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Kitamura, Akihiro; Hirano, Hiroshi*; Yoshida, Masato; Takeuchi, Kentaro
Hoken Butsuri (Internet), 58(2), p.76 - 90, 2023/08
The alpha contaminated gloveboxes have been dismantled for over 20 years in Plutonium Fuel Fabrication Facility. The so called wet recovery equipment gloveboxes, which recover plutonium and uranium from scrap fuel by dissolving and extracting processes, were chosen as the priority gloveboxes to be dismantled. These gloveboxes and other gloveboxes in the same room were size reduced and removed up until 2022. Also, non-radioactive ancillary facility and non-radioactive giant glovebox were removed from 2007 to 2010 for ease of glovebox dismantling activities that follows and for making waste storage spaces. Several incidents were occurred and recidivism prevention measures were implemented on each occasion. In this report, glovebox dismantling activities we conducted in the past 20 years are reviewed and lessons we have learned are summarized.
Kitamura, Ryo; Futatsukawa, Kenta*; Hayashi, Naoki; Hirano, Koichiro; Kondo, Yasuhiro; Kosaka, Satoshi*; Miyao, Tomoaki*; Morishita, Takatoshi; Nemoto, Yasuo*; Oguri, Hidetomo
Physical Review Accelerators and Beams (Internet), 26(3), p.032802_1 - 032802_12, 2023/03
Times Cited Count：0 Percentile：0.02(Physics, Nuclear)A bunch-shape monitor (BSM) is a useful device for performing longitudinal beam tuning using the pointwise longitudinal phase distribution measured at selected points in the beam transportation. To measure the longitudinal phase distribution of a low-energy negative hydrogen (H
) ion beam, highly oriented pyrolytic graphite (HOPG) was adopted for the secondary-electron-emission target to mitigate the thermal damage due to the high-intensity beam loading. The HOPG target enabled the measurement of the longitudinal phase distribution at the center of a 3-MeV H ion beam with a high peak current of about 50 mA. The longitudinal bunch width was measured using HOPG-BSM at the test stand, which was consistent with the beam simulation. The correlation measurement between the beam transverse and longitudinal planes was demonstrated using HOPG-BSM. The longitudinal Twiss and emittance measurement with the longitudinal Q-scan method was conducted using HOPG-BSM.
Di Palma, A.; Adamo, P.*; Dohi, Terumi; Fujiwara, Kenso; Hagiwara, Hiroki; Kitamura, Akihiro; Sakoda, Akihiro; Sato, Kazuhiko; Iijima, Kazuki
Chemosphere, 308, Part 1, p.136179_1 - 136179_13, 2022/12
Times Cited Count：1 Percentile：14.8(Environmental Sciences)The present study shows the use of mosses transplanted in bags, called as moss bags, as biosensors of airborne radioactive dusts in the environment of the evacuated zone of Fukushima. A standardized protocol was applied and three moss species were used. Background sites of Okayama Prefecture were used for comparison. In the Fukushima area, the moss bags were able to accumulate radiocaesium in all exposure sites and periods, with Sphagnum palustre moss acting as the most performant moss. The radiocaesium activity concentrations dectected in mosses were in strong agreement with the Cs deposition levels and decontamination status of each exposure site. The accumulation of soil-derived radiocaesium by moss bags was supported by autoradiography and electron microscopy analyses. The linear dependency of Cs accumulation with the exposure time allowed a radiocaesium quantitative assessment.
Urushidate, Tadayuki*; Yoda, Tomoyuki; Otani, Shuichi*; Yamaguchi, Toshio*; Kunii, Nobuaki*; Kuriki, Kazuki*; Fujiwara, Kenso; Niizato, Tadafumi; Kitamura, Akihiro; Iijima, Kazuki
JAEA-Review 2022-023, 8 Pages, 2022/09
JAEA-Review-2022-023.pdf:1.19MB
After the accident of the Fukushima Daiichi Nuclear Power Station, the Japan Atomic Energy Agency has newly set up a laboratory in Fukushima and started measuring radioactivity concentrations of environmental samples. In October 2015, Fukushima Radiation Measurement Group has been accredited the ISO/IEC 17025 standard by the Japan Accreditation Board (JAB) as a testing laboratory for radioactivity analysis (
Cs, 
Cs) based on Gamma-ray spectrometry with germanium semiconductor detectors. The laboratory has measured approximately 60,000 of various environmental samples at the end of March 2022. The laboratory quality control and measurement techniques have been accredited by regular surveillance of JAB. In September 2019, the laboratory renewed accreditation as a testing laboratory for radioactivity analysis.
