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Nakamura, Satoshi; Ishii, Sho*; Kato, Hitoshi*; Ban, Yasutoshi; Hiruta, Kenta; Yoshida, Takuya; Uehara, Hiroyuki; Obata, Hiroki; Kimura, Yasuhiko; Takano, Masahide
Journal of Nuclear Science and Technology, 62(1), p.56 - 64, 2025/01
Times Cited Count:1 Percentile:68.64(Nuclear Science & Technology)A dissolution method for analyzing the elemental composition of fuel debris using the sodium peroxide (NaO
) fusion technique has been developed. Herein, two different types of simulated debris materials (such as solid solution of (Zr,RE)O
and molten core-concrete interaction products (MCCI)) were taken. At various temperatures, these debris materials were subsequently fused with Na
O
in crucibles, which are made of different materials, such as Ni, Al
O
, Fe, and Zr. Then, the fused samples are dissolved in nitric acid. Furthermore, the effects of the experimental conditions on the elemental composition analysis were evaluated using inductively coupled plasma-atomic emission spectroscopy (ICP-AES), which suggested the use of a Ni crucible at 923 K as an optimum testing condition. The optimum testing condition was then applied to the demonstration tests with Three Mile Island unit-2 (TMI-2) debris in a shielded concrete cell, thereby achieving complete dissolution of the debris. The elemental composition of TMI-2 debris revealed by the proposed dissolution method has good reproducibility and has an insignificant contradiction in the mass balance of the sample. Therefore, this newly developed reproducible dissolution method can be effectively utilized in practical applications by dissolving fuel debris and estimating its elemental composition.
Nauchi, Yasushi*; Sato, Shunsuke*; Hayakawa, Takehito*; Kimura, Yasuhiko; Suyama, Kenya; Kashima, Takao*; Futakami, Kazuhiro*
Nuclear Instruments and Methods in Physics Research A, 1050, p.168109_1 - 168109_9, 2023/05
Times Cited Count:0 Percentile:0.00(Instruments & Instrumentation)Measurement of neutrons from spent nuclear fuel is performed in this study using the H method, which detects 2.223 MeV
rays from neutron capture reaction of hydrogen using a highly pure germanium (HPGe) detector. The detection of the 2.223 MeV
ray is affected by intense
ray emission from fission products (FPs) because the emission rate of
rays from the FP is seven orders of magnitude higher than the emission rate of neutrons. To shield the intense
ray from the FP, the HPGe detector is placed off the axis of a collimator, whereas a polyethylene block is placed on the axis. In this geometry, the detector is shielded from the intense
rays from the FP, but the detector can measure 2.223 MeV
rays from the H
reactions in the polyethylene block. The measured count rate of the 2.223 MeV
rays is consistent with the expected rate within the statistical error, which is calculated based on the nuclide composition, which is primary
Cm, estimated via depletion and decay calculations. Accordingly, the H
method is considered feasible to quantify the number of neutron leakage from spent nuclear fuel assembly, which is applicable to certify burn up of the assembly.
Sato, Shunsuke*; Nauchi, Yasushi*; Hayakawa, Takehito*; Kimura, Yasuhiko; Kashima, Takao*; Futakami, Kazuhiro*; Suyama, Kenya
Journal of Nuclear Science and Technology, 60(6), p.615 - 623, 2022/06
Times Cited Count:0 Percentile:0.00(Nuclear Science & Technology)A new non-destructive method for evaluating Cs activity in spent nuclear fuels was proposed and experimentally demonstrated for physical measurements in burnup credit implementation.
Cs activities were quantified using gamma ray measurements and numerical detector response simulations without reference fuels, in which
Cs activities are well known. Fuel samples were obtained from a lead use assembly (LUA) irradiated in a commercial pressurized water reactor (PWR) up to 53 GWd/t. Gamma rays emitted from the samples were measured using a bismuth germinate (BGO) scintillation detector through a collimator attached to a hot cell. The detection efficiency of gamma rays with the detector was calculated using the PHITS particle transport calculation code considering the measurement geometry. The relative activities of
Cs,
Cs, and
Eu in the sample were measured with a high-purity germanium (HPGe) detector for more accurate simulations of the detector response for the samples. The absolute efficiency of the detector was calibrated by measuring a standard gamma ray source in another geometry.
Cs activity in the fuel samples was quantified using the measured count rate and detection efficiency. The quantified
Cs activities agreed well with those estimated using the MVP-BURN depletion calculation code.
