by the proton flux and the resistivity change per Frankel pair on cryo-cooled sample to maintain damage. Experiments were conducted at the 3 GeV proton synchrotron at the J-PARC Center, and aluminum and copper was used as samples. As a result of comparison between the present experiment and the calculation of the NRT model, which is widely used for calculation of the displacement cross section, it was found that the calculation of the NRT model overestimated the experiment by about 3 times.

Journal Articles

Measurement of displacement cross-sections of copper and iron for proton with kinetic energies in the range 0.4 - 3 GeV

Matsuda, Hiroki; Meigo, Shinichiro; Iwamoto, Yosuke; Yoshida, Makoto*; Hasegawa, Shoichi; Maekawa, Fujio; Iwamoto, Hiroki; Nakamoto, Tatsushi*; Ishida, Taku*; Makimura, Shunsuke*

Journal of Nuclear Science and Technology, 57(10), p.1141 - 1151, 2020/10

 Times Cited Count:9 Percentile:75.92(Nuclear Science & Technology)

To estimate the structural damages of materials in accelerator facilities, displacement per atom (dpa) is widely employed as a damage index, calculated based on the displacement cross-section obtained using a calculation model. Although dpa is applied as standard, the experimental data of the displacement cross-section for a proton in the energy region above 20 MeV are scarce. Among the calculation models, difference of about factor 8 exist, so that the experimental data of the cross-section are crucial to validate the model. To obtain the displacement cross-section, we conducted experiments at J-PARC. The displacement cross-section of copper and iron was successfully obtained for a proton projectile with the kinetic energies, 0.4 - 3 GeV. The results were compared with those obtained using the widely utilized Norgertt-Robinson-Torrens (NRT) model and the athermal-recombination-corrected (arc) model based on molecular dynamics. It was found that the NRT model overestimates the present displacement cross-section by 3.5 times. The calculation results obtained using with the arc model based on the Nordlund parameter show remarkable agreement with the experimental data. It can be concluded that the arc model must be employed for the dpa calculation for the damage estimation of copper and iron.

Journal Articles

Measurement of displacement cross section of structural materials utilized in the proton accelerator facilities with the kinematic energy above 400 MeV

Meigo, Shinichiro; Matsuda, Hiroki; Iwamoto, Yosuke; Yoshida, Makoto*; Hasegawa, Shoichi; Maekawa, Fujio; Iwamoto, Hiroki; Nakamoto, Tatsushi*; Ishida, Taku*; Makimura, Shunsuke*

EPJ Web of Conferences, 239, p.06006_1 - 06006_4, 2020/09

 Times Cited Count:0 Percentile:0.1(Nuclear Science & Technology)

R&D of the beam window is crucial in the ADS, which serves as a partition between the accelerator and the target region. Although the displacement per atom (DPA) is used to evaluate the damage on the window, experimental data on the displacement cross section is scarce in the energy region above 20 MeV. We started to measure the displacement cross section for the protons in the energy region between 0.4 to 3 GeV. The displacement cross section can be derived by resistivity change divided by the proton flux and the resistivity change per Frankel pair on cryo-cooled sample to maintain damage. Experiments were conducted at the 3 GeV proton synchrotron at the J-PARC Center, and copper was used as samples. As a result of comparison between the present experiment and the calculation of the NRT model, which is widely used for calculation of the displacement cross section, it was found that the calculation of the NRT model overestimated the experiment by about 3 times.

Journal Articles

Transverse asymmetry of $$gamma$$ rays from neutron-induced compound states of $$^{140}$$La

Yamamoto, Tomoki*; Okudaira, Takuya; Endo, Shunsuke; Fujioka, Hiroyuki*; Hirota, Katsuya*; Ino, Takashi*; Ishizaki, Kohei*; Kimura, Atsushi; Kitaguchi, Masaaki*; Koga, Jun*; et al.