(Copepoda) from a deep sediment-trap; Abundance and implications for ecological and biogeochemical studiesIkenoue, Takahito*; Otosaka, Shigeyoshi*; Honda, Makio*; Kitamura, Minoru*; Mino, Yoshihisa*; Narita, Hisashi*; Kobayashi, Takuya
Frontiers in Marine Science (Internet), 9, p.884320_1 - 884320_11, 2022/05
Times Cited Count：0 Percentile：0.01(Environmental Sciences)We studied seasonal variations of the mesozooplankton swimmer community collected by a sediment trap moored at 873 m in the Kuroshio & Oyashio Transition region off the east coast of Japan from 5 August 2011 to 23 June 2013. The total flux of mesozooplankton swimmers varied between 0 and 11.1 individuals m-2 d-1, with a mean of 3.1 individuals m-2 d-1 during the sampling period. Among the Copepoda, Neocalanus cristatus was the most dominant taxon. The species composition of the swimmers closely reflected the mid-depth mesozooplankton of the Oyashio region. The fluxes of Neocalanus species reflected ontogenetic vertical migration, but may have been overestimates of active fluxes if they included dormant individuals that accidentally entered the sediment trap.
Sr in cattle bone and tooth samples by inductively coupled plasma mass spectrometryKoarai, Kazuma; Matsueda, Makoto; Aoki, Jo; Yanagisawa, Kayo*; Terashima, Motoki; Fujiwara, Kenso; Kino, Yasushi*; Oka, Toshitaka; Takahashi, Atsushi*; Suzuki, Toshihiko*; et al.
Journal of Analytical Atomic Spectrometry, 36(8), p.1678 - 1682, 2021/08
Times Cited Count：5 Percentile：55.72(Chemistry, Analytical)Rapid analysis of Sr in bone and tooth samples of cattle were achieved by an inductively coupled plasma mass spectrometry (ICP-MS) coupled with mass shift and solid phase extraction techniques. Limit of detection (LOD) in the ICP-MS measurement of 0.1 g samples was lower than that of the radioactivity measurement. Analytical time of the ICP-MS method was reduced from 20 days to 11 hours, compared with the radiometric method. Therefore, the ICP-MS method can be rapid and useful procedure of Sr in small bone and tooth samples derived from terrestrial animals.
Matsueda, Makoto; Yanagisawa, Kayo*; Koarai, Kazuma; Terashima, Motoki; Fujiwara, Kenso; Abe, Hironobu; Kitamura, Akihiro; Takagai, Yoshitaka*
ACS Omega (Internet), 6(29), p.19281 - 19290, 2021/07
Times Cited Count：2 Percentile：14.88(Chemistry, Multidisciplinary)Online solid-phase extraction-inductively coupled plasma-quadrupole mass spectrometry with oxygen dynamic reaction cell (online SPE-ICP-MS-DRC) was shown to be a thorough automatic analytical system, circumventing the need for human handling. At three stepwise separations (SPE-DRC-Q mass filters), we showed that interference materials allowed the coexistence of abundance ratios of 1.5
10
for 
Tc/Mo. Using this optimized system, a detection limit of Tc was 9.3 pg/L (5.9 mBq/L) for a 50 mL injection and sequential measurements were undertaken at a cycle of 24 min/sample.
beam with 3 MeV by the bunch-shape monitorKitamura, Ryo; Futatsukawa, Kenta*; Hayashi, Naoki; Hirano, Koichiro; Kondo, Yasuhiro; Kosaka, Satoshi*; Miyao, Tomoaki*; Nemoto, Yasuo*; Morishita, Takatoshi; Oguri, Hidetomo
JPS Conference Proceedings (Internet), 33, p.011012_1 - 011012_6, 2021/03
The new bunch shape monitor (BSM) is required to measure the bunch size of the high-intensity H beam with 3 MeV at the front-end section in the J-PARC linac. The carbon-nano tube wire and the graphene stick are good candidates for the target wire of the BSM, because these materials have the enough strength to detect the high-intensity beam. However, since the negative high voltage of more than a few kV should be applied to the wire in the BSM, the suppression of the discharge is the challenge to realize the new BSM. After the high-voltage test to investigate the effect of the discharge from the wire, the detection of the signal from the BSM was successful at the beam core with the peak current of 55 mA using the graphene stick. The preliminary result of the bunch-size measurement is reported in this presentation.
