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Journal Articles

Simulation of a gamma-ray imaging technique using detector response patterns

Kitayama, Yoshiharu; Nogami, Mitsuhiro*; Hitomi, Keitaro*

Japanese Journal of Applied Physics, 63(3), p.032005_1 - 032005_6, 2024/03

 Times Cited Count:0 Percentile:0.01(Physics, Applied)

We introduce a novel gamma-ray imaging technique that uses detector response patterns. This method employs multiple shielding cubes randomly positioned in a three-dimensional configuration. Within the volume defined by these cubes, a unique gamma-ray flux pattern is formed based on the incidence direction of the gamma rays. This pattern can be measured using the responses of several scintillator cubes. By pre-measuring the detector response pattern and incidence direction of the gamma rays, the incidence direction can be estimated using an unfolding technique. Simulations were performed using a $$^{137}$$Cs point source. Our results show that a 10 MBq $$^{137}$$Cs source, located 3 m away from the imager, can be imaged with an angular resolution close to 10$$^{circ}$$. These findings suggest that our new method is comparable to existing gamma-ray imaging techniques. Potential applications of this imaging method include nuclear power plant decommissioning, nuclear medicine, security, and astronomy.

Journal Articles

Cu $$K$$-edge X-ray absorption fine structure study of $$T'$$-type $$RE$$$$_{2}$$CuO$$_{4+alpha-delta}$$ ($$RE$$ = Rare Earth); Toward unified understanding of electronic state of $$T'$$-type cuprate

Chen, Y.*; Asano, Shun*; Wang, T.*; Xie, P.*; Kitayama, Shinnosuke*; Ishii, Kenji*; Matsumura, Daiju; Tsuji, Takuya; Taniguchi, Takanori*; Fujita, Masaki*

JPS Conference Proceedings (Internet), 38, p.011050_1 - 011050_6, 2023/05

Journal Articles

Gamma-ray imaging using three-dimensional shadow images created by coded solid

Kitayama, Yoshiharu; Nogami, Mitsuhiro*; Hitomi, Keitaro*

KEK Proceedings 2022-3, p.46 - 53, 2023/01

The position of a streetlight can be predicted from the direction and shape of one's shadow projected on the street at night by the light of the streetlight. The application of this idea to gamma-ray imagers is known as coded aperture. In this study, we proposed the Coded Cube Camera - POrtable (C3PO), which has a three-dimensional shielding and scintillator crystal arrangement, and is composed of lead, scintillator, and depletion cubes randomly arranged in a 3$$times$$3$$times$$3 Rurik's cube shape, with each. The output of each scintillator produces a three-dimensional shadow pattern, which is returned to the source direction distribution by unfolding. In this study, we investigated the characteristics and feasibility of the system by simulation using Geant 4.

Journal Articles

A Phoswich alpha/beta detector for monitoring in the site of Fukushima Daiichi Nuclear Power Station

Morishita, Yuki; Takasaki, Koji; Kitayama, Yoshiharu; Tagawa, Akihiro; Shibata, Takuya; Hoshi, Katsuya; Kaneko, Junichi*; Higuchi, Mikio*; Oura, Masatoshi*

Radiation Measurements, 160, p.106896_1 - 106896_10, 2023/01

 Times Cited Count:0 Percentile:0.01(Nuclear Science & Technology)

This study proposes a newly developed phoswich alpha/beta detector that can discriminate alpha and beta particles emitted from the alpha and beta contaminations in the FDNPS site. The phoswich alpha/beta detector is made up of two layers of scintillators that detect alpha and beta particles. The pulse shape discrimination (PSD) method was used to detect alpha particles in high beta particle and high gamma-ray (comparable to gamma-ray dose rate near the FDNPS reactor building) environments. Due to a 23.3% full width at half maximum (FWHM) energy resolution for alpha particles, the detector can be used to distinguish between nuclear fuel materials such as plutonium and its radon progeny (Po-214). Moreover, the detector could distinguish alpha particles from $$^{137}$$Cs gamma rays with a dose rate background up to 9.0 mSv/h. It is the first to demonstrate that the developed phoswich detector can be used to discriminate and measure alpha and beta particles of the actual contaminated FDNPS samples.