Physical Review C, 101(6), p.064624_1 - 064624_8, 2020/06

 Times Cited Count:9 Percentile:73.66(Physics, Nuclear)

Journal Articles

Measurement of displacement cross section of structural materials utilized in the proton accelerator facilities with the kinematic energy above 400 MeV

Meigo, Shinichiro; Matsuda, Hiroki; Iwamoto, Yosuke; Yoshida, Makoto*; Hasegawa, Shoichi; Maekawa, Fujio; Iwamoto, Hiroki; Nakamoto, Tatsushi*; Ishida, Taku*; Makimura, Shunsuke*

JPS Conference Proceedings (Internet), 28, p.061004_1 - 061004_6, 2020/02

no abstracts in English

Journal Articles

Measurement of displacement cross-section for structural materials in High-Power Proton Accelerator Facility

Meigo, Shinichiro; Matsuda, Hiroki; Iwamoto, Yosuke; Iwamoto, Hiroki; Hasegawa, Shoichi; Maekawa, Fujio; Yoshida, Makoto*; Ishida, Taku*; Makimura, Shunsuke*; Nakamoto, Tatsushi*

Proceedings of 9th International Particle Accelerator Conference (IPAC '18) (Internet), p.499 - 501, 2018/06

no abstracts in English

Journal Articles

Cross section measurements of the radioactive $$^{107}$$Pd and stable $$^{105,108}$$Pd nuclei at J-PARC/MLF/ANNRI

Nakamura, Shoji; Kimura, Atsushi; Kitatani, Fumito; Ota, Masayuki; Furutaka, Kazuyoshi; Goko, Shinji*; Hara, Kaoru; Harada, Hideo; Hirose, Kentaro; Kin, Tadahiro*; et al.

Nuclear Data Sheets, 119, p.143 - 146, 2014/05

 Times Cited Count:10 Percentile:57.34(Physics, Nuclear)

We have started the measurements of the neutron-capture cross sections for stable $$^{105,108}$$Pd nuclei as well as the radioactive $$^{107}$$Pd. The neutron-capture cross-section measurements by the time-of flight method were performed using an apparatus called "Accurate Neutron-Nucleus Reaction measurement Instrument (ANNRI)" installed at the neutron Beam Line No.4 of the Materials and Life science experimental Facility (MLF) in the J-PARC. The neutron-capture cross sections of $$^{107}$$Pd and $$^{105,108}$$Pd have been measured in the neutron energy range from thermal to 300 eV. Some new information was obtained for resonances of these Pd nuclei.

Journal Articles

Energy resolution of pulsed neutron beam provided by the ANNRI beamline at the J-PARC/MLF

Kino, Koichi*; Furusaka, Michihiro*; Hiraga, Fujio*; Kamiyama, Takashi*; Kiyanagi, Yoshiaki*; Furutaka, Kazuyoshi; Goko, Shinji*; Hara, Kaoru; Harada, Hideo; Harada, Masahide; et al.

Nuclear Instruments and Methods in Physics Research A, 736, p.66 - 74, 2014/02

 Times Cited Count:31 Percentile:91.8(Instruments & Instrumentation)

Journal Articles

Measurements of neutron capture cross sections at J-PARC/MLF/ANNRI, 2

Hori, Junichi*; Fujii, Toshiyuki*; Fukutani, Satoshi*; Furusaka, Michihiro*; Furutaka, Kazuyoshi; Goko, Shinji*; Harada, Hideo; Hiraga, Fujio*; Igashira, Masayuki*; Kamiyama, Takashi*; et al.

JAEA-Conf 2011-002, p.29 - 34, 2011/09

The neutron capture cross sections of $$^{93}$$Zr, $$^{99}$$Tc and $$^{107}$$Pd have been measured relative to the $$^{10}$$B(n,$$alphagamma$$) standard cross section by the neutron time-of-flight (TOF) method. Neutron capture $$gamma$$ rays were measured with a 4$$pi$$ Ge spectrometer as a part of the Accurate Neutron-Nucleus Reaction measurement Instrument (ANNRI) installed at the neutron Beam Line No.4 (BL04) of the Material and Life science experimental Facility (MLF) in the Japan Proton Accelerator Research Complex (J-PARC). This paper presents the preliminary results.

Journal Articles

Study of neutron capture reactions using the 4$$pi$$ Ge spectrometer

Harada, Hideo; Goko, Shinji*; Kimura, Atsushi; Ota, Masayuki*; Oshima, Masumi; Kitatani, Fumito; Toh, Yosuke; Furutaka, Kazuyoshi; Kin, Tadahiro; Koizumi, Mitsuo; et al.