Kimura, Takafumi*; Takanami, Takako*; Sakashita, Tetsuya; Wada, Seiichi*; Kobayashi, Yasuhiko; Higashitani, Atsushi*
Radiation Research, 178(4), p.313 - 320, 2012/10
Times Cited Count:9 Percentile:43.51(Biology)Here, we found that exposure to ionizing radiation (IR) induce certain innate immune response gene of in the intestine. Pre-treatment with IR before seeding on
lawn plate, significantly increased survival rate in the nematode. IR induction of
gene was highly dependent on the ELT-2 transcription factor and p38 MAPK. Moreover, the insulin/IGF-1 signal pathway works as an enhancer of induction of this gene. Silencing of the
gene led to growth retardation after IR irradiation. Finally, we describe the cross-tolerance between the responses to radiation exposure and innate immune system.
Sakashita, Tetsuya; Takanami, Takako*; Yanase, Sumino*; Hamada, Nobuyuki*; Suzuki, Michiyo; Kimura, Takafumi*; Kobayashi, Yasuhiko; Ishii, Naoaki*; Higashitani, Atsushi*
Journal of Radiation Research, 51(2), p.107 - 121, 2010/03
Times Cited Count:41 Percentile:67.38(Biology)The study of radiation effect in have been carried out over three decades and now allow for understanding at the molecular, cellular and individual levels. This review describes the current knowledge of the biological effects of ionizing irradiation with a scope of the germ line, aging and behavior.
may be a good
model system in the field of radiation biology.
Shirasu, Noriko; Kuramoto, Kenichi; Nakano, Yoshihiro; Yamashita, Toshiyuki; Kimura, Yasuhiko; Nihei, Yasuo; Ogawa, Toru
Journal of Nuclear Materials, 376(1), p.88 - 97, 2008/05
Times Cited Count:13 Percentile:63.18(Materials Science, Multidisciplinary)The concept of the rock-like oxide (ROX) fuel has been developed for the annihilation of excess plutonium in light water reactors. Irradiation tests and post-irradiation examinations were carried out on candidate ROX fuels. The ternary fuel of YSZ-spinel-corundum system, the single-phase fuels of YSZ, the particle dispersed fuels of YSZ in spinel or corundum matrix, and the blended fuels of YSZ and spinel or corundum matrix were fabricated and submitted to irradiation tests. The fuels containing spinel showed chemical instabilities with the vaporization of MgO component, which caused fuel restructuring. The swelling behavior was improved with the particle-dispersed fuels. However, the particle-dispersed fuels showed higher fractional gas release (FGR) than blended type fuels. The FGR of YSZ single-phase fuels were comparable to what would be expected for UO fuels. The YSZ single-phase fuel showed the best irradiation performance among the ROX fuels investigated.
Fujisato, Toshiya*; Kikuchi, Masahiro; Sakashita, Tetsuya; Funayama, Tomoo; Kobayashi, Yasuhiko; Funamoto, Seiichi*; Kimura, Tsuyoshi*; Kishida, Akio*; Yamaoka, Tetsuji*
JAEA-Review 2007-060, JAEA Takasaki Annual Report 2006, P. 119, 2008/03
Synthetic materials, such as ePTFE or Dacron are not suitable for reconstructing the small-diameter arteries. In contrast, tissue engineering (TE) graft has been attracting great attention recently. One of the promising approaches of TE grafts is using acellular tissues. The acellular scaffold may have the same structure and characteristics as the natural tissue and can be replaced with the host tissues. In this study, we prepared the acellular scaffold using irradiation, which is expected to induce the apoptosis of the cells.
Higashitani, Atsushi*; Mori, Chihiro*; Kimura, Takafumi*; Ikenaga, Takahiko*; Takanami, Takako*; Sakashita, Tetsuya; Wada, Seiichi*; Hamada, Nobuyuki*; Kobayashi, Yasuhiko
JAEA-Review 2007-060, JAEA Takasaki Annual Report 2006, P. 112, 2008/03
We investigated the gene expression of following carbon and
irradiation using DNA microarray analysis. We observed the 187 and 297 upregulated genes after
and carbon irradiation with 100 Gy, respectively, in which 51 genes were upregulated following both irradiations. On the other hand, the 358 and 388 genes were downregulated after
and carbon irradiation, respectively.