Journal Articles

Shield-free directional gamma-ray detector using small-angle Compton scattering

Kitayama, Yoshiharu

Gamma Ray Imaging; Technology and Applications, p.165 - 179, 2023/00

A gamma-ray imager is a powerful tool for visualizing the distribution of radioactive materials. Recently, it has been applied to the decommissioning site of the Fukushima Daiichi Nuclear Power Station. At the decommissioning site, an imager compact, lightweight, and capable of quantitative evaluation of radioactivity is demanded. The Gamma-ray Imager using Small-Angle Scattering (GISAS) was proposed as a gamma-ray imager that meets all these requirements. GISAS consists of several shield-free directional gamma-ray detectors that detect only small-angle Compton scattering. Simulations and experiments verified the feasibility of the shield-free directional gamma-ray detectors. The shield-free directional gamma-ray detector consists of a scatterer that detects small-angle Compton scattering and an absorber that detects the scattered gamma rays. By setting an appropriate energy window for each detector, only scattering events that can be considered almost straightforward are detected. Through simulations and experiments, we have confirmed that using a silicon drift detector as the scatterer and a Gd3Al2Ga3O12 scintillator as the absorber, we can detect only small-angle Compton scattering events and obtain directionality for 662 keV gamma rays.

Journal Articles

Simulation study of a shield-free directional gamma-ray detector using Small-Angle Compton Scattering

Kitayama, Yoshiharu; Terasaka, Yuta; Sato, Yuki; Torii, Tatsuo

Journal of Nuclear Engineering and Radiation Science, 7(4), p.042006_1 - 042006_7, 2021/10

Journal Articles

Electrochemical behavior of carbon steel with bentonite/sand in saline environment

Kitayama, Ayami; Taniguchi, Naoki; Mitsui, Seiichiro

Materials and Corrosion, 72(1-2), p.211 - 217, 2021/01

 Times Cited Count:0 Percentile:0(Materials Science, Multidisciplinary)

Journal Articles

A Study of directional gamma-ray detector without shield by Monte Carlo simulation

Kitayama, Yoshiharu; Terasaka, Yuta; Sato, Yuki; Torii, Tatsuo

Proceedings of International Youth Nuclear Congress 2020 (IYNC 2020) (Internet), 4 Pages, 2020/05

JAEA Reports

Synthesis report on the R&D for the Horonobe Underground Research Laboratory; Project carried out during fiscal years 2015-2019

Nakayama, Masashi; Saiga, Atsushi; Kimura, Shun; Mochizuki, Akihito; Aoyagi, Kazuhei; Ono, Hirokazu; Miyakawa, Kazuya; Takeda, Masaki; Hayano, Akira; Matsuoka, Toshiyuki; et al.

JAEA-Research 2019-013, 276 Pages, 2020/03

JAEA-Research-2019-013.pdf:18.72MB

The Horonobe Underground Research Laboratory (URL) Project is being pursued by the Japan Atomic Energy Agency (JAEA) to enhance the reliability of relevant disposal technologies for geological disposal of High-level Radioactive Waste through investigations of the deep geological environment within the host sedimentary rock at Horonobe Town in Hokkaido, north Japan. The investigations will be conducted in three phases, namely "Phase 1: Surface based investigations", "Phase 2: Construction phase" (investigations during construction of the underground facilities) and "Phase 3: Operation phase" (research in the underground facilities). According to the research plan described in the 3rd Mid- and Long- term Plan of JAEA, "Near-field performance study", "Demonstration of repository design option", and "Verification of crustal-movement buffering capacity of sedimentary rocks" are important issues of the Horonobe URL Project, and schedule of future research and backfill plans of the project will be decided by the end of 2019 Fiscal Year. The present report summarizes the research and development activities of these 3 important issues carried out during 3rd Medium to Long-term Research Phase.