Journal of the Korean Physical Society, 59(2), p.1547 - 1552, 2011/08

 Times Cited Count:9 Percentile:53.69(Physics, Multidisciplinary)

For the improvement of the accuracy on the neutron capture cross sections, a 4$$pi$$ Ge spectrometer was developed. The 4$$pi$$ Ge spectrometer is a unique tool due to its superior energy resolution for studying properties on neutron capture reactions, not only capture cross sections but also resonance identification, $$gamma$$-ray intensity distribution, and spin-parity assignment. For example, its performance on the resonance identification was demonstrated using a $$^{rm nat}$$Ag sample. On the measurement of a $$gamma$$-ray intensity distribution for each resonance, the results of $$^{238}$$U will be shown. Using the 4$$pi$$ Ge spectrometer, the measurements of neutron capture cross sections were started at the J-PARC/MLF/ANNRI. The preliminary results on the measurements of neutron capture cross sections will be discussed mainly based on measurements of neutron capture cross sections for $$^{241}$$Am, together with related techniques.

Journal Articles

The "Study on nuclear data by using a high intensity pulsed neutron source for advanced nuclear system" nuclear data project and the characteristics of the neutron beam line for the capture cross section experiments at J-PARC

Kiyanagi, Yoshiaki*; Kino, Koichi*; Furusaka, Michihiro*; Hiraga, Fujio*; Kamiyama, Takashi*; Kato, Kiyoshi*; Igashira, Masayuki*; Katabuchi, Tatsuya*; Mizumoto, Motoharu*; Oshima, Masumi; et al.

Journal of the Korean Physical Society, 59(2), p.1781 - 1784, 2011/08

 Times Cited Count:13 Percentile:62.2(Physics, Multidisciplinary)

The project of the comprehensive nuclear data research for the development of the advanced reactor systems had been executed successfully by eight organizations from 2005 to 2009. In this project, we constructed the pulsed neutron beamline that was aimed to obtain neutron capture cross-sections of long-lived fission products and minor actinides accurately. The energy spectra, spatial distributions, and pulses of the beam were studied by measurements and simulation calculations, and they were found to be consistent with those of the beamline design. In this paper, we present the overview of the project and the properties of the neutron beam provided by this beam line.

Journal Articles

Measurement of energy spectra and spatial distributions of neutron beams provided by the ANNRI beamline for capture cross-section measurements at the J-PARC/MLF

Kino, Koichi*; Furusaka, Michihiro*; Hiraga, Fujio*; Kamiyama, Takashi*; Kiyanagi, Yoshiaki*; Furutaka, Kazuyoshi; Goko, Shinji*; Harada, Hideo; Harada, Masahide; Kai, Tetsuya; et al.

Nuclear Instruments and Methods in Physics Research A, 626-627, p.58 - 66, 2011/01

 Times Cited Count:45 Percentile:95.09(Instruments & Instrumentation)

We measured the energy spectra and spatial distributions of the neutron beam of ANNRI beamline at the Japan Proton Accelerator Research Complex / Materials and Life Science Experimental Facility (J-PARC/MLF). Our research team designed and built this beamline to measure nuclear data with high precision. The measurements were performed on three types of beams provided by the beamline in the neutron energy range of 1.5 meV to 10 keV. The energy spectra show a typical feature of para-hydrogen moderator, and the absolute intensities almost agree with predictions based on both a simulation calculation of the JSNS (Japan Spallation Neutron Source) and a neutron transmission calculation of the beamline. The available neutron intensities at 21.5 m are 7.5$$times$$10$$^{5}$$, 1.6$$times$$10$$^{4}$$, and 1.1$$times$$10$$^{5}$$ n/cm$$^{2}$$/sec in the energy ranges of 1.5-25 meV, 0.9-1.1 eV, and 0.9-1.1 keV, respectively, under the 17.5 kW JSNS operation. The measured spatial distributions of the beams formed by three different collimators are consistent with those expected from the collimator-system design of the beamline. The beam sizes in FWHM are about 29, 14, and 11 mm for the three different beam collimators. The edges of the spatial distributions are relatively sharp, enabling us to measure the nuclear data successfully.