Sr in hard tissue samplesKoarai, Kazuma; Matsueda, Makoto; Aoki, Jo; Yanagisawa, Kayo*; Fujiwara, Kenso; Terashima, Motoki; Kitamura, Akihiro; Abe, Hironobu
KEK Proceedings 2020-4, p.180 - 185, 2020/11
Strontium-90 and Y, its daughter nuclide, adverse effects on the bone marrow. Monitoring of Sr in the bones have been required after the Fukushima-Daiichi Nuclear Power Plant accident. However, conventional radioactivity measurement method for Sr requires a complicated separation of Y and a time-consuming measurement. ICP-MS system has been applied to Sr concentration survey of water, soil, and edible part of fish. We applied the ICP-MS system for the bones for the first time. In this study, reference bone (JSAC 0785 fish bone) was used as measurement samples. Sample preparation of the bone was performed using a microwave digestion instrument. After sample preparation, Sr was determined using ICP-MS system with cascade separation steps based on on-line column separation and oxygen reaction. Strontium-90 in the bones was successfully separated from Ca, Ba, Y, Zr, Fe, Se, and Ge, which interfered in ICP-MS measurement, in the separation steps.
Hagiwara, Hiroki; Nakanishi, Takahiro; Konishi, Hiromi*; Tsuruta, Tadahiko; Misono, Toshiharu; Fujiwara, Kenso; Kitamura, Akihiro
Journal of Environmental Radioactivity, 220-221, p.106294_1 - 106294_9, 2020/09
Times Cited Count：0 Percentile：0(Environmental Sciences)Kitamura, Ryo; Futatsukawa, Kenta*; Hayashi, Naoki; Hirano, Koichiro; Kondo, Yasuhiro; Kosaka, Satoshi*; Miyao, Tomoaki*; Nemoto, Yasuo*; Morishita, Takatoshi; Oguri, Hidetomo
Proceedings of 17th Annual Meeting of Particle Accelerator Society of Japan (Internet), p.251 - 253, 2020/09
A bunch-shape monitor (BSM) in the low-energy region is being developed in the J-PARC linac to accelerate the high-intensity proton beam with the low emittance. A highly-oriented pyrolytic graphite (HOPG) was introduced as the target of the BSM to mitigate the thermal loading. The stable measurement of the BSM was realized thanks to the HOPG target, while the tungsten target was broken by the thermal loading from the high-intensity beam. However, since the longitudinal distribution measured with the BSM using the HOPG target was wider than the expected one, the improvement of tuning parameters is necessary for the BSM. The BSM consists of an electron multiplier, a bending magnet, and a radio-frequency deflector, which should be tuned appropriately. Behavior of these components were investigated and tuned. The longitudinal distribution measured with the BSM after the tuning was consistent with the expected one.
Sue, Yuki*; Yotsuzuka, Mai*; Futatsukawa, Kenta*; Hasegawa, Kazuo; Iijima, Toru*; Iinuma, Hiromi*; Inami, Kenji*; Ishida, Katsuhiko*; Kawamura, Naritoshi*; Kitamura, Ryo; et al.
Physical Review Accelerators and Beams (Internet), 23(2), p.022804_1 - 022804_7, 2020/02
Times Cited Count：2 Percentile：25.94(Physics, Nuclear)A destructive monitor to measure the longitudinal bunch width of a low-energy and low-intensity muon beam was developed. This bunch-width monitor (BWM) employed microchannel plates to detect a single muon with high time resolution. In addition, constant-fraction discriminators were adopted to suppress the time-walk effect. The time resolution was measured to be 65 ps in rms using a picosecond-pulsed laser. This resolution satisfied the requirements of the muon linac of the J-PARC E34 experiment. We measured the bunch width of negative-muonium ions accelerated with a radio-frequency quadrupole using the BWM. The bunch width was successfully measured to be 
54 
11 ns, which is consistent with the simulation.