Onuki, Toshihiko; Aoyagi, Hisao*; Kitatsuji, Yoshihiro; Samadfam, M.; Kimura, Yasuhiko; Purvis, O. W.*
Journal of Environmental Radioactivity, 77(3), p.339 - 353, 2004/08
Times Cited Count:16 Percentile:33.16(Environmental Sciences)no abstracts in English
Yamashita, Toshiyuki; Kuramoto, Kenichi; Shirasu, Noriko; Nakano, Yoshihiro; Akie, Hiroshi; Nagashima, Hisao; Kimura, Yasuhiko; Omichi, Toshihiko*
Journal of Nuclear Materials, 320(1-2), p.126 - 132, 2003/07
Times Cited Count:10 Percentile:55.56(Materials Science, Multidisciplinary)Two irradiation tests on the rock-like oxide (ROX) fuels, small disk-shape fuel targets and pellet-type fuels, were performed in order to clarify in-pile irradiation stabilities. Swelling, fractional fission gas release (FGR) and phase change were examined by puncture test, profilometry and ceramography. YSZ single-phase fuel showed an excellent irradiation behavior, ie. low fission gas release (less than 3%), negligible swelling and no appreciable restructuring. The particle dispersed fuels showed lower swelling and higher fission gas release than those of mechanically blended fuels. Spinel decomposition and subsequence restructuring in the spinel matrix fuels was observed for the first time in the present investigation. It would be possible to reduce the FGR of the spinel matrix fuels, if the maximum fuels temperature is limited below 1700 K where neither spinel decomposition nor restructuring was observed. Damaged area of spinel matrix due to fission fragment irradiation seemed to be confined to thin layers around the surface of YSZ particles.
Iwai, Takashi; Nakajima, Kunihisa; Kikuchi, Hironobu; Nagashima, Hisao; Kimura, Yasuhiko; Matsui, Hiroki; Arai, Yasuo
JAERI-Research 2002-038, 69 Pages, 2003/01
Uranium-plutonium mixed carbide and nitiride fuel pins were fabricated in JAERI and irradiated at fast test rector JOYO based on the JAERI-JNC joint research program. The results of non-destructive and destructive post irradiation examinations cariied out at JNC were reported elsewhere. This report summarizes the results of destructive post irradiation examinations of (U,Pu)C and (U,Pu)N fuel pins carried out at JAERI.
Shirasu, Noriko; Yamashita, Toshiyuki; Kanazawa, Hiroyuki; Kimura, Yasuhiko; Sudo, Kenji; Magara, Masaaki; Inagawa, Jun; Kono, Nobuaki; Nakahara, Yoshinori
JAERI-Research 2001-018, 23 Pages, 2001/03
no abstracts in English
Iwai, Takashi; Nakajima, Kunihisa; Kikuchi, Hironobu; Kimura, Yasuhiko; Nagashima, Hisao; Sekita, Noriaki; Arai, Yasuo
JAERI-Research 2000-010, p.110 - 0, 2000/03
no abstracts in English
Iwai, Takashi; Nakajima, Kunihisa; Kikuchi, Hironobu; Kimura, Yasuhiko; Kanaitsuka, Fumio; Sekita, Noriaki; Arai, Yasuo
JAERI-Research 2000-009, p.36 - 0, 2000/03
no abstracts in English
Onuki, Toshihiko; Samadfam, M.; Kimura, Yasuhiko; Kitatsuji, Yoshihiro; Aoyagi, Hisao; Purvis, O. W.*
Proceedings of the International Workshop on Distribution and Speciation of Radionuclides in the Environment, p.174 - 180, 2000/00
no abstracts in English
Iwai, Takashi; Arai, Yasuo; Nakajima, Kunihisa; Kimura, Yasuhiko; ;
JAERI-Research 96-066, 26 Pages, 1996/12
no abstracts in English
Iwai, Takashi; Arai, Yasuo; Nakajima, Kunihisa; Kimura, Yasuhiko; ;
JAERI-Research 96-065, 47 Pages, 1996/12
no abstracts in English
Yanagisawa, Kazuaki; Soyama, Kazuhiko; Ichikawa, Hiroki; ; Hoshino, Osamu; ; ; ; Kanazawa, Hiroyuki; Kimura, Yasuhiko; et al.
JAERI-M 91-114, 67 Pages, 1991/08
no abstracts in English
Yanagisawa, Kazuaki; Mimura, Hideaki; Kimura, Yasuhiko
JAERI-M 90-164, 64 Pages, 1990/09
no abstracts in English
Kamada, Yutaka; Yoshino, Ryuji; ; Ozeki, Takahisa; Kawasaki, Kozo; Hiratsuka, Hajime; Miyo, Yasuhiko; Kimura, Haruyuki; Nishitani, Takeo; Yoshida, Hidetoshi; et al.
JAERI-M 89-050, 33 Pages, 1989/05
no abstracts in English