Journal Articles

Status and future perspectives of nuclear data measurements at J-PARC MLF BL04

Harada, Hideo; Oshima, Masumi; Kimura, Atsushi; Goko, Shinji*; Ota, Masayuki*; Furutaka, Kazuyoshi; Kin, Tadahiro; Kitatani, Fumito; Koizumi, Mitsuo; Nakamura, Shoji; et al.

JAEA-Conf 2010-005, p.9 - 14, 2010/12

The neutron-nucleus reaction instrument (NNRI) was installed at the J-PARC MLF BL04, which was designed for measuring neutron cross sections with a neutron time-of-flight technique. This includes two kinds of capture $$gamma$$-ray spectrometers: the 4$$pi$$ Ge spectrometer and the NaI spectrometers. The measurements of neutron capture cross sections for minor actinides and fission products have been started at the NNRI using these spectrometers since 2009. In this paper, the preliminary results and future perspectives are discussed.

Journal Articles

Measurement of neutron capture cross section ratios of $$^{244}$$Cm resonances using NNRI

Goko, Shinji*; Kimura, Atsushi; Harada, Hideo; Oshima, Masumi; Ota, Masayuki*; Furutaka, Kazuyoshi; Kin, Tadahiro; Kitatani, Fumito; Koizumi, Mitsuo; Nakamura, Shoji; et al.

Journal of Nuclear Science and Technology, 47(12), p.1097 - 1100, 2010/12

 Times Cited Count:6 Percentile:35.74(Nuclear Science & Technology)

To obtain the accurate nuclear data of minor actinides required for a nuclear transmutation system or an innovative nuclear fuel cycle system, measurement of neutron-capture cross section of $$^{244}$$Cm was performed using NNRI installed at beam line No.4 (BL04) of MLF in J-PARC. Using "4$$pi$$ Ge spectrometer" that is a component of NNRI, neutron time of flight spectra and prompt $$gamma$$ ray spectra were measured. Then neutron-capture cross section ratios of $$^{244}$$Cm resonances were derived and compared with the evaluated values of JENDL-3.3. The previous experimental data was measured using a nuclear explosion as a pulsed neutron source, and the present result is the first time in the world that such measurements have been carried out at an accelerator facility. By developing techniques for more detailed analysis and improvement of the experimental conditions, the absolute values of capture cross section are expected to be obtained.

Journal Articles

Corrosion resistance of Al-alloying high Cr-ODS steels in stagnant lead-bismuth

Takaya, Shigeru; Furukawa, Tomohiro; Inoue, Masaki; Fujisawa, Toshiharu*; Okuda, Takanari*; Abe, Fujio*; Onuki, Somei*; Kimura, Akihiko*

Journal of Nuclear Materials, 398(1-3), p.132 - 138, 2010/03

 Times Cited Count:59 Percentile:96.05(Materials Science, Multidisciplinary)

Oxide dispersion strengthened (ODS) ferritic steels with excellent high-temperature strength are the candidates for fuel cladding tubes. But, the compatibility with lead bismuth eutectic (LBE) is one of the key issues in accelerator driven system and LBE cooled fast reactors. Addition of Al and increase in Cr may have beneficial influence on the compatibility. Addition of Al, however, causes a decrease in high-temperature strength. A significantly higher Cr concentration results in aging embrittlement. Therefore, we need to find their optimal amount to balance corrosion resistance with high-temperature strength. In this study, the cross sections of the samples after 3,000 h of exposure to LBE with 10$$^{-8}$$ wt% oxygen at 650 $$^{circ}$$C are examined in detail using scanning electron microscope and Auger electron spectroscopy. The observation shows that very thin Al oxide layer is formed continuously between multiple oxide layer/internal oxide zone and matrix, and that such Al oxide layer suppresses further growth of multiple oxide layer/internal oxide zone. The average oxide layer thickness shows a tendency to get thinner by increasing in Al content from about 2 to 4 wt%, although significant dependency on Cr content is not recognized. Furthermore, the additional corrosion test for 5,000 h is conducted. These materials show good corrosion resistance even after 5,000 h of exposure to LBE containing 10$$^{-6}$$ wt% at 650 $$^{circ}$$C. Addition of 3.5 wt% Al is very effective in improving corrosion resistance.

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