Kuwata, Haruka*; Misono, Toshiharu; Fujiwara, Kenso; Takeishi, Minoru; Manabe, Sachi*; Kitamura, Akihiro
Radiation Environment and Medicine, 9(1), p.28 - 34, 2020/02
The analysis of tritium in aquatic biota is one of the most important research areas in Fukushima. The conventional method for measuring the concentration of tritium consists of complicated pretreatment procedures and requires skillful techniques as well as a significant amount of time. Consequently, there are only a few reports on tritium monitoring data in marine products from the coast of Fukushima. In this study, we measured the Tissue Free Water Tritium (TFWT) and Organically Bound Tritium (OBT) in flounders collected from the coast of Fukushima to examine the impacts of the nuclear accident on aquatic biota. The study was done for a period of 4 years; from 2015 to 2018. The conventional method of analysis was firstly used, after which the method was modified by improving the freeze-drying and combustion water recovery processes. Results from both methods show that the most of the concentrations of the TFWT and OBT in the flounder were below the detection or quantitative limit. The effect of the nuclear accident on humans, through internal exposure, was also examined and found to be negligible. Although some uncertainties exist due to the short cut of the processes, the modified version could be considered an effective and practical approximate method.
Hagiwara, Hiroki; Konishi, Hiromi*; Nakanishi, Takahiro; Fujiwara, Kenso; Iijima, Kazuki; Kitamura, Akihiro
Journal of Environmental Radioactivity, 211, p.106042_1 - 106042_10, 2020/01
Times Cited Count：3 Percentile：14.71(Environmental Sciences)Kondo, Yasuhiro; Hirano, Koichiro; Ito, Takashi; Kikuzawa, Nobuhiro; Kitamura, Ryo; Morishita, Takatoshi; Oguri, Hidetomo; Okoshi, Kiyonori; Shinozaki, Shinichi; Shinto, Katsuhiro; et al.
Journal of Physics; Conference Series, 1350, p.012077_1 - 012077_7, 2019/12
Times Cited Count：1 Percentile：52.28(Physics, Particles & Fields)We have upgraded a 3-MeV linac at J-PARC. The ion source is same as the J-PARC linac's, and the old 30-mA RFQ is replaced by a spare 50-mA RFQ, therefore, the beam energy is 3 MeV and the nominal beam current is 50 mA. The main purpose of this system is to test the spare RFQ, but also used for testing of various components required in order to keep the stable operation of the J-PARC accelerator. The accelerator has been already commissioned, and measurement programs have been started. In this paper, present status of this 3-MeV linac is presented.
Otani, Masashi*; Fukao, Yoshinori*; Futatsukawa, Kenta*; Kawamura, Naritoshi*; Matoba, Shiro*; Mibe, Tsutomu*; Miyake, Yasuhiro*; Shimomura, Koichiro*; Yamazaki, Takayuki*; Hasegawa, Kazuo; et al.
Journal of Physics; Conference Series, 1350, p.012067_1 - 012067_6, 2019/12
Times Cited Count：2 Percentile：73.22(Physics, Particles & Fields)Negative muonium atom (
e
e, Mu) has unique features stimulating potential interesting for several scientific fields. Since its discovery in late 1980's in vacuum, it has been discussed that the production efficiency would be improved using a low-work function material. C12A7 was a well-known insulator as a constituent of alumina cement, but was recently confirmed to exhibit electric conductivity by electron doping. The C12A7 electride has relatively low-work function (2.9 eV). In this paper, the negative muonium production measurement with several materials including a C12A7 electride film will be presented. Measured production rate of the Mu were 10
/s for all the Al, electride, and SUS target. Significant enhancement on electride target was not observed, thus it is presumed that the surface condition should be more carefully treated. There was no material dependence of the Mu averaged energy: it was 0.20.1keV.
Otani, Masashi*; Futatsukawa, Kenta*; Mibe, Tsutomu*; Naito, Fujio*; Hasegawa, Kazuo; Ito, Takashi; Kitamura, Ryo; Kondo, Yasuhiro; Morishita, Takatoshi; Iinuma, Hiromi*; et al.
Journal of Physics; Conference Series, 1350, p.012097_1 - 012097_7, 2019/12
Times Cited Count：2 Percentile：73.22(Physics, Particles & Fields)A disk and washer (DAW) coupled cavity linac (CCL) has been developed for a middle velocity part in a muon linac to measure muon anomalous magnetic moment and search for electric dipole moment. I will accelerate muons from 
= 
= 0.3 to 0.7 at an operational frequency of 1.3GHz. In this poster, the cavity design, beam dynamics design, and the cold-model measurements will be presented.