Journal Articles

Extraction behavior of rutherfordium as a cationic fluoride complex with a TTA chelate extractant from HF/HNO $$_{3}$$ acidic solutions

Yokoyama, Akihiko*; Kitayama, Yuta*; Fukuda, Yoshiki*; Kikunaga, Hidetoshi*; Murakami, Masashi*; Komori, Yukiko*; Yano, Shinya*; Haba, Hiromitsu*; Tsukada, Kazuaki; Toyoshima, Atsushi*

Radiochimica Acta, 107(1), p.27 - 32, 2019/01

 Times Cited Count:1 Percentile:10.81(Chemistry, Inorganic & Nuclear)

Journal Articles

Pipe cutting method at high radiation area in FUGEN

Takiya, Hiroaki; Ishiyama, Masahiro; Tezuka, Masashi; Kitayama, Naoki

Proceedings of International Conference on Dismantling Challenges; Industrial Reality, Prospects and Feedback Experience (DEM 2018) (Internet), 8 Pages, 2018/10

In FUGEN, we had isolated the reactor core by cutting pipes of the periphery systems (e.g. reactor cooling system, heavy water system, and helium system) between 2015 and 2017, as preparation for dismantling the reactor core and taking some samples from the reactor core structures. There are three issues to be solved at this isolation work; (1) to shorten the working time at high radiation area which is 1-5mSv/h at air and 10mSv/h at contact, (2) to prevent tritium spreading to working area at cutting work because tritium air is existing with 20-30Bq/cm$$^{3}$$ inside of the heavy water system and helium system, and (3) to minimize the influence of contaminated fume for the accurate radioactivity evaluation of reactor core structure. In this study, considering these problems, we discussed the method for cutting the pipes of heavy water system and helium system at the high radiation area and carried out the pipe cutting in the way.

Journal Articles

Atmospheric modeling of $$^{137}$$Cs plumes from the Fukushima Daiichi Nuclear Power Plant; Evaluation of the model intercomparison data of the Science Council of Japan

Kitayama, Kyo*; Morino, Yu*; Takigawa, Masayuki*; Nakajima, Teruyuki*; Hayami, Hiroshi*; Nagai, Haruyasu; Terada, Hiroaki; Saito, Kazuo*; Shimbori, Toshiki*; Kajino, Mizuo*; et al.

Journal of Geophysical Research; Atmospheres, 123(14), p.7754 - 7770, 2018/07

 Times Cited Count:25 Percentile:69.04(Meteorology & Atmospheric Sciences)

We compared seven atmospheric transport model results for $$^{137}$$Cs released during the Fukushima Daiichi Nuclear Power Plant accident. All the results had been submitted for a model intercomparison project of the Science Council of Japan in 2014. We assessed model performance by comparing model results with observed hourly atmospheric concentrations of $$^{137}$$Cs, focusing on nine plumes over the Tohoku and Kanto regions. The results showed that model performance for $$^{137}$$Cs concentrations was highly variable among models and plumes. We also assessed model performance for accumulated $$^{137}$$Cs deposition. Simulated areas of high deposition were consistent with the plume pathways, though the models that best simulated $$^{137}$$Cs concentrations were different from those that best simulated deposition. The ensemble mean of all models consistently reproduced $$^{137}$$Cs concentrations and deposition well, suggesting that use of a multimodel ensemble results in more effective and consistent model performance.

Journal Articles

Tracing temperature in a nanometer size region in a picosecond time period

Nakajima, Kaoru*; Kitayama, Takumi*; Hayashi, Hiroaki*; Matsuda, Makoto; Sataka, Masao*; Tsujimoto, Masahiko*; Toulemonde, M.*; Bouffard, S.*; Kimura, Kenji*

Scientific Reports (Internet), 5, p.13363_1 - 13363_8, 2015/08

 Times Cited Count:5 Percentile:40.93(Multidisciplinary Sciences)

Journal Articles

Temperature of thermal spikes in amorphous silicon nitride films produced by 1.11 MeV C$$_{60}^{3+}$$ impacts