Sue, Yuki*; Iijima, Toru*; Inami, Kenji*; Yotsuzuka, Mai*; Iinuma, Hiromi*; Nakazawa, Yuga*; Otani, Masashi*; Kawamura, Naritoshi*; Shimomura, Koichiro*; Futatsukawa, Kenta*; et al.
Proceedings of 16th Annual Meeting of Particle Accelerator Society of Japan (Internet), p.55 - 60, 2019/07
The result of bunch size measurement of muon accelerated by RFQ up to 89 keV is presented in this paper. A four-stage muon linac for precise measurement of muon property is under construction in the J-PARC. The demonstration of the first muon RF acceleration with an RFQ linac was conducted and the transverse profile of the accelerated muons was measured in 2017. As one of the remaining issues for the beam diagnostic system, the longitudinal beam profile after the RFQ should be measured to match the profile to the designed acceptance of the subsequent accelerator. For this purpose, the new longitudinal beam monitor using the microchannel plate is under development. The time resolution of the monitor aims to be around 30 to 40 ps corresponding to 1% of a period of an operating frequency of the accelerator, which is 324 MHz. On November 2018, the bunch size of accelerated negative muonium ion of 89 keV with the RFQ was measured using this monitor at the J-PARC MLF. The measured bunch width is 
ns, which is consistent with the simulation.
Yotsuzuka, Mai*; Iijima, Toru*; Iinuma, Hiromi*; Inami, Kenji*; Otani, Masashi*; Kawamura, Naritoshi*; Kitamura, Ryo; Kondo, Yasuhiro; Saito, Naohito; Shimomura, Koichiro*; et al.
Proceedings of 16th Annual Meeting of Particle Accelerator Society of Japan (Internet), p.814 - 817, 2019/07
The J-PARC E34 experiment aims to measure the muon anomalous magnetic moment and the electric dipole moment with a high precision. In this experiment, thermal muonium is produced and ionized by laser resonance to generate ultra-slow muons, which are then accelerated in a multistage muon linac. In order to satisfy the experimental requirements, suppression of the emittance growth during the acceleration is necessary. Because the main cause of the emittance growth is beam mismatching between the accelerating stages, the transverse and longitudinal beam monitoring is important. The longitudinal beam monitor has to measure the bunch length with the resolution equivalent to tens of picoseconds, which is 1% of the acceleration phase of 324 MHz. In addition, it should be sensitive to single muon because the beam intensity is limited during the commissioning phase. To realize above requirements, we are developing a longitudinal beam monitor with a micro channel plate, and the test bench to evaluate the monitor performance. So far, the time resolution of the beam monitor was obtained to be 65 ps in RMS including the jitter on the test bench. We also succeeded in measuring the longitudinal bunch size of the muon beam accelerated by RFQ using the beam monitor. In this paper, the results of the performance evaluation for this beam monitor are reported.
beam with 3 MeV using the carbon materialKitamura, Ryo; Futatsukawa, Kenta*; Hayashi, Naoki; Hirano, Koichiro; Kosaka, Satoshi*; Miyao, Tomoaki*; Moriya, Katsuhiro; Nemoto, Yasuo*; Oguri, Hidetomo
Proceedings of 16th Annual Meeting of Particle Accelerator Society of Japan (Internet), p.51 - 54, 2019/07
The longitudinal measurement and tuning at the beam transport after the RFQ are important to reduce the beam loss and the emittance growth in the J-PARC linac, when the high-intensity H beam of more than 60 mA is supplied. The new bunch shape monitor (BSM) using the carbon-nanotube (CNT) wire is necessary to measure the bunch shape of the high-intensity H beam with 3 MeV, because the CNT wire has a high-temperature tolerance and a small energy deposit. However, when the high voltage was applied to the CNT wire to extract the secondary electron derived, the discharge prevents the power supply from applying the voltage. Therefore, the discharge should be suppressed to measure the bunch shape with stability. Considering the characteristics of the CNT as the emitter, when the length of the CNT wire was short, the high voltage of -10 kV was applied to the CNT wire. The current status and future prospects of the BSM using the CNT wire are reported in this presentation.