Kitayama, Takumi*; Nakajima, Kaoru*; Suzuki, Motofumi*; Narumi, Kazumasa; Saito, Yuichi; Matsuda, Makoto; Sataka, Masao*; Tsujimoto, Masahiko*; Isoda, Shoji*; Kimura, Kenji*

Nuclear Instruments and Methods in Physics Research B, 354, p.183 - 186, 2015/07

 Times Cited Count:2 Percentile:17.52(Instruments & Instrumentation)

Journal Articles

Development of a new continuous dissolution apparatus with a hydrophobic membrane for superheavy element chemistry

Oe, Kazuhiro*; Attallah, M. F.*; Asai, Masato; Goto, Naoya*; Gupta, N. S.*; Haba, Hiromitsu*; Huang, M.*; Kanaya, Jumpei*; Kaneya, Yusuke*; Kasamatsu, Yoshitaka*; et al.

Journal of Radioanalytical and Nuclear Chemistry, 303(2), p.1317 - 1320, 2015/02

 Times Cited Count:10 Percentile:64.26(Chemistry, Analytical)

A new technique for continuous dissolution of nuclear reaction products transported by a gas-jet system was developed for superheavy element (SHE) chemistry. In this technique, a hydrophobic membrane is utilized to separate an aqueous phase from the gas phase. With this technique, the dissolution efficiencies of short-lived radionuclides of $$^{91m,93m}$$Mo and $$^{176}$$W were measured. Yields of more than 80% were observed for short-lived radionuclides at aqueous-phase flow rates of 0.1-0.4 mL/s. The gas flow-rate had no influence on the dissolution efficiency within the studied flow range of 1.0-2.0 L/min. These results show that this technique is applicable for on-line chemical studies of SHEs in the liquid phase.

Journal Articles

Probing strongly correlated 4$$f$$-orbital symmetry of the ground state in Yb compounds by linear dichroism in core-level photoemission

Mori, Takeo*; Kitayama, Satoshi*; Kanai, Yuina*; Naimen, Sho*; Fujiwara, Hidenori*; Higashiya, Atsushi*; Tamasaku, Kenji*; Tanaka, Arata*; Terashima, Kensei*; Imada, Shin*; et al.

Journal of the Physical Society of Japan, 83(12), p.123702_1 - 123702_5, 2014/12

 Times Cited Count:16 Percentile:68.37(Physics, Multidisciplinary)

We show that the strongly correlated 4$$f$$-orbital symmetry of the ground state is revealed by linear dichroism in core-level photoemission spectra, as we have discovered for YbRh$$_{2}$$Si$$_{2}$$ and YbCu$$_{2}$$Si$$_{2}$$. Theoretical analysis shows us that the linear dichroism reflects the anisotropic charge distributions resulting from a crystalline electric field. We have successfully determined the ground-state 4$$f$$ symmetry for both compounds from the polarization-dependent angle resolved core-level spectra at a temperature well below the first excitation energy. The excited-state symmetry is also probed by temperature dependence of the linear dichroism where the high measurement temperatures are on the order of the crystal-field-splitting energies.

Journal Articles

Sputtering of SiN films by 540 keV C$$_{60}$$$$^{2+}$$ ions observed using high-resolution Rutherford backscattering spectroscopy

Nakajima, Kaoru*; Morita, Yosuke*; Kitayama, Takumi*; Suzuki, Motofumi*; Narumi, Kazumasa; Saito, Yuichi; Tsujimoto, Masahiko*; Isoda, Shoji*; Fujii, Yoshikazu*; Kimura, Kenji*

Nuclear Instruments and Methods in Physics Research B, 332, p.117 - 121, 2014/08

 Times Cited Count:7 Percentile:48.18(Instruments & Instrumentation)

Journal Articles

Burning of MOX fuels in LWRs; Fuel history effects on thermal properties of hull and end piece wastes and the repository performance

Hirano, Fumio; Sato, Seichi*; Kozaki, Tamotsu*; Inagaki, Yaohiro*; Iwasaki, Tomohiko*; Oe, Toshiaki*; Kato, Kazuyuki*; Kitayama, Kazumi*; Nagasaki, Shinya*; Niibori, Yuichi*

Journal of Nuclear Science and Technology, 49(3), p.310 - 319, 2012/03

AA2011-0278.pdf:0.56MB

 Times Cited Count:0 Percentile:0.01(Nuclear Science & Technology)

The thermal impacts of hull and end piece wastes from the reprocessing of MOX spent fuels burned in LWRs on repository performance were investigated. The heat generation rates in MOX spent fuels and the resulting heat generation rates in hull and end piece wastes change depending on the fuel histories including the burn-up of UO$$_{2}$$ spent fuels, the cooling period before reprocessing, the storage period of fresh MOX fuels. The heat generation rates of hull and end piece wastes from the reprocessing of MOX spent fuels with any of those histories are significantly larger than those from UO$$_{2}$$ spent fuels with burn-ups of 45 GWd/THM. If a temperature below 80$$^{circ}$$C is specified for cement-based materials used in waste packages after disposal, the allowable number of canisters containing compacted hull and end pieces in a package for 45 GWd-MOX needs to be limited to a value of 0.7 to 1.6, which is significantly lower than the value of 4.0 for 45 GWd-UO$$_{2}$$.

Journal Articles

Study on improvement of reliability on inventory assessment in vitrified waste for long-term safety of geological disposal

Ishikawa, Masumi*; Kaneko, Satoru*; Kitayama, Kazumi*; Ishiguro, Katsuhiko*; Ueda, Hiroyoshi*; Wakasugi, Keiichiro*; Shinohara, Nobuo; Okumura, Keisuke; Chino, Masamichi; Moriya Noriyasu*

Nihon Genshiryoku Gakkai Wabun Rombunshi, 8(4), p.304 - 312, 2009/12

Since quality control issues for vitrified waste are defined mainly with the focus on the transport and storage of the waste rather than the long-term safety of geological disposal, they do not cover inventories of long-lived nuclides which are of most interest in the safety assessment of geological disposal. Therefore we suggest a flow chart for assessment of inventories of long-lived nuclides in the vitrified waste focusing on measured value. We started a programme to examine the applicability as well as to improve reliability of nuclide generation/decay code and nuclear data library using liquid waste from spent fuel with clear irradiation history. To solve the issue of quality control for vitrified waste, comprehensive study is needed in aspects not only of geological disposal field but also of operation of nuclear power plant, reprocessing of spent fuel and vitrification of liquid waste. This study is a pioneering study to integrate them.

JAEA Reports

Discussion on sealing performance required in disposal system; Preliminary study on hydraulic analysis of disposal panel

Sugita, Yutaka*; Takahashi, Yoshiaki*; Uragami, Manabu*; Kitayama, Kazumi*; Fujita, Tomoo; Yui, Mikazu

JAEA-Research 2007-023, 70 Pages, 2007/03

JAEA-Research-2007-023.pdf:26.16MB

The sealing performance of a repository is very important for the safety assessment of the geological disposal system for high-level radioactive waste. NUMO and JAEA set up a technical commission to investigate sealing technology in a repository in 2004 following a cooperation agreement between these two organisations. The objectives of this commission were to present a concept of sealing performance required in the disposal system and to direct future R&D for design requirements of closure components (backfilling material, clay plug, etc.). Hydraulic analyses on tunnel intersections were carried out during the first year in 2004. This was expanded into a hydraulic analysis of a complete disposal panel with all tunnels during the second year in 2005. Since the model structure in 2005 was more complicated than the one used in 2004, the concept of equivalent permeability was adopted in and around each tunnel in the hydraulic analyses. Parameters used in the hydraulic analyses were installation positions of clay plugs, permeability of the backfilling material, permeability of disposal tunnel and directions of hydraulic gradient to estimate influences to the analytical results preliminary. Analytical results showed that flow rate in a disposal tunnel was influenced by directions of hydraulic gradient, installation of the clay plug at the both ends of each disposal tunnel and permeability of the main tunnel.

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